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1. 发明授权

US5883188A Paintable olefinic interpolymer compositions 失效
标题翻译：可涂漆烯烃互聚物组合物
公开(公告)号：US5883188A
公开(公告)日：1999-03-16
申请号：US926760
申请日：1997-09-10
申请人： Yuh-Chin Hwang , Stephen R. Betso , Thomas J. McKeand, Jr. , H. Craig Silvis , Deepak R. Parikh , Don J. Germano , Seema V. Karande
发明人： Yuh-Chin Hwang , Stephen R. Betso , Thomas J. McKeand, Jr. , H. Craig Silvis , Deepak R. Parikh , Don J. Germano , Seema V. Karande
IPC分类号： C08L51/06 , C08L51/00
CPC分类号： C08L51/06 , Y10T428/31938
摘要： Paintable thermoplastic polyolefin compositions are disclosed which comprise (i) about 20 to about 70 wt % of at least one graft-modified polypropylene, (ii) about 10 to about 40 wt % of at least one nongrafted or graft-modified homogeneously branched linear ethylene polymer, ethylene-propylene monomer rubber, ethylene-propylene-diene monomer rubber, heterogeneously branched linear ethylene polymer, styrene block copolymer, or a combination thereof and (iii) about 5 to about 50 wt % of an interpolymer of ethylene and an .alpha.,.beta.-unsaturated carbonyl copolymer, e.g. a copolymer of ethylene and acrylic acid. The polypropylene and, optionally the homogeneously branched linear ethylene polymer, ethylene-propylene monomer rubber, ethylene-propylene-diene monomer rubber, heterogeneously branched linear ethylene polymer, and styrene block copolymer are grafted with an unsaturated organic compound containing at least one site of ethylenic unsaturation and at least one carbonyl group, e.g. maleic anhydride. The compositions exhibit excellent paintability with conventional paints without prior application of a primer or surface treatment, good heat resistance, good low temperature impact resistance, and they can be recycled by melt blending the compositions with thermoplastic materials, e.g., in an extruder.
摘要翻译：公开了可涂覆的热塑性聚烯烃组合物，其包含（i）约20至约70重量％的至少一种接枝改性聚丙烯，（ii）约10至约40重量％的至少一种未接枝或接枝改性的均匀支化的线型乙烯聚合物，乙烯 - 丙烯单体橡胶，乙烯 - 丙烯 - 二烯单体橡胶，非均匀支化的线性乙烯聚合物，苯乙烯嵌段共聚物或其组合，和（iii）约5-约50wt％的乙烯和α的互聚物， β-不饱和羰基共聚物，例如乙烯和丙烯酸的共聚物。聚丙烯和任选的均匀支化的线性乙烯聚合物，乙烯 - 丙烯单体橡胶，乙烯 - 丙烯 - 二烯单体橡胶，非均匀支化的线性乙烯聚合物和苯乙烯嵌段共聚物用含有至少一个烯属的位点的不饱和有机化合物不饱和键和至少一个羰基，例如马来酸酐。组合物在常规涂料中表现出优异的可涂色性，而无需预先施用底漆或表面处理，良好的耐热性，良好的低温耐冲击性，并且它们可以通过将组合物与热塑性材料（例如在挤出机中）熔融共混来再循环。

