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1. 发明专利

JP2012082292A Chemical thermal storage medium and method for manufacturing the same 有权
标题翻译：化学热存储介质及其制造方法
公开(公告)号：JP2012082292A
公开(公告)日：2012-04-26
申请号：JP2010228489
申请日：2010-10-08
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： AOKI MASAKAZU , SHIMAZU TAKASHI , YAMAUCHI TAKASHI , MATSUMOTO MITSURU
IPC分类号： C09K5/16
摘要： PROBLEM TO BE SOLVED: To provide a chemical thermal storage medium capable of stably absorbing or releasing heat.SOLUTION: The chemical thermal storage medium comprises a fired body obtained by firing a molded body of a mixture prepared by mixing thermal storage particles which generate or absorb heat by occlusion or release of ammonia and a binder which binds the thermal storage particles. The thermal storage particles contain a metal chloride which is a compound of at least one alkali metal element, alkaline earth metal element or transition metal element and chlorine. The binder contains a silicate. The chemical thermal storage medium is excellent in mechanical strength and stably exhibits high thermal output because the thermal storage particles of the metal chloride are bound by the binder comprising the silicate.
摘要翻译：要解决的问题：提供能够稳定地吸收或释放热量的化学热存储介质。解决方案：化学热储存介质包括通过烧结通过混合通过闭塞或释放氨产生或吸收热量的蓄热颗粒制备的混合物的成型体而获得的烧结体，以及结合该蓄热颗粒的粘合剂。蓄热颗粒含有金属氯化物，它是至少一种碱金属元素，碱土金属元素或过渡金属元素和氯的化合物。粘合剂含有硅酸盐。化学热存储介质具有优异的机械强度并且稳定地表现出高的热输出，因为金属氯化物的储热颗粒被包含硅酸盐的粘合剂结合。版权所有（C）2012，JPO＆INPIT

2. 发明专利

JP2012082291A Chemical thermal storage medium and method for manufacturing the same 有权
标题翻译：化学热存储介质及其制造方法
公开(公告)号：JP2012082291A
公开(公告)日：2012-04-26
申请号：JP2010228482
申请日：2010-10-08
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： AOKI MASAKAZU , SHIMAZU TAKASHI , YAMAUCHI TAKASHI , MATSUMOTO MITSURU
IPC分类号： C09K5/16
摘要： PROBLEM TO BE SOLVED: To provide a chemical thermal storage medium capable of stably actuating a chemical thermal storage system using ammonia as a working fluid, and a method for manufacturing a chemical thermal storage medium suitable for manufacturing the same.SOLUTION: The chemical thermal storage medium comprises a fired body obtained by firing a molded body of a mixture prepared by mixing thermal storage particles which generate or absorb heat by occlusion or release of ammonia and a binder which binds the thermal storage particles. The thermal storage particles contain a metal chloride which is a compound of at least one alkali metal element, alkaline earth metal element or transition metal element and chlorine. The binder contains a low-melting glass having a glass transition point of ≤600°C.
摘要翻译：解决的问题：提供能够稳定地驱动使用氨作为工作流体的化学热存储系统的化学热存储介质，以及用于制造适于制造它的化学热存储介质的方法。解决方案：化学热储存介质包括通过烧结通过混合通过闭塞或释放氨产生或吸收热量的蓄热颗粒制备的混合物的成型体而获得的烧结体，以及结合蓄热颗粒的粘合剂。蓄热颗粒含有金属氯化物，它是至少一种碱金属元素，碱土金属元素或过渡金属元素和氯的化合物。粘合剂含有玻璃化转变点≤600℃的低熔点玻璃。版权所有（C）2012，JPO＆INPIT

