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11. 发明申请

US20050100494A1 Ferrierite compositions for reducing NOx emissions during fluid catalytic cracking 审中-公开
标题翻译：用于在流化床催化裂化过程中减少NOx排放的镁碱沸石组合物
公开(公告)号：US20050100494A1
公开(公告)日：2005-05-12
申请号：US10909706
申请日：2004-08-02
申请人： George Yaluris , Michael Ziebarth , Xinjin Zhao
发明人： George Yaluris , Michael Ziebarth , Xinjin Zhao
IPC分类号： B01D53/86 , B01J23/42 , B01J23/83 , B01J29/08 , B01J29/65 , B01J29/80 , B01J35/00 , B01J37/00 , C10G11/18 , B01J29/04 , B01J29/87 , B01J21/00 , B01J29/00 , B01J27/14 , B01J27/186 , B01J27/187 , B01J27/199 , C01B21/00 , B01J21/08 , B01J21/12 , B01J21/14
CPC分类号： B01D53/8628 , B01D2255/50 , B01D2258/00 , B01J23/42 , B01J23/83 , B01J29/084 , B01J29/65 , B01J29/80 , B01J35/0006 , B01J35/002 , B01J37/0045 , B01J2229/18 , B01J2229/42 , C10G11/18 , C10G11/182 , C10G2300/405
摘要： Compositions for reduction of NOx generated during a catalytic cracking process, preferably, a fluid catalytic cracking process, are disclosed. The compositions comprise a fluid catalytic cracking catalyst composition, preferably containing a Y-type zeolite, and a particulate NOx reduction composition containing ferrierite zeolite particles. Preferably, the NOx reduction composition contains ferrierite zeolite particles bound with an inorganic binder. In the alternative, the ferrierite zeolite particles are incorporated into the cracking catalyst as an integral component of the catalyst. NOx reduction compositions in accordance with the invention are very effective for the reduction of NOx emissions released from the regenerator of a fluid catalytic cracking unit operating under FCC process conditions without a substantial change in conversion or yield of cracked products. Processes for the use of the compositions are also disclosed.
摘要翻译：公开了在催化裂化过程中产生的用于还原NO x x N的组合物，优选流化催化裂化过程。组合物包含优选含有Y型沸石的流化催化裂化催化剂组合物和含有镁碱沸石颗粒的颗粒状NO x X还原组合物。优选地，NO x X还原组合物含有与无机粘合剂结合的镁碱沸石颗粒。替代方案中，镁碱沸石颗粒作为催化剂的组成成分加入到裂化催化剂中。根据本发明的NO x x还原组合物对于在FCC工艺条件下操作的流化催化裂化装置的再生器中释放的NO x x N 2排放非常有效，破裂产品的转化率或产量大幅度变化。还公开了使用组合物的方法。

12. 发明授权

US09504975B2 System and process for injecting catalyst and/or additives into a fluidized catalytic cracking unit 有权
公开(公告)号：US09504975B2
公开(公告)日：2016-11-29
申请号：US13193052
申请日：2011-07-28
申请人： George Yaluris , Lenny Lee Albin , Alfred Ferdinand Jordan
发明人： George Yaluris , Lenny Lee Albin , Alfred Ferdinand Jordan
IPC分类号： B01J8/24 , B65G53/28 , B01J8/00 , B01J8/32 , B01J8/06 , B01J8/18 , C10G11/18
CPC分类号： B01J8/0015 , B01J8/0025 , B01J8/003 , B01J8/0035 , B01J8/004 , B01J8/006 , B01J8/06 , B01J8/18 , B01J8/24 , B01J8/32 , B01J2208/00548 , B01J2208/00752 , B01J2208/00761 , B01J2208/00769 , B65G53/28 , C10G11/18 , C10G2300/80
摘要： A preferred embodiment of a system for loading catalyst and/or additives into a fluidized catalytic cracking unit includes a bin for storing at least one of the catalyst and/or additives, and a loading unit in fluid communication with the storage bin and the fluidized catalytic cracking unit on a selective basis. The loading unit is capable of being evacuated so that a resulting vacuum within the loading unit draws the catalyst and/or additive from the bin. The loading unit is also capable of being pressurized so that the catalyst and/or additive is transferred from the loading unit to the fluidized catalytic cracking unit.

