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1. 发明授权

EP2133144B1 A NOBLE METAL-CONTAINING TI-SI MATERIAL AND THE PREPARING METHOD THEREOF 有权
公开(公告)号：EP2133144B1
公开(公告)日：2020-08-05
申请号：EP08733849.7
申请日：2008-03-27
申请人： China Petroleum & Chemical Corporation , Research Institute Of Petroleum Processing, Sinopec
发明人： LIN, Min , SHI, Chunfeng , LONG, Jun , ZHU, Bin , SHU, Xingtian , MU, Xuhong , LUO, Yibin , WANG, Xieqing , RU, Yingchun
IPC分类号： B01J29/89 , B01J23/40 , C07D301/04 , C07D305/06

2. 发明公开

EP2868629A1 RARE-EARTH CONTAINED Y TYPE MOLECULAR SIEVE AND PREPARATION METHOD THEREOF 有权
标题翻译：赫尔辛基大学
公开(公告)号：EP2868629A1
公开(公告)日：2015-05-06
申请号：EP13810624.0
申请日：2013-06-27
申请人： China Petroleum & Chemical Corporation , Research Institute Of Petroleum Processing, Sinopec
发明人： ZHENG, Jinyu , LUO, Yibin , SHU, Xingtian
IPC分类号： C01B39/24
CPC分类号： B01J37/30 , B01J29/088 , C01B39/026 , C01B39/24
摘要： The present invention provides a rare earth-containing Y zeolite and a preparation process thereof, said rare earth-containing Y zeolite has a rare earth content as rare earth oxide of 10-25wt%, a unit cell size of 2.440-2.472nm, a crystallinity of 35-65%, a Si/Al atom ratio in the skeleton of 2.5-5.0; and a product of the ratio of the strength I 1 of the peak at 2θ=11.8±0.1° to the strength I 2 of the peak at 2θ=12.3±0.1° in the X-ray diffraction spectrogram of the zeolite and the weight percent of rare earth as rare earth oxide in the zeolite of higher than 48.
摘要翻译：本发明提供了一种含稀土Y沸石及其制备方法，所述含稀土Y沸石的稀土氧化物的稀土含量为10-25wt％，晶胞尺寸为2.440-2.472nm，结晶度为35-65％，骨架中Si / Al原子比为2.5-5.0; 和在2θ= 11.8±0.1°处的峰的强度I 1与在2β= 12.3±0.1°处的峰的强度I 2与沸石的X射线衍射光谱图中的比率的乘积和沸石中稀土稀土氧化物的重量百分比高于48。

3. 发明公开

EP4137456A1 PHOSPHORUS-CONTAINING/PHOSPHORUS-MODIFIED ZSM-5 MOLECULAR SIEVE, PYROLYSIS ADDITIVE AND PYROLYSIS CATALYST CONTAINING SAME, PREPARATION METHOD THEREFOR AND APPLICATION THEREOF 审中-实审
公开(公告)号：EP4137456A1
公开(公告)日：2023-02-22
申请号：EP21788139.0
申请日：2021-04-13
申请人： China Petroleum & Chemical Corporation , Research Institute Of Petroleum Processing, Sinopec
发明人： LUO, Yibin , WANG, Chengqiang , OUYANG, Ying , XING, Enhui , SHU, Xingtian
IPC分类号： C01B39/10 , C01B39/38 , B01J29/40
摘要： The present invention relates to a phosphorus-containing or phosphorus-modified ZSM-5 molecular sieve, which is characterized in that in its 27A1 MAS-NMR, the ratio of peak area for the resonance signal having a chemical shift of 39±3ppm to peak area for the resonance signal having a chemical shift of 54ppm±3ppm is ≥1; or in its surface XPS elemental analysis, the value of n1/n2 is≤0.1; wherein, n1 represents the mole number of phosphorus, n2 represents the total mole number of silicon and aluminum; the present invention also relates to a cracking auxiliary or cracking catalyst containing said phosphorus-containing/phosphorus-modified ZSM-5 molecular sieve, and a process for preparing the same and use thereof.

