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91. 发明公开

EP2143700A1 Process to make olefins from oxygenates 审中-公开
标题翻译：一种用于从含氧化合物制备烯烃的过程
公开(公告)号：EP2143700A1
公开(公告)日：2010-01-13
申请号：EP08158924.4
申请日：2008-06-25
申请人： Total Petrochemicals Research Feluy
发明人： Nesterenko, Nikolai , Vermeiren, Walter , Garcia, Wolfgang
IPC分类号： C07C1/20 , C07C4/06 , B01J37/28 , B01J29/40
CPC分类号： B01J29/06 , B01J29/40 , B01J29/90 , B01J37/0009 , B01J37/28 , B01J38/30 , B01J2229/18 , B01J2229/36 , B01J2229/37 , B01J2229/42 , C07C1/20 , C07C4/06 , C07C11/02 , C07C11/04 , C07C11/06 , C07C2529/40 , C07C2529/70 , Y02P20/52 , Y02P20/584
摘要： The present invention relates to a process to make light olefins, in a combined XTO-OCP process, from an oxygen-containing, halogenide-containing or sulphur-containing organic feedstock comprising :
a) providing a catalyst comprising zeolitic molecular sieves containing 10 member and larger channels in their microporous structure,
b) providing an XTO reaction zone, an OCP reaction zone and a catalyst regeneration zone, said catalyst circulating in the three zones, such that at least a portion of the regenerated catalyst is passed to the OCP reaction zone, at least a portion of the catalyst in the OCP reaction zone is passed to the XTO reaction zone and at least a portion of the catalyst in the XTO reaction zone is passed to the regeneration zone;
c) contacting said oxygen-containing, halogenide-containing or sulphur-containing organic feedstock in the XTO reactor with the catalyst at conditions effective to convert at least a portion of the feedstock to form a XTO reactor effluent comprising light olefins and a heavy hydrocarbon fraction;
d) separating said light olefins from said heavy hydrocarbon fraction;
e) contacting said heavy hydrocarbon fraction in the OCP reactor with the catalyst at conditions effective to convert at least a portion of said heavy hydrocarbon fraction to light olefins.
摘要翻译：本发明涉及一种工艺，使轻烯烃在组合的XTO-OCP方法，从含氧，或有机原料包括含硫的含卤化物-：含有10构件a）提供一种催化剂，包含沸石分子筛和在它们的微孔结构较大的通道，b）在OCP在反应区和催化剂再生区XTO反应区提供，所述催化剂循环在三个区域，求并至少将再生催化剂的一部分被传递到OCP反应区中，至少在OCP反应区中的催化剂的一部分被传递到所述XTO反应区和至少在所述XTO反应区中的催化剂的一部分被传递到所述再生区; c）使所述含氧，卤化物含或含硫在XTO反应器的有机原料与所述催化剂在有效地至少原料的一部分转化以形成XTO反应器流出物包括轻质烯烃和重质烃级分的条件 ; d）分离与所述重质烃级分。所述轻质烯烃; E）中接触所述与在有效条件下催化剂中的OCP反应器的重质烃馏分的至少所述重质烃馏分的一部分转化为轻质烯烃。