3. 发明专利

JP2010215464A Hydride complex and method for producing hydrogen gas 有权
标题翻译：氢化物复合物和生产氢气的方法
公开(公告)号：JP2010215464A
公开(公告)日：2010-09-30
申请号：JP2009065490
申请日：2009-03-18
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： MATSUMOTO MITSURU
IPC分类号： C01B3/00 , B01J20/04 , C01B3/04 , C01B3/06 , C01B6/04
CPC分类号： C01B3/065 , C01B3/0078 , C01B6/04 , Y02E60/324 , Y02E60/362 , Y02E60/364
摘要： PROBLEM TO BE SOLVED: To provide a hydride complex which generates a hydrogen gas with a relatively high purity at 200°C or lower and is easily regenerated, and a method for producing a hydrogen gas by using a hydride complex.
SOLUTION: There is provided a hydride complex which includes NaH and a metal salt containing an alkaline earth metal or a transition metal, and in this case, the method for producing a hydrogen gas has a reaction process for reacting the hydride complex with an ammonia gas. Further provided is a hydride complex which includes NaH, a metal salt containing an alkaline earth metal or a transition metal, and an ammonia source which is solid at a normal temperature and generates an ammonia gas by decomposition, and in this case, the method for producing a hydrogen gas has a reaction process for heating the hydride complex.
COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：待解决的问题：提供一种在200℃以下生成具有较高纯度且易于再生的氢气的氢化物配合物，以及使用氢化物络合物制造氢气的方法。解决方案：提供了包含NaH和含有碱土金属或过渡金属的金属盐的氢化物络合物，在这种情况下，氢气的制备方法具有使氢化物络合物与一种氨气。此外还提供了氢化物络合物，其包括NaH，含有碱土金属或过渡金属的金属盐和在常温下为固体并通过分解产生氨气的氨源，在这种情况下，产生氢气具有加热氢化物络合物的反应过程。版权所有（C）2010，JPO＆INPIT

4. 发明专利

JP2011173967A Manufacturing method of energy gas, and energy gas storage material 有权
标题翻译：能源气体的制造方法和能源储气体材料
公开(公告)号：JP2011173967A
公开(公告)日：2011-09-08
申请号：JP2010037931
申请日：2010-02-23
申请人： Tohoku Univ , Toyota Central R&D Labs Inc , 国立大学法人東北大学 , 株式会社豊田中央研究所
发明人： KAWAI YASUAKI , MATSUMOTO MITSURU , TOWATA SHINICHI , FUKUSHIMA YOSHIAKI , CHO KIBU , SAITO FUMIYOSHI
IPC分类号： C10J3/00 , C01B3/02 , C01B32/40
CPC分类号： Y02P20/52
摘要： PROBLEM TO BE SOLVED: To provide a manufacturing method of an energy gas that requires a relatively small charged amount of energy for a mixing treatment of raw materials, gives an energy gas by heating at a relatively low temperature and permits employment of an additive abundant in resources, and an energy gas storage material.
SOLUTION: The manufacturing method of an energy gas has the following constitutions. (1) The manufacturing method of an energy gas comprises a mixing step of adding a formic acid-iron additive or an aqueous solution thereof to a compound containing carbon, hydrogen and/or oxygen and subsequently mixing these and a heating step of heating the mixture obtained in the mixing step in an inert atmosphere. (2) The formic acid-iron additive is at least one selected from among a mixture of formic acid with an iron-based additive, a reaction product of formic acid with the iron-based additive and iron formate. The energy gas storage material is obtained by the mixing step above.
COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：为了提供一种需要相对较少的用于混合处理原料的能量的能量气体的制造方法，通过在较低的温度下加热而产生能量气体，并允许使用资源丰富的添加剂和能源气体储存材料。解决方案：能量气体的制造方法具有以下构成。（1）能量气体的制造方法包括将甲酸 - 铁添加剂或其水溶液添加到含有碳，氢和/或氧的化合物中并随后将其混合的加热步骤和加热混合物的加热步骤在惰性气氛中在混合步骤中得到。（2）甲酸 - 铁添加剂是选自甲酸与铁基添加剂的混合物中的至少一种，甲酸与铁基添加剂的反应产物和甲酸铁。通过上述混合步骤获得能量气体储存材料。版权所有（C）2011，JPO＆INPIT