13. 发明授权

US09120090B2 Modified zeolite catalyst 有权
标题翻译：改性沸石催化剂
公开(公告)号：US09120090B2
公开(公告)日：2015-09-01
申请号：US13377725
申请日：2010-06-22
申请人： Avelino Corma , Cristina Martinez , Eric J. Doskocil , George Yaluris
发明人： Avelino Corma , Cristina Martinez , Eric J. Doskocil , George Yaluris
IPC分类号： B01J29/06 , B01J35/10 , B01J29/44 , B01J29/70 , B01J29/72 , B01J29/78 , B01J37/06 , C01B39/02 , C07C1/20 , C10G50/00
CPC分类号： B01J35/1038 , B01J29/44 , B01J29/7042 , B01J29/7092 , B01J29/7284 , B01J29/7884 , B01J35/1061 , B01J35/109 , B01J37/06 , B01J2229/16 , B01J2229/22 , B01J2229/32 , B01J2229/37 , B01J2229/38 , C01B39/026 , C07C1/20 , C07C2521/04 , C07C2521/08 , C07C2521/12 , C07C2529/70 , C07C2529/76 , C07C2529/78 , C10G50/00 , C10G2300/70
摘要： A modified zeolite catalyst derived from a zeolite of a structural type which consists of a one-dimensional micropore structure of channels made from rings containing between 8 and 12 silicon/aluminum atoms is disclosed. It consists substantially of a plurality of crystallites having additional mesoporosity whose volume is in the range 0.09 to 0.25 cc/g as mentioned by nitrogen adsorption at 77° K and calculated by the BJH method. The mesoporosity may be introduced into the crystallites by e.g. treatment with aqueous sodium hydroxide at a pH at 25° C. in excess of 8 for an extended period at elevated temperature. The catalyst shows improved resistance to catalyst deactivation and greater selectivity to higher hydrocarbons when used to e.g. oligomerize light alkenes e.g. propene or the butenes.
摘要翻译：公开了一种衍生自结构类型的沸石的改性沸石催化剂，其由包含8和12个硅/铝原子的环制成的通道的一维微孔结构组成。它基本上由具有额外介孔度的多个微晶组成，其体积在0.09至0.25cc / g的范围内，如通过77°K的氮气吸附所提及的，并通过BJH方法计算。可以通过例如，将介孔导入微晶。在25℃的pH下在高温下长时间处理超过8的氢氧化钠水溶液处理。该催化剂显示出改进的对催化剂失活的抵抗性和当用于例如高分子量化合物时对高级烃的更高选择性。低聚轻链烯，例如丙烯或丁烯。

14. 发明授权

US08967919B2 System and process for injecting catalyst and/or additives into a fluidized catalytic cracking unit 有权
标题翻译：将催化剂和/或添加剂注入到流化催化裂化装置中的系统和方法
公开(公告)号：US08967919B2
公开(公告)日：2015-03-03
申请号：US13193012
申请日：2011-07-28
申请人： George Yaluris , Lenny Albin , Alfred Jordan
发明人： George Yaluris , Lenny Albin , Alfred Jordan
IPC分类号： B65G53/66 , C10G11/18 , B01J8/00 , B01J8/06 , B01J8/18 , B01J8/24
CPC分类号： C10G11/18 , B01J8/0015 , B01J8/0025 , B01J8/003 , B01J8/0035 , B01J8/004 , B01J8/006 , B01J8/06 , B01J8/18 , B01J8/24 , B01J2208/00548 , B01J2208/00752 , B01J2208/00761 , B01J2208/00769 , C10G2300/80
摘要： A preferred embodiment of a system for loading catalyst and/or additives into a fluidized catalytic cracking unit includes a bin for storing at least one of the catalyst and/or additives, and a loading unit in fluid communication with the storage bin and the fluidized catalytic cracking unit on a selective basis. The loading unit is capable of being evacuated so that a resulting vacuum within the loading unit draws the catalyst and/or additive from the bin. The loading unit is also capable of being pressurized so that the catalyst and/or additive is transferred from the loading unit to the fluidized catalytic cracking unit.
摘要翻译：用于将催化剂和/或添加剂加载到流化催化裂化装置中的系统的优选实施方案包括用于储存催化剂和/或添加剂中的至少一种的容器以及与储存箱和流化催化剂流体连通的装载单元选择性地开裂单元。装载单元能够被排空，使得装载单元内的所得真空从箱中抽出催化剂和/或添加剂。加载单元还能够被加压，使得催化剂和/或添加剂从装载单元转移到流化催化裂化装置。

