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1. 发明授权

US5990261A Organic optical component 失效
标题翻译：有机光学元件
公开(公告)号：US5990261A
公开(公告)日：1999-11-23
申请号：US917387
申请日：1997-08-26
申请人： Wataru Yamashita , Tomomi Yoshimura , Atsushi Shibuya , Yoshihiro Sakata , Hideaki Oikawa , Keisuke Takuma , Masahiro Ohta
发明人： Wataru Yamashita , Tomomi Yoshimura , Atsushi Shibuya , Yoshihiro Sakata , Hideaki Oikawa , Keisuke Takuma , Masahiro Ohta
IPC分类号： C08G69/42 , C08G69/12 , C08G69/32 , C08G69/40 , C08G73/10 , C08G63/00 , C08G69/26
CPC分类号： C08G69/40 , C08G69/32 , C08G73/1039
摘要： A low birefringent organic optical component prepared from a resin consisting essentially of one or more repetitive structural units selected from the group consisting of structures represented by general formula (1); ##STR1## wherein A is either of the groups below. ##STR2## The organic optical component can exhibit excellent transparency, heat resistance and mechanical strength as well as a low birefringence. Also provided is a novel aromatic polyamide with a low permitivity and excellent transparency, processability and thermal stability, besides excellent heat resistance inherent in an aromatic polyamide.
摘要翻译：由基本上由选自由通式（1）表示的结构的一个或多个重复结构单元组成的树脂制成的低双折射有机光学部件; 其中A是下面的组之一。有机光学部件可以表现出优异的透明性，耐热性和机械强度以及低双折射性。还提供了具有低介电常数和优异的透明性，加工性和热稳定性的新型芳族聚酰胺，以及芳族聚酰胺固有的优异的耐热性。

2. 发明授权

US6080833A Low-birefringent organic optical component and a spirobiindan polymer 失效
标题翻译：低双折射有机光学组件和螺二茚聚合物
公开(公告)号：US6080833A
公开(公告)日：2000-06-27
申请号：US896008
申请日：1997-07-17
申请人： Atsuo Otsuji , Keisuke Takuma , Rihoko Suzuki , Tatsuhiro Urakami , Toshihiro Motoshima , Wataru Yamashita , Tomomi Yoshimura , Atsushi Shibuya , Yoshihiro Sakata , Hideaki Oikawa , Masahiro Ohta , Masanobu Ajioka , Masatoshi Takagi , Akio Karasawa
发明人： Atsuo Otsuji , Keisuke Takuma , Rihoko Suzuki , Tatsuhiro Urakami , Toshihiro Motoshima , Wataru Yamashita , Tomomi Yoshimura , Atsushi Shibuya , Yoshihiro Sakata , Hideaki Oikawa , Masahiro Ohta , Masanobu Ajioka , Masatoshi Takagi , Akio Karasawa
IPC分类号： C08G83/00 , C08F222/10 , C08G18/32 , C08G59/17 , C08G59/24 , C08G63/193 , C08G63/672 , C08G64/06 , C08G73/10 , G11B7/243 , G11B7/253 , G11B7/2533 , G11B7/2534 , G11B7/2535 , G11B7/2536 , G11B7/257 , G11B7/2578 , G11B7/258 , G11B7/2585 , C08G64/00
CPC分类号： G11B7/2535 , C08F222/1006 , C08G18/3215 , C08G59/1466 , C08G59/245 , C08G63/193 , C08G63/672 , C08G64/06 , C08G73/105 , G11B7/2533 , G11B7/2534 , G11B2007/24304 , G11B7/2536 , G11B7/2578 , G11B7/2585
摘要： A low-birefringent organic optical component comprising a polymer prepared by polymerizing a racemic mixture of the monomer with an asymmetric spiro ring represented by general formula (1) as an essential ingredient; wherein ring A represents a monocyclic or polycyclic organic group, wherein two ring As are mutually bound each other via a spiro bond to form a spiro ring which has a molecular asymmetric structure; n is an integer of 0 to 10; X.sub.1 and Y.sub.1 are binding groups; and Z.sub.1 is a polymerization-active group. The component has excellent transparency, mechanical strength and heat resistance, as well as a low birefringence.
摘要翻译：一种低双折射有机光学元件，包括通过将单体的外消旋混合物与通式（1）表示的不对称螺环作为必要成分聚合而制备的聚合物; 其中环A表示单环或多环有机基团，其中两个环彼此通过螺键彼此相互结合以形成具有分子不对称结构的螺环; n为0〜10的整数。 X1和Y1是结合基团; Z1是聚合活性基团。该组分具有优异的透明性，机械强度和耐热性，以及低双折射。

