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11. 发明申请

US20100120926A1 Processes for Gasification of a Carbonaceous Feedstock 审中-公开
标题翻译：碳质原料气化工艺
公开(公告)号：US20100120926A1
公开(公告)日：2010-05-13
申请号：US12562921
申请日：2009-09-18
申请人： Earl T. Robinson , Avinash Sirdeshpande , Eli Gal , Vincent G. Reiling , Nicholas Charles Nahas
发明人： Earl T. Robinson , Avinash Sirdeshpande , Eli Gal , Vincent G. Reiling , Nicholas Charles Nahas
IPC分类号： C07C1/04
CPC分类号： C10J3/00 , C01B3/34 , C01B3/48 , C01B2203/0233 , C01B2203/0244 , C01B2203/025 , C01B2203/0283 , C01B2203/0405 , C01B2203/0415 , C01B2203/0445 , C01B2203/045 , C01B2203/0455 , C01B2203/046 , C01B2203/047 , C01B2203/0475 , C01B2203/048 , C01B2203/0485 , C01B2203/06 , C01B2203/1058 , C01B2203/1064 , C01B2203/147 , C10J3/482 , C10J3/721 , C10J2300/093 , C10J2300/0956 , C10J2300/0959 , C10J2300/0973 , C10J2300/0986 , C10J2300/1662 , C10J2300/1671 , C10J2300/1675 , C10J2300/1687 , C10J2300/1807 , C10J2300/1884 , C10K1/004 , C10K1/005 , C10K1/122 , C10K1/143 , C10K1/16 , C10K1/165 , C10K3/04 , C10L3/08
摘要： The present invention relates to processes for preparing gaseous products, and in particular, methane via the catalytic gasification of carbonaceous feedstocks in the presence of steam. The processes comprise using at least one methanation step to convert carbon monoxide and hydrogen in the gaseous products to methane and do not recycle carbon monoxide or hydrogen to the catalytic gasifier.
摘要翻译：本发明涉及通过在蒸汽存在下通过碳质原料的催化气化来制备气态产物，特别是甲烷的方法。该方法包括使用至少一个甲烷化步骤将气态产物中的一氧化碳和氢气转化成甲烷，并且不将一氧化碳或氢气循环到催化气化器中。

12. 发明授权

US08999020B2 Processes for the separation of methane from a gas stream 有权
标题翻译：从气流中分离甲烷的方法
公开(公告)号：US08999020B2
公开(公告)日：2015-04-07
申请号：US12415042
申请日：2009-03-31
申请人： Pattabhi K. Raman , Francis S. Lau , Earl T. Robinson
发明人： Pattabhi K. Raman , Francis S. Lau , Earl T. Robinson
IPC分类号： C10J3/46 , C10J3/00 , C01B3/34 , C01B3/52 , C01B3/58 , C10J3/48 , C10J3/72 , C10J3/82 , C10K3/04 , C10L3/08 , C10L3/10 , F25J3/02
CPC分类号： C10J3/00 , C01B3/34 , C01B3/52 , C01B3/58 , C01B2203/0205 , C01B2203/0283 , C01B2203/0405 , C01B2203/0415 , C01B2203/0435 , C01B2203/0465 , C01B2203/047 , C01B2203/0475 , C01B2203/048 , C01B2203/0485 , C01B2203/06 , C01B2203/1241 , C01B2203/84 , C10J3/482 , C10J3/72 , C10J3/82 , C10J2300/0903 , C10J2300/0973 , C10J2300/0986 , C10J2300/1662 , C10J2300/1807 , C10J2300/1823 , C10J2300/1853 , C10K3/04 , C10L3/08 , C10L3/10 , F25J3/0223 , F25J3/0233 , F25J3/0252 , F25J3/0261 , F25J3/0271 , F25J2205/40 , F25J2205/80 , F25J2215/02 , F25J2245/02
摘要： Processes for the catalytic conversion of a carbonaceous composition into a gas stream comprising methane are provided. In addition, the processes provide for the generation of a hydrogen-enriched gas stream and, optionally, a carbon monoxide-enriched gas stream, which can be mixed or used separately as an energy source for subsequent catalytic gasification processes.
摘要翻译：提供了将碳质组合物催化转化成包含甲烷的气流的方法。此外，这些方法提供了产生富含氢气的气流和任选地富含一氧化碳的气流，其可以单独混合或使用作为后续催化气化过程的能量源。