2. 发明授权

US5424362A Paintable olefinic interpolymer compositions 失效
标题翻译：可涂漆烯烃互聚物组合物
公开(公告)号：US5424362A
公开(公告)日：1995-06-13
申请号：US54384
申请日：1993-04-28
申请人： Yuh-Chin Hwang , Thomas J. McKeand, Jr. , Stephen R. Betso , H. Craig Silvis , Deepak R. Parikh , Don J. Germano
发明人： Yuh-Chin Hwang , Thomas J. McKeand, Jr. , Stephen R. Betso , H. Craig Silvis , Deepak R. Parikh , Don J. Germano
IPC分类号： B60K37/00 , B29C43/02 , B29C45/00 , B29C47/00 , B29K23/00 , C08F255/00 , C08F255/02 , C08J5/00 , C08L23/00 , C08L23/08 , C08L23/10 , C08L23/12 , C08L51/00 , C08L51/06 , C09D151/06
CPC分类号： C08F255/02 , C08F255/00 , C08L23/12 , C08L51/06 , C09D151/06 , C08L2205/02 , C08L2205/03 , C08L23/0815 , C08L23/0846 , C08L23/0869 , Y10T428/31938
摘要： Paintable thermoplastic polyolefin compositions are disclosed which comprise (i) 30 to about 70 wt % of at least one polypropylene or graft-modified polypropylene, (ii) 0 to about 40 wt % of at least one nongrafted or graft-modified substantially linear ethylene polymer, and (iii) 0 to about 50 wt % of an interpolymer of ethylene and an .alpha.,.beta.-unsaturated carbonyl copolymer, e.g. a copolymer of ethylene and acrylic acid. The polypropylene and substantially linear ethylene polymer are grafted with an unsaturated organic compound containing at least on ethylenic unsaturation and at least one carbonyl group, e.g. maleic anhydride. The compositions exhibit excellent paintability with conventional paints without prior application of a primer or surface treatment, good heat resistance, and good low temperature impact resistance and they can be recycled by melt blending the compositions with thermoplastic materials, e.g., in an extruder.
摘要翻译：公开了可涂覆的热塑性聚烯烃组合物，其包含（i）30至约70重量％的至少一种聚丙烯或接枝改性聚丙烯，（ii）0至约40重量％的至少一种未接枝或接枝改性的基本线性的乙烯聚合物，和（iii）0至约50wt％的乙烯和α，β-不饱和羰基共聚物的互聚物，例如乙烯和丙烯酸的共聚物。聚丙烯和基本上线性的乙烯聚合物用至少含有不饱和键和不少于一个羰基的不饱和有机化合物接枝。马来酸酐。该组合物在常规涂料中表现出优异的可涂色性，而无需预先施用底漆或表面处理，良好的耐热性和良好的低温耐冲击性，并且它们可以通过将组合物与热塑性材料（例如在挤出机中）熔融共混来再循环。

3. 发明授权

US5681897A Impact modification of thermoplastics 失效
标题翻译：热塑性塑料的冲击改性
公开(公告)号：US5681897A
公开(公告)日：1997-10-28
申请号：US468695
申请日：1995-06-06
申请人： H. Craig Silvis , Daniel J. Murray , Thomas R. Fiske , Stephen R. Betso , Robert R. Turley
发明人： H. Craig Silvis , Daniel J. Murray , Thomas R. Fiske , Stephen R. Betso , Robert R. Turley
IPC分类号： C08L23/00 , C08L23/08 , C08L23/10 , C08L23/12 , C08L23/14 , C08L23/16 , C08L25/00 , C08L27/06 , C08L75/00 , C08L75/04 , C08L101/00 , C08F8/00
CPC分类号： C08L23/0815 , B60C19/002 , C08L101/00 , C08L23/10 , C08L23/12 , C08L2314/06 , Y10S138/07
摘要： Compositions having good low temperature impact performance made from a thermoplastic (e.g., a polyolefin such as polypropylene) and either at least one linear ethylene/C.sub.5 -C.sub.20 .alpha.-olefin or at least one substantially linear ethylene/C.sub.3 -C.sub.20 .alpha.-olefin polymer are disclosed. The compositions are easily molded and have particular utility in making automotive facia, parts and other household articles.
摘要翻译：具有由热塑性塑料（例如聚烯烃如聚丙烯）和至少一种直链乙烯/ C5-C20α-烯烃或至少一种基本上线性的乙烯/ C 3 -C 20α-烯烃聚合物制成的良好低温冲击性能的组合物是披露组合物易于模塑，并且在制造汽车面板，零件和其它家用制品方面具有特别的用途。

4. 发明授权

US5856406A Impact modification of thermoplastics 失效
标题翻译：热塑性塑料的冲击改性
公开(公告)号：US5856406A
公开(公告)日：1999-01-05
申请号：US980142
申请日：1997-11-26
申请人： H. Craig Silvis , Daniel J. Murray , Thomas R. Fiske , Stephen R. Betso , Robert R. Turley
发明人： H. Craig Silvis , Daniel J. Murray , Thomas R. Fiske , Stephen R. Betso , Robert R. Turley
IPC分类号： C08L23/00 , C08L23/08 , C08L23/10 , C08L23/12 , C08L23/14 , C08L23/16 , C08L25/00 , C08L27/06 , C08L75/00 , C08L75/04 , C08L101/00
CPC分类号： C08L23/0815 , B60C19/002 , C08L101/00 , C08L23/10 , C08L23/12 , C08L2314/06 , Y10S138/07
摘要： Compositions having good low temperature impact performance made from a thermoplastic (e.g., a polyolefin such as polypropylene) and either at least one linear ethylene/C.sub.5 -C.sub.20 .alpha.-olefin or at least one substantially linear ethylene/C.sub.3 -C.sub.20 .alpha.-olefin polymer are disclosed. The compositions are easily molded and have particular utility in making automotive facia, parts and other household articles.
摘要翻译：具有由热塑性塑料（例如聚烯烃如聚丙烯）和至少一种直链乙烯/ C5-C20α-烯烃或至少一种基本上线性的乙烯/ C 3 -C 20α-烯烃聚合物制成的良好低温冲击性能的组合物是披露组合物易于模塑，并且在制造汽车面板，零件和其它家用制品方面具有特别的用途。

