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    • 3. 发明专利
    • METHOD FOR TREATING SPENT FUEL
    • JPH11248880A
    • 1999-09-17
    • JP5550798
    • 1998-03-06
    • MITSUBISHI HEAVY IND LTDNEW CLEAR DEV KK
    • FUJIOKA TSUNAAKIIIZUKA TATSUYAKOSAKA YUJI
    • G21C3/62G21C19/44
    • PROBLEM TO BE SOLVED: To collect uranium in the form of nitride by heating a spent fuel with uranium nitride as a main constituent in a nitrogen atmosphere containing N that is at least a specific nitrogen partial pressure at a specific temperature of a specific amount of time and removing the covering of uranium nitride and pulverizing it and at the same time separating and eliminating a volatile unclear reaction product. SOLUTION: A reaction container 2 is provided with a nitrogen gas supply line 4 for supplying a nitrogen gas containing N to a reaction container 2, an inert gas supply line 5 for supplying an inert gas to the reaction container 2, a gas exhaust line 6, and a heating heater 3, and heats a spent fuel 1 in a nitrogen gas atmosphere. In this configuration, the spent fuel that mainly consists of uranium nitride is heated for approximately 10-30 minutes within the range of 600 deg.C-800 deg.C in a nitrogen gas atmosphere containing N where a nitrogen partial pressure is at least 0.01 atmospheric pressure, and then the spent fuel is heated at least for 30 minutes within the range of 800 deg.C-1,450 deg.C in an atmosphere where nitrogen is set to a partial pressure of 1 atmospheric pressure or less, vacuum, or inert gas atmosphere.