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121. 发明授权

US09163041B2 Metal utilization in supported, metal-containing catalysts 有权
标题翻译：负载金属催化剂中的金属利用
公开(公告)号：US09163041B2
公开(公告)日：2015-10-20
申请号：US13557700
申请日：2012-07-25
申请人： Kam-To Wan
发明人： Kam-To Wan
IPC分类号： B01J23/75 , B01J23/745 , B01J21/18 , C07F9/38 , B01J23/70 , B01J23/42 , B01J23/74
CPC分类号： C07F9/3813 , B01J21/18 , B01J23/42 , B01J23/626 , B01J23/70 , B01J23/74 , B01J23/745 , B01J23/75 , B01J23/8906 , B01J23/8913 , B01J23/8926
摘要： Generally, the present invention relates to improvements in metal utilization in supported, metal-containing catalysts. For example, the present invention relates to methods for directing and/or controlling metal deposition onto surfaces of porous substrates. The present invention also relates to methods for preparing catalysts in which a first metal is deposited onto a support (e.g., a porous carbon support) to provide one or more regions of a first metal at the surface of the support, and a second metal is deposited at the surface of the one or more regions of the first metal. The invention further relates to use of catalysts prepared as detailed herein in catalytic oxidation reactions, such as oxidation of a substrate selected from the group consisting of N-(phosphonomethyl)iminodiacetic acid or a salt thereof, formaldehyde, and/or formic acid.
摘要翻译：通常，本发明涉及负载的含金属催化剂中金属利用的改进。例如，本发明涉及用于引导和/或控制金属沉积到多孔基底表面上的方法。本发明还涉及制备催化剂的方法，其中第一金属沉积在载体（例如，多孔碳载体）上以在载体的表面提供一个或多个第一金属的区域，第二金属是沉积在第一金属的一个或多个区域的表面上。本发明还涉及在催化氧化反应中如本文详述制备的催化剂的用途，例如氧化选自N-（膦酰基甲基）亚氨基二乙酸或其盐，甲醛和/或甲酸的底物。

122. 发明授权

US09150968B2 Platinum-based electrocatalysts synthesized by depositing contiguous adlayers on carbon nanostructures 有权
标题翻译：通过在碳纳米结构上沉积连续的层，合成铂基电催化剂
公开(公告)号：US09150968B2
公开(公告)日：2015-10-06
申请号：US13775674
申请日：2013-02-25
申请人： Brookhaven Science Associates, LLC
发明人： Radoslav R. Adzic , Alexander Harris
IPC分类号： B05D3/00 , C08J7/04 , H05H1/32 , C23C28/02 , B82Y30/00 , B82Y40/00 , C01B31/02 , H01G11/36 , H01M4/92 , C23C28/00 , H01G11/24 , B01J37/34 , B01J35/00 , B01J21/18 , B01J23/42 , B01J23/44 , B01J23/60 , B01J23/89 , B01J23/56
CPC分类号： H01G11/36 , B01J21/185 , B01J23/42 , B01J23/44 , B01J23/56 , B01J23/60 , B01J23/892 , B01J23/8926 , B01J35/0006 , B01J35/0033 , B01J35/008 , B01J37/348 , B82Y30/00 , B82Y40/00 , C01B32/18 , C23C28/321 , C23C28/322 , C23C28/34 , C23C28/345 , C23C28/347 , C23C28/42 , H01G11/04 , H01G11/24 , H01G11/28 , H01G11/58 , H01M4/92 , H01M4/926 , Y02E60/13
摘要： High-surface-area carbon nanostructures coated with a smooth and conformal submonolayer-to-multilayer thin metal films and their method of manufacture are described. The manufacturing process may involve initial oxidation of the carbon nanostructures followed by immersion in a solution with the desired pH to create negative surface dipoles. The nanostructures are subsequently immersed in an alkaline solution containing non-noble metal ions which adsorb at surface reaction sites. The metal ions are then reduced via chemical or electrical means and the nanostructures are exposed to a solution containing a salt of one or more noble metals which replace adsorbed non-noble surface metal atoms by galvanic displacement. Subsequent film growth may be performed via the initial quasi-underpotential deposition of a non-noble metal followed by immersion in a solution comprising a more noble metal. The resulting coated nanostructures may be used, for example, as high-performance electrodes in supercapacitors, batteries, or other electric storage devices.
摘要翻译：描述了涂覆有平滑且适形的亚单层至多层薄金属薄膜的高表面积碳纳米结构及其制造方法。制造方法可以包括碳纳米结构的初始氧化，然后浸入具有所需pH的溶液中以产生负表面偶极子。随后将纳米结构浸入含有非表面反应位点吸附的非贵金属离子的碱性溶液中。然后通过化学或电气方式还原金属离子，并且将纳米结构暴露于含有一种或多种贵金属盐的溶液，其通过电位移代替了吸附的非贵重表面金属原子。随后的膜生长可以通过非贵金属的初始准低电位沉积进行，然后浸入包含更贵贵金属的溶液中。所得到的涂覆的纳米结构可以用作例如超级电容器，电池或其它蓄电装置中的高性能电极。

