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1. 发明授权

US07387981B1 Direct epoxidation catalyst and process 失效
标题翻译：直接环氧化催化剂和工艺
公开(公告)号：US07387981B1
公开(公告)日：2008-06-17
申请号：US11823651
申请日：2007-06-28
申请人： Mark P. Kaminsky , Roger A. Grey , Jay F. Miller
发明人： Mark P. Kaminsky , Roger A. Grey , Jay F. Miller
IPC分类号： B01J23/44
CPC分类号： B01J29/89 , B01J21/063 , B01J23/38 , B01J23/44 , B01J23/52 , B01J23/66 , B01J35/0006 , B01J35/023 , B01J35/1019 , B01J37/0009 , B01J2229/20 , C07D301/10
摘要： A catalyst comprising a transition metal zeolite and a supported noble metal is disclosed. The mean mass diameter of the catalyst is greater than 0.5 mm. The catalyst is formed from transition metal zeolite particles and the supported noble metal particles each having a mean mass diameter of less than 0.1 mm. An epoxidation process by reacting an olefin, hydrogen, and oxygen in the presence of the catalyst is disclosed.
摘要翻译：公开了一种包含过渡金属沸石和负载的贵金属的催化剂。催化剂的平均质量直径大于0.5mm。催化剂由平均质量直径小于0.1mm的过渡金属沸石颗粒和负载的贵金属颗粒形成。公开了在催化剂存在下使烯烃，氢气和氧气反应的环氧化方法。

2. 发明授权

US07671222B2 Direct epoxidation process using a mixed catalyst system 失效
标题翻译：直接环氧化工艺采用混合催化剂体系
公开(公告)号：US07671222B2
公开(公告)日：2010-03-02
申请号：US11484906
申请日：2006-07-12
申请人： Mark P. Kaminsky , Roger A. Grey
发明人： Mark P. Kaminsky , Roger A. Grey
IPC分类号： C07D301/06 , C07D301/12
CPC分类号： C07D301/06 , B01J21/063 , B01J21/066 , B01J23/6567 , B01J29/89 , B01J35/0006 , B01J35/1014 , B01J37/0205
摘要： The invention is a process for epoxidizing an olefin with hydrogen and oxygen in the presence of a catalyst mixture containing a titanium or vanadium zeolite and a supported catalyst comprising palladium, rhenium and a carrier. The process results in significantly reduced alkane byproduct formed by the hydrogenation of olefin.
摘要翻译：本发明是在含有钛或钒沸石的催化剂混合物和包含钯，铼和载体的负载催化剂存在下，用氢和氧环氧化烯烃的方法。该方法可显着减少由烯烃氢化形成的烷烃副产物。

3. 发明授权

US07615654B2 Direct epoxidation process 失效
标题翻译：直接环氧化工艺
公开(公告)号：US07615654B2
公开(公告)日：2009-11-10
申请号：US11254829
申请日：2005-10-20
申请人： Bi Le-Khac , Mark P. Kaminsky , Kun Qin , Roger A. Grey
发明人： Bi Le-Khac , Mark P. Kaminsky , Kun Qin , Roger A. Grey
IPC分类号： C07D301/10 , C07D303/00
CPC分类号： C07D301/06
摘要： A process is disclosed for the epoxidation of an olefin with hydrogen and oxygen in the presence of an oxidation catalyst comprising a transition metal zeolite, and a noble metal catalyst comprising a noble metal and an ion-exchange resin. The process is highly productive and selective in making epoxides. A noble metal catalyst comprising a cation-exchanged resin further improves the productivity and/or the selectivity of the process.
摘要翻译：公开了在含有过渡金属沸石的氧化催化剂和包含贵金属和离子交换树脂的贵金属催化剂存在下，用氢和氧环氧化烯烃的方法。该方法在制备环氧化物方面具有高生产率和选择性。包含阳离子交换树脂的贵金属催化剂进一步提高了工艺的生产率和/或选择性。

