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1. 发明专利

JP2012038737A Non-aqueous electrolyte secondary battery and the nonaqueous electrolyte 审中-公开
标题翻译：非电解电解质二次电池和非电解电解质
公开(公告)号：JP2012038737A
公开(公告)日：2012-02-23
申请号：JP2011220640
申请日：2011-10-05
申请人： Mitsubishi Chemicals Corp , Sanyo Electric Co Ltd , 三洋電機株式会社 , 三菱化学株式会社
发明人： TAKEHARA MASAHIRO , KOTADO MIWA , TAMURA NOBUYUKI , JINNO MARUO
IPC分类号： H01M10/0567 , H01M4/134 , H01M10/052 , H01M10/0568 , H01M10/0569
CPC分类号： Y02E60/122
摘要： PROBLEM TO BE SOLVED: To obtain superior charge/discharge cycle characteristics together with high charge/discharge capacity by suppressing a reaction or the like between a negative electrode active material and a nonaqueous electrolyte in a nonaqueous electrolyte secondary battery in which a thin film of the negative electrode active material containing amorphous or microcrystal silicon or its alloy is formed on a current collector and the thin film of the negative electrode active material is separated into a columnar shape by a gap.SOLUTION: The nonaqueous electrolyte secondary battery includes: a negative electrode 2 in which the thin film of the negative electrode active material comprising the amorphous or microcrystal silicon thin film to store/release lithium is formed on a current collector 2b, and the thin film of the negative electrode active material is separated into the columnar shape by the gap formed in the thickness direction; a positive electrode 1 using a positive electrode active material to store/release lithium; and a nonaqueous electrolyte solution in which lithium salt is dissolved into a nonaqueous solvent. In the battery, a carbonate compound having alkyl group combined with fluorine or alkylene group is contained in the nonaqueous electrolyte solution.
摘要翻译：要解决的问题：为了通过抑制非水电解质二次电池中的负极活性物质和非水电解质之间的反应等来获得优异的充电/放电循环特性以及高的充电/放电容量，其中薄的含有非晶或微晶硅或其合金的负极活性物质的膜形成在集电体上，负极活性物质的薄膜通过间隙分离为柱状。解决方案：非水电解质二次电池包括：在集电体2b上形成负极2，其中包含用于储存/释放锂的非晶或微晶硅薄膜的负极活性材料的薄膜形成在集电体2b上，通过沿厚度方向形成的间隙将负极活性物质的薄膜分离成柱状，使用正极活性物质来储存/释放锂的正极1; 以及将锂盐溶解在非水溶剂中的非水电解液。在电池中，在非水电解液中含有具有与氟或亚烷基结合的烷基的碳酸酯化合物。版权所有（C）2012，JPO＆INPIT

2. 发明专利

JP2006092748A Non-aqueous electrolyte secondary battery and the nonaqueous electrolyte 有权
标题翻译：非电解电解质二次电池和非电解电解质
公开(公告)号：JP2006092748A
公开(公告)日：2006-04-06
申请号：JP2004272661
申请日：2004-09-21
申请人： Mitsubishi Chemicals Corp , Sanyo Electric Co Ltd , 三洋電機株式会社 , 三菱化学株式会社
发明人： TAKEHARA MASAHIRO , KOTADO YOSHIKAZU , TAMURA NOBUYUKI , JINNO MARUO
IPC分类号： H01M4/02 , H01M4/134 , H01M4/38 , H01M10/05 , H01M10/052 , H01M10/0567 , H01M10/0568 , H01M10/0569
CPC分类号： Y02E60/122
摘要： PROBLEM TO BE SOLVED: To provide a nonaqueous electrolyte secondary battery which inhibits the reaction of a cathode active substance and a nonaqueous electrolyte and the like, and can attain a high charge-discharge capacity and excellent charge-discharge cycle performance, where a thin film made of the cathode active substance including a metal to store/emit lithium is formed on a collector of the nonaqueous electrolyte secondary battery, and the thin film made of the cathode active substance is divided into pillars by cuts. SOLUTION: The nonaqueous electrolyte secondary battery is constituted such that: a cathode of the pillars is formed into which the thin film made of a cathode active substance 2a is divided by cuts 2c, where the cathode active substance 2a includes the metal to store/emit lithium, and the thin film is formed on a collector 2b; an anode which uses an anode active substance to store/emit lithium; and a nonaqueous electrolyte made of a nonaqueous solvent into which a lithium salt is dissolved where other lithium salt than LiBF 4 is dissolved into the nonaqueous electrolyte, and the nonaqueous electrolyte is doped with BF 4 salt. COPYRIGHT: (C)2006,JPO&NCIPI
摘要翻译：解决的问题：提供抑制阴极活性物质和非水电解质等的反应的非水电解质二次电池，能够获得高的充放电容量和优异的充放电循环性能，其中在非水电解质二次电池的集电体上形成由包含存储/放出锂的金属的阴极活性物质制成的薄膜，由阴极活性物质制成的薄膜通过切割分割为支柱。解决方案：非水电解质二次电池被构成为：形成由阴极活性物质2a制成的薄膜被切割部分2c分割成柱状的阴极，阴极活性物质2a包括金属，存储/发射锂，并且薄膜形成在集电体2b上; 使用阳极活性物质来储存/释放锂的阳极; 以及由非水溶剂制成的非水电解质，其中将锂盐溶解在其中比LiBF 4 的其它锂盐溶解在其中的非水溶剂中，并且非水电解质掺杂有BF / SB>盐。版权所有（C）2006，JPO＆NCIPI