3. 发明授权

US6103860A Fluorine-containing polyamide 失效
标题翻译：含氟聚酰胺
公开(公告)号：US6103860A
公开(公告)日：2000-08-15
申请号：US332534
申请日：1999-06-14
申请人： Wataru Yamashita , Tomomi Yoshimura , Atsushi Shibuya , Yoshihiro Sakata , Hideaki Oikawa , Masahiro Ohta
发明人： Wataru Yamashita , Tomomi Yoshimura , Atsushi Shibuya , Yoshihiro Sakata , Hideaki Oikawa , Masahiro Ohta
IPC分类号： C08G69/42 , C08G69/12 , C08G69/32 , C08G69/40 , C08G73/10 , C08G69/02
CPC分类号： C08G69/40 , C08G69/32 , C08G73/1039
摘要： There is disclosed an organic optical component prepared from a resin essentially comprising one or more repetitive structural units selected from the group consisting of structures represented by general formula (1); ##STR1## wherein A is either of the groups below. ##STR2## This invention provides an organic optical component with excellent transparency, heat resistance and mechanical strength as well as a low birefringence. This invention also provides a novel aromatic polyamide with a low permitivity and excellent transparency, processability and thermal stability, besides excellent heat resistance inherent in an aromatic polyamide.
摘要翻译：公开了一种由基本上包含一个或多个重复结构单元的树脂制备的有机光学组件，所述重复结构单元选自由通式（1）表示的结构; 其中A是下面的组之一。本发明提供了具有优异的透明性，耐热性和机械强度以及低双折射性的有机光学部件。本发明还提供了芳香族聚酰胺固有的耐热性优异的低介电常数和优异的透明性，加工性和热稳定性的芳香族聚酰胺。

4. 发明授权

US5354839A Polyimide and preparation process of same 失效
标题翻译：聚酰亚胺及其制备方法相同
公开(公告)号：US5354839A
公开(公告)日：1994-10-11
申请号：US40608
申请日：1993-03-31
申请人： Wataru Yamashita , Yoshihiro Sakata , Toshiyuki Kataoka , Yuichi Okawa , Hideaki Oikawa , Tadashi Asanuma , Mitsunori Matsuo , Tsutomu Ishida , Keizaburo Yamaguchi , Akihiro Yamaguchi
发明人： Wataru Yamashita , Yoshihiro Sakata , Toshiyuki Kataoka , Yuichi Okawa , Hideaki Oikawa , Tadashi Asanuma , Mitsunori Matsuo , Tsutomu Ishida , Keizaburo Yamaguchi , Akihiro Yamaguchi
IPC分类号： C07C217/90 , C08G73/10 , H05K1/00 , H05K1/03 , C08G69/26
CPC分类号： C08G73/105 , C07C217/90 , C08G73/10 , C08G73/1014 , C08G73/1017 , H05K1/0346 , H05K3/4676
摘要： A polyimide comprising a requisite structural unit having one or more recurring structural units of the formula: ##STR1## such as the structural units of the formula ##STR2## The polyimide can have an extremely low dielectric constant and is colorless, transparent and excellent in processability and heat resistance, and also provides an aromatic diamine which is useful as a raw material monomer of the polyimide or a raw material of other various engineering plastics.
摘要翻译：一种聚酰亚胺，其包含具有一个或多个下式的重复结构单元的必需结构单元：例如下式的结构单元：该聚酰亚胺可以具有极低的介电常数，为无色透明且加工性优异和耐热性，并且还提供可用作聚酰亚胺的原料单体或其它各种工程塑料的原料的芳族二胺。