123. 发明授权

US09138732B2 Copper CHA zeolite catalysts 有权
公开(公告)号：US09138732B2
公开(公告)日：2015-09-22
申请号：US14598854
申请日：2015-01-16
申请人： BASF Corporation
发明人： Ivor Bull , Wen-Mei Xue , Patrick Burk , R. Samuel Boorse , William M. Jaglowski , Gerald Stephen Koermer , Ahmad Moini , Joseph A. Patchett , Joseph C. Dettling , Matthew Tyler Caudle
IPC分类号： B01D53/56 , B01J29/80 , B01D53/94 , B01J23/42 , B01J23/89 , B01J29/072 , B01J29/72 , B01J29/76 , B01J35/00 , B01J35/04 , B01J37/02 , B01J29/74 , B01D53/86 , B01J29/06 , C01B39/46
CPC分类号： B01J29/723 , B01D53/56 , B01D53/8628 , B01D53/9413 , B01D53/9418 , B01D53/9431 , B01D53/9477 , B01D2251/206 , B01D2251/2062 , B01D2251/2067 , B01D2255/20715 , B01D2255/20738 , B01D2255/20761 , B01D2255/50 , B01D2255/9032 , B01D2255/904 , B01D2255/9155 , B01D2257/40 , B01D2257/404 , B01D2258/012 , B01J23/42 , B01J23/8926 , B01J29/061 , B01J29/068 , B01J29/072 , B01J29/743 , B01J29/76 , B01J29/763 , B01J29/80 , B01J35/0006 , B01J35/04 , B01J37/0246 , B01J2029/062 , C01B39/46 , Y02T10/24 , Y10T428/24149
摘要： Zeolite catalysts and systems and methods for preparing and using zeolite catalysts having the CHA crystal structure are disclosed. The catalysts can be used to remove nitrogen oxides from a gaseous medium across a broad temperature range and exhibit hydrothermal stable at high reaction temperatures. The zeolite catalysts include a zeolite carrier having a silica to alumina ratio from about 15:1 to about 256:1 and a copper to alumina ratio from about 0.25:1 to about 1:1.

124. 发明授权

US09126189B2 Method of making pyrochlores 有权
标题翻译：制作烧绿石的方法
公开(公告)号：US09126189B2
公开(公告)日：2015-09-08
申请号：US14311925
申请日：2014-06-23
申请人： SABIC Global Technologies B.V.
发明人： Lawrence D'Souza , Vinu Viswanath
IPC分类号： B01J23/63 , B01J23/83 , C01B3/40 , B01J21/16 , B01J23/10 , B01J37/08 , B01J23/42 , B01J23/46 , B01J23/755 , B01J37/02 , C01G25/00 , C01G51/00 , C01G53/00 , C01G55/00 , C01B3/32
CPC分类号： B01J23/83 , B01J21/16 , B01J23/002 , B01J23/10 , B01J23/42 , B01J23/462 , B01J23/464 , B01J23/63 , B01J23/755 , B01J35/002 , B01J35/1009 , B01J35/1014 , B01J37/0201 , B01J37/0236 , B01J37/035 , B01J37/08 , B01J2523/00 , C01B3/326 , C01B3/40 , C01B2203/0238 , C01B2203/0405 , C01B2203/1052 , C01B2203/1058 , C01B2203/1064 , C01B2203/107 , C01B2203/1082 , C01B2203/1088 , C01G25/00 , C01G51/70 , C01G53/70 , C01G55/002 , C01P2002/36 , C01P2002/72 , C01P2004/04 , C01P2006/12 , Y02P20/52 , B01J2523/3706 , B01J2523/48 , B01J2523/822 , B01J2523/821 , B01J2523/827 , B01J2523/847 , B01J2523/845 , B01J2523/828 , B01J2523/824
摘要： Disclosed is a method of making a pyrochlore comprising, obtaining a solution comprising a solvent and a metal precursor or salt thereof capable of forming a pyrochlore, wherein the metal precursor or salt thereof is dissolved in the solvent, subjecting the solution to a drying step to obtain a non-gelled or non-polymerized pyrochlore precursor material in powdered form, and subjecting the pyrochlore precursor material to a calcination step to obtain a pyrochlore.
摘要翻译：公开了制备烧绿石的方法，其包括：获得包含能够形成烧绿石的溶剂和金属前体或其盐的溶液，其中金属前体或其盐溶解在溶剂中，使溶液进行干燥步骤获得粉末形式的非胶凝或未聚合的烧绿石前体材料，并对烧绿石前体材料进行煅烧步骤以获得烧绿石。