92. 发明公开

EP2130585A1 Process for making crystalline metallosilicates 审中-公开
标题翻译：制造结晶金属硅酸盐的方法
公开(公告)号：EP2130585A1
公开(公告)日：2009-12-09
申请号：EP08157768.6
申请日：2008-06-06
申请人： Total Petrochemicals Research Feluy
发明人： Bulut, Metin , Jacobs, Pierre , Minoux, Delphine , Nesterenko, Nikolai , Dath, Jean-Pierre , Van Donk, Sander
IPC分类号： B01J29/40 , C01B39/36 , C10G11/05 , C01B39/40
CPC分类号： C01B39/02 , B01J29/06 , B01J29/40 , B01J2229/62 , C01B39/38 , C01B39/40 , C01B39/44 , C01B39/445 , C01B39/46 , C01B39/48 , C07C2/66 , C07C2529/70 , C10G11/05 , C10G45/64 , C07C15/02
摘要： The present invention relates to a process for making a crystalline metallosilicate composition and comprising crystallites having an inner part (the core) and an outer part (the outer layer or shell) such that :
the ratio Si/Metal is higher in the outer part than in the inner part,
the crystallites have a continuous distribution of metal and silicon over the crystalline cross-section,
said process comprising :
a) providing an aqueous medium comprising OH - anions and a metal source,
b) providing an aqueous medium comprising an inorganic source of silicon and optionally a templating agent,
c) optionally providing a non aqueous liquid medium comprising optionally an organic source of silica,
d) mixing the medium a), b) and the optional c) at conditions effective to partly crystallize the desired metallosilicate,
e) cooling down the reaction mixture a)+b)+c) to about room temperature,
f) decreasing the pH of the reaction mixture by at least 0.1 preferably by 0.3 to 4, more preferably by 0.5 to 3,
g) subjecting the resulting mixture of step f) at conditions effective to continue the crystallization of the desired metallosilicate,
h) recovering the desired metallosilicate,

wherein at step d) in the mixture a)+b)+c), before crystallization,
the ratio Si org/Si inorganic is
the molar ratio OH - /SiO 2 is at least 0.3, preferably from 0.3 to 0.6 and more preferably from 0.33 to 0.6 .
摘要翻译：本发明涉及一种制造结晶金属硅酸盐组合物的方法，该方法包括具有内部部分（芯部）和外部部分（外层或外壳）的微晶，使得：外部部分中Si /金属的比率高于在内部，微晶在结晶横截面上具有金属和硅的连续分布，所述方法包括：a）提供包含OH-阴离子和金属源的水性介质，b）提供包含无机物硅源和任选的模板剂，c）任选地提供包含任选有机二氧化硅源的非水性液体介质，d）在有效部分结晶所需金属硅酸盐的条件下混合介质a），b）和任选c） e）将反应混合物a）+ b）+ c）冷却至约室温，f）将反应混合物的pH降低至少0.1，优选0.3至4，更优选0 g）使得到的步骤f）的混合物在有效继续所需金属硅酸盐结晶的条件下进行，h）回收所需的金属硅酸盐，其中在步骤d）中混合物a）+ b）+ c），在结晶之前，Si org / Si无机比率<0.3，有利地<0.2且优选0，OH- / SiO 2摩尔比至少为0.3，优选为0.3-0.6，更优选为0.33-0.6。

93. 发明公开

EP1773737A4 OLIGOMERIZATION PROCESS 有权
标题翻译： OLIGOMERISATIONSVERFAHREN
公开(公告)号：EP1773737A4
公开(公告)日：2009-11-25
申请号：EP05705397
申请日：2005-01-10
申请人： CATALYTIC DISTILLATION TECH
发明人： LOESCHER MITCHELL E , WOODS DAVID G , KEENAN MICHAEL J , SILVERBERG STEVEN E , ALLEN PAUL W
IPC分类号： C07C2/04 , C07C2/02 , C07C2/12 , C07C5/23
CPC分类号： C07C2/12 , C07C2529/70 , Y02P20/127 , C07C11/02