13. 发明授权

US08647402B2 Processes for gasification of a carbonaceous feedstock 有权
标题翻译：碳质原料气化方法
公开(公告)号：US08647402B2
公开(公告)日：2014-02-11
申请号：US12562922
申请日：2009-09-18
申请人： Earl T. Robinson , Francis S. Lau , Pattabhi K. Raman , Vincent G. Reiling , Dwain Dodson , Mustafiz Rahman , Nicholas Charles Nahas
发明人： Earl T. Robinson , Francis S. Lau , Pattabhi K. Raman , Vincent G. Reiling , Dwain Dodson , Mustafiz Rahman , Nicholas Charles Nahas
IPC分类号： B23K35/38
CPC分类号： C10J3/00 , C01B3/586 , C01B2203/0445 , C01B2203/047 , C10G2/32 , C10J3/482 , C10J3/721 , C10J2300/093 , C10J2300/0956 , C10J2300/0959 , C10J2300/0973 , C10J2300/0986 , C10J2300/1662 , C10J2300/1671 , C10J2300/1675 , C10J2300/1687 , C10J2300/1807 , C10J2300/1884 , C10L3/08 , C10L3/102 , C10L9/10
摘要： The present invention relates to processes and continuous processes for preparing gaseous products, and in particular, methane via the catalytic gasification of carbonaceous feedstocks in the presence of steam. In one aspect of the invention, the processes comprise at least partially combusting a first carbonaceous feedstock with an oxygen-rich gas stream in an oxygen-blown gasifier, under suitable temperature and pressure, to generate a first gas stream comprising hydrogen, carbon monoxide and superheated steam; and reacting a second carbonaceous feedstock and the first gas stream in a catalytic gasifier in the presence of a gasification catalyst under suitable temperature and pressure to form a second gas stream comprising a plurality of gaseous products comprising methane, carbon dioxide, hydrogen, carbon monoxide and hydrogen sulfide. The processes can comprise using at least one catalytic methanator to convert carbon monoxide and hydrogen in the gaseous products to methane and in certain embodiments do not recycle carbon monoxide or hydrogen to the gasifier.
摘要翻译：本发明涉及用于在蒸汽存在下通过碳质原料的催化气化来制备气态产物，特别是甲烷的方法和连续方法。在本发明的一个方面，该方法包括在合适的温度和压力下，在吹氧气化器中至少部分地将第一含碳原料与富氧气流一起燃烧，以产生包含氢气，一氧化碳和过热蒸汽以及在气化催化剂存在下，在合适的温度和压力下使催化气化器中的第二碳质原料与第一气流反应，形成第二气流，其包含多个包含甲烷，二氧化碳，氢气，一氧化碳和硫化氢。该方法可以包括使用至少一种催化甲烷化器将气态产物中的一氧化碳和氢气转化成甲烷，并且在某些实施方案中不将一氧化碳或氢气循环到气化器。

14. 发明授权

US08123827B2 Processes for making syngas-derived products 有权
标题翻译：制造合成气衍生产品的方法
公开(公告)号：US08123827B2
公开(公告)日：2012-02-28
申请号：US12342628
申请日：2008-12-23
申请人： Earl T. Robinson
发明人： Earl T. Robinson
IPC分类号： C07C27/00 , C10J3/46
CPC分类号： C10J3/00 , C10G2/00 , C10G2/32 , C10G2300/807 , C10J3/463 , C10J2300/0903 , C10J2300/093 , C10J2300/0943 , C10J2300/0986 , C10J2300/16 , C10J2300/1659 , C10J2300/1665 , C10J2300/1853 , C10J2300/1861 , C10K1/003 , C10K3/00 , C10K3/04
摘要： The present invention provides processes for making syngas-derived products. For example, one aspect of the present invention provides a process for making a syngas-derived product, the process comprising (a) providing a carbonaceous feedstock; (b) converting the carbonaceous feedstock in a syngas formation zone at least in part to a synthesis gas stream comprising hydrogen and carbon monoxide; (c) conveying the synthesis gas stream to a syngas reaction zone; (d) reacting the synthesis gas stream in the syngas reaction zone to form the syngas-derived product and heat energy, a combustible tail gas mixture, or both; (e) recovering the syngas-derived product; and (f) recovering the heat energy formed from the reaction of the synthesis gas stream, burning the combustible tail gas mixture to form heat energy, or both.
摘要翻译：本发明提供了制备合成气衍生产品的方法。例如，本发明的一个方面提供了制备合成气衍生产品的方法，该方法包括（a）提供含碳原料; （b）将合成气形成区中的含碳原料至少部分转化成包含氢气和一氧化碳的合成气流; （c）将合成气流输送到合成气反应区; （d）使合成气流在合成气反应区中反应以形成合成气衍生的产物和热能，可燃尾气混合物或两者; （e）回收合成气衍生产品; 和（f）回收由合成气流的反应形成的热能，燃烧可燃尾气混合物以形成热能，或两者兼而有之。

