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11. 发明申请

US20090318740A1 METHOD OF CONVERTING FEEDSTOCKS FROM RENEWABLE SOURCES TO GOOD-QUALITY DIESEL FUEL BASES USING A ZEOLITE TYPE CATALYST 有权
标题翻译：使用沸石型催化剂将可再生来源的原料转化为优质柴油燃料的方法
公开(公告)号：US20090318740A1
公开(公告)日：2009-12-24
申请号：US12489885
申请日：2009-06-23
申请人： Emmanuelle GUILLON , Christophe Bouchy , Nathalie Dupassieux , Antoine Daudin , Thierry Chapus
发明人： Emmanuelle GUILLON , Christophe Bouchy , Nathalie Dupassieux , Antoine Daudin , Thierry Chapus
IPC分类号： C07C5/27
CPC分类号： C10G3/50 , B01J23/883 , B01J29/74 , B01J29/78 , B01J37/20 , B01J37/28 , C10G3/46 , C10G3/54 , C10G45/02 , C10G45/08 , C10G45/64 , C10G65/043 , C10G2300/1014 , C10G2300/1018 , C10G2300/4006 , C10G2300/4012 , C10G2300/4018 , Y02P30/20
摘要： The invention relates to a method of treating feedstocks from renewable sources in order to produce diesel fuel bases of excellent quality. The feedstocks used can be, for example, raw vegetable oils or such oils that have been previously subjected to a prerefining stage, animal fats, or mixtures of such feedstocks. The invention relates to a method allowing high diesel fuel base yields to be obtained from such feedstocks.
摘要翻译：本发明涉及一种从可再生能源处理原料以生产质量优良的柴油燃料基料的方法。所使用的原料可以是例如以前经受预精制阶段，动物脂肪或这些原料的混合物的生植物油或这种油。本发明涉及允许从这些原料获得高柴油燃料碱产率的方法。

12. 发明授权

US09447334B2 Process for converting feeds derived from renewable sources with pre-treatment of feeds by hot dephosphatation 有权
标题翻译：通过热脱磷预处理饲料来转化源自可再生能源的饲料的方法
公开(公告)号：US09447334B2
公开(公告)日：2016-09-20
申请号：US12968354
申请日：2010-12-15
申请人： Aurelie Dandeu , Vincent Coupard , Thierry Chapus
发明人： Aurelie Dandeu , Vincent Coupard , Thierry Chapus
IPC分类号： C10L1/00 , C10G3/00 , C11B3/00 , C11B3/04 , C11B3/12 , C11B3/10
CPC分类号： C10G3/48 , C10G3/46 , C10G3/50 , C10G3/54 , C10G2300/1014 , C10G2300/1018 , C10G2300/205 , C10G2300/4006 , C10G2300/4012 , C10G2300/4018 , C10G2400/04 , C11B3/001 , C11B3/04 , C11B3/10 , C11B3/12 , Y02E50/13 , Y02P30/20
摘要： The invention concerns a process for the pre-treatment of an unrefined vegetable or animal oil, consisting of passing said oil through a reactor comprising at least one fixed bed of at least one adsorbent comprising a porous refractory oxide which is free of catalytic metals, at a temperature in the range 130° C. to 320° C., at a pressure in the range 0.1 to 7 MPa and with a residence time for said oil on said fixed bed in the range 0.1 to 1 hour. The invention concerns a process for pre-treatment of a semi-refined vegetable or animal oil, integrated upstream of a hydrotreatment step for the production of green gas oil.
摘要翻译：本发明涉及一种用于预处理未精制植物油或动物油的方法，该方法包括使所述油通过包含至少一个至少一个吸附剂的固定床的反应器，所述至少一个吸附剂包含不含催化金属的多孔难熔氧化物，温度范围为130℃至320℃，压力为0.1至7MPa，所述固定床上油的停留时间为0.1至1小时。本发明涉及一种用于预处理半精制蔬菜或动物油的方法，该方法在用于生产绿瓦斯油的加氢处理步骤的上游整合。