15. 发明授权

US08901364B2 Alkene oligomerization process 有权
标题翻译：烯烃低聚过程
公开(公告)号：US08901364B2
公开(公告)日：2014-12-02
申请号：US13377959
申请日：2010-06-22
申请人： Avelino Corma , Cristina Martinez , Eric J. Doskocil , George Yaluris
发明人： Avelino Corma , Cristina Martinez , Eric J. Doskocil , George Yaluris
IPC分类号： C07C2/12 , B01J29/70 , B01J29/06 , B01J35/10 , C10G50/00 , C10L1/08
CPC分类号： B01J29/7042 , B01J29/06 , B01J35/1061 , B01J2229/16 , B01J2229/22 , B01J2229/38 , C10G50/00 , C10G2300/1088 , C10G2300/4018 , C10G2300/70 , C10G2400/04 , C10L1/08
摘要： Disclosed is a process for producing a hydrocarbon fraction rich in components boiling in the range typical for diesel fuel comprising contacting a feedstock comprising one or more C2 to C10 alkenes with a modified zeolite catalyst having a one-dimensional micropore structure consisting of channels made from rings containing between 8 and 12 silicon/aluminum atoms at a temperature in the range 100 to 500° C. and pressure in the range 0.1 to 200 bar characterized in that the modified zeolite catalyst is one which has been prepared by treating a corresponding zeolite precursor with an alkaline solution. The alkaline solution used to treat the zeolite precursor can be for example aqueous sodium hydroxide solution. Relative to equivalent untreated zeolites the modified zeolite catalysts described show improved catalyst life and selectivity to hydrocarbons boiling in the range 250 to 350° C.
摘要翻译：公开了一种制备富含柴油特征典型沸点的组分的烃馏分的方法，包括使包含一种或多种C 2至C 10烯烃的原料与具有由环制成的通道组成的一维微孔结构的改性沸石催化剂接触在100〜500℃的温度范围内含有8〜12个硅/铝原子，压力在0.1〜200巴的范围内，其特征在于改性沸石催化剂是通过用相应的沸石前体处理碱性溶液。用于处理沸石前体的碱溶液可以是例如氢氧化钠水溶液。相对于等效的未处理的沸石，所述改性的沸石催化剂显示改善的催化剂寿命和沸点为250-350℃的烃的选择性。

16. 发明申请

US20110284588A1 SYSTEM AND PROCESS FOR INJECTING CATALYST AND/OR ADDITIVES INTO A FLUIDIZED CATALYTIC CRACKING UNIT 有权
公开(公告)号：US20110284588A1
公开(公告)日：2011-11-24
申请号：US13193012
申请日：2011-07-28
申请人： George Yaluris , Lenny Lee Albin , Alfred Ferdinand Jordan
发明人： George Yaluris , Lenny Lee Albin , Alfred Ferdinand Jordan
IPC分类号： B67D7/06
CPC分类号： C10G11/18 , B01J8/0015 , B01J8/0025 , B01J8/003 , B01J8/0035 , B01J8/004 , B01J8/006 , B01J8/06 , B01J8/18 , B01J8/24 , B01J2208/00548 , B01J2208/00752 , B01J2208/00761 , B01J2208/00769 , C10G2300/80
摘要： A preferred embodiment of a system for loading catalyst and/or additives into a fluidized catalytic cracking unit includes a bin for storing at least one of the catalyst and/or additives, and a loading unit in fluid communication with the storage bin and the fluidized catalytic cracking unit on a selective basis. The loading unit is capable of being evacuated so that a resulting vacuum within the loading unit draws the catalyst and/or additive from the bin. The loading unit is also capable of being pressurized so that the catalyst and/or additive is transferred from the loading unit to the fluidized catalytic cracking unit.