94. 发明公开

EP2072484A1 Olefin oligomerization process 有权
标题翻译： OlefisierungsverfahrenfürOlefine
公开(公告)号：EP2072484A1
公开(公告)日：2009-06-24
申请号：EP09157119.0
申请日：2005-05-26
申请人： ExxonMobil Chemical Patents Inc.
发明人： Brown, Stephen , Mathys, Georges , Godsmark, John
IPC分类号： C07C2/12 , B01J29/04
CPC分类号： B01J29/7042 , B01J29/06 , B01J29/7026 , B01J29/703 , B01J29/7046 , B01J37/0009 , B01J2229/42 , C07C2/12 , C07C2529/70 , C07C2529/80 , C10G50/00 , C07C11/02
摘要： In a process for oligomerizing an olefinic hydrocarbon feedstock comprising at least 65 wt% olefins, the feedstock is contacted under oligomerization conditions with (a) a first unidimensional 10-ring molecular sieve catalyst and (b) a second multidimensional crystalline molecular sieve catalyst. The first and second catalysts may be contained in separate reactors or as separate beds in a single reactor.
摘要翻译：在包含至少65重量％的烯烃的烯烃原料的低聚方法中，原料在低聚条件下与（a）第一单维10环分子筛催化剂和（b）第二多维结晶分子筛催化剂接触。第一和第二催化剂可以包含在单独的反应器中或作为单个反应器中的分离床。

95. 发明公开

EP2060551A1 Process for producing triptane 审中-公开
标题翻译：生产triptane的过程
公开(公告)号：EP2060551A1
公开(公告)日：2009-05-20
申请号：EP07254491.9
申请日：2007-11-16
申请人： BP p.l.c.
发明人： The designation of the inventor has not yet been filed
IPC分类号： C07C2/86 , C07C9/16 , C07C11/02 , B01J29/06
CPC分类号： C07C2/865 , B01J29/06 , B01J29/082 , B01J29/084 , B01J29/123 , B01J29/126 , B01J29/143 , B01J29/146 , B01J29/40 , B01J29/44 , B01J29/46 , B01J29/70 , B01J29/7007 , B01J29/74 , B01J29/7415 , B01J29/76 , B01J29/7615 , C07C2/864 , C07C2529/08 , C07C2529/12 , C07C2529/14 , C07C2529/40 , C07C2529/44 , C07C2529/46 , C07C2529/70 , C07C2529/74 , C07C2529/76 , C07C9/16 , C07C11/02
摘要： A process for the production of triptane and/or triptene from methanol and/or one or more derivatives thereof and one or more olefins in the presence of a catalyst at a temperature in the range of from 150 to 400°C, in which the catalyst is a zeolite having Brønsted acidity and has a structure selected from:
i. Zeolites having frameworks comprising silicon and aluminium atoms and having a channel structure comprising a ring size of 12 or more non-oxygen framework atoms in 2 or 3 dimensions;
ii. Zeolites having frameworks comprising silicon and aluminium atoms and which have a framework ring comprising 12 or more non-oxygen atoms accessible on the external surface of the zeolite, and a channel structure in which all of the channels have a ring-size of less than 12 non-oxygen framework atoms,

and wherein zeolites of type (ii) comprise alkali metal where methanol is not a reactant.
摘要翻译：在催化剂存在下，在150-400℃范围内的温度下由甲醇和/或其一种或多种衍生物和一种或多种烯烃生产三癸烷和/或三萜的方法，其中催化剂是具有布朗斯台德酸性并具有选自以下的结构的沸石：i。具有包含硅和铝原子并且具有包含12或更多个2维或3维的非氧骨架原子的环尺寸的通道结构的骨架的沸石; II。具有包含硅和铝原子的骨架并且具有包含可在沸石的外表面上获得的12个或更多个非氧原子的骨架环的沸石以及其中所有通道的环尺寸均小于12的通道结构非氧骨架原子，并且其中类型（ii）的沸石包含碱金属，其中甲醇不是反应物。