13. 发明授权

US08674151B2 Two-step hydrotreatment of a feed derived from a renewable source using a first, metallic, catalyst and a second, sulphurized, catalyst 失效
标题翻译：使用第一种金属催化剂和第二种硫化催化剂对来自可再生能源的原料进行两步加氢处理
公开(公告)号：US08674151B2
公开(公告)日：2014-03-18
申请号：US12664136
申请日：2008-06-03
申请人： Quentin Debuisschert , Jean Cosyns , Thierry Chapus , Damien Hudebine
发明人： Quentin Debuisschert , Jean Cosyns , Thierry Chapus , Damien Hudebine
IPC分类号： C07C1/00 , C10G3/00 , C10G51/02 , C10G45/08
CPC分类号： C10G3/42 , C07C1/2078 , C10G3/46 , C10G3/47 , C10G3/48 , C10G3/50 , C10G45/08 , C10G51/02 , C10G2300/1014 , C10G2300/1018 , C10G2300/4018 , C11C3/123 , Y02P30/20
摘要： The invention describes a two-step process for hydrotreatment of a feed derived from a renewable source, comprising: a) a first step, termed a mild pre-hydrogenation step, operating in the presence of a first, metallic, catalyst comprising an active hydrodehydrogenating phase constituted by at least one metal from group VIII and/or at least one metal from group VIB and an amorphous mineral support; and b) a second step, termed the second treatment step, operating in the presence of a second, sulphurized, catalyst comprising an active hydrodehydrogenating phase constituted by at least one non-noble metal from group VIII and/or at least one metal from group VIB and an amorphous mineral support.
摘要翻译：本发明描述了用于加氢处理源自可再生源的进料的两步法，该方法包括：a）第一步骤，称为温和预氢化步骤，在第一金属催化剂存在下操作，其包含活性氢化氢由至少一种来自第VIII族的金属和/或至少一种来自VIB族的金属和无定形矿物载体构成; 和b）称为第二处理步骤的第二步骤，在第二种硫化催化剂存在下操作，该催化剂包含由至少一种来自第VIII族的非贵金属和/或至少一种来自基团的金属构成的活性氢化氢化相 VIB和无定形矿物支持。

14. 发明申请

US20110098494A1 METHOD OF HYDROTREATING FEEDS FROM RENEWABLE SOURCES WITH INDIRECT HEATING USING A CATALYST BASED ON NICKEL AND MOLYBDENUM HAVING A PARTICULAR ATOMIC RATIO 审中-公开
标题翻译：使用基于镍的催化剂和具有特定原子比的钼的间接加热从可再生来源进料的方法
公开(公告)号：US20110098494A1
公开(公告)日：2011-04-28
申请号：US12911983
申请日：2010-10-26
申请人： Wilfried WEISS , Laurent Bournay , Thierry Chapus , Antoine Daudin
发明人： Wilfried WEISS , Laurent Bournay , Thierry Chapus , Antoine Daudin
IPC分类号： C11B3/02
CPC分类号： C10G3/46 , C10G3/48 , C10G3/50 , C10G65/04 , C10G2300/1014 , C10G2300/1018 , C10G2300/4006 , C10G2300/4081 , Y02P30/20
摘要： The invention describes a method of treating feeds from renewable sources comprising a hydrotreatment stage comprising at least two catalytic zones in which the entry stream comprising said feed mixed with at least a part of a hydrotreated liquid effluent from stage b) is introduced into the first catalytic zone at a temperature comprised between 150 and 260° C., and the effluent from the first catalytic zone is then introduced, mixed with at least a part of a hydrotreated liquid effluent from stage b) and preheated, into the following catalytic zone or zones at a temperature comprised between 260 and 320° C., and a stage of separation of the effluent from the hydrotreatment stage permitting the separation of a gaseous effluent and a hydrotreated liquid effluent of which at least a part is recycled at the top of each catalytic zone, said method using, in at least the catalytic zone or zones following the first, a bulk or supported catalyst comprising an active phase constituted by at least one group VIB element and at least one group VIII element, said elements being in sulphide form and the atomic ratio of the group VIII metal to the group VIB metal being strictly greater than 0 and less than 0.095.
摘要翻译：本发明描述了一种处理来自可再生来源的饲料的方法，该方法包括加氢处理阶段，该加氢处理阶段包括至少两个催化区，其中将包含所述进料的进料与至少一部分来自步骤b）的加氢处理液体流出物混合进入第一催化剂区域，然后引入来自第一催化区域的流出物，与来自阶段b）的加氢处理的液体流出物的至少一部分混合并预热到以下催化区或区域在260至320℃之间的温度下，流出物与加氢处理阶段的分离阶段允许分离气态流出物和加氢处理的液体流出物，其中至少一部分在每个催化剂的顶部被再循环所述方法在至少在第一个催化区域之后使用本体或负载型催化剂，其包含由下式构成的活性相：至少一种VIB族元素和至少一种VIII族元素，所述元素为硫化物形式，并且VIII族金属与VIB族金属的原子比严格大于0且小于0.095。