4. 发明授权

EP2075068B1 A CATALYST FOR CONVERTING HYDROCARBONS 有权
标题翻译：一种转化烃的催化剂
公开(公告)号：EP2075068B1
公开(公告)日：2018-02-28
申请号：EP06791146.1
申请日：2006-09-28
申请人： China Petroleum & Chemical Corporation , Research Institute Of Petroleum Processing, Sinopec
发明人： LIU, Yujian , TIAN, Huiping , SHU, Xingtian , LONG, Jun , LUO, Yibin , XIE, Chaogang , CHEN, Zhenyu , ZHAO, Liuzhou , ZHU, Yuxia , LU, Youbao
IPC分类号： B01J35/10 , B01J35/02 , B01J37/02 , B01J35/04
CPC分类号： B01J29/80 , B01J29/40 , B01J29/7007 , B01J29/7057 , B01J29/7615 , B01J29/7815 , B01J35/023 , B01J35/04 , B01J35/1076 , B01J35/1095 , B01J37/0045 , B01J37/0219 , B01J37/0234 , B01J2229/20 , B01J2229/42 , C04B35/18 , C04B2235/3201 , C04B2235/3262 , C04B2235/3272 , C04B2235/3275 , C04B2235/3279 , C04B2235/3281 , C04B2235/3284 , C04B2235/3293 , C04B2235/447 , C10G2400/20
摘要： A hydrocarbon conversion catalyst, which comprises, based on the total weight of the catalyst, 1-60 wt% of a zeolite mixture, 5-99 wt% of a thermotolerant inorganic oxide and 0-70 wt% of clay, wherein said zeolite mixture comprises, based on the total weight of said zeolite mixture, 1-75 wt% of a zeolite beta modified with phosphorus and a transition metal M, 25-99 wt% of a zeolite having a MFI structure and 0-74 wt% of a large pore zeolite, wherein the anhydrous chemical formula of the zeolite beta modified with phosphorus and the transition metal M is represented in the mass percent of the oxides as (0-0.3)Na 2 O·(0.5-10)Al 2 O 3 ·(1.3-10)P 2 O 5 ·(0.7-15)M x O y ·(64-97)SiO 2 , in which the transition metal M is one or more selected from the group consisting of Fe, Co, Ni, Cu, Mn, Zn and Sn; x represents the atom number of the transition metal M, and y represents a number needed for satisfying the oxidation state of the transition metal M. The catalysts provided in the present invention have higher ability to convert petroleum hydrocarbons and higher yields for light olefins, particularly for propylene. The catalysts can be used for the selectively producing light olefins.

5. 发明授权

EP1892040B1 MODIFIED ZEOLITE BETA 有权
标题翻译：修改后的Beta沸石
公开(公告)号：EP1892040B1
公开(公告)日：2010-07-07
申请号：EP06742051.3
申请日：2006-05-31
申请人： China Petroleum & Chemical Corporation , RESEARCH INSTITUTE OF PETROLEUM PROCESSING, SINOPEC
发明人： LUO, Yibin , DA, Zhijian , OUYANG, Ying , ZHUANG, Li , LONG, Jun , SHU, Xingtian , ZONG, Baoning
IPC分类号： B01J29/72 , C10G11/05
CPC分类号： C01B39/10 , B01J29/7057 , B01J29/7615 , B01J29/7815 , B01J29/85 , B01J2229/18 , C01B39/06 , C10G11/05

6. 发明公开

EP2072604A1 A PROCESS FOR CATALYTIC CONVERTING HYDROCARBONS 有权
标题翻译：工艺用于烃的催化转化
公开(公告)号：EP2072604A1
公开(公告)日：2009-06-24
申请号：EP06791147.9
申请日：2006-09-28
申请人： China Petroleum & Chemical Corporation , Research Institute Of Petroleum Processing, Sinopec
发明人： XIE, Chaogang , ZHU, Genquan , YANG, Yihua , LUO, Yibin , LONG, Jun , SHU, Xingtian , ZHANG, Jiushun
IPC分类号： C10G11/05 , B01J29/80 , B01J29/072 , B01J29/076 , B01J29/40
CPC分类号： B01J29/80 , B01J29/084 , B01J29/18 , B01J29/40 , B01J29/60 , B01J29/7057 , B01J29/7615 , B01J29/7815 , B01J37/0045 , B01J2229/18 , B01J2229/42 , C10G11/02 , C10G11/05 , C10G11/14 , C10G11/16 , C10G11/18 , C10G2300/1033 , C10G2300/104 , C10G2300/1044 , C10G2300/1055 , C10G2300/107 , C10G2300/1074 , C10G2300/1077 , C10G2300/4018 , C10G2300/4093 , C10G2300/807 , C10G2400/02 , C10G2400/04 , C10G2400/20
摘要： A process for the catalytic conversion of hydrocarbons, said process comprising the following steps:
a feedstock of hydrocarbons is contacted with a hydrocarbon-converting catalyst to conduct a catalytic cracking reaction in a reactor, then the reaction products are taken from said reactor and fractionated to give light olefins, gasoline, diesel, heavy oil and other saturated hydrocarbons with low molecular weight,
wherein said hydrocarbon-converting catalyst comprises, based on the total weight of the catalyst, 1-60 wt% of a zeolite mixture, 5-99 wt% of a thermotolerant inorganic oxide and 0-70 wt% of clay, wherein said zeolite mixture comprises, based on the total weight of said zeolite mixture, 1-75 wt% of a zeolite beta modified with phosphorus and a transition metal M, 25-99 wt% of a zeolite having a MFI structure and 0-74 wt% of a large pore zeolite,
wherein the anhydrous chemical formula of the zeolite beta modified with phosphorus and the transition metal M is represented in the mass percent of the oxides as (0-0.3)Na 2 O·(0.5-10)Al 2 O 3 ·(1.3-10)P 2 O 5 ·(0.7-15)M x O y ·(64-97)SiO 2 ,
in which the transition metal M is one or more selected from the group consisting of Fe, Co, Ni, Cu, Mn, Zn and Sn; x represents the atom number of the transition metal M, and y represents a number needed for satisfying the oxidation state of the transition metal M.
The process of the present invention has a higher ability to convert petroleum hydrocarbon in a higher yield for light olefins, particularly for propylene.

