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1. 发明公开

EP3203561A1 ODORANT FOR FUEL GASES FOR ANION MEMBRANE FUEL CELLS, FUEL GAS AND POWER GENERATION SYSTEM USING ANION MEMBRANE FUEL CELL 审中-公开
标题翻译：用阴离子膜燃料电池研究阴离子膜燃料电池，燃料气体和发电系统的燃料气体
公开(公告)号：EP3203561A1
公开(公告)日：2017-08-09
申请号：EP15845749.9
申请日：2015-09-29
申请人： Tokuyama Corporation
发明人： NEGISHI, Takayuki , WATANABE, Shin
IPC分类号： H01M8/04 , H01M8/10
CPC分类号： H01M8/04671 , C01B3/02 , C01C1/02 , G01M3/00 , G01N21/80 , H01M4/926 , H01M8/04 , H01M8/0662 , H01M8/10 , H01M2008/1095
摘要： To provide an odorant for fuel gases for anion membrane fuel cells, which does not generate a harmful sulfur compound after combustion and does not deteriorate the performance of a fuel cell, while enabling leakage detection at low concentrations, and which enables detection of leakage of a gas by a means other than odor, for example, by visual observation. An odorant for fuel gases for anion membrane fuel cells, which imparts a fuel gas with an odor, and which is characterized in that the odorant contains at least one or more substances selected from the group consisting of ammonia, trimethylamine, triethylamine, N,N-diethylmethylamine, N,N-dipropylmethylamine, N,N-dipropylethylamine, N,N-diisopropylmethylamine, N,N-diisopropylethylamine, dimethylamine, diethylamine, dipropylamine, ethylmethylamine, propylmethylamine, propylethylamine, methylamine, ethylamine and propylamine.
摘要翻译：本发明提供一种阴极隔膜型燃料电池用燃料气体用加臭剂，其燃烧后不会产生有害的硫化合物，不会使燃料电池的性能下降，并且能够在低浓度下进行泄漏检测，并且能够检测出例如通过视觉观察，通过气味以外的手段来获得气体。一种阴离子膜燃料电池用燃料气体用加味剂，其赋予燃料气体臭味，其特征在于，加味剂含有选自氨，三甲胺，三乙胺，N，N N-二丙基甲胺，N，N-二丙基乙胺，N，N-二异丙基甲基胺，N，N-二异丙基乙胺，二甲胺，二乙胺，二丙胺，乙基甲胺，丙基甲胺，丙基乙胺，甲胺，乙胺和丙胺。

2. 发明授权

EP1338588B1 METHOD OF RESOLVING OPTICAL ISOMERS OF AMINO ACID DERIVATIVE 有权
标题翻译：氨基衍生物的方法解析
公开(公告)号：EP1338588B1
公开(公告)日：2007-09-26
申请号：EP01980906.0
申请日：2001-10-25
申请人： TOKUYAMA CORPORATION
发明人： WATANABE, Shin , KAWAHARA, Mizue
IPC分类号： C07C231/20 , C07C233/83 , C07C269/08 , C07C271/22 , C07C319/28 , C07C323/58 , C07D207/16 , C07D209/20 , C07B57/00
CPC分类号： C07C269/08 , C07B2200/07 , C07C231/20 , C07C319/28 , C07D207/16 , C07C233/83 , C07C271/22 , C07C323/58 , C07C323/59
摘要： A method of resolving optical isomers which comprises mixing in an aqueous solution an amino acid derivative in the form of a mixture of D- and L-isomers (for example, N-(tert-butoxycarbonyl)-DL-alanine) with a hydrophilic compound isomers (for example, β-cyclodextrin), and then bringing the resultant aqueous solution or aqueous suspension into contact with a hydrophobic substance (for example, a solid having been subjected to a hydrophobic surface treatment) at pH 3.5 or lower or in the coexistence of an ion containing an atomic group capable of serving as a counter ion to the above-described amino acid derivative (for example, triethylammonium ion) to thereby resolve the D-amino acid derivative from the L-amino acid derivative which are contained in the aqueous solution or the aqueous suspension.