15. 发明申请

US20080156694A1 PROCESS FOR THE CONVERSION OF FEEDSTOCKS RESULTING FROM RENEWABLE SOURCES FOR PRODUCING GAS OIL FUEL BASES WITH A LOW SULPHUR CONTENT AND WITH AN IMPROVED CETANE NUMBER 有权
标题翻译：用于生产具有低硫含量和改进的CETANE号码的燃气油的可再生能源转化的进料的方法
公开(公告)号：US20080156694A1
公开(公告)日：2008-07-03
申请号：US11963231
申请日：2007-12-21
申请人： Thierry Chapus , Karin Marchand
发明人： Thierry Chapus , Karin Marchand
IPC分类号： C10G69/00
CPC分类号： C10G65/12 , C10G3/46 , C10G3/48 , C10G3/50 , C10G3/54 , C10G45/02 , C10G45/08 , C10G2300/1003 , C10G2300/1014 , C10G2300/1018 , C10G2300/1074 , C10G2300/202 , C10G2300/207 , C10G2300/301 , C10G2300/4006 , C10G2300/4012 , C10G2300/4018 , C10G2400/04 , Y02P30/20
摘要： The invention relates to a process for the treatment of heavy petroleum feedstocks in order to produce a gas oil fraction having a sulphur content of less than 50 ppm and generally 10 ppm which comprises the following stages: a) mild hydrocracking in a catalyst fixed bed, b) separation of the hydrogen sulphide, of a distillate cut including a gas oil fraction and of a fraction which is heavier than the gas oil, c) hydrotreating, by contact with at least one catalyst, of at least a portion of the said distillate cut obtained in stage b) including the gas oil fraction, as a mixture with a feedstock resulting from a crude or refined renewable source, d) separation of a gas oil cut comprising less than 50 ppm of sulphur. Advantageously, the heavy fraction is sent for catalytic cracking. Preferably, the process is carried out with makeup hydrogen introduced in stage c) and very advantageously all the makeup hydrogen for the process is introduced in stage c).The invention also relates to a plant which can be used for implementing this process.
摘要翻译：本发明涉及一种处理重质石油原料的方法，以生产硫含量小于50ppm，通常为10ppm的瓦斯油馏分，其包括以下阶段：a）催化剂固定床中的轻度加氢裂化， b）分离硫化氢，馏分馏分，其包括粗柴油馏分和比粗柴油重的馏分，c）通过与至少一种催化剂接触加氢处理所述馏出物的至少一部分在包括粗油或精制可再生来源的原料的混合物中包含粗柴油馏分的步骤b）中得到的切割，d）分离包含小于50ppm硫的瓦斯油馏分。有利地，将重馏分送入催化裂化。优选地，通过在阶段c）中引入的补充氢来进行该方法，并且非常有利地，用于该方法的所有补充氢在阶段c）中引入。本发明还涉及可用于实施该方法的设备。