96. 发明公开

EP2038059A1 TREATMENT OF CHA-TYPE MOLECULAR SIEVES AND THEIR USE IN THE CONVERSION OF OXYGENATES TO OLEFINS 审中-公开
标题翻译： THE CHA分子筛TYPE治疗和它们在含氧物至烯烃的转化
公开(公告)号：EP2038059A1
公开(公告)日：2009-03-25
申请号：EP07776686.3
申请日：2007-05-01
申请人： Exxonmobil Chemical Patents Inc. A Corporation Of The State Of Delaware
发明人： CAO, Guang , SHAH, Matu, J.
IPC分类号： B01J29/70 , B01J37/10 , C01B39/00 , C10G3/00 , C07C1/20
CPC分类号： C01B39/46 , B01J29/7015 , B01J37/10 , B01J2229/24 , B01J2229/36 , C01B39/026 , C01B39/48 , C07C1/20 , C07C2529/70 , C10G3/49 , C10G3/62 , C10G2300/807 , C10G2400/20 , Y02P30/20 , C07C11/02
摘要： A method is disclosed of treating a crystalline material comprising a CHA framework-type molecular sieve, wherein said crystalline material has a composition and involving the molar relationship: (n)X2O3:YO2, where X is a trivalent element, Y is a tetravalent element, and n is less than 0.07, and wherein the crystalline material does not comprise a silicoaluminophosphate, is substantially free of framework phosphorus, or both. The method can comprise treating the crystalline material with steam under conditions such that the prime olefin selectivity of the treated material in an oxygenate conversion process is greater than the prime olefin selectivity of the untreated material in the same process.

97. 发明公开

EP2032245A1 REAKTOR ZUR HERSTELLUNG VON C2- BIS C8- OLEFINEN AUS EINEM OXYGENAT, WASSERDAMPF UND EINEN ODER MEHRERE KOHLENWASSERSTOFFE ENTHALTENDEM STOFFSTROM 有权转让
标题翻译：反应器用于由含氧，蒸汽C2-C8烯烃和一种或多种烃材料包含电源
公开(公告)号：EP2032245A1
公开(公告)日：2009-03-11
申请号：EP07724448.1
申请日：2007-04-21
申请人： Lurgi AG
发明人： BACH, Hermann , BREHM, Lothar , BOHLE, Jürgen , QUASS, Gunter , HEINZ, Günther , BARTELS, Katja , DÖRR, Heinrich , KÖMPEL, Harald
IPC分类号： B01J8/04 , C07C1/20 , C07C11/06
CPC分类号： B01J8/0496 , B01J4/002 , B01J8/0453 , B01J8/0492 , B01J19/26 , B01J19/30 , B01J19/32 , B01J2208/00176 , B01J2208/00212 , B01J2208/00362 , B01J2208/00663 , B01J2208/00672 , B01J2208/00805 , B01J2208/00814 , B01J2208/00884 , B01J2208/025 , B01J2219/185 , B01J2219/1943 , B01J2219/30207 , B01J2219/30416 , B01J2219/32286 , C07C1/20 , C07C2529/40 , C07C2529/70 , F28D9/00 , Y02P30/42 , C07C11/06 , C07C11/02
摘要： The invention relates to a reactor for the production of C2 to C8 olefins from gaseous oxygenate and H2O and one or more material flows containing C2 C4, C5, C6, C7, C8 olefin and paraffin at 400° to 470° C, wherein several reaction stages which the material flow can pass through from the top to the bottom, each consisting of a support base with a catalyst layer situated on it, are arranged in a closed, upright container. In order to be able in each case to lower the temperature of the reaction mixture leaving the reaction stages before it enters into the next reaction stage, it is provided that each support base consists of cells which are placed closely next to each other with no gaps and which are securely attached to each other and filled with catalyst, and in the space formed by two neighboring reaction stages, respectively, an assembly of nozzle tubes is installed for spraying a liquid phase containing H2O and DME and/or MEOH, using a water-saturated gas phase containing mainly DME and/or MEOH, in the direction of the following reaction stage downstream.