15. 发明申请

US20090324460A1 Four-Train Catalytic Gasification Systems 审中-公开
标题翻译：四列车催化气化系统
公开(公告)号：US20090324460A1
公开(公告)日：2009-12-31
申请号：US12492484
申请日：2009-06-26
申请人： Earl T. Robinson , Francis S. Lau , Dwain Dodson
发明人： Earl T. Robinson , Francis S. Lau , Dwain Dodson
IPC分类号： B01J8/00
CPC分类号： C10J3/00 , C01B3/34 , C01B3/501 , C01B3/506 , C01B3/52 , C01B2203/0205 , C01B2203/0405 , C01B2203/0415 , C01B2203/042 , C01B2203/046 , C01B2203/0465 , C01B2203/0475 , C01B2203/048 , C01B2203/0485 , C01B2203/0894 , C01B2203/1241 , C01B2203/84 , C10J3/482 , C10J3/721 , C10J2300/0903 , C10J2300/0906 , C10J2300/0916 , C10J2300/093 , C10J2300/0973 , C10J2300/0986 , C10J2300/1662 , C10J2300/1671 , C10J2300/1675 , C10J2300/1687 , C10J2300/169 , C10J2300/1807 , C10J2300/1823 , C10J2300/1853 , C10J2300/1884 , C10K1/003 , C10K1/004 , C10K1/006 , C10K1/007 , C10K1/101 , C10K1/102 , C10K1/103 , C10K1/14 , C10K1/143 , C10K1/16 , C10K1/20 , C10K1/32 , C10K3/04 , C10L3/08 , C10L3/10 , C10L3/102
摘要： Systems to convert a carbonaceous feedstock into a plurality of gaseous products are described. The systems include, among other units, four separate gasification reactors for the gasification of a carbonaceous feedstock in the presence of an alkali metal catalyst into the plurality of gaseous products including at least methane. Each of the gasification reactors may be supplied with the feedstock from a single or separate catalyst loading and/or feedstock preparation unit operations. Similarly, the hot gas streams from each gasification reactor may be purified via their combination at a heat exchanger, acid gas removal, or methane removal unit operations. Product purification may comprise trace contaminant removal units, ammonia removal and recovery units, and sour shift units.
摘要翻译：描述了将碳质原料转化成多种气体产物的系统。这些系统包括四个单独的气化反应器，用于在碱金属催化剂存在下将碳质原料气化成至少包括甲烷的多种气态产物。可以从单个或单独的催化剂装载和/或原料制备单元操作向每个气化反应器供应原料。类似地，来自每个气化反应器的热气流可以通过它们的组合在热交换器，酸性气体去除或甲烷去除单元操作中纯化。产品净化可以包括痕量污染物去除单元，氨去除和回收单元以及酸转移单元。