16. 发明申请

US20060289338A1 Process of mild hydrocracking including a dilution of the feedstock 有权
标题翻译：轻度加氢裂化的方法，包括原料稀释
公开(公告)号：US20060289338A1
公开(公告)日：2006-12-28
申请号：US11449867
申请日：2006-06-09
申请人： Christophe Gueret , Thierry Chapus , Damien Hudebine
发明人： Christophe Gueret , Thierry Chapus , Damien Hudebine
IPC分类号： C10G57/00 , B01J8/18
CPC分类号： C10G69/04 , C10G11/18 , C10G47/00
摘要： The invention relates to a process for FCC pretreatment by mild hydrocracking of a hydrocarbon feedstock that comprises a vacuum distillate fraction or a deasphalted oil or else a mixture of these two fractions, said primary feedstock, to produce gas oil and an effluent having an initial boiling point of more than 320° C., said effluent (FCC feedstock) then being subjected to a catalytic cracking, process in which at least 85% by weight of said primary feedstock ends above 375° C. and at least 95% by weight of said primary feedstock ends below 650° C., whereby the mild hydrocracking is performed under an absolute pressure of 2 to 12 MPa and at a temperature of between 300 and 500° C., characterized in that the hydrocarbon feedstock also comprises a lighter hydrocarbon fraction, a so-called secondary feedstock, of which at least 50% by weight ends below 375° C. and at least 80% ends above 200° C.
摘要翻译：本发明涉及通过烃原料的轻度加氢裂化来进行FCC预处理的方法，所述烃原料包括真空蒸馏馏分或脱沥青油，或者所述主要原料的这两个馏分的混合物，以产生瓦斯油和具有初始沸点的流出物所述流出物（FCC原料）然后进行催化裂化，其中至少85重量％的所述主要原料在375℃以上终止，并且至少95重量％所述主要原料终止于650℃以下，由此在2至12MPa的绝对压力和300至500℃的温度下进行轻度加氢裂化，其特征在于，烃原料还包含较轻的烃馏分，所谓的二次原料，其中至少50重量％终止于375℃以下且至少80％在200℃以上结束。

17. 发明授权

US06838060B1 Process and apparatus for the production of catalytic cracking gasoline with a low sulphur content 失效
标题翻译：用于生产硫含量低的催化裂化汽油的方法和装置
公开(公告)号：US06838060B1
公开(公告)日：2005-01-04
申请号：US09434282
申请日：1999-11-05
申请人： Thierry Chapus , Blaise Didillon , Christian Marcilly , Charles Cameron
发明人： Thierry Chapus , Blaise Didillon , Christian Marcilly , Charles Cameron
IPC分类号： B01J23/42 , B01J23/85 , B01J31/12 , C10G27/00 , C10G29/06 , C10G45/06 , C10G45/10 , C10G45/40 , C10G65/00 , C10G65/06 , C10G67/00 , C10G67/04 , C10G67/12 , B01J8/00 , C10G45/00
CPC分类号： C10G65/00 , C10G2400/02
摘要： An apparatus for the production of gasolines with a low sulphur content from a catalytic cracking gasoline, comprising a fractionation column (1) provided with a line (2) for introducing raw gasoline from a catalytic cracking step and comprising at least two lines, one (3) in the upper portion of the column for taking off a light cut, and the other (4) in the lower portion of the column for taking off the heavy cut; a zone (5) for hydrotreatment in the presence of hydrogen, comprising a catalytic bed, an inlet line (6) for the light gasoline cut to be treated, said line being connected either to the fractionation column (I), or to the zone (7) for treatment over a palladium catalyst, said hydrotreatment zone also comprising an outlet line (8) for hydrotreated effluent; a stripping zone (9) comprising a line for introducing light hydrotreated gasoline, a line (10) for evacuating H2S and an outlet line (11) for stripped light gasoline; and said apparatus also comprising at least one of the following sweetening zones: a sweetening zone (12) located after the stripping zone, comprising a line for introducing the stripped light gasoline and a line (14) for supplying an oxidizing agent to said zone; a treatment zone (7) located after the hydrotreatment zone and comprising a line (3) for introducing the light gasoline cut from the fractionation column, an outlet line for the treated light gasoline cut, said zone also comprising at least one catalyst bed containing 0.1-1% of palladium deposited on a support, and said apparatus further comprising a line (13) for taking the stripped and sweetened light gasoline out of the apparatus, and connected either to the zone (12) or to the zone (9).