7. 发明公开

EP2042477A1 A PROCESS FOR PRODUCING ETHYLENE FROM ETHANOL COMBINING THE CATALYTIC CONVERSION OF HYDROCARBONS 有权
标题翻译：工艺生产乙烯从乙醇能够产生碳氢化合物的催化转化将结合
公开(公告)号：EP2042477A1
公开(公告)日：2009-04-01
申请号：EP07764038.1
申请日：2007-07-12
申请人： China Petroleum & Chemical Corporation , RESEARCH INSTITUTE OF PETROLEUM PROCESSING, SINOPEC
发明人： WU, Zhiguo , XIE, Wenhua , XIE, Chaogang , LIU, Qiang , MU, Xuhong , ZHANG, Jiushun , LUO, Yibin , SHU, Xingtian , YAN, Chenghan
IPC分类号： C07C1/24 , C07C11/04
CPC分类号： C10G57/00 , C07C1/24 , C07C2529/08 , C10G11/05 , C10G2300/1033 , C10G2300/104 , C10G2300/1044 , C10G2300/1055 , C10G2300/107 , C10G2300/1074 , C10G2300/1077 , C10G2300/4018 , C10G2400/20 , Y02P20/52 , Y02P20/584 , C07C11/04
摘要： A process for producing ethylene from ethanol combining the catalytic conversion of hydrocarbons: an ethanol feedstock is contacted with a Y-zeolite containing catalyst to give a product stream, and a coked catalyst and an target product of ethylene are obtained after separating the reaction stream; a hydrocarbon feedstock is contacted with a Y-zeolite containing catalyst to give a product stream, a spent catalyst and an oil vapor are obtained after separating the reaction stream, and the oil vapor is further separated to give the products such as gas, gasoline and the like; a part or all of the coked catalyst and a part or all of the spent catalyst enter the regenerator for the coke-burning regeneration, and the regenerated catalyst is divided into two portions, wherein one portion returns to be contacted with the hydrocarbon feedstock, and the other portion, after cooling, returns to be contacted with ethanol feedstock. This process not only reasonably utilizes the excessive thermal energy of the hydrocarbon conversion, but also solves the problem of heat supply for the conversion of ethanol, thus ensuring the continuous catalytic conversion of ethanol and generating enormous economic benefits. For the catalytic conversion of the ethanol, the content of ethylene is 95 vol% or more in the gas product; and the conversion of ethylene is not less than 99%. For the catalytic conversion of the hydrocarbons, the yield for the light olefins increases slightly by at least 2 mol%.
摘要翻译：一种用于从乙醇组合烃的催化转化生产乙烯的方法：乙醇原料与Y型沸石含催化剂，得到的产物料流，和结焦的催化剂与乙烯的目标产物分离反应流之后获得接触; 的烃原料与Y型沸石含催化剂，得到的产物料流，废催化剂和油蒸汽被分离反应流之后获得接触，和油蒸汽被进一步分离，得到产品：如天然气，汽油和等; 的一部分或全部的结焦催化剂和部分或全部的废催化剂进入用于烧焦的再生的再生器，和再生的催化剂分成两个部分，worin一个部分返回到与所述烃原料接触，并另一部分，冷却后，返回到与乙醇原料接触。这个过程不仅合理利用烃转化的过量的热能，因此解决了但热供应用于乙醇转化的麻烦，从而确保了乙醇的连续催化转化并产生巨大的经济效益。对于乙醇的催化转化中，乙烯的含量是在气体产品95体积％以上; 和乙烯的转化率不小于99％。用于烃的催化转化，产量为轻质烯烃稍微增加至少2摩尔％。

