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1. 发明专利

JP2012104244A Composition for forming catalyst layer, gas diffusion electrode, membrane-electrode assembly and fuel cell 审中-公开
标题翻译：形成催化层，气体扩散电极，膜电极组件和燃料电池的组合物
公开(公告)号：JP2012104244A
公开(公告)日：2012-05-31
申请号：JP2010249168
申请日：2010-11-05
申请人： Kuraray Co Ltd , Nagoya Univ , 国立大学法人名古屋大学 , 株式会社クラレ
发明人： NAKANO TAKESHI , YAMASHITA TAKETOMO , ONO TOMOHIRO , SUGO NOZOMI , HIBINO TAKASHI
IPC分类号： H01M4/86 , H01M4/90 , H01M4/92 , H01M8/10
CPC分类号： Y02E60/521
摘要： PROBLEM TO BE SOLVED: To provide a fuel cell that can be used at temperatures of 100°C or higher and can especially reduce the cathode overvoltage, and to provide a gas diffusion electrode having a catalyst layer used in the fuel cell, a membrane-electrode assembly having the gas diffusion electrodes on both sides of a polymer electrolyte membrane, and a composition for forming catalyst layer.SOLUTION: A composition for forming a catalyst layer contains, based on 100 pts.mass of a block copolymer (P) containing a polymer block (A) having an ion conductive group and a polymer block (B) having no ion conductive group, 25 to 400 pts.mass of an ion conductive metal phosphate, and 50 to 300 pts.mass in terms of metal of a metal catalyst (X) containing at least one kind of metal selected from metals belonging to group VIII to X on the periodic table (long period type). A gas diffusion electrode having a catalyst layer formed using the composition for forming a catalyst layer, a membrane-electrode assembly and a fuel cell are also provided.
摘要翻译：要解决的问题：为了提供可以在100℃以上的温度下使用并能够特别地降低阴极过电压的燃料电池，并且提供具有在燃料电池中使用的催化剂层的气体扩散电极，在聚合物电解质膜的两侧具有气体扩散电极的膜 - 电极组件和用于形成催化剂层的组合物。
解决方案：用于形成催化剂层的组合物基于100质量份含有具有离子传导性基团的聚合物嵌段（A）和不具有离子传导性的聚合物嵌段（B）的嵌段共聚物（P）基团，离子导电金属磷酸盐为25〜400质量份，金属催化剂（X）为50〜300质量份，含有选自属于VIII〜X族的金属中的至少一种金属周期表（长周期型）。还提供了一种具有使用该催化剂层形成用组合物形成的催化剂层的气体扩散电极，膜 - 电极组件和燃料电池。版权所有（C）2012，JPO＆INPIT

2. 发明专利

JP2013206669A Polymer electrolyte membrane 审中-公开
标题翻译：聚合物电解质膜
公开(公告)号：JP2013206669A
公开(公告)日：2013-10-07
申请号：JP2012073172
申请日：2012-03-28
申请人： Kuraray Co Ltd , 株式会社クラレ
发明人： YAMASHITA TAKETOMO , TOSHINARI KENTA , ONO TOMOHIRO , SUGO NOZOMI
IPC分类号： H01M8/02 , C08K5/05 , C08L53/00 , H01B1/06
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide a polymer electrolyte membrane which is made of a non-fluorine-based material, flexible and hard to crack, and excellent in hot water resistance.SOLUTION: There is provided the polymer electrolyte membrane in which a block copolymer (Z) containing a polymer block (A), which is composed of a structural unit derived from an aromatic vinyl compound and has an ion conductive group, and an amorphous polymer block (B), which is composed of a structural unit derived from an unsaturated aliphatic hydrocarbon, is crosslinked with a crosslinking agent (X) having three or more allyl groups and one or more hydroxyl groups.
摘要翻译：要解决的问题：提供一种由非氟基材料制成的高分子电解质膜，其柔软且难裂纹，并且具有优异的耐热水性。解决方案：提供了一种聚合物电解质膜，其中嵌段共聚物（Z），其含有由芳香族乙烯基化合物衍生的具有离子导电性基团的结构单元构成的聚合物嵌段（A）和非结晶性聚合物嵌段（B），其由来自不饱和脂肪族烃与具有三个以上烯丙基和一个以上羟基的交联剂（X）交联。