18. 发明授权

US06187173B1 Process for purification of raw gasoline from catalytic cracking 失效
标题翻译：原料汽油从催化裂化中提纯的工艺
公开(公告)号：US06187173B1
公开(公告)日：2001-02-13
申请号：US08935896
申请日：1997-09-23
申请人： Thierry Chapus , Blaise Didillon , Christian Marcilly , Charles Cameron
发明人： Thierry Chapus , Blaise Didillon , Christian Marcilly , Charles Cameron
IPC分类号： C10G6700
CPC分类号： C10G67/12 , C10G2400/02
摘要： A process and apparatus for treating raw gasoline from catalytic cracking to obtain gasoline with the qualities required for use as motor fuel comprises selective hydrogenation followed by stabilization and optional cooling of the effluent, then sweetening followed by degassing to obtain a dedienized, stabilized and sweetened gasoline. The hydrogenation catalyst preferably comprises 0.1-1% of palladium deposited on a support, sweetening is preferably carried out on a solid catalyst containing an aluminosilicate of an alkali metal (for example sodalite), a metal chelate and activated charcoal. The product from this process can be placed directly in the gasoline pool or, advantageously, fractionated to obtain one or more cuts which can be used as feeds for etherification.
摘要翻译：用催化裂化处理原汽油以获得汽油作为汽油使用所需要的质量的方法和装置包括选择性氢化，然后进行稳定化和任选的冷却流出物，然后进行脱气，然后进行脱气以获得脱气，稳定和增甜的汽油。氢化催化剂优选包含沉积在载体上的0.1-1％的钯，优选在含有碱金属（例如钠盐）的铝硅酸盐，金属螯合物和活性炭的固体催化剂上进行。来自该方法的产物可以直接放置在汽油池中，或者有利地分馏以获得一个或多个可用作醚化进料的切口。

19. 发明授权

US6117306A Catalytic process for conversion of a petroleum residue using a fixed bed hydrodemetallization catalyst 失效
标题翻译：使用固定床加氢脱金属催化剂转化石油残渣的催化方法
公开(公告)号：US6117306A
公开(公告)日：2000-09-12
申请号：US942051
申请日：1997-10-01
申请人： Frederic Morel , Jean-Luc Duplan , Thierry Chapus , Alain Billon , Stephane Kressmann , Gerard Heinrich
发明人： Frederic Morel , Jean-Luc Duplan , Thierry Chapus , Alain Billon , Stephane Kressmann , Gerard Heinrich
IPC分类号： C10G69/04 , C10G45/00
CPC分类号： C10G69/04 , Y10S208/95
摘要： A process for converting a heavy hydrocarbon fraction comprises treating the hydrocarbon feed in a hydrodemetallization section, the section containing at least one fixed bed hydrodemetallization catalyst. At least a portion of the hydrotreated liquid effluent from step a) is sent to an atmospheric distillation zone from which a distillate and an atmospheric residue are recovered; at least a portion of the atmospheric residue is sent to a vacuum distillation zone from which a vacuum distillate and a vacuum residue are recovered; at least a portion of the vacuum residue is sent to a deasphalting section from which a deasphalted hydrocarbon cut and residual asphalt are recovered; at least a portion of the deasphalted hydrocarbon cut is sent to a hydrotreatment section from which a gas fraction, a fuel fraction and a heavier liquid fraction of the hydrotreated feed are recovered, and at least a portion of the heavier liquid fraction of the hydrotreated feed is sent to a catalytic cracking section in which it is treated under conditions such that a gaseous fraction, a gasoline fraction, a gas oil fraction and a slurry fraction are produced.
摘要翻译：用于转化重质烃馏分的方法包括在加氢脱金属部分中处理烃进料，所述部分含有至少一个固定床加氢脱金属催化剂。将来自步骤a）的加氢处理的液体流出物的至少一部分送至常压蒸馏区，回收馏出物和大气残留物; 将至少一部分大气残留物送至减压蒸馏区，从真空蒸馏区回收真空馏分和真空残渣; 将至少一部分真空残渣送至脱沥青部分，从其中回收脱沥青烃馏分和残余沥青; 将脱沥青烃馏分的至少一部分送到加氢处理部分，加氢处理的进料的气体馏分，燃料馏分和较重液体馏分从该加氢处理部分回收，加氢处理的进料的至少一部分较重液体馏分被送到催化裂化部分，其中在气态馏分，汽油馏分，粗柴油馏分和淤浆馏分产生的条件下进行处理。