3. 发明公开

EP3125346A9 ANION CONDUCTOR AND LAYERED METAL HYDROXIDE 审中-公开
标题翻译：阴离子导体和层状金属氢氧化物
公开(公告)号：EP3125346A9
公开(公告)日：2017-05-10
申请号：EP15769786.3
申请日：2015-03-25
申请人： Tokuyama Corporation
发明人： KAMADA, Kai , WATANABE, Shin , YANAGI, Hiroyuki
IPC分类号： H01M8/02 , C01F17/00 , C01G3/00 , C01G9/00 , H01B1/06 , H01M8/10
CPC分类号： H01M8/1016 , C01F17/00 , C01F17/0043 , C01F17/005 , C01F17/0075 , C01G3/00 , C01G3/02 , C01G3/08 , C01G9/00 , C01G9/02 , C01P2002/22 , C01P2002/72 , C01P2004/61 , C01P2004/62 , C01P2004/64 , C01P2006/40 , C01P2006/60 , H01B1/04 , H01B1/06 , H01M2/1646 , H01M4/926 , H01M8/083 , H01M12/08 , H01M2300/0014 , H01M2300/0068 , Y02E60/128
摘要： The present invention provides a novel anion conductor which comprises a layered metal hydroxide and can be used as an alkaline electrolyte film for use in a fuel cell or the like. An anion conductor characterized by comprising a molded product of a layered metal hydroxide represented by formula (1): [M x (OH) y (A) (αx-y)/z -nH 2 O] (wherein M represents a metal that can serve as a bivalent or trivalent cation; α represents the number of valency of the metal M, A represents an atom or an atomic group that can serve as an anion, and z represents the number of valency of the anion A, wherein, when (αx-y)/z is 2 or greater, A's may be different types of anions which can serve as anions having the same valencies as each other, or may be anions having different valencies from each other; and n represents the average number of molecules of interlayer water contained per one repeating unit). The anion conductor according to the present invention is composed of an inorganic material, and therefore has excellent heat resistance and physical strength and can be operated for a longer period at a higher temperature compared with the conventional ones when used as an anion conductor for a fuel cell, an air cell or the like.
摘要翻译：本发明提供一种新型阴离子导体，其包含层状金属氢氧化物并且可用作用于燃料电池等的碱性电解质膜。一种阴离子导体，其特征在于，含有由式（1）表示的层状金属氢氧化物的成型体：[Mx（OH）y（A）（αx-y）/ z-nH2O]（式中，M表示可作为二价或三价阳离子，α表示金属M的价数，A表示可以作为阴离子的原子或原子团，z表示阴离子A的价数，其中当（αx- y）/ z为2以上时，A可以是可以作为具有相同价态的阴离子的不同种类的阴离子，也可以是价态不同的阴离子，n表示中间层的平均分子数每个重复单位含有的水）。根据本发明的阴离子导体由无机材料组成，因此具有优异的耐热性和物理强度，并且当用作燃料的阴离子导体时，与传统的阴极导体相比，可以在更高的温度下运行更长的时间细胞，空气细胞等。

4. 发明授权

EP2343764B1 OPERATING METHOD FOR NEGATIVE ION EXCHANGE MEMBRANE-TYPE FUEL CELL 有权
标题翻译：操作方法与膜的燃料电池FOR阴离子交换
公开(公告)号：EP2343764B1
公开(公告)日：2015-08-12
申请号：EP09819176.0
申请日：2009-10-06
申请人： Tokuyama Corporation
发明人： INOUE, Hiroshi , WATANABE, Shin , FUKUTA, Kenji , YANAGI, Hiroyuki
IPC分类号： H01M8/04 , H01M8/02 , H01M8/10 , H01M8/06
CPC分类号： H01M8/0668 , H01M8/1004 , H01M2008/1095

