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1. 发明授权

US5036111A Expanded materials with nadimide resin base 失效
标题翻译：膨胀材料与纳迪尔树脂基体
公开(公告)号：US5036111A
公开(公告)日：1991-07-30
申请号：US597666
申请日：1990-10-17
申请人： Michel Senneron , Gilbert Parrain , Guy Rabilloud , Bernard Sillion
发明人： Michel Senneron , Gilbert Parrain , Guy Rabilloud , Bernard Sillion
IPC分类号： C08G65/48 , C08G73/10 , C08J9/02 , C08L67/00 , C08L67/02 , C08L71/12 , C08L77/00 , C08L79/08 , C08L81/00 , C08L81/06
CPC分类号： C08J9/02 , C08G73/101 , C08L79/085 , C08J2379/08
摘要： Expanded material obtained by heating a composition comprising at least onehermosetting nadimide resin, said heating being performed at a temperature and during a period which are sufficient to cause the expansion of said composition by release of cyclopentadiene. A nadimide resin of the polyimide type and having a number average molecular weight of 600 to 10,000 is preferably used. The composition further comprises preferably 1% to 50% by weight of a linear, preferably thermostable polymer.
摘要翻译：通过加热包含至少一种热固性nadimide树脂的组合物获得的膨胀材料，所述加热在足以通过释放环戊二烯而使所述组合物膨胀的温度和时间内进行。优选使用数均分子量为600〜10000的聚酰亚胺型纳米二酰亚胺树脂。组合物还优选包含1重量％至50重量％的线性，优选热稳定性聚合物。

2. 发明授权

US5093202A Method of gluing substrates using a composition comprising an arylaliphatic copolyimide with ether chain formations and an epoxy resin 失效
标题翻译：使用包含ARYLALIPHATIC COPOLYIMIDE与醚链和环氧树脂的组合物制备基材的方法
公开(公告)号：US5093202A
公开(公告)日：1992-03-03
申请号：US561999
申请日：1990-08-02
申请人： Paul Mariaggi , Serge Gonzalez , Guy Rabilloud , Bernard Sillion
发明人： Paul Mariaggi , Serge Gonzalez , Guy Rabilloud , Bernard Sillion
IPC分类号： B32B15/08 , C08G59/00 , C08G59/40 , C08G73/10 , C08L63/00 , C08L79/08 , C09J5/00 , C09J5/06 , C09J179/08
CPC分类号： C09J179/08 , C08G73/1042 , C08G73/105 , C08L63/00 , C08L79/08 , Y10T428/31515 , Y10T428/31522
摘要： Adhesive compositions are described comprising at least an arylaliphatic olyimide with ether chain formations, obtained by the polycondensation reaction of a tetracarboxylic aromatic acid or of one of its derivatives with at least two primary diamines, one of these diamines consisting of a polyether chain ending with the two amine functional groups and at least an epoxy resin possessing more than one epoxy group per molecular.These adhesive compositions can be used particularly for the gluing of films of polymers to thin metal sheets.
摘要翻译：描述了粘合剂组合物，其至少包括具有醚链形成的芳基脂族共聚酰亚胺，其通过四羧酸芳族酸或其衍生物与至少两种伯二胺的缩聚反应获得，这些二胺中的一种由结束于两个胺官能团和至少一个每分子具有多于一个环氧基团的环氧树脂。这些粘合剂组合物可以特别用于将聚合物膜粘合到薄金属片材上。