5. 发明授权

US5494996A Polyimide resin composition 失效
标题翻译：聚酰亚胺树脂组合物
公开(公告)号：US5494996A
公开(公告)日：1996-02-27
申请号：US277568
申请日：1994-07-20
申请人： Shoji Tamai , Yuichi Okawa , Wataru Yamashita , Yoshihiro Sakata , Hideaki Oikawa , Keizaburo Yamaguchi , Tadashi Asanuma , Akihiro Yamaguchi , Mitsunori Matsuo
发明人： Shoji Tamai , Yuichi Okawa , Wataru Yamashita , Yoshihiro Sakata , Hideaki Oikawa , Keizaburo Yamaguchi , Tadashi Asanuma , Akihiro Yamaguchi , Mitsunori Matsuo
IPC分类号： C08L71/10 , C08G73/10 , C08L71/08 , C08L79/04 , C08L79/08
CPC分类号： C08L79/08 , C08L79/04
摘要： A polyimide resin composition substantially comprising 1 99.9.about.50 parts by weight of polyimide having recurring structural units of the formula ##STR1## and 2 0.1.about.50 parts by weight of a polyimide which improved melt flowability and is prepared by using 1,3-bis(3-aminophenoxy)benzene or 6,6'-bis(3-aminophenoxy)-3,3,3',3'-tetramethyl-1,1'-spirobiindane as essential diamine component, or polyether pyridine having recurring structural units of the formula: ##STR2## is disclosed. Further, a polyimide based resin composition comprising the polyimide resin composition or a polyimide copolymer obtained by using the above diamines and a fibrous reinforcement is disclosed. These compositions have remarkably good processability, excellent heat stability and repeated fatigue characteristics.
摘要翻译：一种聚酰亚胺树脂组合物，其基本上包含+ E，crc / 1 / 99.9差异50重量份具有式（1）的重复结构单元的聚酰亚胺和+ E，crc / 2 / 0.1差异50重量份的通过使用1,3-双（3-氨基苯氧基）苯或6,6'-双（3-氨基苯氧基）-3,3,3'，3'-四甲基-1,1' - 螺环丁烷作为必需二胺组分，或具有下式重复结构单元的聚醚吡啶：。此外，公开了一种聚酰亚胺系树脂组合物，其包含使用上述二胺和纤维增强剂而得到的聚酰亚胺树脂组合物或聚酰亚胺共聚物。这些组合物具有非常好的加工性能，优异的热稳定性和重复的疲劳特性。

6. 发明授权

US06531568B1 Polyimide containing crosslinkable group and process for producing the same 有权
标题翻译：含交联性基团的聚酰亚胺及其制造方法
公开(公告)号：US06531568B1
公开(公告)日：2003-03-11
申请号：US09762260
申请日：2001-04-09
申请人： Atsushi Shibuya , Tomomi Okumura , Hideaki Oikawa , Yoshihiro Sakata , Takashi Kuroki , Yuichi Okawa , Shoji Tamai
发明人： Atsushi Shibuya , Tomomi Okumura , Hideaki Oikawa , Yoshihiro Sakata , Takashi Kuroki , Yuichi Okawa , Shoji Tamai
IPC分类号： C08G7310
CPC分类号： C08G73/10 , C08G73/101
摘要： This invention provides crosslinkable-group-containing polyimides of various known thermoplastic polyimide backbone structures, which are provided with far better heat resistance, chemical resistance and mechanical properties than known polyimides of the structures without impairing excellent moldability or formability, superb sliding property, low water absorption property, outstanding electrical properties, high thermal oxidation stability and high radiation resistance, all of which are inherent to the structures.
摘要翻译：本发明提供了各种已知的热塑性聚酰亚胺骨架结构的含交联性基团的聚酰亚胺，其具有比已知结构的聚酰亚胺更好的耐热性，耐化学性和机械性能，而不损害优异的成型性或成型性，优异的滑动性，低水吸收性能，优异的电性能，高热氧化稳定性和高耐辐射性，所有这些都是结构固有的。