3. 发明专利

JP2013194194A Method for producing polymer compound having proton-conducting group 有权
标题翻译：用于生产具有原子导体组的聚合物化合物的方法
公开(公告)号：JP2013194194A
公开(公告)日：2013-09-30
申请号：JP2012064828
申请日：2012-03-22
申请人： Kuraray Co Ltd , 株式会社クラレ
发明人： SHIMIZU KAZUYA , YAMASHITA TAKETOMO , SUGO NOZOMI
IPC分类号： C08F8/00 , C08F6/06 , C08G85/00 , H01B13/00 , H01M8/02 , H01M8/10
CPC分类号： Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide an industrially advantageous production method of a polymer compound which is free from a water-soluble acid and has a proton-conducting group.SOLUTION: A method for producing a polymer compound having a proton-conducting group includes: a reaction step of introducing the proton-conducting group to a polymer compound having no proton-conducting group; a precipitation step of precipitating a solid content by adding water after the reaction step; and a cleaning step of disposing the solid content and an ion exchange resin through a water permeable diaphragm to bring the solid content into contact therewith through water.
摘要翻译：要解决的问题：提供一种不含水溶性酸并具有质子传导基团的高分子化合物的工业上有利的制备方法。溶液：具有质子传导基团的高分子化合物的制造方法包括：将质子传导基团引入到不具有质子传导基团的高分子化合物的反应步骤; 沉淀步骤，通过在反应步骤后加水来沉淀固体含量; 以及通过透水膜将固体成分和离子交换树脂配置成使固体成分与水接触的清洗工序。

4. 发明专利

JP2011204467A Membrane-electrode assembly and method of manufacturing the same, and polymer electrolyte fuel cell 有权
标题翻译：膜电极组件及其制造方法和聚合物电解质燃料电池
公开(公告)号：JP2011204467A
公开(公告)日：2011-10-13
申请号：JP2010070654
申请日：2010-03-25
申请人： Kuraray Co Ltd , 株式会社クラレ
发明人： SHIMIZU KAZUYA , ONO TOMOHIRO , NAKANO TAKESHI , YAMASHITA TAKETOMO , SUZUKI CHIE , SUGO NOZOMI
IPC分类号： H01M4/86 , H01M8/10
CPC分类号： Y02P70/56
摘要： PROBLEM TO BE SOLVED: To supply a polymer electrolyte fuel cell having high cell voltage in a high current density region and high maximum output density.SOLUTION: In this membrane-electrode assembly, the intensity ratio of a crystal peak to be measured with the wide-angle X-ray diffraction of polymer electrolyte in a catalyst layer, to an amorphism peak is in a range of 1.09-1.19. The polymer electrolyte fuel cell equipped with the membrane-electrode assembly is supplied.
摘要翻译：要解决的问题：在高电流密度区域提供具有高电池电压的高分子电解质型燃料电池，并且具有高的最大输出密度。解决方案：在该膜 - 电极组件中，测量的结晶峰的强度比与宽聚合物电解质在催化剂层中的X射线衍射峰到异性峰的范围为1.09-1.19。提供配备有膜 - 电极组件的聚合物电解质燃料电池。