5. 发明专利

JP2011046583A Mixed body and method for producing the same, method for producing gaseous hydrogen, and hydrogen generator 有权
标题翻译：混合体及其制造方法，生产氢气的方法和氢发生器
公开(公告)号：JP2011046583A
公开(公告)日：2011-03-10
申请号：JP2009198827
申请日：2009-08-28
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： AOKI MASAKAZU , MATSUMOTO MITSURU , TOWATA SHINICHI , NORITAKE TATSUO , KITAJIMA SATSUKI , SATO MASAHIRO
IPC分类号： C01B3/06 , H01M8/06
CPC分类号： Y02E60/362
摘要： PROBLEM TO BE SOLVED: To provide a mixed body which enables LiBH
4 and NH
3 to be reacted with each other at low temperature and also under low pressure and also can release a relatively large quantity of hydrogen, to provide a method for producing the mixed body, to provide a method for producing gaseous hydrogen, and to provide a hydrogen generator.
SOLUTION: The mixed body is obtained by mixing a blend comprising LiBH
4 and NiCl
2 , and is used for being reacted with ammonia, and the method for producing the mixed body is also provided. The method for producing a gaseous hydrogen includes a step where the mixed body is reacted with ammonia. The hydrogen generator includes a mixed body vessel for storing the mixed body; an ammonia vessel for storing ammonia; an ammonia feeder for feeding the ammonia from the ammonia vessel to the mixed body vessel, and a hydrogen exhaust apparatus which, in the mixed body vessel, exhausts the hydrogen produced by the reaction between the mixed body and the ammonia from the mixed body vessel.
COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：为了提供使LiBH 4 和NH 3 在低温和低压下彼此反应的混合体，并且还可以释放相当大量的氢气，以提供制造混合体的方法，提供一种生产气态氢的方法，并提供氢气发生器。解决方案：通过混合包含LiBH 4 和NiCl SB SB2的共混物获得混合体，并用于与氨反应，还提供混合体。制造气态氢的方法包括使混合体与氨反应的工序。氢气发生器包括用于储存混合体的混合体容器; 用于储存氨的氨容器; 用于将氨从氨容器供给到混合体容器的氨供料器，以及在混合体容器中从混合体容器排出由混合体和氨之间的反应产生的氢的氢气排出装置。版权所有（C）2011，JPO＆INPIT

6. 发明专利

JP2009143790A Hydride complex and hydrogen storage material 审中-公开
标题翻译：氢化复合物和氢储存材料
公开(公告)号：JP2009143790A
公开(公告)日：2009-07-02
申请号：JP2008202274
申请日：2008-08-05
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： AOKI MASAKAZU , MATSUMOTO MITSURU , TOWATA SHINICHI , NORITAKE TATSUO
IPC分类号： C01B3/00 , B01J20/04 , C01B6/00
CPC分类号： Y02E60/327 , Y02P20/129
摘要： PROBLEM TO BE SOLVED: To provide a hydride complex which has low rare element content, is lightweight and from/in which a large quantity of hydrogen can be released/absorbed at relatively low temperature and to provide a hydrogen storage material. SOLUTION: The hydride complex comprises Mg(BH 4 ) 2 and Mg(NH 2 ) 2 . The hydrogen storage material is obtained by releasing the whole or a part of the hydrogen contained in the hydride complex. The hydride complex shown by (Mg(BH 4 ) 2 +xMg(NH 2 ) 2 (1/3≤x≤3.0)) is preferably used. COPYRIGHT: (C)2009,JPO&INPIT
摘要翻译：要解决的问题：为了提供稀有元素含量低的氢化物络合物，其重量轻且能够在较低温度下释放/吸收大量氢并提供储氢材料。解决方案：氢化物配合物包含Mg（BH 4 ） 2 和Mg（NH SB 2）。通过释放氢化物络合物中所含的全部或一部分氢来获得储氢材料。由（Mg（BH 4 ） + xMg（NH SB 2）/ SB> 2（/ 3≤x≤3.0））。版权所有（C）2009，JPO＆INPIT