3. 发明授权

US5064934A Thermosetting polyimide schiff base resins, their preparation and their applications 失效
标题翻译：热固性聚酰亚胺席夫碱树脂，其制备及应用
公开(公告)号：US5064934A
公开(公告)日：1991-11-12
申请号：US502275
申请日：1990-04-02
申请人： Regis Mercier , Thierry Pascal , Bernard Sillion
发明人： Regis Mercier , Thierry Pascal , Bernard Sillion
IPC分类号： C07D209/48 , C08F38/00
CPC分类号： C07D209/48 , C08F38/00
摘要： Thermosetting Schiff base resins, their preparation and their applicationsre described.These thermosetting Schiff base resins can be defined as responding to the general formula: ##STR1## Radicals Ar.sub.1, Ar.sub.2 and Ar.sub.3 are chosen so that the softening temperature of the resins is less than about 150.degree. C.The resins can be prepared by direct condensation of an ethynyl benzaldehyde or acetophenone on a telechelic diamine oligomer obtained by reaction of a diamine containing flexibilizing groups on a derivative of benzhydrol tetracarboxylic acid. These Schiff base resins can be used by bulk thermal polymerization particularly to prepare adhesives or composite matrices.
摘要翻译：描述了热固性席夫碱树脂及其制备及其应用。这些热固性希夫碱树脂可以定义为响应于以下通式：选择Ar1，Ar2和Ar3的自由基，使得树脂的软化温度低于约150℃。树脂可以通过直接冷凝通过在二苯甲醇四羧酸的衍生物上使含有柔性基团的二胺反应得到的遥爪二胺低聚物上的乙炔基苯甲醛或苯乙酮。这些席夫碱树脂可以通过本体热聚合使用，特别是制备粘合剂或复合基质。

4. 发明授权

US4931541A Thermosetting quinazolone resins their preparation and their applications 失效
标题翻译：热固性喹唑啉酮树脂的制备及应用
公开(公告)号：US4931541A
公开(公告)日：1990-06-05
申请号：US313679
申请日：1989-02-22
申请人： Regis Mercier , Bernard Sillion
发明人： Regis Mercier , Bernard Sillion
IPC分类号： C07D239/91 , C08F38/00 , C08F138/00 , C08G73/06
CPC分类号： C08G73/0694 , C08F38/00
摘要： Thermosetting quinazolone resins, their preparation and their applicationsre described.These thermosetting quinazolone resins can be defined as having the following general formula: ##STR1## in which Ar.sup.1 is a bivalent mono- or polycyclic aromatic radical and Ar.sup.2 is a bivalent aromatic radical of several simple aromatic rings bound two by two by atoms or bivalent groups.These Ar.sup.1 and Ar.sup.2 radicals are chosen so that the melting or emollescence temperature is between 80.degree. C. and 170.degree. C.The resins can be prepared from condensation of an ethynylarylbenzoxazinone with an aromatic diamine containing flexibilizing groups.These quinazolone resins can be polymerized in bulk in order to prepare adhesives or composite matrices in particular.
摘要翻译：热固性喹唑啉酮树脂及其制备方法及应用。这些热固性喹唑啉酮树脂可以定义为具有以下通式：其中Ar1是二价单环或多环芳族基团，Ar2是几个由原子或二价基团键合的两个简单芳环的二价芳族基团。选择这些Ar1和Ar2基团，使得熔融或发泡温度在80℃和170℃之间。树脂可以由乙炔基芳基苯并恶嗪酮与含有柔性基团的芳族二胺的缩合制备。这些喹唑啉酮树脂可以大量聚合，以便制备粘合剂或复合基质。

5. 发明授权

US4814403A Oligomer compositions of polyaryloxypyridines with acetylenic end groups, their manufacture and lattices obtained by thermal polymerization thereof 失效
标题翻译：具有炔末端基的聚芳氧基吡啶的低聚物组合物，其制备和通过其热聚合获得的晶格
公开(公告)号：US4814403A
公开(公告)日：1989-03-21
申请号：US105745
申请日：1987-10-08
申请人： Annie Dussart-Lermusiaux , Michel Senneron , Guy Rabilloud , Bernard Sillion
发明人： Annie Dussart-Lermusiaux , Michel Senneron , Guy Rabilloud , Bernard Sillion
IPC分类号： C07D213/63 , C07D213/64 , C07D213/643 , C07F7/08 , C08F38/00 , C08F290/00 , C08F299/00 , C08G65/40 , C08G65/48 , C08F26/06
CPC分类号： C07D213/643 , C07F7/0812 , C08G65/4006 , C08G65/48 , C08G2650/48 , C08G2650/60
摘要： Oligomer compositions of polyaryloxypyridine with acetylenic end groups arebtained by formation of an oligomer composition of polyaryloxypyridine with halogenated end groups from an alkaline diphenolate and a dihalogenopyridine, followed with an ethynylation reaction. The average polycondensation degree may range from 1 to 50. Theses compositions can be used to form cross-linked lattices by polyaddition of the ethynyl groups.
摘要翻译：具有炔末端基的聚芳氧基吡啶的低聚物组成通过由碱式二酚盐和二卤代吡啶形成具有卤化端基的聚芳氧基吡啶的低聚物组合物，然后进行乙炔化反应而获得。平均缩聚度可以在1至50之间。这些组合物可用于通过乙炔基的加成形成交联晶格。