7. 发明授权

US06458912B1 Crystalline polyimide for melt molding with satisfactory thermal stability 有权
标题翻译：用于熔体模塑的结晶聚酰亚胺，具有令人满意的热稳定性
公开(公告)号：US06458912B1
公开(公告)日：2002-10-01
申请号：US09674916
申请日：2001-02-05
申请人： Takashi Kuroki , Yoshihiro Sakata , Tomomi Okumura , Atsushi Shibuya , Yuichi Okawa , Hideaki Oikawa , Kayako Yanagihara , Yasunori Yoshida , Masaji Yoshimura , Hiroyasu Kido , Shoji Tamai
发明人： Takashi Kuroki , Yoshihiro Sakata , Tomomi Okumura , Atsushi Shibuya , Yuichi Okawa , Hideaki Oikawa , Kayako Yanagihara , Yasunori Yoshida , Masaji Yoshimura , Hiroyasu Kido , Shoji Tamai
IPC分类号： C08G7300
CPC分类号： C08G73/1042 , C08G73/101 , C08G73/105
摘要： A thermoplastic polyimide having good thermal stability, comprising a repeating unit represented by the chemical formula (1), a molecular terminal being composed of the chemical formula (2) and/or chemical formula (3), characterized in that: a melt viscosity ratio calculated by the numerical formula (1) and/or the numerical formula (3) is within a numerical range shown in the numerical formula (2) and/or the numerical formula (4) and 1,3-bis(4-aminophenoxy)benzene represented by the chemical formula (3) for production of the above polyimide, characterized in that the content of an azo compound is from 0.0 to 0.2%. The thermoplastic polyimide of the present invention has excellent characteristics {circle around (1)} to {circle around (4)} described below. {circle around (1)} It is superior in thermal stability on melting. That is, the degree of lowering of the fluidity on melting with a lapse of time is small and it is possible to apply to conventional melt molding. {circle around (2)} It has high heat resistance. {circle around (3)} It is superior in productivity. {circle around (4)} It is superior in dimensional accuracy.
摘要翻译：一种具有良好热稳定性的热塑性聚酰亚胺，其包含由化学式（1）表示的重复单元，由化学式（2）和/或化学式（3）组成的分子末端，其特征在于：熔体粘度比由式（1）和/或数值式（3）计算的数值在数值式（2）和/或数值式（4）和1,3-双（4-氨基苯氧基）由化学式（3）表示的用于制备上述聚酰亚胺的苯，其特征在于偶氮化合物的含量为0.0-0.2％。本发明的热塑性聚酰亚胺具有以下所述的{圆周（1）}〜{圆周（4）}的特性。 {circle around（1）}熔融时的热稳定性优异。也就是说，随着时间的流逝，熔融流动性的降低程度小，可以适用于常规的熔融成型。 {circle around（2）}它具有很高的耐热性。 {circle around（3）}它的生产力优越。 {circle around（4）}尺寸精度优越。