16. 发明申请

US20090246120A1 Sour Shift Process for the Removal of Carbon Monoxide from a Gas Stream 有权
标题翻译：从气流中去除一氧化碳的酸转移过程
公开(公告)号：US20090246120A1
公开(公告)日：2009-10-01
申请号：US12415050
申请日：2009-03-31
申请人： Pattabhi K. Raman , Francis S. Lau , Earl T. Robinson
发明人： Pattabhi K. Raman , Francis S. Lau , Earl T. Robinson
IPC分类号： C01B3/26
CPC分类号： C10J3/82 , C01B3/12 , C01B3/34 , C01B3/50 , C01B3/52 , C01B2203/0205 , C01B2203/0283 , C01B2203/04 , C01B2203/0405 , C01B2203/0415 , C01B2203/0435 , C01B2203/0445 , C01B2203/046 , C01B2203/0465 , C01B2203/0475 , C01B2203/048 , C01B2203/0485 , C01B2203/1241 , C01B2203/147 , C10J3/00 , C10J3/482 , C10J3/72 , C10J3/721 , C10J2300/0903 , C10J2300/094 , C10J2300/0959 , C10J2300/0966 , C10J2300/0973 , C10J2300/1662 , C10J2300/1687 , C10J2300/1807 , C10J2300/1823 , C10J2300/1846 , C10J2300/1853 , C10K3/04 , C10L3/10
摘要： Processes for the catalytic conversion of a carbonaceous composition into a gas stream comprising methane are provided, where a sour shift reaction is used to remove carbon monoxide gas stream produced by the gasification process. The incorporation of the sour shift reaction provides an efficient and cost-effective means of eliminating carbon monoxide from the gas stream. In addition, the sour shift reaction also generates additional hydrogen, thus increasing the amount of hydrogen produced from the gasification process.
摘要翻译：提供了将碳质组合物催化转化成包含甲烷的气流的方法，其中使用酸转移反应来除去由气化过程产生的一氧化碳气流。引入酸转移反应提供了从气流中除去一氧化碳的有效且成本有效的手段。此外，酸转化反应还产生额外的氢，从而增加从气化过程产生的氢气的量。

17. 发明申请

US20090217589A1 Carbonaceous Fines Recycle 有权
标题翻译：碳质细粉回收
公开(公告)号：US20090217589A1
公开(公告)日：2009-09-03
申请号：US12395385
申请日：2009-02-27
申请人： Earl T. Robinson
发明人： Earl T. Robinson
IPC分类号： C10J3/46 , B01J27/20
CPC分类号： C10L3/08 , C10J3/00 , C10J3/482 , C10J2300/0903 , C10J2300/0906 , C10J2300/0973 , C10J2300/0986 , C10J2300/1662 , C10J2300/1807 , C10J2300/1853 , Y02P20/52
摘要： Processes are provided for capturing and recycling carbonaceous fines generated during a gasification process. In particular, the recycled fines are processed into a particulate composition which is useable as a carbonaceous feedstock and is conversion into a gas stream comprising methane.
摘要翻译：提供了用于捕获和回收在气化过程中产生的碳质细粉的方法。特别地，回收的细粉被加工成可用作碳质原料并转化成包含甲烷的气流的颗粒组合物。

18. 发明申请

US20090170968A1 Processes for Making Synthesis Gas and Syngas-Derived Products 审中-公开
标题翻译：制备合成气和合成气产品的工艺
公开(公告)号：US20090170968A1
公开(公告)日：2009-07-02
申请号：US12342596
申请日：2008-12-23
申请人： Nicholas Charles Nahas , Earl T. Robinson
发明人： Nicholas Charles Nahas , Earl T. Robinson
IPC分类号： C07C1/04 , C01B3/34 , F01K13/00
CPC分类号： C10J3/00 , C10J3/463 , C10J2300/093 , C10J2300/0943 , C10J2300/0973 , C10J2300/0986 , C10J2300/16 , C10J2300/1618 , C10J2300/1671 , C10J2300/1675 , C10J2300/1687 , C10J2300/1823 , C10J2300/1853 , C10J2300/1884 , C10K1/003 , C10K3/006 , C10K3/02 , C10L3/08 , C10L3/102
摘要： The present invention provides processes for making synthesis gas and processes for making syngas-derived products. For example, one aspect of the present invention provides a process for making a synthesis gas stream comprising hydrogen and carbon monoxide, the process comprising (a) providing a carbonaceous feedstock; (b) reacting the carbonaceous feedstock in a gasification reactor in the presence of steam and a gasification catalyst under suitable temperature and pressure to form a raw product gas stream comprising a plurality of gases comprising methane, hydrogen and carbon monoxide; (c) removing steam from and sweetening the raw product gas stream to form a sweetened gas stream; (d) separating and adding steam to the sweetened gas stream to form a first reformer input gas stream having a first steam/methane ratio; and a second reformer input stream having a second steam/methane ratio, in which the first steam/methane ratio is smaller than the second steam/methane ratio; (e) reforming the second reformer input stream to form a recycle gas stream comprising steam, carbon monoxide and hydrogen; (f) introducing the recycle gas stream to the gasification reactor; and (g) reforming the first reformer input stream to form the synthesis gas stream.
摘要翻译：本发明提供了制备合成气的方法和制备合成气衍生产物的方法。例如，本发明的一个方面提供了一种制备包含氢气和一氧化碳的合成气流的方法，该方法包括（a）提供碳质原料; （b）在合适的温度和压力下，在蒸汽和气化催化剂的存在下在气化反应器中使碳质原料反应，形成包含甲烷，氢气和一氧化碳的多种气体的原始产物气流; （c）从原料气流中除去蒸汽并使其变质，形成增甜的气流; （d）将蒸汽分离并加入到所述增甜气流中以形成具有第一蒸汽/甲烷比的第一重整器输入气流; 以及第二蒸汽/甲烷比小于第二蒸汽/甲烷比的第二蒸汽/甲烷比的第二重整器输入流; （e）重整所述第二重整器输入流以形成包含蒸汽，一氧化碳和氢气的循环气流; （f）将再循环气流引入气化反应器; 和（g）重整第一重整器输入流以形成合成气流。