17. 发明申请

US20110280769A1 SYSTEM AND PROCESS FOR INJECTING CATALYST AND/OR ADDITIVES INTO A FLUIDIZED CATALYTIC CRACKING UNIT 有权
标题翻译：将催化剂和/或添加剂注入流化催化裂化装置的系统和方法
公开(公告)号：US20110280769A1
公开(公告)日：2011-11-17
申请号：US13193052
申请日：2011-07-28
申请人： George Yaluris , Lenny Lee Albin , Alfred Ferdinand Jordan
发明人： George Yaluris , Lenny Lee Albin , Alfred Ferdinand Jordan
IPC分类号： F27B15/08
CPC分类号： B01J8/0015 , B01J8/0025 , B01J8/003 , B01J8/0035 , B01J8/004 , B01J8/006 , B01J8/06 , B01J8/18 , B01J8/24 , B01J8/32 , B01J2208/00548 , B01J2208/00752 , B01J2208/00761 , B01J2208/00769 , B65G53/28 , C10G11/18 , C10G2300/80
摘要： A preferred embodiment of a system for loading catalyst and/or additives into a fluidized catalytic cracking unit includes a bin for storing at least one of the catalyst and/or additives, and a loading unit in fluid communication with the storage bin and the fluidized catalytic cracking unit on a selective basis. The loading unit is capable of being evacuated so that a resulting vacuum within the loading unit draws the catalyst and/or additive from the bin. The loading unit is also capable of being pressurized so that the catalyst and/or additive is transferred from the loading unit to the fluidized catalytic cracking unit.
摘要翻译：用于将催化剂和/或添加剂加载到流化催化裂化装置中的系统的优选实施方案包括用于储存催化剂和/或添加剂中的至少一种的容器以及与储存箱和流化催化剂流体连通的装载单元选择性地开裂单元。装载单元能够被排空，使得装载单元内的所得真空从箱中抽出催化剂和/或添加剂。加载单元还能够被加压，使得催化剂和/或添加剂从装载单元转移到流化催化裂化装置。

18. 发明授权

US07906015B2 Reduction of gas phase reduced nitrogen species in partial burn FCC processes 有权
标题翻译：部分燃烧FCC工艺中减少气相减少了氮物质
公开(公告)号：US07906015B2
公开(公告)日：2011-03-15
申请号：US11238745
申请日：2005-09-29
申请人： George Yaluris , John Allen Rudesill
发明人： George Yaluris , John Allen Rudesill
IPC分类号： C10G11/00
CPC分类号： B01D53/8621 , B01D53/96 , Y02P30/446
摘要： Reduced emissions of gas phase reduced nitrogen species in the off gas of an FCC regenerator operated in a partial or incomplete mode of combustion is achieved by contacting the off gas with an oxidative catalyst/additive composition having the ability to reduce gas phase nitrogen species to molecular nitrogen and to oxidize CO under catalytic cracking conditions. The oxidative catalyst/additive composition is used in an amount less than the amount necessary to prevent afterburn. Fluidizable particles of the oxidative catalyst/additives are circulated throughout the partial or incomplete burn FCC unit along with the FCC catalyst inventory. The flue gas having a reduced content of gas phase reduced nitrogen species and NOx is passed to a downstream CO boiler, preferably a low NOx CO boiler. In the CO boiler, as CO is oxidized to CO2, a reduced amount of gas phase reduced nitrogen species is oxidized to NOx, thereby providing an increase in the overall reduction of NOx emitted into the environment.
摘要翻译：通过使脱气与具有将气相氮物质还原成分子的能力的氧化催化剂/添加剂组合物接触来实现在部分或不完全燃烧模式下操作的FCC再生器的废气中减少的气相排放减少的氮物质并在催化裂化条件下氧化CO。氧化催化剂/添加剂组合物的用量小于防止后燃烧所需的量。氧化催化剂/添加剂的可流化颗粒与FCC催化剂库存一起循环遍及部分或不完全燃烧的FCC单元。具有减少的氮气种类的气相含量降低的烟道气被排放到下游CO锅炉，优选低NOx CO锅炉。在CO锅炉中，当CO被氧化成CO 2时，减少的氮气种类的气相被氧化成NOx，从而提高了排放到环境中的NO x的总体还原。