125. 发明申请

US20150225869A1 Underpotential Deposition-Mediated Layer-by-Layer Growth of Thin Films 有权
标题翻译：低电位沉积介导的薄膜逐层生长
公开(公告)号：US20150225869A1
公开(公告)日：2015-08-13
申请号：US14689708
申请日：2015-04-17
申请人： Brookhaven Science Associates, LLC
发明人： Jia Xu Wang , Radoslav R. Adzic
IPC分类号： C25D21/12 , C25D3/50
CPC分类号： C25D21/12 , B01J21/18 , B01J23/42 , B01J23/44 , B01J37/0215 , B01J37/0228 , B01J37/341 , C25D3/50 , C25D5/18 , C25D5/34 , C25D7/006 , H01M4/8657 , H01M4/8853 , H01M4/921 , H01M4/926 , Y02E60/50
摘要： A method of depositing contiguous, conformal submonolayer-to-multilayer thin films with atomic-level control is described. The process involves electrochemically exchanging a mediating element on a substrate with a noble metal film by alternatingly sweeping potential in forward and reverse directions for a predetermined number of times in an electrochemical cell. By cycling the applied voltage between the bulk deposition potential for the mediating element and the material to be deposited, repeated desorption/adsorption of the mediating element during each potential cycle can be used to precisely control film growth on a layer-by-layer basis.
摘要翻译：描述了一种沉积具有原子级控制的连续的共形亚单层到多层薄膜的方法。该方法包括通过在电化学电池中交替地将正向和反向的电位扫描预定次数，在衬底上用介电元件电化学交换介质元件与贵金属膜。通过在介质元件的体积沉积电位和待沉积的材料之间循环施加的电压，可以使用在每个电位循环期间重复解吸/吸附中间元件以逐层地精确地控制膜生长。

126. 发明授权

US09101879B2 Catalysts 有权
标题翻译：催化剂
公开(公告)号：US09101879B2
公开(公告)日：2015-08-11
申请号：US13139132
申请日：2009-12-10
申请人： Martyn Vincent Twigg
发明人： Martyn Vincent Twigg
IPC分类号： B01J21/06 , B01J21/08 , B01J23/34 , B01J23/50 , B01D53/02 , B01D53/14 , B01D53/66 , B01D53/86 , B01J23/68 , B01J23/96 , B01J35/02 , B01J35/04 , B01J37/02 , A61L2/20 , B01J23/42
CPC分类号： B01D53/8675 , A61L2/202 , A61L2202/13 , B01D2255/104 , B01D2255/20707 , B01D2255/2073 , B01D2255/30 , B01J21/063 , B01J21/08 , B01J23/34 , B01J23/42 , B01J23/50 , B01J23/688 , B01J23/96 , B01J35/023 , B01J35/04 , B01J37/0215
摘要： A sterilant such as ozone used for large scale decontamination of, for example, a hospital room, may be destroyed and the room made safe, by passing the atmosphere in the room over a catalyst which is silver oxide in combination with titania. The catalyst may be readily regenerated and used again.
摘要翻译：例如医院房间用于大规模去污的臭氧等消毒剂可能被破坏，并且通过将氧化银与二氧化钛组合的催化剂通过房间中的气氛而使房间安全。催化剂可以容易地再生并再次使用。