8. 发明公开

EP1688392A1 MOLECULAR SIEVE WITH MFI STRUCTURE CONTAINING PHOSPHORUS AND METAL COMPONENTS, PREPARATION PROCESS AND USE THEREOF 有权转让
标题翻译：磷和金属部件含有MFI结构，工艺分子筛用于其与用来生成
公开(公告)号：EP1688392A1
公开(公告)日：2006-08-09
申请号：EP04789889.5
申请日：2004-10-28
申请人： China Petroleum & Chemical Corporation , RESEARCH INSTITUTE OF PETROLEUM PROCESSING, SINOPEC
发明人： LUO, Yibin , OUYANG, Ying , SHU, Xingtian , HE, Mingyuan , WANG, Dianzhong , ZONG, Baoning , LI, Minggang
IPC分类号： C01B39/38
CPC分类号： C01B39/026 , B01J29/084 , B01J29/405 , B01J29/46 , B01J29/48 , B01J29/80 , B01J2229/18 , B01J2229/42 , C10G11/02
摘要： A MFI-structured molecular sieve containing phosphorus and metal components has a formula expressed in anhydrous form and on the basis of oxide weight, as follows: (0 ~ 0.3) Na 2 O (0.5 ∼ 5.5) Al 2 O 3 (1.3 ~ 10) P 2 O 5 (0.7 ~ 15) M1 x O y (0.01 ~ 5) M2 m O n (70 ~ 97) SiO 2 , wherein M1 is one of transition metals selected from the group consisting of Fe, Co and Ni, and M2 is any one of metals selected from the group consisting of Zn, Mn, Ga and Sn. Preparation processes and uses of the instant molecular sieve are also provided. The molecular sieve has an excellent performance for increasing the yield of lower olefins and increasing the aromatics content in gasoline, and can be used as a shape-selective active component for the catalytic cracking catalyst of petroleum hydrocarbons or its additives.
摘要翻译：甲MFI结构分子筛含有磷和金属组分在无水形式和氧化物重量的基础上过表达的公式，如下：（0〜0.3）的Na 2 O（0.5¼5.5）的Al 2 O 3（1.3〜10 ）P 2 O 5（0.7〜15）M1×○Y（0.01〜5）M2 M O对N（70〜97）的SiO 2，worin M1是选自Fe，Co和Ni中选择的过渡金属中的一种，和M2是选自锌，锰，镓和Sn的选择的金属的任何一种。因此，提供的制备方法和本发明分子筛的用途。分子筛具有用于提高低级烯烃和芳烃的增加在汽油含量收率优良的性能，并且可以用作用于石油烃的催化剂或它的添加剂的催化裂化择形活性组分。

9. 发明公开

EP1650288A1 A CRACKING CATALYST WITH DESULFURIZATION 有权
标题翻译：采用催化剂脱硫裂纹
公开(公告)号：EP1650288A1
公开(公告)日：2006-04-26
申请号：EP04738281.7
申请日：2004-06-24
申请人： China Petroleum & Chemical Corporation , RESEARCH INSTITUTE OF PETROLEUM PROCESSING, SINOPEC
发明人： ZONG, Baoning , ZHENG, Jinyu , XIE, Wenhua , XU, Yong , MU, Xuhong , LUO, Yibin , LI, Minggang , SHU, Xingtian
IPC分类号： C10G45/02
CPC分类号： B01J29/84 , B01J29/084 , B01J29/088 , B01J29/40 , B01J29/405 , B01J29/80 , B01J2229/42 , C10G45/12 , C10G47/20
摘要： This invention relates to a composition with desulfurization property, in which the desulfurization component is a kind of molecular sieves with incorporation of vanadium into the skeleton. The composition has high hydrothermal stability and the vanadium is hard to lose.

10. 发明授权

EP2868629B1 RARE-EARTH CONTAINED Y TYPE MOLECULAR SIEVE AND PREPARATION METHOD THEREOF 有权
公开(公告)号：EP2868629B1
公开(公告)日：2019-05-22
申请号：EP13810624.0
申请日：2013-06-27
申请人： China Petroleum & Chemical Corporation , Research Institute Of Petroleum Processing, Sinopec
发明人： ZHENG, Jinyu , LUO, Yibin , SHU, Xingtian
IPC分类号： C01B39/02 , C01B39/24

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