6. 发明授权

US4645821A Precursor of copolyphthalocyanine-imide lattice, preparation, and the resultant lattice 失效
标题翻译：共聚酞菁 - 酰亚胺晶格的前体，制备和所得的晶格
公开(公告)号：US4645821A
公开(公告)日：1987-02-24
申请号：US758949
申请日：1985-07-25
申请人： Jean Malinge , Guy Rabilloud , Bernard Sillion
发明人： Jean Malinge , Guy Rabilloud , Bernard Sillion
IPC分类号： C08G73/00 , C07D209/48 , C08G73/10 , C08G73/06
CPC分类号： C07D209/48 , C08G73/10 , C08G73/1035
摘要： Aromatic polyimide compositions, precursors of copolyphthalocyanine-imides,heir manufacturing process and the resultant copolyphthalocyanine-imides, are described.These compositions may result for the reaction of 80.degree.-300.degree. C. of an aromatic tetra acid, diester-diacid, tetraester or dianhydride compound of formula: ##STR1## with an aromatic amino-dinitrile ##STR2## and optionally an aromatic diamine NH.sub.2 --Ar--NH.sub.2. A subsequent heating at 200.degree.-300.degree. C. provides, by cross-linking, copolyphthalocyanine-imides, which are hardened resins, stable at 250.degree.-300.degree. C. in continuous use.
摘要翻译：描述了芳族聚酰亚胺组合物，共聚酞菁 - 酰亚胺的前体，它们的制备方法和所得的共聚酞菁 - 酰亚胺。这些组合物可能导致80-300℃的芳香族四酸，二酯 - 二酸，四酯或二酐化合物与芳香族氨基二腈和任选的芳族二胺NH 2 -Ar-NH2。随后在200-300℃下加热，通过交联，共聚酞菁 - 酰亚胺，它们是硬化树脂，在250-300℃下连续使用时稳定。

7. 发明授权

US5104968A Polyimide precursor composition and application therefrom 失效
标题翻译：聚酰亚胺前体组合物及其应用
公开(公告)号：US5104968A
公开(公告)日：1992-04-14
申请号：US564236
申请日：1990-08-08
申请人： Serge Gonzalez , Paul Mariaggi , Guy Rabilloud , Bernard Sillion
发明人： Serge Gonzalez , Paul Mariaggi , Guy Rabilloud , Bernard Sillion
IPC分类号： C08G73/10 , C09D5/25 , H01B3/30
CPC分类号： C08G73/1003 , C08G73/1007 , C08G73/1042 , H01B3/306 , Y10T428/31504
摘要： Polyimide precursor compositions incorporating at least one compound of fula (1), at least one compound of formula (2), at least one compound of formula (3) and at least one compound of formula (4) ##STR1## in which one of the groups R.sup.3 and R.sup.4 represents a hydrogen atom and the other, in the same way as the groups R.sup.1 and R.sup.2, which can be the same or different, in each case represent a hydrocarbon group having 1 to 16 carbon atoms, m is a number between 5 and 20, n is an integer between 1 and 5 and R.sup.5 represents a hydrogen atom, a halogen atom, a hydrocarbon group with 1 to 16 carbon atoms, or a group of formula R.sup.6 --O-- in which R.sup.6 represents a hydrocarbon group having 1 to 16 carbon atoms. The preferred composition contains 30 to 70% by weight of dry matter of compounds of formulas (1), (2) and (3), in which the groups R.sup.1, R.sup.2 and one of the groups R.sup.3 and R.sup.4 is a methyl or ethyl group and the compound of formula (4) is benzyl alcohol. These compositions are usable as smoothing and/or protective coatings for metals, metal alloys or other substrates and in particular in the electrical and electronic industries, e.g. for the formation of dielectric films.
摘要翻译：引入至少一种式（1）化合物，至少一种式（2）化合物，至少一种式（3）化合物和至少一种式（4）化合物的聚酰亚胺前体组合物图像（2）（3）（4）其中R3和R4中的一个代表氢原子，另一个与R1和R2基团相同，可以相同或者不同，在每种情况下都表示具有1至16个碳原子的烃基，m是5至20之间的数，n是1和5之间的整数，R 5表示氢原子，卤素原子，具有1个至16个碳原子的基团，或其中R 6表示具有1至16个碳原子的烃基的式R6-O-基团。优选的组合物包含30至70重量％的式（1），（2）和（3）化合物的干物质，其中基团R 1，R 2和基团R 3和R 4中的一个是甲基或乙基并且式（4）的化合物是苄醇。这些组合物可用作金属，金属合金或其它基材的平滑和/或保护涂层，特别是在电气和电子工业中。用于形成介电膜。