4. 发明申请

US20080015372A1 Direct epoxidation process using a mixed catalyst system 失效
标题翻译：直接环氧化工艺采用混合催化剂体系
公开(公告)号：US20080015372A1
公开(公告)日：2008-01-17
申请号：US11484906
申请日：2006-07-12
申请人： Mark P. Kaminsky , Roger A. Grey
发明人： Mark P. Kaminsky , Roger A. Grey
IPC分类号： C07D301/06
CPC分类号： C07D301/06 , B01J21/063 , B01J21/066 , B01J23/6567 , B01J29/89 , B01J35/0006 , B01J35/1014 , B01J37/0205
摘要： The invention is a process for epoxidizing an olefin with hydrogen and oxygen in the presence of a catalyst mixture containing a titanium or vanadium zeolite and a supported catalyst comprising palladium, rhenium and a carrier. The process results in significantly reduced alkane byproduct formed by the hydrogenation of olefin.
摘要翻译：本发明是在含有钛或钒沸石的催化剂混合物和包含钯，铼和载体的负载催化剂存在下，用氢和氧环氧化烯烃的方法。该方法可显着减少由烯烃氢化形成的烷烃副产物。

5. 发明授权

US07256149B2 Catalyst regeneration process 有权
标题翻译：催化剂再生过程
公开(公告)号：US07256149B2
公开(公告)日：2007-08-14
申请号：US10785455
申请日：2004-02-24
申请人： Roger A. Grey , Mark P. Kaminsky
发明人： Roger A. Grey , Mark P. Kaminsky
IPC分类号： B01J20/34
CPC分类号： B01J38/12 , B01J29/89 , B01J29/90 , B01J37/0045 , B01J38/10 , B01J2229/42
摘要： Used noble metal-containing titanium zeolite catalysts, that have been employed in the liquid-phase epoxidation of olefins with hydrogen and oxygen in the presence of a buffer, are regenerated by heating the used catalyst at a temperature of at least 250° C. in the presence of a oxygen-containing gas stream, followed by reduction at a temperature of at least 20° C. in the presence of a hydrogen-containing gas stream to form a reactivated catalyst.
摘要翻译：在缓冲液存在下用于氢气和氧气的烯烃的液相环氧化中使用的含贵金属的钛沸石催化剂通过在至少250℃的温度下加热所用的催化剂来再生存在含氧气流，然后在含氢气流的存在下在至少20℃的温度下还原以形成再活化的催化剂。

6. 发明申请

US20090042718A1 Direct epoxidation catalyst and process 审中-公开
标题翻译：直接环氧化催化剂和工艺
公开(公告)号：US20090042718A1
公开(公告)日：2009-02-12
申请号：US11891460
申请日：2007-08-10
申请人： Mark P. Kaminsky , Roger A. Grey , Edrick Morales
发明人： Mark P. Kaminsky , Roger A. Grey , Edrick Morales
IPC分类号： B01J29/068 , C07D301/03
CPC分类号： C07D301/06 , B01J23/44 , B01J23/52 , B01J29/89 , B01J35/0006 , B01J35/006 , B01J37/0045
摘要： A catalyst comprising a transition metal zeolite and a noble metal supported on a titania-containing carrier is disclosed. The supported noble metal has a mean mass diameter of from 2 to 200 μm. The catalyst is used in an epoxidation process comprising reacting an olefin, hydrogen, and oxygen. The supported noble metal is well dispersed in the reaction media.
摘要翻译：公开了一种包含过渡金属沸石和负载在含二氧化钛的载体上的贵金属的催化剂。负载的贵金属的平均质量直径为2〜200μm。催化剂用于环氧化方法，包括使烯烃，氢气和氧气反应。负载的贵金属良好地分散在反应介质中。