7. 发明专利

JP2009067668A Method of manufacturing metal amide, amide compound complex and its manufacturing method, and hydrogen storage material and its manufacturing method 审中-公开
标题翻译：制备金属酰胺，复合复合材料及其制造方法，氢储存材料及其制造方法
公开(公告)号：JP2009067668A
公开(公告)日：2009-04-02
申请号：JP2008081186
申请日：2008-03-26
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： AOKI MASAKAZU , MATSUMOTO MITSURU , NORITAKE TATSUO , TOWATA SHINICHI , KITAJIMA SATSUKI , SATO MASAHIRO
IPC分类号： C01B21/092 , C01B3/00 , C01B6/04 , H01M8/06
CPC分类号： Y02E60/327 , Y02E60/328 , Y02P20/129
摘要： PROBLEM TO BE SOLVED: To provide a method of manufacturing a metal amide compound which is thermally unstable, and easy to take out hydrogen, an amide compound complex using the metal amide compound prepared by the method and a hydrogen storage material, and methods of manufacturing the compounds. SOLUTION: The method of manufacturing the metal amide comprises reacting an organic metal compound expressed by the general formula: (R) x M and ammonia. In the formula, R is any of one or more organic groups chosen from a group consisting of a 1-10C normal chain alkyl group, branched alkyl group, and an aromatic group. M is a metallic element. X is the valence of M. The amide compound complex is obtained by reacting the organic metal compound: (R) x M and ammonia and mixing an obtained solid and the second component and its manufacture method is disclosed. The hydrogen storage material is obtained by reacting the organic compound: (R) x M containing two or more metallic elements and ammonia and heat-treating under reduced pressure or inert gas atmosphere, and its manufacturing method is disclosed. COPYRIGHT: (C)2009,JPO&INPIT
摘要翻译：待解决的问题：提供一种使用通过该方法制备的金属酰胺化合物和储氢材料制造热不稳定并易于除去氢的金属酰胺化合物的方法和酰胺化合物络合物，以及制造化合物的方法。解决方案：制备金属酰胺的方法包括使由通式（R）-Si x SB / M表示的有机金属化合物与氨反应。在该式中，R是选自1-10C正链烷基，支链烷基和芳族基团中的一种或多种有机基团中的任何一种。 M是金属元素。酰胺化合物络合物是通过使有机金属化合物：（R）＆lt; SB＆gt; M＆amp; M＆amp; M与氨反应，并将得到的固体和第2成分并公开了其制造方法。储氢材料通过使含有两种或更多种金属元素的氨基的有机化合物（R） xS / M与氨反应并在减压或惰性气体气氛下进行热处理而得到，其制造方法公开。版权所有（C）2009，JPO＆INPIT

8. 发明专利

JP2011011936A Hydride composite and hydrogen storage material 审中-公开
标题翻译：氢化复合材料和氢储存材料
公开(公告)号：JP2011011936A
公开(公告)日：2011-01-20
申请号：JP2009156394
申请日：2009-06-30
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： MATSUMOTO MITSURU , AOKI MASAKAZU , NORITAKE TATSUO , TOWATA SHINICHI
IPC分类号： C01B6/24 , B01J20/02 , C01B3/00 , H01M8/06
CPC分类号： Y02E60/327 , Y02P20/129
摘要： PROBLEM TO BE SOLVED: To provide a novel hydride composite from which hydrogen can be taken out, even at ≤200°C, and a hydrogen storage material that can be obtained by releasing the hydrogen from the hydride composite.SOLUTION: The hydride composite is obtained by mixing and pulverizing a mixture of a metal borohydride M(BH)(wherein M is a first metal element; and n is the oxidation number of M) and a metal aluminum hydride compound M'(AlH)(wherein M' is a second metal element; and n' is the oxidation number of M'). The hydrogen storage material is obtained by releasing all or a portion of the hydrogen contained in the hydride composite.
摘要翻译：要解决的问题：提供即使在≤200℃也可以从其中取出氢的新型氢化物复合物，以及可以通过从氢化物复合物中释放氢而获得的储氢材料。溶液：氢化物复合物通过混合并粉碎金属硼氢化物M（BH）（其中M是第一金属元素; n是M的氧化数）和金属氢化铝化合物M'（AlH）（其中M'是第二金属元素; n'是M'的氧化数）。通过释放氢化物复合材料中所含的全部或一部分氢来获得储氢材料。