19. 发明授权

US07030055B2 NOx reduction compositions for use in FCC processes 失效
标题翻译：用于FCC工艺的NOx还原组合物
公开(公告)号：US07030055B2
公开(公告)日：2006-04-18
申请号：US10837846
申请日：2004-05-03
申请人： George Yaluris , John Allen Rudesill
发明人： George Yaluris , John Allen Rudesill
IPC分类号： B01J23/00 , B01J23/40 , B01J23/42 , B01J23/44 , B01J21/00
CPC分类号： B01J35/023 , B01D53/8628 , B01J21/12 , B01J23/10 , B01J23/58 , B01J23/63 , B01J29/08 , B01J35/0006 , B01J35/1019 , B01J37/0045 , C10G11/182 , Y02P30/446
摘要： Compositions for reduction of gas phase reduced nitrogen species and NOx generated during a partial or incomplete combustion catalytic cracking process, preferably, a fluid catalytic cracking process, are disclosed. The compositions comprise (i) an acidic metal oxide containing substantially no zeolite, (ii) an alkali metal, alkaline earth metal, and mixtures thereof, (iii) an oxygen storage component, and (iv) a noble metal component, preferably rhodium or iridium, and mixtures thereof, are disclosed. Preferably, the compositions are used as separate additives particles circulated along with the circulating FCC catalyst inventory. Reduced emissions of gas phase reduced nitrogen species and NOx in an effluent off gas of a partial or incomplete combustion FCC regenerator provide for an overall NOx reduction as the effluent gas stream is passed from the FCC regenerator to a CO boiler, whereby as CO is oxidized to CO2 a lesser amount of the reduced nitrogen species is oxidized to NOx.
摘要翻译：公开了在部分或不完全燃烧催化裂化过程中产生的气相还原氮和NO x的组合物，优选流化催化裂化过程。组合物包含（i）基本上不含沸石的酸性金属氧化物，（ii）碱金属，碱土金属及其混合物，（iii）储氧组分，和（iv）贵金属组分，优选铑或铱及其混合物。优选地，组合物用作与循环FCC催化剂库存一起循环的单独的添加剂颗粒。在部分或不完全燃烧的FCC再生器的排出物气体中减少的气相排放减少了氮物质和NO x，从而提供了总体NO x SO 2还原作为流出气流从FCC再生器传递到CO锅炉，由此当CO被氧化成CO 2时，较少量的还原氮物质被氧化成NO 2。

20. 发明申请

US20050042158A1 NOx reduction compositions for use in FCC processes 失效
标题翻译：用于FCC工艺的NOx还原组合物
公开(公告)号：US20050042158A1
公开(公告)日：2005-02-24
申请号：US10837846
申请日：2004-05-03
申请人： George Yaluris , John Rudesill
发明人： George Yaluris , John Rudesill
IPC分类号： B01D53/86 , B01J21/12 , B01J23/10 , B01J23/58 , B01J23/63 , B01J29/08 , B01J35/00 , B01J35/02 , B01J35/10 , B01J37/00 , C10G11/18
CPC分类号： B01J35/023 , B01D53/8628 , B01J21/12 , B01J23/10 , B01J23/58 , B01J23/63 , B01J29/08 , B01J35/0006 , B01J35/1019 , B01J37/0045 , C10G11/182 , Y02P30/446
摘要： Compositions for reduction of gas phase reduced nitrogen species and NOx generated during a partial or incomplete combustion catalytic cracking process, preferably, a fluid catalytic cracking process, are disclosed. The compositions comprise (i) an acidic metal oxide containing substantially no zeolite, (ii) an alkali metal, alkaline earth metal, and mixtures thereof, (iii) an oxygen storage component, and (iv) a noble metal component, preferably rhodium or iridium, and mixtures thereof, are disclosed. Preferably, the compositions are used as separate additives particles circulated along with the circulating FCC catalyst inventory. Reduced emissions of gas phase reduced nitrogen species and NOx in an effluent off gas of a partial or incomplete combustion FCC regenerator provide for an overall NOx reduction as the effluent gas stream is passed from the FCC regenerator to a CO boiler, whereby as CO is oxidized to CO2 a lesser amount of the reduced nitrogen species is oxidized to NOx.
摘要翻译：公开了在部分或不完全燃烧催化裂化过程（优选流化催化裂化过程）中产生的气相还原氮和氮氧化合物的组合物。组合物包含（i）基本上不含沸石的酸性金属氧化物，（ii）碱金属，碱土金属及其混合物，（iii）储氧组分，和（iv）贵金属组分，优选铑或铱及其混合物。优选地，组合物用作与循环FCC催化剂库存一起循环的单独的添加剂颗粒。在部分或不完全燃烧的废气中，气相的减少排放减少了氮物质和NOx。随着废气流从FCC再生器通入CO锅炉，FCC再生器提供总的NOx还原，从而当CO被氧化对于二氧化碳，较少量的还原氮物质被氧化成NOx。

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