7. 发明申请

US20110042273A1 Method for Reducing Coke Fouling in a Burner Tip 有权
标题翻译：减少燃烧器中焦炭污垢的方法
公开(公告)号：US20110042273A1
公开(公告)日：2011-02-24
申请号：US12583313
申请日：2009-08-18
申请人： Mark P. Kaminsky , Bala S. Devakottai , Sellamuthu G. Chellappan
发明人： Mark P. Kaminsky , Bala S. Devakottai , Sellamuthu G. Chellappan
IPC分类号： C10G9/16
CPC分类号： B01J23/883 , B01J23/85 , B01J37/349 , F23D2900/00016
摘要： A method for reducing coke fouling in a burner tip when a waste gas stream containing unsaturated hydrocarbons is combusted by coating the interior of the burner tip and/or impregnating the body of the burner tip with a hydrocarbon hydrogenation promoting catalyst and/or a combustion catalyst.
摘要翻译：当包含不饱和烃的废气流通过涂覆燃烧器尖端的内部和/或用烃氢化促进催化剂和/或燃烧催化剂浸渍燃烧器尖端的主体来燃烧时，减少燃烧器尖端中的焦炭结垢的方法。

8. 发明授权

US06548725B2 Process for manufacturing olefins 失效
标题翻译：制造烯烃的方法
公开(公告)号：US06548725B2
公开(公告)日：2003-04-15
申请号：US09918925
申请日：2001-07-31
申请人： Gilbert Fernand Alphonse Froment , Wilfried Jozef Hippolyte Dehertog , Mark P. Kaminsky
发明人： Gilbert Fernand Alphonse Froment , Wilfried Jozef Hippolyte Dehertog , Mark P. Kaminsky
IPC分类号： C07C406
CPC分类号： C07C4/06 , B01J29/061 , B01J29/405 , B01J29/82 , B01J2229/26 , B01J2229/42 , C07C2529/40 , C10G2400/20 , Y02P30/40
摘要： A catalyst and an improved process for producing olefins by catalytic naphtha cracking are described. The process provides relatively higher yields over a commercially important range of naphtha conversion, while providing about the same or lower yields of aromatics and methane over the range. In the process, a hydrocarbon naphtha feedstock including a hydrocarbon having about three to about twenty carbon atoms per molecule is passed into a reactor containing a pentasil zeolite catalyst. The catalyst includes about 0.1 to about 10 weight percent phosphorus and about 0.1 to about 10 weight percent of a promoter metal selected from the group consisting of gallium, germanium, tin and mixtures thereof. The hydrocarbon may be passed into the reactor together with a diluent selected from the group consisting of steam, nitrogen, methane, and ethane and mixtures thereof. Alternatively, the hydrocarbon may be passed into the reactor together with additional propane.
摘要翻译：描述了通过催化石脑油裂解生产烯烃的催化剂和改进方法。该方法在商业上重要的石脑油转化范围上提供相对较高的产率，同时在该范围内提供大约相同或更低的芳族化合物和甲烷的产率。在此过程中，将包含每分子约3至约20个碳原子的烃类石脑油原料进入含有pentasil沸石催化剂的反应器中。催化剂包括约0.1至约10重量％的磷和约0.1至约10重量％的选自镓，锗，锡及其混合物的助催化剂金属。烃可以与选自蒸汽，氮气，甲烷和乙烷的稀释剂及其混合物一起进入反应器。或者，烃可以与另外的丙烷一起进入反应器。