5. 发明公开

EP2333887A1 METHOD FOR PRODUCING ANION EXCHANGE MEMBRANE FOR SOLID POLYMER ELECTROLYTE-TYPE FUEL CELL 有权
标题翻译： METHOD FOR PRODUCING阴离子交换膜与固体高分子电解质的燃料电池
公开(公告)号：EP2333887A1
公开(公告)日：2011-06-15
申请号：EP09819175.2
申请日：2009-10-06
申请人： Tokuyama Corporation
发明人： FUKUTA, Kenji , WATANABE, Shin , YANAGI, Hiroyuki
IPC分类号： H01M8/02 , C08J5/22 , H01M8/10
CPC分类号： C08J5/2287 , C08J2323/12 , H01M8/1025 , H01M8/1027 , H01M8/103 , H01M8/1039 , H01M8/1088 , Y02P70/56
摘要： Provided is a method for the simple and stable production of an anion exchange membrane for an anion exchange membrane-type fuel cell. An anion-exchange membrane having quaternary ammonium groups or quaternary phosphonium groups wherein halogen ions serve as the counter ions is obtained and rather than being subjected to ion exchange with an OH-type membrane using a toxic substance such as sodium hydroxide, the halogen-type anion exchange membrane is brought into contact with a carbonate solution and/or bicarbonate solution to directly obtain an anion exchange membrane where at least some of the counterions of the quaternary ammonium groups or quaternary phosphonium groups are CO 3 2- and/or HCO 3 - .
摘要翻译：提供了一种用于简单和稳定的生产的阴离子交换膜的对阴离子交换膜型燃料电池的方法。具有季铵基团或季基团的阴离子交换膜worin卤离子作为抗衡离子获得和，而不是使用一种有毒物质经受与OH型膜的离子交换：诸如氢氧化钠，卤素型阴离子交换膜进入与碳酸盐溶液和/或碳酸氢盐溶液对阴离子交换膜，其中至少一些所述季铵基团或季基团的抗衡离子的是CO 3 2-得到直接接触和/或HCO 3 - ，

6. 发明公开

EP3125346A1 ANION CONDUCTOR AND LAYERED METAL HYDROXIDE 审中-公开
标题翻译： ANIONENLEITER和层状金属氢氧化物
公开(公告)号：EP3125346A1
公开(公告)日：2017-02-01
申请号：EP15769786.3
申请日：2015-03-25
申请人： Tokuyama Corporation
发明人： KAMADA, Kai , WATANABE, Shin , YANAGI, Hiroyuki
IPC分类号： H01M8/02 , C01F17/00 , C01G3/00 , C01G9/00 , H01B1/06 , H01M8/10
CPC分类号： H01M8/1016 , C01F17/00 , C01F17/0043 , C01F17/005 , C01F17/0075 , C01G3/00 , C01G3/02 , C01G3/08 , C01G9/00 , C01G9/02 , C01P2002/22 , C01P2002/72 , C01P2004/61 , C01P2004/62 , C01P2004/64 , C01P2006/40 , C01P2006/60 , H01B1/04 , H01B1/06 , H01M2/1646 , H01M4/926 , H01M8/083 , H01M12/08 , H01M2300/0014 , H01M2300/0068 , Y02E60/128
摘要： The present invention provides a novel anion conductor which comprises a layered metal hydroxide and can be used as an alkaline electrolyte film for use in a fuel cell or the like. An anion conductor characterized by comprising a molded product of a layered metal hydroxide represented by formula (1): [M x (OH) y (A) (αx-y)/z -nH 2 O] (wherein M represents a metal that can serve as a bivalent or trivalent cation; α represents the number of valency of the metal M, A represents an atom or an atomic group that can serve as an anion, and z represents the number of valency of the anion A, wherein, when (αx-y)/z is 2 or greater, A's may be different types of anions which can serve as anions having the same valencies as each other, or may be anions having different valencies from each other; and n represents the average number of molecules of interlayer water contained per one repeating unit). The anion conductor according to the present invention is composed of an inorganic material, and therefore has excellent heat resistance and physical strength and can be operated for a longer period at a higher temperature compared with the conventional ones when used as an anion conductor for a fuel cell, an air cell or the like.