127. 发明申请

US20150209761A1 Vertically Aligned Arrays of Carbon Nanotubes Formed on Multilayer Substrates 有权
标题翻译：在多层基板上形成的碳纳米管的垂直对准阵列
公开(公告)号：US20150209761A1
公开(公告)日：2015-07-30
申请号：US14414227
申请日：2013-07-10
申请人： Carbice Nanotechnologies, Inc.
发明人： Baratunde A. Cola
IPC分类号： B01J23/745 , B01J21/02 , C01B31/02 , B01J35/00 , B01J35/02 , B01J23/72 , C09K5/14
CPC分类号： B01J23/745 , B01J21/02 , B01J23/42 , B01J23/44 , B01J23/464 , B01J23/466 , B01J23/468 , B01J23/72 , B01J23/75 , B01J23/755 , B01J35/0006 , B01J35/02 , B82Y30/00 , B82Y40/00 , C01B32/162 , C01B2202/08 , C09K5/14 , Y10S977/742 , Y10S977/81 , Y10T428/12431 , Y10T428/12493 , Y10T428/12576 , Y10T428/12611 , Y10T428/24975 , Y10T428/25 , Y10T428/265 , Y10T428/30
摘要： Multilayer substrates for the growth and/or support of CNT arrays are provided. These multilayer substrates both promote the growth of dense vertically aligned CNT arrays and provide excellent adhesion between the CNTs and metal surfaces. Carbon nanotube arrays formed using multilayer substrates, which exhibit high thermal conductivity and excellent durability, are also provided. These arrays can be used as thermal interface materials.
摘要翻译：提供了用于CNT阵列生长和/或支持的多层基底。这些多层基板都促进了紧密垂直排列的CNT阵列的生长，并且在CNT和金属表面之间提供优异的粘合性。还提供了使用多层基板形成的具有高导热性和优异耐久性的碳纳米管阵列。这些阵列可以用作热界面材料。

128. 发明授权

US09090475B1 In situ oxide removal, dispersal and drying for silicon SiO2 有权
标题翻译：硅SiO 2的原位氧化物去除，分散和干燥
公开(公告)号：US09090475B1
公开(公告)日：2015-07-28
申请号：US12961108
申请日：2010-12-06
申请人： Stephen Edward Lehman, Jr.
发明人： Stephen Edward Lehman, Jr.
IPC分类号： C01B33/027 , C23C18/14
CPC分类号： H05K1/0306 , B01J23/42 , B01J23/8926 , B01J37/00 , B22F2001/0092 , B28B3/025 , B28B23/0081 , B28B23/0087 , B32B5/30 , B32B7/12 , B32B37/14 , B32B2037/1253 , B32B2262/0253 , B32B2264/104 , B32B2264/107 , B32B2307/558 , B32B2571/02 , B82Y30/00 , B82Y40/00 , C01B33/027 , C23C4/134 , C23C18/14 , F41H1/02 , F41H5/0471 , F41H5/0492 , H01B1/02 , H01L21/6835 , H01L23/64 , H01L2924/0002 , H05K1/16 , Y02E60/122 , Y02P70/54 , Y10T428/12576 , Y10T428/24983 , Y10T428/25 , Y10T428/252 , Y10T428/26 , Y10T428/28 , Y10T428/2916 , H01L2924/00
摘要： A method of removing silicon-dioxide from silicon powder. The method comprises: providing a silicon powder defined by each particle having a silicon core and a silicon dioxide layer surrounding the silicon core; dispersing the particles in a dispersing solution; adding an etching solution, wherein the etching solution removes the silicon dioxide layer; adding an organic solvent, thereby producing an organic phase and an aqueous phase, the organic phase comprising the silicon cores and the organic solvent, and the aqueous phase comprising the dispersing solution, the etching solution, and the etching by-products; coating each silicon core with an organic material; draining out the aqueous phase; washing the organic phase, wherein the remaining material from the aqueous phase is removed; and providing the silicon powder as a plurality of silicon cores each absent a silicon dioxide layer and having an organic coating.
摘要翻译：从硅粉中除去二氧化硅的方法。该方法包括：提供由具有硅芯的每个颗粒限定的硅粉末和围绕硅芯的二氧化硅层; 将颗粒分散在分散溶液中; 添加蚀刻溶液，其中所述蚀刻溶液除去二氧化硅层; 加入有机溶剂，从而制备有机相和水相，包含硅芯和有机溶剂的有机相和包含分散溶液，蚀刻溶液和蚀刻副产物的水相; 用有机材料涂覆每个硅芯; 排出水相; 洗涤有机相，其中除去来自水相的剩余物质; 并且将硅粉末提供为多个硅芯，每个硅芯都不含二氧化硅层并具有有机涂层。

