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1. 发明专利

JP2006181399A Hydrocarbon reforming catalyst, production method for the catalyst and reforming method by the catalyst 有权
标题翻译：碳氢化合物改性催化剂，催化剂生产方法和催化剂改性方法
公开(公告)号：JP2006181399A
公开(公告)日：2006-07-13
申请号：JP2004356491
申请日：2004-12-09
申请人： Nikki Universal Co Ltd , Teikoku Oil Co Ltd , 帝国石油株式会社 , 日揮ユニバーサル株式会社
发明人： AKIYAMA KAZUYA , GOTO TAKASHI , HARA KOJI , KAGANOI SHOICHI , YAMAZAKI TOSHINORI , KURIMURA HIDEKI
IPC分类号： B01J23/46 , B01J21/16 , B01J37/08 , B01J37/18 , C01B3/40
CPC分类号： Y02P20/52
摘要： PROBLEM TO BE SOLVED: To provide a catalyst having high activity, stable at a high temperature and excellent in durability, a production method for the catalyst and a reforming method using the catalyst in order to obtain hydrogen and a synthesis gas by reforming hydrocarbon.
SOLUTION: The catalyst has a molded body of a heat-resistant inorganic oxide; and a covering layer on a surface of the molded body containing a metal-containing solid-solution composition (M+HT/S) obtained by heating an active metal-containing hydrotalcite compound (M-HT) is active in a reforming reaction, has sufficient mechanical strength even in a reaction condition of 700-1,200°C and is excellent in durability. The catalyst can be manufactured by the production method including a step for coating the surface of the molded body constituted by the heat-resistant inorganic oxide with a water slurry containing the active metal-containing hydrotalcite compound (M-HT) and forming the covering layer containing M-HT; and a step for heating the molded body provided with the covering layer to the temperature of 500°C or higher under a reduction atmosphere and reducing/treating it.
COPYRIGHT: (C)2006,JPO&NCIPI
摘要翻译：要解决的问题：为了提供具有高活性，高温稳定和耐久性优异的催化剂，催化剂的制备方法和使用该催化剂的重整方法以通过重整获得氢气和合成气烃。解决方案：催化剂具有耐热无机氧化物的成型体; 在含有含活性金属的水滑石化合物（M-HT）得到的含金属固溶体组合物（M + HT / S）的成形体表面上的覆盖层在重整反应中具有活性，即使在700-1200℃的反应条件下也具有足够的机械强度，并且耐久性优异。催化剂可以通过包括用含有活性金属的水滑石化合物（M-HT）的水浆料涂覆由耐热无机氧化物构成的成型体的表面的步骤的制造方法制造，并形成覆盖层含有M-HT; 以及在还原气氛下将设置有覆盖层的成型体加热至500℃以上的温度并进行还原处理的工序。版权所有（C）2006，JPO＆NCIPI

2. 发明专利

JP2006298664A Solid electrolyte membrane-type reactor 有权
标题翻译：固体电解膜型反应器
公开(公告)号：JP2006298664A
公开(公告)日：2006-11-02
申请号：JP2005118794
申请日：2005-04-15
申请人： Nippon Steel Corp , Teikoku Oil Co Ltd , 帝国石油株式会社 , 新日本製鐵株式会社
发明人： ITO WATARU , SAKON TADASHI , HIRANO KENJI , NAGAI TORU , KURIMURA HIDEKI , YAMAZAKI TOSHINORI
IPC分类号： C01B3/38 , B01D53/22 , B01D69/10
CPC分类号： Y02P20/52
摘要： PROBLEM TO BE SOLVED: To provide a supporting membrane-type membrane-type reactor having a new structure which provides gas species having high utilization value, such as synthesis gases, by a high efficiency chemical conversion reaction by employing a structure for eliminating the influence of the gas diffusion in a porous support. SOLUTION: The solid electrolyte membrane-type reactor has reaction structure of a three layer structure comprising a porous support 1, a dense layer 2 comprising an oxygen ion-electron mixed conductive solid electrolyte formed on the support 1, and a catalyst layer 3 formed on the dense layer 2, wherein a gas 4 to be treated containing a hydrocarbon as main component is supplied onto the surface of the catalyst layer 3 and a high purity oxygen gas 5 is supplied onto the surface of the porous support 1 side, respectively. COPYRIGHT: (C)2007,JPO&INPIT
摘要翻译：要解决的问题：提供一种具有新结构的支撑膜型膜型反应器，其通过采用消除结构的方式通过高效率化学转化反应提供诸如合成气体的具有高利用价值的气体种类多孔载体中气体扩散的影响。解决方案：固体电解质膜型反应器具有包括多孔载体1的三层结构的反应结构，包含形成在载体1上的氧离子电子混合导电固体电解质的致密层2和催化剂层 3，其中将含有烃作为主要成分的待处理气体4供应到催化剂层3的表面上，并将高纯度氧气5供应到多孔载体1侧的表面上，分别。版权所有（C）2007，JPO＆INPIT

