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11. 发明公开

EP1414886A2 VERFAHREN ZUR HERSTELLUNG VON THERMOPLASTISCHEN POLY(3-HYDROXYALKANOATEN) 有权
标题翻译：用于生产热塑性聚（3-羟基链烷酸酯）
公开(公告)号：EP1414886A2
公开(公告)日：2004-05-06
申请号：EP02767222.9
申请日：2002-07-17
申请人： BASF AKTIENGESELLSCHAFT
发明人： SLANY, Michael , LUINSTRA, Gerrit , SAVA, Xavier
IPC分类号： C08G63/82 , C08G63/78
CPC分类号： C08G63/823 , C08G63/06
摘要： A method for the production of thermoplastic poly(3-hydroxyalkanoates) having a molecular weight of more than 6.000 g/mol and a melting point of 70 -170°C by reacting an oxirane compound with carbon monoxide in the presence of a transition metal catalyst chelated with neutral Lewis bases with rhodium (0), nickel(0), iron (0), cobalt (0) or palladium (0) as a central metal and in the presence of diisocyanates, orthoesters, acetalene, anhydrides, P2O5, MgO, MgCl2, MgSO4, zeolites or mixtures thereof at a pressure of 1 - 250 bars and at a temperature ranging from room temperature to 150°C.

12. 发明公开

EP1360005A2 VON EINEM BIS-PHOSPHORINAN ABGELEITETE UND ALS KATALYSATOR ODER ZUR HERSTELLUNG EINES KATALYSATORSYSTEMS GEEIGNETE VERBINDUNG 有权
标题翻译：从A到-phosphorinane衍生物及其生产羰基化催化剂系统的合适的连接
公开(公告)号：EP1360005A2
公开(公告)日：2003-11-12
申请号：EP02704673.9
申请日：2002-01-26
申请人： BASF AKTIENGESELLSCHAFT
发明人： SLANY, Michael , SCHÄFER, Martin , RÖPER, Michael
IPC分类号： B01J31/24 , C07F9/6568 , C07C67/38 , C07F9/50
CPC分类号： B01J31/2433 , B01J2231/321 , B01J2531/80 , B01J2531/822 , B01J2531/824 , B01J2531/827 , B01J2531/828 , C07C67/38 , C07C253/30 , C07F9/65683 , C07C69/44 , C07C69/24 , C07C255/19
摘要： .he invention relates to a compound of formula (I) wherein X represents a low alkylen group, an arylene group or an alkarylene group, L1 has formula (II) wherein Y1 represents oxygen, sulphur or N-R17, R11, R12, R13, R14, R15, R16, R17 independently represent hydrogen, alkyl or aryl, L2 has formula (III) wherein Y2 represents oxygen, sulphur or N-R27, R21, R22, R23, R24, R25, R26, R27 independently represent hydrogen, alkyl or aryl wherein L1 and L2 can be identical or different. The inventive compound is suitable for use as a catalyst or for producing a catalyst system.

13. 发明授权

EP1071689B1 CIS-VERBRÜCKTE METALLKOMPLEXE UND DIESE ENTHALTENDE KATALYSATORSYSTEME 有权
标题翻译： CIS桥联配合和含金属催化剂体系
公开(公告)号：EP1071689B1
公开(公告)日：2002-07-03
申请号：EP99919184.4
申请日：1999-04-01
申请人： BASF AKTIENGESELLSCHAFT
发明人： QUEISSER, Joachim , SLANY, Michael , SCHÄFER, Ansgar , SCHULZ, Michael
IPC分类号： C07F15/00 , C08G67/02 , B01J31/24
CPC分类号： B01J31/24 , C07F9/50 , C07F9/6568 , C07F15/00 , C08G67/02 , C08L73/00 , C09D173/00 , D01F6/76 , D02G3/00 , Y10T428/2913
摘要： The invention relates to a Cis-bridged metal complex of general formula (I), wherein the subsituent R represents an electron-attracting radical. The invention also relates to catalyst systems based on said complexes for copolymerization of carbon monoxide and olefinically non-saturated compounds.