20. 发明授权

US09109168B2 Production of paraffinic fuels from renewable materials using a continuous hydrotreatment process 有权
标题翻译：使用连续加氢处理工艺从可再生材料生产石蜡燃料
公开(公告)号：US09109168B2
公开(公告)日：2015-08-18
申请号：US13332442
申请日：2011-12-21
申请人： Nathalie Dupassieux , Thierry Chapus
发明人： Nathalie Dupassieux , Thierry Chapus
IPC分类号： C07C1/00 , C10G3/00 , C10G45/60 , C10G65/04 , C10L1/04 , C10L1/08 , C10L1/06
CPC分类号： C10G3/54 , C10G3/42 , C10G3/44 , C10G3/45 , C10G3/46 , C10G3/50 , C10G3/52 , C10G3/60 , C10G45/60 , C10G65/043 , C10G2300/1011 , C10G2300/1014 , C10G2300/1018 , C10G2300/1048 , C10G2300/4018 , C10G2300/4081 , C10G2400/02 , C10G2400/04 , C10L1/04 , C10L1/06 , C10L1/08 , Y02E50/13 , Y02E50/32 , Y02P30/20 , Y02T50/678
摘要： A process for hydrotreating a feed originating from renewable sources such as vegetable oils to produce paraffinic hydrocarbons in the presence of hydrogen in excess over the theoretical hydrogen consumption and under hydrotreatment conditions in a fixed bed reactor having a plurality of catalytic zones disposed in series and comprising a hydrotreatment catalyst. The total feed flow is divided into a certain number of different part flows equal to the number of catalytic zones in the reactor; the various part flows are injected into the successive catalytic zones in increasing proportions to produce an effluent comprising paraffinic hydrocarbons. The effluent undergoes a separation step in order to separate a gas fraction and a liquid fraction containing the paraffinic hydrocarbons. At least a portion of said this liquid fraction is recycled to the first catalytic zone so that the weight ratio between said recycle and the part flow introduced into the first catalytic zone is 10 or more.
摘要翻译：在诸如植物油的可再生来源的加氢处理方法中，在具有超过理论氢消耗的氢气存在下，在加氢处理条件下，在具有多个串联设置的催化剂区域的固定床反应器中产生链烷烃，并且包含加氢处理催化剂。总进料流分为等于反应器中催化剂区数的一定数量的不同部分流动; 各种部分流量以增加的比例注入连续的催化区域中以产生包含链烷烃的流出物。流出物经历分离步骤以分离气体馏分和含有链烷烃的液体馏分。将所述液体馏分的至少一部分再循环到第一催化区域，使得引入第一催化区域的所述再循环物和部件流之间的重量比为10以上。

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