129. 发明申请

US20150202572A1 DIESEL OXIDATION CATALYST AND EXHAUST SYSTEM 有权
标题翻译：柴油氧化催化剂和排气系统
公开(公告)号：US20150202572A1
公开(公告)日：2015-07-23
申请号：US14603523
申请日：2015-01-23
申请人： Johnson Matthey Public Limited Company
发明人： Andrew Francis CHIFFEY , John Benjamin GOODWIN , James LEELAND , Francois MOREAU
IPC分类号： B01D53/94 , B01J21/12 , B01J23/656
CPC分类号： B01D53/944 , B01D53/56 , B01D53/62 , B01D53/72 , B01D53/922 , B01D53/945 , B01D53/9454 , B01D53/9459 , B01D53/9468 , B01D53/9472 , B01D53/9477 , B01D2201/62 , B01D2255/1021 , B01D2255/1023 , B01D2255/2042 , B01D2255/2065 , B01D2255/20707 , B01D2255/20715 , B01D2255/2073 , B01D2255/20776 , B01D2255/2092 , B01D2255/30 , B01D2255/40 , B01D2255/50 , B01D2255/502 , B01D2255/504 , B01D2255/902 , B01D2255/9022 , B01D2255/903 , B01D2255/9032 , B01D2255/91 , B01D2255/912 , B01D2257/404 , B01D2257/502 , B01D2257/702 , B01J21/12 , B01J23/02 , B01J23/10 , B01J23/34 , B01J23/38 , B01J23/42 , B01J23/44 , B01J23/58 , B01J23/63 , B01J23/6562 , B01J23/66 , B01J29/40 , B01J29/7007 , B01J29/7015 , B01J29/7415 , B01J29/743 , B01J35/0006 , B01J35/023 , B01J35/04 , B01J37/0036 , B01J37/0219 , B01J37/0228 , B01J37/0234 , B01J37/0236 , B01J37/0244 , B01J37/0246 , B01J37/086 , B01J37/10 , F01N3/035 , F01N3/103 , F01N3/106 , F01N3/281 , F01N3/2828 , F01N3/2882 , F01N2330/02 , F01N2330/06 , F01N2370/02 , F01N2510/06 , F01N2510/0682 , F01N2510/0684 , F01N2570/10 , F01N2570/12 , F01N2570/14 , Y02A50/2325 , Y02A50/2341
摘要： An oxidation catalyst for treating an exhaust gas from a diesel engine and an exhaust system comprising the oxidation catalyst are described. The oxidation catalyst comprises: a first washcoat region for oxidising carbon monoxide (CO) and hydrocarbons (HCs), wherein the first washcoat region comprises a first platinum group metal (PGM) and a first support material; a second washcoat region for oxidising nitric oxide (NO), wherein the second washcoat region comprises platinum (Pt), manganese (Mn) and a second support material; and a substrate having an inlet end and an outlet end; wherein the second washcoat region is arranged to contact the exhaust gas at the outlet end of the substrate and after contact of the exhaust gas with the first washcoat region.
摘要翻译：描述了用于处理来自柴油发动机的废气的氧化催化剂和包含氧化催化剂的排气系统。氧化催化剂包括：用于氧化一氧化碳（CO）和烃（HC））的第一修补基面涂层区域，其中第一修补基面涂层区域包含第一铂族金属（PGM）和第一载体材料; 用于氧化一氧化氮（NO）的第二修补基面涂层区域，其中所述第二修补基面涂层区域包含铂（Pt），锰（Mn）和第二载体材料; 以及具有入口端和出口端的基底; 其中所述第二修补基面涂层区域布置成在所述基板的出口端处和所述废气与所述第一修补基面涂层区域接触之后接触所述废气。

130. 发明申请

US20150197465A1 Bimetallic Catalyst and Use in Xylene Production 有权
标题翻译：双金属催化剂和二甲苯生产中的应用
公开(公告)号：US20150197465A1
公开(公告)日：2015-07-16
申请号：US14669179
申请日：2015-03-26
申请人： ExxonMobil Chemical Patents Inc.
发明人： April D. Ross , Jane C. Cheng
IPC分类号： C07C5/27 , B01J29/44 , B01J37/08 , C07C7/148
CPC分类号： C07C5/2708 , B01J16/005 , B01J23/42 , B01J23/50 , B01J23/60 , B01J23/62 , B01J23/626 , B01J23/628 , B01J23/8926 , B01J29/405 , B01J29/44 , B01J29/46 , B01J37/0018 , B01J2229/186 , B01J2229/36 , B01J2229/42 , C07C5/222 , C07C5/2556 , C07C5/2737 , C07C5/2754 , C07C15/08 , C07C2529/44 , Y02P20/52
摘要： The invention is directed to a bimetallic catalyst system adapted for the manufacture of xylenes, a process for making said catalyst system, and to the process of manufacture of xylenes using said catalyst system, providing, in embodiments, improved selectivity by at least one of higher ethylene saturation and low xylene loss, decreased susceptibility to poisoning from feedstream impurities, and ability to operate at less severe conditions.
摘要翻译：本发明涉及适用于制造二甲苯的双金属催化剂体系，制备所述催化剂体系的方法，以及使用所述催化剂体系制备二甲苯的方法，在实施方案中，提供了至少一种较高的选择性乙烯饱和度低，二甲苯损失低，对原料杂质中毒的易感性降低，在恶劣条件下操作能力差。

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