14. 发明公开

EP1499579A1 VERFAHREN ZUR HERSTELLUNG VON METHYLFORMIAT 审中-公开
标题翻译：用于生产甲酸甲酯
公开(公告)号：EP1499579A1
公开(公告)日：2005-01-26
申请号：EP03746771.9
申请日：2003-04-15
申请人： BASF AKTIENGESELLSCHAFT
发明人： ADAMI, Christoph , SLANY, Michael , KARL, Jörn , KAIBEL, Gerd , SCHÄFER, Martin , ZEHNER, Peter , RÖPER, Michael
IPC分类号： C07C67/36 , C07C69/06
CPC分类号： C07C67/36 , C07C69/06
摘要： The invention relates to a method for producing methyl formate by reacting methanol with carbon monoxide at a pressure between 0.5 - 10 MPa abs and at a temperature between 50 - 150 °C in the presence of a metal alcoholate as a catalyst in a reactor, wherein a gas flow is extracted from the reactor, methyl formate carried with said gas flows is separated by condensation and the remaining flow of gas is feed back into the reactor either totally or partially as a circulatory gas flow. In at least one area of the reactor, in which the gas flows essentially in one direction, the average empty tube speed of the gas is adjusted to between 1 - 20 cm/s.

15. 发明公开

EP1434781A1 DIPHOSPHIN 有权
标题翻译：双膦
公开(公告)号：EP1434781A1
公开(公告)日：2004-07-07
申请号：EP02800574.2
申请日：2002-09-26
申请人： BASF AKTIENGESELLSCHAFT
发明人： SAVA, Xavier , SLANY, Michael , RÖPER, Michael
IPC分类号： C07F9/6568
CPC分类号： B01J31/2485 , B01J2231/321 , B01J2531/824 , C07C67/38 , C07F9/65683 , C07F9/657163 , C07C69/533
摘要： The invention relates to diphosphine of formula Rl⊃P-(CH)¿n-PR?2R3 wherein Rl is a bivalent radical which together with the phosphorous atom to which it is linked represents an unsubstituted or substituted 2-phospha-tricyclo[3.3.1.1{3,7}]decyl-group or a derivative thereof, wherein one or several carbon atoms are replaced by heteroatoms, R2, R3 independently represent a monovalent radical having 1 -20 atoms or a joint bivalent radical having 2 - 20 atoms, n is 4 or 5, and the mixtures thereof as a suitable carboxylation system containing palladium or a palladium compound and said type of diphosphin. The invention also relates to a method for the carbonylation of a conjugated diene in the presence of said system.

16. 发明公开

EP1341750A1 VERFAHREN ZUR CARBONYLIERUNG VON PENTENSAEURE UND DEREN DERIVATE 审中-公开
标题翻译：方法羰基戊及其衍生物
公开(公告)号：EP1341750A1
公开(公告)日：2003-09-10
申请号：EP01985838.0
申请日：2001-12-03
申请人： BASF AKTIENGESELLSCHAFT
发明人： SLANY, Michael , SCHÄFER, Martin , RÖPER, Michael
IPC分类号： C07C255/19 , C07C53/00 , C07C51/02 , C07C253/30 , C07C67/36
CPC分类号： C07C253/30 , C07C51/14 , C07C67/38 , C07C55/02 , C07C69/44
摘要： The invention relates to a method for the carbonylation of n-pentenoic acid or derivatives thereof of formula (I), wherein R1 represents CN or COOR?2 and R2¿ represents hydrogen, alkyl or aryl. According to said method, a compound of formula (I) is reacted with carbon monoxide and a compound (II) containing a hydroxyl group in the presence of a catalyst system. The method is characterised in that the catalyst system is obtained by reacting a) a source of a metallic ion of a metal (III) of the 8th subgroup of the periodic table with b) a bidentate phosphine ligand of formula (IV), wherein R?3, R4, R5, R6, R7, R8, R9, R10, R11, R12, R13 and R14¿ independently of one another represent an inorganic group, which contains a respective carbon atom, by means of which the respective group is linked to the relevant tertiary carbon atom given in formula (IV), L1, L2represent independently of one another a lower alkylene group and X represents an arylene group.