5. 发明授权

US5688866A Impact modification of theremoplastics 失效
标题翻译：冲击改性塑料
公开(公告)号：US5688866A
公开(公告)日：1997-11-18
申请号：US469300
申请日：1995-06-06
申请人： H. Craig Silvis , Daniel J. Murray , Thomas R. Fiske , Stephen R. Betso , Robert R. Turley
发明人： H. Craig Silvis , Daniel J. Murray , Thomas R. Fiske , Stephen R. Betso , Robert R. Turley
IPC分类号： C08L23/00 , C08L23/08 , C08L23/10 , C08L23/12 , C08L23/14 , C08L23/16 , C08L25/00 , C08L27/06 , C08L75/00 , C08L75/04 , C08L101/00 , C08F8/30
CPC分类号： C08L23/0815 , B60C19/002 , C08L101/00 , C08L23/10 , C08L23/12 , C08L2314/06 , Y10S138/07
摘要： Compositions having good low temperature impact performance made from a thermoplastic (e.g., a polyolefin such as polypropylene) and either at least one linear ethylene/C.sub.5 -C.sub.20 .alpha.-olefin or at least one substantially linear ethylene/C.sub.3 -C.sub.20 .alpha.-olefin polymer are disclosed. The compositions are easily molded and have particular utility in making automotive facia, parts and other household articles.
摘要翻译：具有由热塑性塑料（例如聚烯烃如聚丙烯）和至少一种直链乙烯/ C5-C20α-烯烃或至少一种基本上线性的乙烯/ C 3 -C 20α-烯烃聚合物制成的良好低温冲击性能的组合物是披露组合物易于模塑，并且在制造汽车面板，零件和其它家用制品方面具有特别的用途。

6. 发明授权

US08288470B2 Polyolefin compositions and articles prepared therefrom, and methods for making the same 有权
标题翻译：聚烯烃组合物及其制备的制品及其制备方法
公开(公告)号：US08288470B2
公开(公告)日：2012-10-16
申请号：US12520380
申请日：2007-12-21
申请人： Patricia Ansems , Ashish Batra , Laura Bauerle Weaver , Lawrence J. Effler , H. Craig Silvis , Hamed Lakrout , Laura K. Mergenhagen
发明人： Patricia Ansems , Ashish Batra , Laura Bauerle Weaver , Lawrence J. Effler , H. Craig Silvis , Hamed Lakrout , Laura K. Mergenhagen
IPC分类号： C08G63/48 , C08J3/22 , C08K3/34 , C08F8/00 , C08F32/00 , C08F132/00 , C08F232/00 , C08F8/32 , C08C19/22
CPC分类号： C08L51/06 , B32B27/08 , B32B27/32 , C08F8/32 , C08F10/00 , C08F255/00 , C08F255/02 , C08F287/00 , C08L23/36 , C08L51/00 , C08L51/003 , C08L51/006 , C08L53/00 , C08L75/04 , C08L2205/02 , C08L2666/02 , C08L2666/04 , C08L2666/06 , C08L2666/14 , C08L2666/20 , C08L2666/24
摘要： The invention provides a composition comprising at least one olefin multi-block interpolymer; at least one functionalized olefin-based polymer; and optionally at least one thermoplastic polyurethane. The invention also provides for articles prepared from the inventive compositions and for methods for making the same.
摘要翻译：本发明提供包含至少一种烯烃多嵌段互聚物的组合物; 至少一种官能化烯烃基聚合物; 和任选的至少一种热塑性聚氨酯。本发明还提供了由本发明组合物制备的制品及其制备方法。