3. 发明专利

JP2011238440A Nonaqueous electrolyte secondary battery and nonaqueous electrolyte for the same 有权
标题翻译：非电解电解质二次电池和非电解电解质
公开(公告)号：JP2011238440A
公开(公告)日：2011-11-24
申请号：JP2010108224
申请日：2010-05-10
申请人： Mitsubishi Chemicals Corp , Sanyo Electric Co Ltd , 三洋電機株式会社 , 三菱化学株式会社
发明人： YAMAMOTO HIDEKAZU , TSUZUKI KOHEI , SUNANO TAIZO , JINNO MARUO , OHASHI YOICHI , KOTADO MINORU
IPC分类号： H01M10/0567 , H01M10/052 , H01M10/0568 , H01M10/0569
CPC分类号： H01M4/134 , H01M10/0567 , H01M10/0568 , H01M10/0569 , Y02E60/122
摘要： PROBLEM TO BE SOLVED: To provide a nonaqueous electrolyte secondary battery which uses powder-type silicon and/or silicon alloy as an anode active material, the battery being capable of suppressing a side reaction of the anode active material with an electrolyte in a charging/discharging state and improving a charge/discharge cycle characteristics.SOLUTION: In a nonaqueous electrolyte secondary battery provided with a cathode containing a cathode active material, an anode containing an anode active material, and a nonaqueous electrolyte composed of a solute dissolved in a nonaqueous solvent, powder-type silicon and/or silicon alloys are used as an anode active material, a diisocyanate compound as well as at least one type of lithium fluorophosphate selected from a group consisting of lithium monofluorophosphate, lithium difluorophosphate and lithium trifluorophosphate are contained in the nonaqueous electrolyte as an additive, and a chain carbonate compound is contained as the nonaqueous solvent.
摘要翻译：解决问题的方案为了提供使用粉末型硅和/或硅合金作为负极活性物质的非水电解质二次电池，该电池能够抑制负极活性物质与电解质的副反应充电/放电状态，并且提高充电/放电循环特性。解决方案：在设置有包含正极活性物质的阴极的非水电解质二次电池中，含有负极活性物质的阳极和溶解在非水溶剂中的溶质构成的非水电解质，粉末型硅和/或作为负极活性物质使用硅合金，作为添加剂的非水电解质含有二异氰酸酯化合物以及选自单氟磷酸锂，二氟磷酸锂和三氟磷酸锂中的至少一种类型的氟化锂锂，链条含有碳酸酯化合物作为非水溶剂。版权所有（C）2012，JPO＆INPIT