17. 发明授权

EP0944638B1 CIS-VERBRÜCKTE METALLKOMPLEXE 失效
标题翻译： CIS-VERBRÜCKTEMETALLKOMPLEXE
公开(公告)号：EP0944638B1
公开(公告)日：2003-06-11
申请号：EP97952029.3
申请日：1997-12-02
申请人： BASF AKTIENGESELLSCHAFT
发明人： SLANY, Michael , HÖHN, Arthur
IPC分类号： C07F15/00 , C07F9/50 , C08G67/02 , B01J31/16
CPC分类号： C08G67/02 , B01J31/18 , B01J31/189 , B01J31/2409 , B01J2531/824 , C07F9/5004 , C07F15/0066
摘要： Cis-bridged metal complexes have the general formula (I), in which the substituents and indexes have the following meanings: R5 stands for hydrogen or for substituents selected from the group of substituted or unsubstituted organic C¿1?-C20 carbon radicals and organic C3-C30 silicon radicals, NR?6R7¿ substituents or a radical of general formula (II), in which q is an integer from 0 to 20; R', R'' stand for hydrogen or substituents selected from the group of organic C¿1?-C20 carbon radicals and organic C3-C30 silicon radicals; and the other substituents in (II) and (I) have the following meanings: M stands for a metal of group VIIIB of the periodic table of elements; E?1, E2¿ stand for an element of group VA of the periodic table of elements; Z stands for an element of group VA of the periodic table of elements; R1 to R4 stand for substituents independently selected from the group of substituted or unsubstituted organic C¿1?-C20 carbon radicals and organic C3-C30 silicon radicals; A', B' stand for substituted and unsubstituted C1-C4-alkylene units, silylene-bridged organic radicals and NR?8¿ radicals; R6 to R8 stand for hydrogen or for substituents selected from the group of organic C¿1?-C20 carbon radicals and organic C3-C30 silicon radicals; L?1, L2¿ are formally charged or neutral ligands, with the exception of L1 = L2 = chloride when R5 ¸ (II); X stands for formally monovalent or polyvalent anions; p equals 0, 1, 2, 3 or 4; m, n equal 0, 1, 2, 3 or 4, whereas p = m x n.

18. 发明授权

EP1091967B1 WASSERLÖSLICHE ÜBERGANGSMETALLKOMPLEXE 有权
标题翻译：水溶性过渡金属络合物
公开(公告)号：EP1091967B1
公开(公告)日：2002-06-05
申请号：EP99929298.0
申请日：1999-06-22
申请人： BASF AKTIENGESELLSCHAFT
发明人： QUEISSER, Joachim , SLANY, Michael , GEPRÄGS, Michael , LINDNER, Ekkehard , SCHMID, Markus , WALD, Joachim , WEGNER, Peter
IPC分类号： C07F15/00 , C07F9/50 , C08G67/02 , B01J31/16
CPC分类号： C08G67/02 , B01J31/18 , B01J31/24 , B01J2531/10 , B01J2531/20 , B01J2531/80 , B01J2531/824 , C07F9/5004 , C07F9/5027 , C07F15/0066

19. 发明公开

EP1071689A1 CIS-VERBRÜCKTE METALLKOMPLEXE UND DIESE ENTHALTENDE KATALYSATORSYSTEME 有权
标题翻译： CIS桥联配合和含金属催化剂体系
公开(公告)号：EP1071689A1
公开(公告)日：2001-01-31
申请号：EP99919184.4
申请日：1999-04-01
申请人： BASF AKTIENGESELLSCHAFT
发明人： QUEISSER, Joachim , SLANY, Michael , SCHÄFER, Ansgar , SCHULZ, Michael
IPC分类号： C07F15/00 , C08G67/02 , B01J31/24
CPC分类号： B01J31/24 , C07F9/50 , C07F9/6568 , C07F15/00 , C08G67/02 , C08L73/00 , C09D173/00 , D01F6/76 , D02G3/00 , Y10T428/2913
摘要： The invention relates to a Cis-bridged metal complex of general formula (I), wherein the subsituent R5 represents an electron-attracting radical. The invention also relates to catalyst systems based on said complexes for copolymerization of carbon monoxide and olefinically non-saturated compounds.

20. 发明公开

EP1024899A1 VERFAHREN ZUR HERSTELLUNG VON GETRÄGERTEN ÜBERGANGSMETALLKATALYSATOREN 审中-公开
标题翻译：工艺生产负载过渡金属催化剂
公开(公告)号：EP1024899A1
公开(公告)日：2000-08-09
申请号：EP98954331.9
申请日：1998-10-05
申请人： BASF AKTIENGESELLSCHAFT
发明人： QUEISSER, Joachim , SLANY, Michael , LUDWIG, Alfons
IPC分类号： B01J37/02 , B01J37/03 , C08G67/02
CPC分类号： C08G67/02 , B01J31/1625 , B01J31/18 , B01J31/1815 , B01J31/2409 , B01J37/031 , B01J2531/824 , C08F10/00 , Y02P20/588 , C08F4/26 , C08F4/7006
摘要： The invention relates to a method for producing supported transition metal catalysts. The support material is suspended in a non-polar aprotic liquid medium, and a metal complex is added to the suspension under control, said metal complex being dissolved in a polar aprotic liquid medium and chelated with at least one bi- or tridentate ligand and containing a metal of group VIIIB, IB or IIB of the periodic table as the metal centre. This mixture is filtered, the resulting residue is optionally washed with a non-polar aprotic liquid medium and the resulting supported transition metal catalyst is optionally liberated advantageously from the liquid residue using inert gas.

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