8. 发明授权

US06710160B2 Polyamic acid, polyimide, process for producing these, and film of the polyimide 有权
标题翻译：聚酰胺酸，聚酰亚胺，其制造方法和聚酰亚胺薄膜
公开(公告)号：US06710160B2
公开(公告)日：2004-03-23
申请号：US10088481
申请日：2002-03-20
申请人： Wataru Yamashita , Katsuji Watanabe , Hideaki Oikawa , Hisato Ito
发明人： Wataru Yamashita , Katsuji Watanabe , Hideaki Oikawa , Hisato Ito
IPC分类号： C08G7310
CPC分类号： G01N33/54346 , C08G73/10 , C08G73/1082
摘要： Disclosed are a polyamic acid having repeating units represented by the formula (1): wherein the norbornane skeleton of comprises four components of and their contents satisfy the following: 1%≦2,5-[diexo]≦90%, 1%≦2,5-[exo,endo]≦90%, 1%≦2,6-[diexo]≦90%, 1% ≦2,6-[exo,endo]≦90%, provided that (2,5-[diexo])+(2,5-[exo,endo])+(2,6-[diexo])+(2,6-[exo,endo])=100%, R represents from 4 to 27 carbon atoms, and represents a tetravalent group selected from the group consisting of an aliphatic group, a monocyclic aliphatic group, a condensed polycyclic aliphatic group, a monocyclic aromatic group, a condensed polycyclic aromatic group, and a non-condensed polycyclic aliphatic or aromatic group which is composed of cycloaliphatic or aromatic groups mutually bonded to each other either directly or via a crosslinking member; and a polyimide which is obtained by imidizing the polyamic acid and which has good properties intrinsic to polyimides, or that is, thermal resistance, mechanical properties, slidability, low water absorption, electric properties and radiation resistance intrinsic thereto. By varying the composition ratio of the starting diamine isomers, various polyimides having controlled thermal resistance, melt flowability, optical properties, chemical resistance and electric properties and capable of forming films of various forms can be obtained.
摘要翻译：公开了具有由式（1）表示的重复单元的聚酰胺酸：其中含有四种成分及其含量的降冰片烷骨架满足以下条件：1％<= 2,5- [阴离子] <= 90％，1％<= 2,5- [外，内] <= 90％，1％<= 2,6- [阴离子] <= 90％，1％<= 2,6- [外，内] <= 90％表示4〜27个碳原子，表示选自脂肪族基团，单环脂族基团，缩合多环脂族基团，单环芳香族基团，缩合多环芳香族基团和未缩合的四价基团由脂环族或芳族基团组成的多环脂肪族或芳香族基团直接或通过交联成分彼此相互结合; 和通过酰亚胺化聚酰胺酸而获得的聚酰亚胺，其具有聚酰亚胺所固有的良好性能，或者其本身具有的热阻，机械性能，滑动性，低吸水性，电性能和耐辐射性。通过改变起始二胺异构体的组成比，可以获得具有受控热阻，熔体流动性，光学性能，耐化学性和电性能并且能够形成各种形式的膜的各种聚酰亚胺。

9. 发明授权

US5480965A Readily soluble, amorphous polyimide, and preparation process of same 失效
标题翻译：易溶，无定形聚酰亚胺及其制备方法相同
公开(公告)号：US5480965A
公开(公告)日：1996-01-02
申请号：US280551
申请日：1994-07-26
申请人： Wataru Yamashita , Yuichi Okawa , Hideaki Oikawa , Tadashi Asanuma , Yuko Ishihara , Mitsunori Matsuo , Keizaburo Yamaguchi , Akihiro Yamaguchi , Shoji Tamai
发明人： Wataru Yamashita , Yuichi Okawa , Hideaki Oikawa , Tadashi Asanuma , Yuko Ishihara , Mitsunori Matsuo , Keizaburo Yamaguchi , Akihiro Yamaguchi , Shoji Tamai
IPC分类号： C07C201/12 , C07C205/45 , C07C221/00 , C07C225/22 , C08G73/10 , C08G73/12 , C08J5/18 , C08L79/08 , C08G69/26 , C08L77/00
CPC分类号： C08G73/10 , C08G73/1007 , C08G73/1014 , C08G73/1017 , C08G73/1067 , Y10T428/31504 , Y10T428/31721
摘要： This invention relates to a novel thermoplastic and amorphous polyimide which is readily soluble in organic solvent, a novel aromatic diamino compound used for the polyimide, a preparation process thereof, a polyimide-based resin composition comprising the thermoplastic polyimide and a fibrous reinforcement, a process for preparing the resin composition, an injection molded article of the resin composition, a polyimide-based composite obtained by molding the above soluble and thermoplastic polyimide in combination with a fibrous reinforcement, and a fibrous reinforcement having a surface modified with the above polyimide.The polyimide comprise a requisite structural unit having one or more recurring structural units of the formula: ##STR1## wherein m and n are individually an integer of 0 or 1, and R is ##STR2## The polyimide of the invention is essentially amorphous, excellent in melt flow stability in the decreased temperature as compared with conventionally known polyimide and has greatly improved processability.The polyimide of the invention obtained by using a novel aromatic diamino compound as a monomer can control various properties such as melt flow ability and solubility in solvents by side chains and not by principal chain of polyimide. Thus, excellent melt flow property and solubility in solvents can be obtained while maintaining high heat resistance and adhesive property which are derived from benzophenone structure of the diamino compound of the the invention.
摘要翻译：本发明涉及易溶于有机溶剂的新型热塑性和无定形聚酰亚胺，用于聚酰亚胺的新型芳族二氨基化合物及其制备方法，包含热塑性聚酰亚胺和纤维增强剂的聚酰亚胺基树脂组合物，用于制备树脂组合物的树脂组合物的注塑制品，通过将上述可溶性和热塑性聚酰亚胺与纤维增强剂组合成型而获得的聚酰亚胺类复合材料和具有用上述聚酰亚胺改性的表面的纤维增强剂。聚酰亚胺包含必需的结构单元，其具有一个或多个下式的重复结构单元：其中m和n分别为0或1的整数，R为本发明的聚酰亚胺基本上为与常规已知的聚酰亚胺相比，在降低的温度下的熔体流动稳定性优异并且具有极大的改进的加工性。通过使用新颖的芳族二氨基化合物作为单体获得的本发明的聚酰亚胺可以通过侧链而不是聚酰亚胺的主链来控制各种性能如熔体流动性和在溶剂中的溶解度。因此，在保持由本发明的二氨基化合物的二苯甲酮结构得到的高耐热性和粘合性的同时，可以获得优异的熔体流动性和溶剂中的溶解性。