5. 发明专利

JP2013080599A Polyelectrolyte membrane, membrane-electrode assembly, and solid polymer fuel cell 有权
标题翻译：聚电解质膜，膜电极组件和固体聚合物燃料电池
公开(公告)号：JP2013080599A
公开(公告)日：2013-05-02
申请号：JP2011219479
申请日：2011-10-03
申请人： Kuraray Co Ltd , 株式会社クラレ
发明人： YAMASHITA TAKETOMO , IDE AYAKA , ONO TOMOHIRO , SUGO NOZOMI
IPC分类号： H01M8/02 , C08J5/22 , H01B1/06 , H01M8/10
CPC分类号： Y02E60/521
摘要： PROBLEM TO BE SOLVED: To provide a polyelectrolyte membrane excellent in durability and ionic conductivity in a low-humidity atmosphere, a membrane-electrode assembly, and a solid polymer fuel cell.SOLUTION: A block copolymer (Z) includes 7 or 8 polymer blocks including a polymer block (A) which has no ion-conducting group, an amorphous olefin polymer block (B), and aromatic vinyl polymer blocks (C), the terminal polymer blocks are selected from the polymer block (A) and the polymer blocks (C), and the polymer blocks attached to both ends of the polymer block (B) are the polymer blocks (C) only. A block copolymer (Z) is made from the block copolymer (Z) by introducing an ion-conducting group into the polymer block (A), and the percentage of breaking elongation of the block copolymer (Z) is equal to or higher than 300% under a condition where the temperature is 25°C, the relative humidity is 50%, and the tensile rate is 500 mm/min. A polyelectrolyte membrane contains the block copolymer (Z). A membrane-electrode assembly includes the polyelectrolyte membrane. A solid polymer fuel cell includes the membrane-electrode assembly.
摘要翻译：要解决的问题：提供在低湿度气氛下，耐久性和离子传导性优异的聚电解质膜，膜 - 电极组件和固体聚合物燃料电池。解决方案：嵌段共聚物（Z 0 ）包括7或8个聚合物嵌段，包括聚合物嵌段（A 0 ）不含离子导电基团，无定形烯烃聚合物嵌段（B）和芳香族乙烯基聚合物嵌段（C），末端聚合物嵌段选自聚合物嵌段（A 0 ）和聚合物嵌段（C），并且附着于聚合物嵌段（B）两端的聚合物嵌段仅为聚合物嵌段（C）。嵌段共聚物（Z）由嵌段共聚物（Z > 0 SB”）通过将离子导电基团引入聚合物嵌段（A 0 ），嵌段共聚物（Z）的断裂伸长率在温度为25℃，相对湿度为50％的条件下为300％以上，拉伸倍率为 500毫米/分。聚电解质膜含有嵌段共聚物（Z）。膜 - 电极组件包括聚电解质膜。固体聚合物燃料电池包括膜 - 电极组件。版权所有（C）2013，JPO＆INPIT

6. 发明专利

JP2011216244A Polymer electrolyte, polymer electrolyte membrane, membrane-electrode assembly, and fuel cell 审中-公开
标题翻译：聚合物电解质，聚合物电解质膜，膜电极组件和燃料电池
公开(公告)号：JP2011216244A
公开(公告)日：2011-10-27
申请号：JP2010081463
申请日：2010-03-31
申请人： Kuraray Co Ltd , 株式会社クラレ
发明人： ONO TOMOHIRO , YAMASHITA TAKETOMO , TOSHINARI KENTA , SHIMIZU KAZUYA , KUBO KEIJI , SUGO NOZOMI
IPC分类号： H01M8/02 , C08F297/04 , C08J5/22 , H01B1/06 , H01M8/10
CPC分类号： Y02E60/521
摘要： PROBLEM TO BE SOLVED: To provide a new polymer electrolyte, a polymer electrolyte membrane formed of the polymer electrolyte, a membrane-electrode assembly having the polymer electrolyte membrane, and a fuel cell including the membrane-electrode assembly and having output characteristics and mechanical durability in wetting.SOLUTION: The polymer electrolyte is characterized by that it contains a star polymer having 2.5 or more straight-chain arm structures on average, the arm structure contains a polymer block (A) having an ion conductive group, and a polymer block (C) having no ion conductive group, and a terminal of the arm structure of the star polymer has a block structure of (C)-(A)-. This invention provides the polymer electrolyte membrane formed of the above polymer electrolyte, the membrane-electrode assembly having the polymer electrolyte membrane, and the fuel cell having the membrane-electrode assembly.
摘要翻译：要解决的问题：为了提供新的聚合物电解质，由聚合物电解质形成的聚合物电解质膜，具有聚合物电解质膜的膜 - 电极组件和包括膜 - 电极组件的燃料电池，具有输出特性和机械耐久性溶液：聚合物电解质的特征在于它含有平均具有2.5个或更多个直链臂结构的星形聚合物，该臂结构包含具有离子导电基团的聚合物嵌段（A）和聚合物嵌段（ C）没有离子导电基团，并且星形聚合物的臂结构的末端具有（C） - （A） - 的嵌段结构。本发明提供由上述聚合物电解质形成的聚合物电解质膜，具有聚合物电解质膜的膜 - 电极组件和具有膜 - 电极组件的燃料电池。