7. 发明公开

EP2461411A9 POWER GENERATION SYSTEM UTILIZING ALKALINE FUEL CELL, AND FUEL GAS FOR ALKALINE FUEL CELL FOR USE IN THE SYSTEM 审中-公开
标题翻译：在本系统为碱性燃料电池碱性燃料电池和燃料气体用发电系统
公开(公告)号：EP2461411A9
公开(公告)日：2012-08-15
申请号：EP10804311.8
申请日：2010-07-22
申请人： Tokuyama Corporation
发明人： WATANABE, Shin , FUKUTA, Kenji , YANAGI, Hiroyuki
IPC分类号： H01M8/06 , H01M8/02 , H01M8/10
CPC分类号： H01M8/083 , H01M8/222 , Y02E60/50
摘要： Disclosed is a method for producing a higher output in an alkaline fuel cell that utilizes an electrolyte membrane comprising an anion exchange membrane, compared to the outputs produced in the conventional alkaline fuel cells. Specifically disclosed is a power generation system which utilizes an alkaline fuel cell that comprises an electrolyte membrane comprising an anion exchange membrane and a pair of electrodes (an anode and a cathode) arranged on the both sides of the electrolyte membrane, wherein the alkaline fuel cell can generate an electric power by supplying a fuel gas and an oxidizer gas to the anode side and the cathode side, respectively. The power generation system is characterized by using a hydrogen gas containing a basic compound such as ammonia as the fuel gas to be supplied to the anode side.

8. 发明公开

EP2461411A1 POWER GENERATION SYSTEM UTILIZING ALKALINE FUEL CELL, AND FUEL GAS FOR ALKALINE FUEL CELL FOR USE IN THE SYSTEM 审中-公开
标题翻译：在本系统为碱性燃料电池碱性燃料电池和燃料气体用发电系统
公开(公告)号：EP2461411A1
公开(公告)日：2012-06-06
申请号：EP10804311.8
申请日：2010-07-22
申请人： Tokuyama Corporation
发明人： WATANABE, Shin , FUKUTA, Kenji , YANAGI, Hiroyuki
IPC分类号： H01M8/06 , H01M8/02 , H01M8/10
CPC分类号： H01M8/083 , H01M8/222 , Y02E60/50
摘要： Disclosed is a method for producing a higher output in an alkaline fuel cell that utilizes an electrolyte membrane comprising an anion exchange membrane, compared to the outputs produced in the conventional alkaline fuel cells. Specifically disclosed is a power generation system which utilizes an alkaline fuel cell that comprises an electrolyte membrane comprising an anion exchange membrane and a pair of electrodes (an anode and a cathode) arranged on the both sides of the electrolyte membrane, wherein the alkaline fuel cell can generate an electric power by supplying a fuel gas and an oxidizer gas to the anode side and the cathode side, respectively. The power generation system is characterized by using a hydrogen gas containing a basic compound such as ammonia as the fuel gas to be supplied to the anode side.
摘要翻译：公开了用于在给碱性燃料电池产生更高的输出的方法并利用到电解质膜包含阴离子交换膜的，相比于在常规的碱性燃料电池所产生的输出。具体地说游离缺失盘是发电系统，其利用给碱性燃料电池那样电解质膜包括包含布置在所述电解质膜的bothsides阴离子交换膜和一对电极（阳极和阴极）的，worin的碱性燃料电池可以通过分别供给燃料气体和氧化剂气体向阳极侧至阴极侧，并且产生电力。发电系统是通过使用含有碱性化合物氢气特点：如氨作为燃料气体被供给到阳极侧。