3. 发明专利

JP2005281077A Ceramic composition, composite material, and chemical reaction apparatus 审中-公开
标题翻译：陶瓷组合物，复合材料和化学反应装置
公开(公告)号：JP2005281077A
公开(公告)日：2005-10-13
申请号：JP2004098895
申请日：2004-03-30
申请人： Teikoku Oil Co Ltd , 帝国石油株式会社
发明人： KURIMURA HIDEKI , KAGANOI SHOICHI , YAMAZAKI TOSHINORI , ITO TAKASHI , TAKAMURA HITOSHI
IPC分类号： B01D53/22 , B01D71/02 , B01J19/24 , B01J23/89 , C01B3/40 , C01B13/02 , C01F17/00 , C04B35/50 , H01B1/06 , H01B1/08 , H01M4/90
CPC分类号： Y02P20/52
摘要： PROBLEM TO BE SOLVED: To provide a composition which is a composite-type oxide ion mixed conductor composition and excellent in stability and oxygen permeability; and to provide a composite material obtained by using the composition and a chemical reaction apparatus. SOLUTION: The composite-type oxide ion mixed conductor composition includes an oxygen ion conduction phase comprising a rare earth element-added cerium oxide expressed by compositional formula: Ce a A 1-a O γ and a perovskite-type compound oxide expressed by compositional formula: Sr b X 1-b Co c Fe d Z e O δ , wherein the molar ratio of the rare earth element-added cerium oxide to the perovskite-type compound oxide is 0.1 to 20. The composite material is composed of the composition and a porous support body part. The chemical reaction apparatus utilizing the composition or the composite material is used. COPYRIGHT: (C)2006,JPO&NCIPI
摘要翻译：要解决的问题：提供一种复合型氧化物离子混合导体组合物，稳定性和透氧性优异的组合物; 并提供通过使用该组合物和化学反应装置获得的复合材料。解决方案：复合型氧化物离子混合导体组合物包括由以下组成式表示的含有稀土元素的氧化铈的氧离子传导相：Ce < 由组成式表示的钙钛矿型复合氧化物：＆lt; SB＆gt;＆lt; SB＆gt; X＆lt; SB＆gt; 稀土元素添加的二氧化铈与钙钛矿型的摩尔比复合氧化物为0.1〜20。复合材料由组合物和多孔支撑体部分构成。使用利用组合物或复合材料的化学反应装置。版权所有（C）2006，JPO＆NCIPI

4. 发明专利

JP2005288259A Catalyst for reforming methane-containing gas and method for manufacturing synthetic gas 审中-公开
标题翻译：用于改造含甲烷气体的催化剂和制造合成气的方法
公开(公告)号：JP2005288259A
公开(公告)日：2005-10-20
申请号：JP2004105009
申请日：2004-03-31
申请人： National Institute Of Advanced Industrial & Technology , Teikoku Oil Co Ltd , 帝国石油株式会社 , 独立行政法人産業技術総合研究所
发明人： KURIMURA HIDEKI , KAGANOI SHOICHI , YAMAZAKI TOSHINORI , ITO TAKASHI , HAYAKAWA TAKASHI , INABA MIEKO , ANDREI TSUIGANOKU
IPC分类号： B01J23/46
摘要： PROBLEM TO BE SOLVED: To produce an inexpensive and high-performance catalyst used in a reforming reaction of a methane-containing gas, and to provide a method for manufacturing a synthetic gas using the same.
SOLUTION: The method comprises manufacturing the synthetic gas using the catalyst for reforming of the methane-containing gas produced by sintering a hydrotalcite-like layered compound represented by the formula (I); [(M(II)
2+ )
1-x (M(III)
3+ )
x (OH
- )
2 ]
x+ [(A
n- )
x/n ].mH
2 O (I) (wherein M(II)
2+ is Mg
2+ alone or a combination of Mg
2+ with Ni
2+ , Co
2+ , Zn
2+ , Cr
2+ or Fe
2+ ; M(III)
3+ is Al
3+ alone or a combination of Al
3+ with Co
3+ , Cr
3+ or Fe
3+ ; the sum of ions other than Mg
2+ and Al
3+ is 30.0 mol% or lower based on the total of the metal cations; (x) is ≥0.24 and ≤0.33; A
n- are n-valent anions present between layers and on surfaces of the layered compound; and at least a part of A
n- ions is anions derived from an organic metal complex of Ru, Pt, Pd, Rh or Ir).
COPYRIGHT: (C)2006,JPO&NCIPI
摘要翻译：要解决的问题：为了生产用于含甲烷气体的重整反应中使用的便宜且高性能的催化剂，并提供使用该催化剂制造合成气体的方法。解决方案：该方法包括使用通过烧结由式（I）表示的类水滑石层状化合物制备的含甲烷气体的重整用催化剂来制造合成气体; [（M（II） 2 + ） 1-x （M（III） 3 + ） X （ OH - ） 2 ] X + [（A N - ） X / N ]其中M（II） 2 + 单独使用Mg或SP + 2 + ，具有Ni 2 + ，Co 2 + ，Zn 2 + ，Cr 2 + 或Fe 2 + ; M（III） 3 + 是单独的A1 3 + 或Al 3 + > Co 3 + ，Cr 3 + 或Fe 3 + ; Mg以外的离子之和 2 + 并且Al 3 + 基于金属阳离子的总量为30.0mol％或更低;（x）≥0.24和≤0.33; A n - 存在于层之间和层状化合物的表面上的价阴离子;并且至少一部分A n - / SP>离子是衍生自Ru，Pt，Pd，Rh或Ir的有机金属络合物的阴离子）。版权所有（C）2006，JPO＆NCIPI

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