7. 发明专利

JP2011204468A Membrane-electrode assembly and solid polymer fuel cell 审中-公开
标题翻译：膜电极组件和固体聚合物燃料电池
公开(公告)号：JP2011204468A
公开(公告)日：2011-10-13
申请号：JP2010070655
申请日：2010-03-25
申请人： Kuraray Co Ltd , 株式会社クラレ
发明人： SHIMIZU KAZUYA , ONO TOMOHIRO , NAKANO TAKESHI , YAMASHITA TAKETOMO , SUZUKI CHIE , SUGO NOZOMI
IPC分类号： H01M8/02 , H01M8/10
CPC分类号： Y02E60/521
摘要： PROBLEM TO BE SOLVED: To supply a polymer electrolyte fuel cell having high cell voltage in a high current density region and high maximum output density.SOLUTION: The membrane-electrode assembly includes two gas diffusion electrodes, and polymer electrolyte membrane arranged therebetween. 180° peel strength on an interface between each gas diffusion electrode and the polymer electrolyte membrane is 0.20 N/cm or more. The solid polymer fuel cell including the membrane-electrode assembly is supplied.
摘要翻译：要解决的问题：提供具有高电流密度区域和高最大输出密度的高电池电压的聚合物电解质燃料电池。解决方案：膜 - 电极组件包括两个气体扩散电极和布置在其间的聚合物电解质膜。每个气体扩散电极和聚合物电解质膜之间的界面上的180°剥离强度为0.20N / cm以上。提供包括膜 - 电极组件的固体聚合物燃料电池。

8. 发明专利

JP2011108553A Catalyst layer, and method of manufacturing the same 有权
标题翻译：催化剂层及其制造方法
公开(公告)号：JP2011108553A
公开(公告)日：2011-06-02
申请号：JP2009264332
申请日：2009-11-19
申请人： Kuraray Co Ltd , 株式会社クラレ
发明人： NAKAI SHINJI , KUBO KEIJI , YAMASHITA TAKETOMO , ONO TOMOHIRO , SUGO NOZOMI
IPC分类号： H01M4/88 , C08F297/04 , H01M4/86 , H01M8/02 , H01M8/10
CPC分类号： Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide a method of manufacturing a catalyst layer which structures a gas diffusion electrode for a solid polymer fuel cell which achieves excellent catalyst utilization efficiency, and to provide a catalyst layer obtained by the manufacturing method. SOLUTION: The method of manufacturing the catalyst layer formed of catalyst particles and at least one kind of ion conductive binders, includes a first process for mixing a solution formed of a first ion conductive binder and an organic solvent with the catalyst particles which are not dissolved in the organic solvent substantially; a second process for eliminating the organic solvent and obtaining binder coated particles; and a third process for mixing the binder coated catalyst particles with a diffusion liquid formed by diffusing a second ion conductive binder in an aqueous diffusion medium with a diffusion particle diameter of 1 μm or less. The catalyst layer is obtained by the same manufacturing method. COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：提供一种制造催化剂层的方法，该催化剂层构成固体高分子型燃料电池用气体扩散电极，其能够获得优异的催化剂利用效率，并提供通过该制造方法获得的催化剂层。解决方案：制造由催化剂颗粒和至少一种离子导电粘合剂形成的催化剂层的方法包括将由第一离子导电粘合剂和有机溶剂形成的溶液与催化剂颗粒混合的第一方法，基本上不溶于有机溶剂; 用于消除有机溶剂并获得粘合剂涂覆颗粒的第二种方法; 以及第三种方法，用于将粘合剂涂覆的催化剂颗粒与扩散液混合，所述扩散液通过使扩散粒径为1μm以下的水性扩散介质中的第二离子导电性粘合剂扩散而形成。催化剂层通过相同的制造方法获得。版权所有（C）2011，JPO＆INPIT

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