7. 发明授权

US06777502B2 Rheology modification of polymers prepared using metallocenes 有权
标题翻译：使用金属茂制备的聚合物的流变改性
公开(公告)号：US06777502B2
公开(公告)日：2004-08-17
申请号：US10347713
申请日：2003-01-21
申请人： Thoi H. Ho , Wendy D. Hoenig , Che-l Kao , Michael E. Rowland , Clark H. Cummins , Michael J. Mullins , H. Craig Silvis
发明人： Thoi H. Ho , Wendy D. Hoenig , Che-l Kao , Michael E. Rowland , Clark H. Cummins , Michael J. Mullins , H. Craig Silvis
IPC分类号： C08C1900
CPC分类号： C08L23/02 , C08G81/02 , C08K5/43 , C08L23/04 , C08L23/06 , C08L23/08 , C08L23/0815 , C08L23/0838 , C08L23/0853 , C08L23/16 , C08L2205/22 , C08L2312/00 , C08L2314/06 , Y10T428/1334 , Y10T428/1352 , Y10T428/1386 , Y10T428/139 , Y10T428/31913 , Y10T428/31917 , C08L2666/04
摘要： Coupled polymers are prepared by a process comprising heating an admixture containing (1) at least one polyolefin comprising ethylene and optionally at least one comonomer and (2) a coupling amount at least one poly(sulfonyl azide) to at least the decomposition temperature of the poly(sulfonyl azide) for a period sufficient for decomposition of at least 80 weight percent of the poly(sulfonyl azide) and sufficient to result in a coupled polymer; particularly where the polyolefin is the product of polymerization of ethylene and optionally at least one other alpha-olefin in the presence of a single site catalyst.
摘要翻译：通过包括加热含有（1）至少一种包含乙烯和任选的至少一种共聚单体的聚烯烃和（2）偶联量的至少一种聚（磺酰基叠氮化物）的聚烯烃至少至少分解温度的混合物来制备偶联聚合物聚（磺酰基叠氮化物）足以分解至少80重量％的聚（磺酰基叠氮化物）并足以产生偶联聚合物的时间; 特别是当聚烯烃是在单一位点催化剂存在下乙烯和任选的至少一种其它α-烯烃聚合的产物时。

8. 发明授权

US06521306B1 Rheology modification of low density polyethylene 有权
标题翻译：低密度聚乙烯的流变改性
公开(公告)号：US06521306B1
公开(公告)日：2003-02-18
申请号：US09129163
申请日：1998-08-05
申请人： Wendy D. Hoenig , Teresa Karjala , Li-Min Tau , Clark H. Cummins , Michael J. Mullins , H. Craig Silvis , Thoi H. Ho
发明人： Wendy D. Hoenig , Teresa Karjala , Li-Min Tau , Clark H. Cummins , Michael J. Mullins , H. Craig Silvis , Thoi H. Ho
IPC分类号： B29D2200
CPC分类号： C08L23/02 , C08G81/02 , C08K5/43 , C08L23/04 , C08L23/06 , C08L23/08 , C08L23/0815 , C08L23/0838 , C08L23/0853 , C08L23/16 , C08L2205/22 , C08L2312/00 , C08L2314/06 , Y10T428/1334 , Y10T428/1352 , Y10T428/1386 , Y10T428/139 , Y10T428/31913 , Y10T428/31917 , C08L2666/04
摘要： The invention includes a process of preparing a coupled polymer characterized by heating an admixture containing (1) at least one ethylene polymer or blend of ethylene polymers having a density of at least about 0.89 g/mL and less than about 0.935 g/mL and a comonomer content between about 0.5 and 50 weight percent of an alpha olefin having greater than 2 and less than 20 carbon atoms per molecule and (2) a coupling amount of at least one poly(sulfonyl azide) to at least the decomposition temperature of the poly(sulfonyl azide) for a period sufficient for decomposition of at least about 80 weight percent of the poly(sulfonyl azide) and sufficient to result in a coupled polymer. The amount of poly(sulfonyl azide) is preferably from about 0.01 to about 5 weight percent of polymers in the admixture. The invention also includes any composition which is the product of any of the processes of the invention and articles made from those compositions, particularly any film of any composition of the invention. Additionally the invention includes a use of any composition of the invention in a process of blowing, casting or calendaring a film. More particularly the invention includes articles of compositions of the invention which are trash bags, agricultural films, construction films, or geomembranes, grocery sacks, sealant layers, tie layers, produce bags, garment bags, shipping sacks, medical films, stretch films, shrink films, agricultural films, greenhouse films, construction films, or stretch hooders.
摘要翻译：本发明包括一种制备偶联聚合物的方法，其特征在于加热含有（1）至少一种乙烯聚合物或密度为至少约0.89g / mL且小于约0.935g / mL的乙烯聚合物的共混物的混合物，共聚单体含量为约0.5至50重量％的每分子具有大于2个且小于20个碳原子的α-烯烃，和（2）至少一个聚（磺酰基叠氮化物）的偶联量至少达到聚（磺酰基叠氮化物）足以分解至少约80重量％的聚（磺酰基叠氮化物）并足够导致偶联聚合物的时间。聚（磺酰基叠氮化物）的量优选为混合物中约0.01至约5重量％的聚合物。本发明还包括任何组合物，其是本发明任何方法的产物和由这些组合物制成的制品，特别是本发明任何组合物的任何薄膜。此外，本发明包括在吹塑，浇铸或压延膜的方法中使用本发明的任何组合物。更具体地，本发明包括本发明的制品，其为垃圾袋，农用膜，建筑膜或土工膜，杂货袋，密封剂层，连接层，生产袋，服装袋，运输袋，医疗膜，拉伸膜，收缩电影，农膜，温室膜，建筑膜或拉伸罩。