9. 发明专利

JP2010265136A Hydride composite, imide material and method for producing hydrogen gas 审中-公开
标题翻译：氢化物复合材料，生产氢气的材料和方法
公开(公告)号：JP2010265136A
公开(公告)日：2010-11-25
申请号：JP2009117054
申请日：2009-05-13
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： AOKI MASAKAZU , MATSUMOTO MITSURU , TOWATA SHINICHI , NORITAKE TATSUO , KITAJIMA SATSUKI , SATO MASAHIRO
IPC分类号： C01B6/24 , C01B3/04 , C01B21/092
CPC分类号： Y02E60/364 , Y02P20/129
摘要： PROBLEM TO BE SOLVED: To provide a hydride composite from which hydrogen can be taken out even at ≤100°C, an imide compound that can be obtained by releasing hydrogen from the hydride composite material, and a method for producing hydrogen gas using the hydride composite. SOLUTION: The hydride composite comprises LiAlH x (NH 2 ) 4-x (wherein x=0 or 1) and LiAlH 4 . The imide material is obtained by releasing all or a portion of hydrogen contained in the hydride composite. The method for producing the hydrogen gas comprises a hydrogen releasing step of releasing hydrogen from the hydride composite. COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：为了提供即使在≤100℃也可以取出氢的氢化物复合物，可以通过从氢化物复合材料中释放氢而获得的酰亚胺化合物，以及氢气的制造方法使用氢化物复合材料。解决方案：氢化物复合材料包含LiAlH x SB SB（4）x-x SB（x = 0或1）和LiAlH < SB> 4 。酰亚胺材料是通过释放氢化物复合材料中所含的全部或部分氢而获得的。制造氢气的方法包括从氢化物复合物中释放氢的氢释放步骤。版权所有（C）2011，JPO＆INPIT

10. 发明专利

JP2009023857A Hydrogen generation apparatus 有权
标题翻译：氢气发生装置
公开(公告)号：JP2009023857A
公开(公告)日：2009-02-05
申请号：JP2007186419
申请日：2007-07-18
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： AOKI MASAKAZU , OBA NOBUKO , MATSUMOTO MITSURU , WAKAYAMA HIROAKI
IPC分类号： C01B3/06 , C01B3/00 , C01B3/56
CPC分类号： Y02E60/324 , Y02E60/36
摘要： PROBLEM TO BE SOLVED: To provide a hydrogen generation apparatus which applies a reaction for generating hydrogen from two or more kinds of material. SOLUTION: The hydrogen generation apparatus comprises a liquid material tank 12 for storing a liquid material; a second material tank 18 which is divided into a plurality of subtanks A-D, each of the subtanks A-D being filled with a second material for generating hydrogen by the reaction with the liquid raw material or its gas; a liquid material supplying means (V1 A -V1 D valves) for supplying the liquid material or its gas separately into the subtanks A-D; a hydrogen discharge means (V2 A -V2 B valves) for separately discharging a gas containing hydrogen from the subtanks A-D; and a control means for controlling both of the liquid material supply means and the hydrogen discharge means. COPYRIGHT: (C)2009,JPO&INPIT
摘要翻译：要解决的问题：提供一种从两种或更多种材料产生氢的反应的氢气产生装置。解决方案：氢气产生装置包括用于储存液体材料的液体料箱12; 被分成多个子容器A-D的第二材料槽18，每个副容器A-D填充有通过与液体原料或其气体的反应产生氢气的第二材料; 用于将液体材料或其气体分别供入到子容器A-D中的液体材料供给装置（V1 A -V1 D ）; 用于从副容器A-D分别排放含氢气体的氢气排出装置（V2 A -V2 B ）; 以及用于控制液体材料供应装置和氢气排出装置两者的控制装置。版权所有（C）2009，JPO＆INPIT

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