4. 发明专利

JP2004296105A Non-aqueous electrolyte for secondary batteries and non-aqueous electrolyte secondary battery 有权
标题翻译：二次电池非水电解液和非水电解质二次电池
公开(公告)号：JP2004296105A
公开(公告)日：2004-10-21
申请号：JP2003083086
申请日：2003-03-25
申请人： Mitsubishi Chemicals Corp , Sanyo Electric Co Ltd , 三洋電機株式会社 , 三菱化学株式会社
发明人： TAMURA NOBUYUKI , YOSHIDA TOMOKAZU , JINNO MARUO , FUJITANI SHIN , TAKEHARA MASAHIRO , UE MAKOTO
IPC分类号： H01M4/66 , H01M4/134 , H01M4/1395 , H01M4/38 , H01M10/05 , H01M10/052 , H01M10/0567 , H01M10/0568 , H01M10/0569 , H01M10/40 , H01M4/02 , H01M4/04 , H01M4/58
CPC分类号： H01M4/139 , H01M4/045 , H01M4/134 , H01M4/525 , H01M4/661 , H01M4/70 , H01M10/052 , H01M10/0567 , H01M10/0569 , H01M2300/0025
摘要： PROBLEM TO BE SOLVED: To provide a non-aqueous electrolyte secondary battery of a high energy density suppressing decomposition of electrolyte, with a high charging and discharging efficiency and indicating excellent charging and recharging cycle characteristic. SOLUTION: An active substance thin film storing and discharging lithium is deposited on a collector by CVD (chemical vapor deposition) method, spattering method, vapor deposition method, thermal spraying method or plating method. The active substance thin film is separated into columnar state by slits formed in the thickness direction and a cathode in which a bottom of the column is adhered to the collector, a (positive electrode) storing and discharging lithium, and electrolyte which is produced by having lithium salt dissolved in the non-aqueous solvent, are provided. A compound expressed by a general formula(I) below is contained in the electrolyte. General formula (I): R n -M=0.In the formula, R expresses alkyl which can be provided with a substituent, they may be the same or different from each other, and may either be independent substituents or joined with each other wound in a ring. Furthermore, M is either S or P, n is 2 when M is S and 3 when P. COPYRIGHT: (C)2005,JPO&NCIPI
摘要翻译：解决的问题：提供一种能够抑制电解质分解的高能量密度的非水电解质二次电池，具有高的充放电效率，并表现出优异的充电和再充电循环特性。解决方案：通过CVD（化学气相沉积）法，溅射法，气相沉积法，热喷涂法或电镀法将收集和放电锂的活性物质薄膜沉积在集电体上。活性物质薄膜通过在厚度方向上形成的狭缝和柱的底部附着到集电体上的阴极分离成柱状，存储和放出锂的正电极和通过具有提供了溶解在非水溶剂中的锂盐。由电解液中含有下述通式（I）表示的化合物。通式（I）：R SB = -M = 0。式中，R表示可带有取代基的烷基，它们可以相同或不同，可以是独立的取代基或彼此缠绕在环中。此外，M是S或P，当M是S时，n是2，当P是3时。（C）2005，JPO和NCIPI

5. 发明专利

JP2004296103A Non-aqueous electrolyte for secondary battery and non-aqueous electrolyte secondary battery 审中-公开
公开(公告)号：JP2004296103A
公开(公告)日：2004-10-21
申请号：JP2003083084
申请日：2003-03-25
申请人： Mitsubishi Chemicals Corp , Sanyo Electric Co Ltd , 三洋電機株式会社 , 三菱化学株式会社
发明人： TAMURA NOBUYUKI , YOSHIDA TOMOKAZU , JINNO MARUO , FUJITANI SHIN , TAKEHARA MASAHIRO , UE MAKOTO
IPC分类号： H01M4/66 , H01M4/134 , H01M4/1395 , H01M4/38 , H01M10/05 , H01M10/052 , H01M10/0567 , H01M10/0568 , H01M10/0569 , H01M10/40 , H01M4/02 , H01M4/58
CPC分类号： H01M4/139 , H01M4/04 , H01M4/0402 , H01M4/0421 , H01M4/13 , H01M4/134 , H01M4/661 , H01M4/70 , H01M10/052 , H01M10/0567 , H01M10/0569 , H01M2004/027
摘要： PROBLEM TO BE SOLVED: To provide a high energy density non-aqueous electrolyte secondary battery suppressing decomposition of electrolyte with a high charging and discharging efficiency and superior charging and discharging cycle characteristic.
SOLUTION: Active substance thin film storing and discharging lithium is deposited on a collector by CVD (chemical vapor deposition) method, spattering method, vapor deposition method, thermal spraying method or plating method in the non-aqueous electrolyte secondary battery. The active substance thin film is separated into columnar states by slits formed in the thickness direction, and a (negative electrode) in which the bottom of the column is adhered to the collector, a (positive electrode) storing and discharging lithium, and electrolyte which is produced by having lithium salt dissolved in the non-aqueous solvent, are provided. A compound expressed by a general formula(I) is contained in the electrolyte. In the formula, X expresses a perfluoro alkyl group, in which the number of fluorine or carbon is 1 to 3 and 2n units of X may either be mually the same or different. 'n' expresses an integer which is 1 or more.
COPYRIGHT: (C)2005,JPO&NCIPI