9. 发明授权

US5354932A Catalytic hydrocarbon conversion using thermally activated hydrotalcite-type clays 失效
标题翻译：使用热活化水滑石型粘土催化烃转化
公开(公告)号：US5354932A
公开(公告)日：1994-10-11
申请号：US93768
申请日：1993-07-19
申请人： Alakananda Bhattacharyya , Mark P. Kaminsky
发明人： Alakananda Bhattacharyya , Mark P. Kaminsky
IPC分类号： B01J21/16 , B01J23/00 , C01B13/14 , C01B13/36 , C01B33/20 , C01B39/06 , C01F7/00 , C01G9/00 , C01G31/00 , C07B61/00 , C07C2/00
CPC分类号： C01G9/006 , B01J23/007 , C01B13/14 , C01B13/363 , C01G31/006 , C01B2203/0261 , C01B2203/1011 , C01B2203/1041 , C01B2203/1047 , C01B2203/1052 , C01B2203/1076 , C01B2203/1082 , C01B2203/1088 , C01B2203/1241 , C01P2002/22 , C01P2002/72 , C01P2002/78 , C01P2006/12 , C01P2006/80 , C01P2006/82 , Y10S585/943
摘要： A catalytic process for the conversion of hydrocarbons is described. Catalyst in this improved process is made by thermally activating a hydrotalcite-type clay of formula:M.sup.2+.sub.2x M.sup.3+.sub.2 (OH).sub.4x+4 A.sup.n-.sub.2/n.ZH.sub.2 Owhere M.sup.2+ is one or more metal ion selected from the group consisting of Mg.sup.2+, Zn.sup.2+ Cu.sup.2+, Ni.sup.2+, Co.sup.2+, Mn.sup.2+ and Fe.sup.2+ and M.sup.3+ is one or more metal ion selected from the group consisting of Al.sup.3+, Fe.sup.3+, Co.sup.3+, Mn.sup.3+ and Cr.sup.3+, x runs between 1.5 and 5, A is one or more anions selected from the group consisting of B(OH).sub.4.sup.-, [B.sub.3 O.sub.3 (OH).sub.4 ].sup.-, V.sub.2 O.sub.7.sup.4-, V.sub.4 O.sub.12.sup.4-, and V.sub.3 O.sub.9.sup.3-, n is 1, 3 or 4, and Z runs between 0 and about 4. These hydrotalcite-type clays have an X-ray diffraction d(001) value greater than about 7.7 Angstroms.
摘要翻译：描述了用于烃转化的催化方法。该改进方法中的催化剂是通过热活化下式的水滑石型粘土制备的：M2 + 2xM3 + 2（OH）4x + 4An-2 / n.ZH2O，其中M2 +是一种或多种金属离子，选自Mg2 + ，Zn2 + Cu2 +，Ni2 +，Co2 +，Mn2 +和Fe2 +和M3 +是选自Al3 +，Fe3 +，Co3 +，Mn3 +和Cr3 +的一种或多种金属离子，x在1.5和5之间运行，A是选择一种或多种阴离子由B（OH）4，[B3O3（OH）4] - ，V2O74-，V4O124-和V3O93-组成的组中，n为1,3或4，Z为0至约4.这些水滑石型粘土具有大于约7.7埃的X射线衍射d（001）值。

10. 发明授权

US5316995A Hydrocarbon conversion catalyst 失效
标题翻译：烃转化催化剂
公开(公告)号：US5316995A
公开(公告)日：1994-05-31
申请号：US32666
申请日：1993-03-17
申请人： Mark P. Kaminsky , Mark S. Kleefisch , George A. Huff, Jr. , Don M. Washecheck , Mark K. Barr
发明人： Mark P. Kaminsky , Mark S. Kleefisch , George A. Huff, Jr. , Don M. Washecheck , Mark K. Barr
IPC分类号： C07C2/84 , B01J27/06 , B01J27/08 , B01J27/125 , B01J27/138
CPC分类号： C07C2/84 , C07C2523/02 , C07C2523/10 , C07C2523/14 , C07C2527/138 , Y10S585/943
摘要： A contact material composition of an intimately mixed halogen-containing mixed oxide of at least one cationic species of a naturally occurring Group IIIB element, at least one cationic species of a Group IIA metal of magnesium, calcium, strontium and barium and at least one cationic species of germanium and gallium, as well as methods for hydrocarbon conversion using such contact material compositions are provided.
摘要翻译：天然存在的IIIB族元素的至少一种阳离子物质的至少一种阳离子种类，镁，钙，锶和钡的IIA族金属的至少一种阳离子物质和至少一种阳离子提供锗和镓的种类，以及使用这种接触材料组合物的烃转化方法。

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