98. 发明公开

EP1968919A4 DILUTE LIQUID PHASE ALKYLATION 审中-公开
标题翻译：稀释的液体相
公开(公告)号：EP1968919A4
公开(公告)日：2009-01-21
申请号：EP07716344
申请日：2007-01-05
申请人： FINA TECHNOLOGY
发明人： BUTLER JAMES R
IPC分类号： C07C2/64
CPC分类号： C07C2/66 , C07C2523/10 , C07C2529/08 , C07C2529/70 , C07C15/073
摘要： Methods of forming ethylbenzene are described herein. In one embodiment, the method includes contacting dilute ethylene with benzene in the presence of an alkylation catalyst to form ethylbenzene, wherein such contact occurs in a liquid phase reaction zone and recovering ethylbenzene from the reaction zone.

99. 发明公开

EP1659096A3 Improved zeolites and molecular sieves and the use thereof 审中-公开
标题翻译：沸石，分子筛和其用途
公开(公告)号：EP1659096A3
公开(公告)日：2009-01-07
申请号：EP06002100.3
申请日：2001-10-19
申请人： ABB LUMMUS GLOBAL INC.
发明人： Overbeek, Rudolf A. , Van der Puil, Nelleke , Chang, Yun-Feng , Angevine, Philip Jay , Koegler, Johannes, Hendrik , Yeh, Chuen Y. , Murrell, Lawrence L.
IPC分类号： C01B39/26 , C01B39/42 , C01B39/48 , B01J29/04 , C10G45/64 , C10G47/16 , C07C5/22 , C07C2/66 , C07B37/02
CPC分类号： C01B39/48 , B01J29/18 , B01J29/7007 , B01J29/7034 , B01J35/002 , B01J37/08 , B01J2229/64 , C01B39/265 , C01B39/42 , C07C2/66 , C07C2529/18 , C07C2529/40 , C07C2529/70 , C10G29/20 , C10G45/64 , C07C15/073
摘要： This invention relates to a process for producing a zeolite wherein said process includes removal of an organic templating agent, the improvement comprising: removing said templating agent at a temperature of no greater than 550°C and under conditions wherein after the removal of the templating agent, said zeolite has an AAI of at least 1.2 and is selected from the group consisting of zeolite Beta, TEA-mordenite, and TEA-ZSM-12.

100. 发明公开

EP1965914A1 CATALYSEUR COMPRENANT UNE ZEOLITHE EUO, UNE ZEOLITHE 10 MR ET UNE ZEOLITHE 12 MR ET SON UTILISATION EN ISOMERISATION DES COMPOSES C8 AROMATIQUES 有权
标题翻译：催化剂，其包含EUO沸石，10-MR沸石和12-MR沸石及其USE IN C8芳族化合物的异构化
公开(公告)号：EP1965914A1
公开(公告)日：2008-09-10
申请号：EP06841855.7
申请日：2006-12-01
申请人： Institut Français du Pétrole
发明人： GUILLON, Emmanuelle , SANCHEZ, Eric , LACOMBE, Sylvie
IPC分类号： B01J29/80 , C07C5/27
CPC分类号： B01J29/80 , B01J29/084 , B01J29/126 , B01J29/18 , B01J29/22 , B01J29/40 , B01J29/44 , B01J29/70 , B01J29/7007 , B01J29/74 , B01J29/7415 , B01J2229/186 , B01J2229/20 , B01J2229/37 , B01J2229/42 , C07C5/2708 , C07C2529/08 , C07C2529/18 , C07C2529/70 , C07C2529/80 , C07C2529/88 , Y02P20/52 , C07C15/08
摘要： A catalyst is described, comprising at least one zeolite of EUO structural type, at least one zeolite exhibiting channels whose aperture is defined by a ring with 10 oxygen atoms (10 MR), at least one zeolite exhibiting channels whose aperture is defined by a ring with 12 oxygen atoms (12 MR) and at least one porous mineral matrix. Said catalyst optionally contains in addition at least one metal from group VIII. The catalyst according to the invention is used in an isomerisation process for a charge comprising aromatic compounds with 8 carbon atoms per molecule.

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