10. 发明授权

US5380805A Polyimides, process for the preparation thereof and polyimide resin compositions 失效
标题翻译：聚酰亚胺，其制备方法和聚酰亚胺树脂组合物
公开(公告)号：US5380805A
公开(公告)日：1995-01-10
申请号：US143105
申请日：1993-10-29
申请人： Shoji Tamai , Masahiro Ohta , Saburo Kawashima , Katsuaki Iiyama , Hideaki Oikawa , Akihiro Yamaguchi , Kouji Ohkoshi , Masao Yoshikawa
发明人： Shoji Tamai , Masahiro Ohta , Saburo Kawashima , Katsuaki Iiyama , Hideaki Oikawa , Akihiro Yamaguchi , Kouji Ohkoshi , Masao Yoshikawa
IPC分类号： C08G73/10 , C08L79/08
CPC分类号： C08G73/1042 , C08G73/105 , C08G73/1071 , C08L79/08
摘要： In one aspect, the present invention relates to polyimides having excellent thermal resistance and process for preparing the same comprising carrying out condensation of 4,4'-bis(3-aminophenoxy)biphenyl with pyromellitic dianhydride in the presence of a different diamine compound and optionally with a different tetracarboxylic acid dianhydride.In a second aspect, the present invention relates to a heat resistant resin composition consisting essentially of an aromatic polyetherimide and a defined polyimide.In a third aspect, the present invention relates to a polyimide resin composition comprised on a defined polyimide and a separate high-temperature engineering polymer.In a fourth aspect, the present invention relates to a resin composition comprised of a defined polyimide and an aromatic polyamideimide.
摘要翻译：一方面，本发明涉及具有优异耐热性的聚酰亚胺及其制备方法，包括在不同的二胺化合物和任选地存在下进行4,4'-双（3-氨基苯氧基）联苯与均苯四酸二酐的缩合与不同的四羧酸二酐。在第二方面，本发明涉及一种主要由芳族聚醚酰亚胺和所定义的聚酰亚胺组成的耐热树脂组合物。在第三方面，本发明涉及包含在限定的聚酰亚胺和单独的高温工程聚合物上的聚酰亚胺树脂组合物。在第四方面，本发明涉及由限定的聚酰亚胺和芳族聚酰胺酰亚胺组成的树脂组合物。

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