6. 发明专利

JP2004296104A Non-aqueous electrolyte for secondary battery and non-aqueous electrolyte secondary battery 有权
公开(公告)号：JP2004296104A
公开(公告)日：2004-10-21
申请号：JP2003083085
申请日：2003-03-25
申请人： Mitsubishi Chemicals Corp , Sanyo Electric Co Ltd , 三洋電機株式会社 , 三菱化学株式会社
发明人： TAMURA NOBUYUKI , YOSHIDA TOMOKAZU , JINNO MARUO , FUJITANI SHIN , TAKEHARA MASAHIRO , UE MAKOTO
IPC分类号： H01M4/66 , H01M4/134 , H01M4/1395 , H01M4/38 , H01M4/64 , H01M10/05 , H01M10/052 , H01M10/0567 , H01M10/0568 , H01M10/0569 , H01M10/40 , H01M4/02 , H01M4/58
CPC分类号： H01M4/133 , H01M4/04 , H01M4/0404 , H01M4/0419 , H01M4/0426 , H01M4/0428 , H01M4/0438 , H01M4/0452 , H01M4/1391 , H01M4/64 , H01M10/052 , H01M10/0568 , H01M10/0569
摘要： PROBLEM TO BE SOLVED: To provide a non-aqueous electrolyte secondary battery of a high energy density suppressing decomposition of the electrolyte with a high charging and discharging efficiency and excellent charging and discharging cycle characteristic.
SOLUTION: An active substance thin film storing and discharging lithium is deposited on a collector by CVD (chemical vapor deposition) method, spattering method, vapor deposition method, thermal spraying method or plating method in the non-aqueous electrolyte secondary battery. The active substance thin film is separated into columns by slits formed in the thickness direction. A (negative electrode) in which a bottom of the column is adhered to the collector, an anode storing and discharging lithium, and electrolyte which is produced by having lithium salt dissolved in the non-aqueous solvent, are provided. A compound expressed by a general formula(I) is contained in the electrolyte. In the formula, R
1 , R
2 and R
3 express an alkyl in which hydrogen or a substituent can be provided, each may either be the same or different from each other and they can either be independent substituents or joined with each other wound in a ring.
COPYRIGHT: (C)2005,JPO&NCIPI