8. 发明授权

US4764578A Compositions of polyaryloxypyridine oligomers with phthalonitrile end groups, their preparation and use for manufacturing polyaryloxypyridine co-phthalocyanine lattices 失效
标题翻译：具有邻苯二甲腈端基的聚芳氧基吡啶低聚物的组成及其制备和用于制备聚芳氧基吡啶共酞菁晶格
公开(公告)号：US4764578A
公开(公告)日：1988-08-16
申请号：US907905
申请日：1986-09-16
申请人： Jean Malinge , Guy Rabilloud , Bernard Sillion
发明人： Jean Malinge , Guy Rabilloud , Bernard Sillion
IPC分类号： C08G65/40 , C08G65/48 , C08G73/06 , C08G83/00 , C08G73/00
CPC分类号： C08G65/48 , C08G65/4006 , C08G73/0627 , C08G2650/64
摘要： The disclosed compositions of polyaryloxypyridine oligomers with phthalonile end groups are obtained by formation of a composition of polyaryloxypyridine oligomers with alkali phenolate end groups, followed with the reaction of said composition with 4-nitrophthalonitrile. Their average polycondensation degree may range from 1 to 50. They can be used in combination with a co-reactant derived from benzhydrol and containing one or two ortho-dinitrile functional groups, to constitute polyaryloxypyridine co-polyphthalocyanine lattices.
摘要翻译：所公开的具有邻苯二甲腈端基的聚芳氧基吡啶低聚物的组合物通过用碱性酚盐端基形成聚芳氧基吡啶低聚物的组合物，随后将所述组合物与4-硝基邻苯二腈反应而获得。它们的平均缩聚度可以在1至50之间。它们可以与衍生自二苯甲醛并含有一个或两个邻二甲苯基官能团的共反应物组合使用，以构成聚芳氧基吡啶共聚酞菁晶格。

9. 发明授权

EP0170591B1 Procédé de préparation de compositions de précurseurs de polyimides 失效
标题翻译：制备聚酰亚胺前体组合物的方法
公开(公告)号：EP0170591B1
公开(公告)日：1989-04-05
申请号：EP85401502.1
申请日：1985-07-22
申请人： CENTRE D'ETUDE DES MATERIAUX ORGANIQUES POUR TECHNOLOGIES AVANCEES
发明人： Rabilloud, Guy , Mariaggi, Paul , Gonzalez, Serge , Sillion, Bernard
IPC分类号： C08G73/10 , H01B3/30
CPC分类号： C08G73/1067 , C08G73/1042 , H01B3/306

10. 发明授权

EP0424224B1 Matériaux expansés à base de résine nadimide 失效
标题翻译：基于Nadimidharz发泡材料。
公开(公告)号：EP0424224B1
公开(公告)日：1995-01-04
申请号：EP90402862.8
申请日：1990-10-12
申请人： CENTRE D'ETUDE DES MATERIAUX ORGANIQUES POUR TECHNOLOGIES AVANCEES
发明人： Senneron, Michel , Parrain, Gilbert , Rabilloud, Guy , Sillion, Bernard
IPC分类号： C08J9/02 , C08L79/08 , C08G73/12
CPC分类号： C08J9/02 , C08G73/101 , C08J2379/08 , C08L79/085 , C08L79/08 , C08L2666/22 , C08L81/00 , C08L2666/14

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