9. 发明公开

EP2296210A1 METHOD FOR PRODUCING ION CONDUCTIVITY-IMPARTING AGENT FOR CATALYST ELECTRODE LAYER OF ANION-EXCHANGE MEMBRANE FUEL CELL 审中-公开
标题翻译：方法HERSTELUNG的离子电导率剂催化剂电极层中的阴离子燃料电池
公开(公告)号：EP2296210A1
公开(公告)日：2011-03-16
申请号：EP09758318.1
申请日：2009-06-02
申请人： Tokuyama Corporation
发明人： FUKUTA, Kenji , WATANABE, Shin , YAMASHITA, Yoshinobu , YANAGI, Hiroyuki
IPC分类号： H01M4/88 , H01M4/86 , H01M8/10
CPC分类号： H01M4/8663 , H01M8/1018
摘要： Disclosed is a method for producing an ion-conductivity providing agent for a catalyst electrode layer of an anion-exchange membrane type fuel cell comprising: producing anionic conductive resin including a quaternary onium base having a halogeno ion as its counterion, and bringing the halogen type anionic conductive resin into contact with carbonate solution and/or bicarbonate solution to directly obtain anionic conductive resin in which at least a part of the counterion of said quaternary onium base is CO 3 2- and/or HCO 3 - , without ion exchange of the counterion to OH-type by using deleterious substance such as sodium hydroxide. The purpose is to provide a method for stably producing an ion-conductivity providing agent used for giving ion conductivity to a catalyst electrode layer of an anion-exchange membrane type fuel cell, the method being easy to operate, the ion-conductivity providing agent showing constant effect for giving ion conductivity.
摘要翻译：公开了一种用于在离子传导性产生用于阴离子交换膜型燃料电池，其包含的催化剂电极层中提供剂的方法：生产阴离子导电性树脂，其包括具有卤代离子作为其抗衡离子的季鎓基，并且使卤素型阴离子的导电性树脂与碳酸盐溶液和/或碳酸氢盐溶液接触，以获得直接阴离子导电性树脂至少在所述季鎓基的抗衡离子的一部分是CO 3 2-和/或HCO 3 - ，而不的离子交换如氢氧化钠：通过使用有害物质抗衡OH型。目的是提供一种用于稳定地制造在离子传导性，提供用于给出离子传导性的阴离子交换膜型燃料电池的催化剂电极层剂，该方法易于操作，离子导电性赋予剂显示提供一种方法用于给出离子传导性常数的效果。

10. 发明公开

EP2822070A1 CATALYST ELECTRODE LAYER AND METHOD FOR PRODUCING SAME 审中-公开
标题翻译：哈萨克斯坦共和国人权大臣KATALYSATORELEKTRODENSCHICHT
公开(公告)号：EP2822070A1
公开(公告)日：2015-01-07
申请号：EP13755212.1
申请日：2013-02-27
申请人： Tokuyama Corporation
发明人： WATANABE, Shin , FUKUTA, Kenji , INOUE, Fumie
IPC分类号： H01M4/86 , H01M4/88 , H01M8/02 , H01M8/10 , H01B1/06
CPC分类号： H01M4/8673 , H01M4/8668 , H01M4/8825 , H01M4/8828 , H01M4/8892 , H01M4/926 , H01M8/1004 , H01M2008/1095 , H01M2300/0082
摘要： [Problem] To provide a catalyst electrode layer which has excellent durability and is easily controlled with respect to the cross-linking degree. [Solution] Provided is a catalyst electrode layer which is characterized by containing a catalyst for electrodes and an anion-conducting elastomer that is obtained by introducing a quaternary base-type anion exchange group into at least some aromatic rings in a copolymer of an aromatic vinyl compound and a conjugated diene compound or in a copolymer that is obtained by saturating some or all of the double bonds in the main chain by hydrogenating the conjugated diene part of the above-mentioned copolymer, in said anion-conducting elastomer, at least some quaternary base-type anion exchange groups forming a cross-linked structure.
摘要翻译： [问题]提供一种具有优异的耐久性并且易于相对于交联度控制的催化剂电极层。 [方案]提供一种催化剂电极层，其特征在于含有电极用催化剂和阴离子导电性弹性体，其通过在芳香族乙烯基共聚物的共聚物中的至少一些芳香环中引入季碱型阴离子交换基团化合物和共轭二烯化合物或通过在所述阴离子导电弹性体中氢化所述共聚物的共轭二烯部分而使主链中的一部分或全部双键饱和而获得的共聚物中的至少一种四形成交联结构的碱式阴离子交换基团。

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