19. 发明申请

US20090165376A1 Steam Generating Slurry Gasifier for the Catalytic Gasification of a Carbonaceous Feedstock 审中-公开
标题翻译：用于碳质原料催化气化的蒸汽发生浆料气化器
公开(公告)号：US20090165376A1
公开(公告)日：2009-07-02
申请号：US12343149
申请日：2008-12-23
申请人： Francis S. Lau , Earl T. Robinson
发明人： Francis S. Lau , Earl T. Robinson
IPC分类号： C10J3/60
CPC分类号： C10J3/82 , C10J3/463 , C10J3/721 , C10J2300/0903 , C10J2300/093 , C10J2300/094 , C10J2300/0943 , C10J2300/0959 , C10J2300/0973 , C10J2300/0986 , C10J2300/1807 , C10J2300/1823 , C10J2300/1846 , C10J2300/1853 , C10J2300/1884 , C10K1/004 , C10K1/101 , C10K1/122 , C10K1/143 , C10K1/16 , C10K1/165 , C10K3/02 , C10L3/08 , C10L3/102
摘要： Steam generating gasification reactors for providing high-pressure and high-temperature steam for catalytic gasification of a carbonaceous feedstock can be based on oxygen blown gasification reactors adapted for processing a slurry feedstock comprising at least 40% water. The exhaust from the slurry gasifier comprises at least steam, carbon monoxide and hydrogen. The slurry composition and the oxygen to fuel ratio can be varied to control the ratio of carbonaceous gases in the generator exhaust. By directing substantially all of exhaust gases produced from the slurry gasification reactor through the catalytic gasifier and subsequent gas separation and sequestration processes, a greatly higher energy efficiency and decreased carbon footprint can be realized.
摘要翻译：用于提供用于碳质原料的催化气化的高压和高温蒸汽的蒸汽发生气化反应器可以基于适于处理包含至少40％水的浆料原料的吹氧气化反应器。来自浆料气化器的废气至少包括蒸汽，一氧化碳和氢气。可以改变浆料组成和氧气与燃料比以控制发电机排气中的碳质气体的比例。通过将从浆料气化反应器产生的废气基本上引导通过催化气化器和随后的气体分离和封存方法，可以实现极高的能量效率和减少的碳足迹。

20. 发明授权

US08653149B2 Conversion of liquid heavy hydrocarbon feedstocks to gaseous products 有权
标题翻译：将液体重质烃原料转化为气态产物
公开(公告)号：US08653149B2
公开(公告)日：2014-02-18
申请号：US13116647
申请日：2011-05-26
申请人： Earl T. Robinson , Pattabhi K. Raman , Wenyuan Wu
发明人： Earl T. Robinson , Pattabhi K. Raman , Wenyuan Wu
IPC分类号： C07C27/00
CPC分类号： C10G11/02 , C01B3/36 , C01B3/382 , C01B2203/0244 , C01B2203/0255 , C01B2203/0894 , C10G2/30 , C10G11/20 , C10G11/22 , C10G2300/807 , C10G2400/20 , C10J3/02 , C10J3/46 , C10J2300/0906 , C10J2300/0969 , C10J2300/0976 , C10J2300/0986 , C10J2300/0989 , C10J2300/1807 , C10L3/08 , C10L3/12 , Y02P30/40
摘要： The present invention relates to processes and apparatuses for generating light olefins, methane and other higher-value gaseous hydrocarbons from “liquid” heavy hydrocarbon feedstocks.
摘要翻译：本发明涉及从“液体”重质烃原料产生轻质烯烃，甲烷和其它较高价值的气态烃的方法和装置。

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