9. 发明授权

US06359073B1 Process of rheology modification of polymers 有权
标题翻译：聚合物流变改性工艺
公开(公告)号：US06359073B1
公开(公告)日：2002-03-19
申请号：US09694649
申请日：2000-10-23
申请人： David A. Babb , Che-I Kao , Wendy D. Hoenig , Michael E. Rowland , Clark H. Cummins , H. Craig Silvis , Michael J. Mullins , Thoi H. Ho
发明人： David A. Babb , Che-I Kao , Wendy D. Hoenig , Michael E. Rowland , Clark H. Cummins , H. Craig Silvis , Michael J. Mullins , Thoi H. Ho
IPC分类号： C08F800
CPC分类号： C08L23/02 , C08G81/02 , C08K5/43 , C08L23/04 , C08L23/06 , C08L23/08 , C08L23/0815 , C08L23/0838 , C08L23/0853 , C08L23/16 , C08L2205/22 , C08L2312/00 , C08L2314/06 , Y10T428/1334 , Y10T428/1352 , Y10T428/1386 , Y10T428/139 , Y10T428/31913 , Y10T428/31917 , C08L2666/04
摘要： The invention includes a process of reacting a poly(sulfonyl azide) with a polymer comprising steps (a) forming a first admixture of a first amount of a first polymer or in a liquid which does not require removal from the polymer and a poly(sulfonyl azide); (b) then forming a second admixture of the first admixture with a second amount of at least one second polymer; and (c) heating the second admixture at lest to the decomposition temperature of the coupling agent for a time sufficient to result in coupling of polymer chains. The invention further includes all compositions obtainable by processes of the invention as well as blends of those compositions with one or more polymers of compositions different from the first or second polymer or the product of a process of the invention. Additionally the invention includes articles made from compositions of the invention, and shaping those articles particularly by processes which comprise shaping the compositions in a melted state into an article, more preferably when the process comprises thermoforming, injection molding, extrusion, casting, blow molding, foaming or blowing as well as the use of the compositions in those processes.
摘要翻译：本发明包括使聚（磺酰基叠氮化物）与聚合物反应的方法，包括步骤（a）形成第一量的第一聚合物的第一混合物或不需要从聚合物中除去的液体和聚（磺酰基叠氮化物）; （b）然后形成第一混合物与第二量的至少一种第二聚合物的第二混合物; 和（c）加热第二混合物至少达到偶联剂的分解温度足以导致聚合物链偶联的时间。本发明还包括可通过本发明的方法获得的所有组合物以及这些组合物与一种或多种不同于第一或第二聚合物或本发明方法的产物的组合物的一种或多种聚合物的共混物。另外，本发明包括由本发明的组合物制成的制品，并且特别通过包括将熔融状态的组合物成型成制品的方法成型那些制品，更优选当该方法包括热成型，注射成型，挤出，浇铸，吹塑成型，发泡或吹塑以及在这些方法中使用组合物。

10. 发明授权

US5112934A Epoxy polymeric nonolinear optical materials based on glycidyl amines 失效
标题翻译：基于甘氨酸的环氧聚合非线性光学材料
公开(公告)号：US5112934A
公开(公告)日：1992-05-12
申请号：US441805
申请日：1989-11-27
申请人： John J. Kester , H. Craig Silvis
发明人： John J. Kester , H. Craig Silvis
IPC分类号： G02F1/35 , C08G59/10 , C08G59/20 , C08G59/32 , C08G59/50 , G02F1/355 , G02F1/361
CPC分类号： C08G59/32 , C08G59/20 , C08G59/5033 , G02F1/3611 , G02F1/3613 , G02F1/3616
摘要： The present invention is directed to an epoxy-containing polymeric material having nonlinear optical properties, particularly a glycidyl amine polymer, and a process for making the nonlinear optical (NLO) epoxy-containing polymeric material including poling the polymeric material under high voltage at elevated temperature for a period of time to bring about orientation of the nonlinear optical functionalities in the polymer. The polymers have enhanced thermal stability and good NLO properties.

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