7. 发明专利

JP2006086058A Non-aqueous electrolytic solution secondary battery, and non-aqueous electrolytic solution 有权
标题翻译：非水电解液二次电池和非水电解液
公开(公告)号：JP2006086058A
公开(公告)日：2006-03-30
申请号：JP2004271042
申请日：2004-09-17
申请人： Mitsubishi Chemicals Corp , Sanyo Electric Co Ltd , 三洋電機株式会社 , 三菱化学株式会社
发明人： TAKEHARA MASAHIRO , KOTADO YOSHIKAZU , TAMURA NOBUYUKI , JINNO MARUO
IPC分类号： H01M4/02 , H01M4/134 , H01M4/38 , H01M10/05 , H01M10/052 , H01M10/0567 , H01M10/0568 , H01M10/0569
CPC分类号： H01M10/0569 , H01M4/04 , H01M4/134 , H01M4/38 , H01M4/386 , H01M4/387 , H01M4/661 , H01M10/0525 , H01M10/0567 , H01M2004/027 , H01M2300/0025
摘要： PROBLEM TO BE SOLVED: To suppress reaction or the like of a cathode active material with a non-aqueous electrolytic solution so that a superior charge and discharge cycle characteristic can be obtained together with a high charge and discharge capacity in the non-aqueous electrolytic secondary battery in which a thin film of cathode active material containing metals that store and release lithium on a current collector is formed and this thin film of the cathode active material is separated by gaps into pillar shapes. SOLUTION: In the non-aqueous electrolytic secondary battery that has the cathode 2, in which the film of cathode active material containing the metals that store and release lithium is formed on the current collector 2b and this thin film of cathode active material is separated by the gaps into the pillar shapes formed in the thickness direction, the anode 1 using the anode active material that stores and releases lithium, and the non-aqueous electrolytic solution in which lithium salts are dissolved into the non-aqueous solvent, the non-aqueous electrolytic solution is made to contain carbonate compounds having alkyl groups bonded with fluorine. COPYRIGHT: (C)2006,JPO&NCIPI
摘要翻译：要解决的问题：为了抑制正极活性物质与非水电解液的反应等，从而可以获得优异的充放电循环特性，同时在非极性电解液中具有高充电和放电容量，形成含有在集电体上储存和释放锂的金属的阴极活性物质的薄膜的阴极活性物质的薄膜由间隙分离为柱状的水性电解质二次电池。解决方案：在具有阴极2的非水电解质二次电池中，其中在集电体2b上形成含有储存和释放锂的金属的正极活性物质的膜，并且该阴极活性物质薄膜由间隙分离成在厚度方向形成的柱状，使用负极活性物质储存和释放锂的阳极1和其中锂盐溶解在非水溶剂中的非水电解液，使非水电解液含有具有与氟键合的烷基的碳酸酯化合物。版权所有（C）2006，JPO＆NCIPI

8. 发明专利

JP2011048921A Lithium secondary battery, and method of manufacturing the same 审中-公开
标题翻译：锂二次电池及其制造方法
公开(公告)号：JP2011048921A
公开(公告)日：2011-03-10
申请号：JP2009194071
申请日：2009-08-25
申请人： Sanyo Electric Co Ltd , 三洋電機株式会社
发明人： FUKUI ATSUSHI , SUNANO TAIZO , JINNO MARUO
IPC分类号： H01M4/134 , H01M4/1395 , H01M4/62 , H01M10/052 , H01M10/058
CPC分类号： H01M10/052 , C08G73/10 , C08G73/1085 , H01M4/134 , H01M4/386 , H01M4/525 , H01M4/621 , H01M4/622 , Y02T10/7011 , Y10T29/49115
摘要： PROBLEM TO BE SOLVED: To provide a lithium secondary battery with good charge/discharge cycle characteristics having at least either silicon or a silicon alloy used as a negative electrode active material. SOLUTION: The lithium secondary battery includes an electrode including a negative electrode with a negative electrode current collector and a negative electrode mixture layer formed on the negative electrode current collector and including negative electrode active material particles having at least either silicon or silicon alloy and a binder, a positive electrode, and a separator arranged between the negative electrode and the positive electrode, and nonaqueous electrolyte impregnated in the electrode. The binder contains polyimide resin having a branch structure prepared by imidization of a trivalent or more polyvalent amine with tetracarboxylic dianhydride. COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：提供具有至少用作负极活性材料的硅或硅合金的充电/放电循环特性良好的锂二次电池。解决方案：锂二次电池包括具有负极集电体的负极和在负极集电体上形成的负极合剂层的电极，并且包括至少具有硅或硅合金的负极活性物质粒子以及布置在负极和正极之间的粘合剂，正极和隔膜以及浸渍在电极中的非水电解质。粘合剂含有具有通过三价以上的多元胺与四羧酸二酐的酰亚胺化而制备的分支结构的聚酰亚胺树脂。版权所有（C）2011，JPO＆INPIT

9. 发明专利

JP2011034943A Nonaqueous electrolyte secondary battery 审中-公开
标题翻译：非电解电解质二次电池
公开(公告)号：JP2011034943A
公开(公告)日：2011-02-17
申请号：JP2009193903
申请日：2009-08-25
申请人： Sanyo Electric Co Ltd , 三洋電機株式会社
发明人： YANAGIDA KATSUISA , YU DENISUYAUWAI , MASAHARA SHINOGI , CHITO DAIZO , JINNO MARUO , OGASAWARA TAKESHI
IPC分类号： H01M10/052 , H01M4/131 , H01M4/36 , H01M4/505 , H01M4/525 , H01M4/62 , H01M10/0569
CPC分类号： H01M4/505 , H01M4/364 , H01M4/366 , H01M4/525 , H01M4/5825 , H01M10/052 , H01M10/0569 , H01M10/446 , H01M2300/0025
摘要： PROBLEM TO BE SOLVED: To provide a nonaqueous electrolyte secondary battery containing a lithium-containing transition metal oxide that releases oxygen during the initial charge as a positive active material and having high discharge capacity and excellent cycle characteristics at high voltage. SOLUTION: The nonaqueous electrolyte secondary battery includes a positive electrode containing an active material, a negative electrode, and a nonaqueous electrolyte solution in which an electrolyte is dissolved in a nonaqueous solvent, and the positive active material contains the lithium-containing transition metal oxide that releases oxygen during the initial charge, and the nonaqueous solvent contains a fluorinated cyclic carbonate in which fluorine atoms are directly bonded to a carbonate ring. COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：解决的问题：提供一种含有含锂过渡金属氧化物的非水电解质二次电池，其在初始充电期间作为正极活性物质释放氧并且具有高放电容量和高电压下优异的循环特性。解决方案：非水电解质二次电池包括含有活性物质的正极，负极和电解质溶解在非水溶剂中的非水电解质溶液，正极活性物质含有含锂过渡体在初始充电期间释放氧的金属氧化物，非水溶剂含有其中氟原子直接键合到碳酸酯环上的氟化环状碳酸酯。版权所有（C）2011，JPO＆INPIT

10. 发明专利

JP2010198904A Manufacturing method of lithium secondary battery 审中-公开
标题翻译：锂二次电池的制造方法
公开(公告)号：JP2010198904A
公开(公告)日：2010-09-09
申请号：JP2009042289
申请日：2009-02-25
申请人： Sanyo Electric Co Ltd , 三洋電機株式会社
发明人： FUKUI ATSUSHI , OGASAWARA TAKESHI , JINNO MARUO
IPC分类号： H01M10/052 , H01M4/36 , H01M4/505 , H01M4/525 , H01M10/0569 , H01M10/058
CPC分类号： Y02P70/54
摘要： PROBLEM TO BE SOLVED: To provide a manufacturing method of a lithium secondary battery having a lithium transition metal complex oxide positive electrode and a silicon negative electrode, and capable of manufacturing the lithium secondary battery superior in cycle characteristics in the case of carrying out charge and discharge at a high charging rate. SOLUTION: Lithium transition metal complex oxide particles having a layered structure expressed by a chemical formula Li a Ni x Mn y Co z O 2 (0≤a≤1.1, x+y+z=1, 0≤x≤1, 0≤y≤1, and 0≤z≤1) is mixed into an Al 3+ aqueous solution, and by making pH of the aqueous solution 7 or more, Al(OH) 3 particles are arranged on a surface of the lithium transition metal complex oxide particles, and after that, by applying heat-treatment to the lithium transition metal complex oxide particles in which the Al(OH) 3 particles are arranged on the surface in an oxidized atmosphere at 450°C to 650°C, the Al(OH) 3 particles are converted into Al 2 O 3 particles, and they are stuck to the surface of the lithium transition metal complex oxide particles. COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：解决的问题：提供具有锂过渡金属复合氧化物正极和硅负极的锂二次电池的制造方法，并且能够制造在携带时具有优异的循环特性的锂二次电池以高充电率进行充放电。解决方案：具有由化学式Li表示的层状结构的锂过渡金属复合氧化物颗粒Ni x Y Co 3 + 水溶液，通过使水溶液的pH为7以上，将Al（OH）3 SB 3颗粒排列在锂过渡层的表面上金属复合氧化物粒子，然后通过对在氧化气氛中的450℃的表面上配置Al（OH） 3 粒子的锂过渡金属络合物氧化物粒子进行热处理在350℃至650℃之间，将Al（OH）3 SB 3颗粒转化为AlS / SiO 3 SB 3颗粒，并将它们粘附到表面的锂过渡金属复合氧化物颗粒。版权所有（C）2010，JPO＆INPIT

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