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1. 发明授权

US06759500B1 High-molecular polypropylene with a broad distribution of the molecular weight and a short isotactic sequence length 失效
标题翻译：高分子量聚丙烯具有广泛的分子量分布和短的全同立构序列长度
公开(公告)号：US06759500B1
公开(公告)日：2004-07-06
申请号：US10130045
申请日：2002-05-13
申请人： Volker Dolle , Volker Fraaije , Herbert Terwyen , Thomas Boehm
发明人： Volker Dolle , Volker Fraaije , Herbert Terwyen , Thomas Boehm
IPC分类号： C08F11006
CPC分类号： C08F10/06 , C08F4/65912 , C08F10/00 , C08F110/06 , C08F4/65916 , C08F4/65927 , C08F2500/12 , C08F2500/17 , C08F2500/04 , C08F2500/15 , C08F2500/01
摘要： Propylene polymers containing from 0 to 2.5% by weight of C2-C10-olefin comonomers have an Mw of from 350,000 to 1,000,000 g/mol, an Mw/Mn of from 4 to 10, a proportion by weight of the polymer fraction having a viscosity number of from 500 to 1400 ml/g of from 20 to 80% of the total polymer and a proportion by weight of a polymer fraction having a viscosity number of from 200 to 400 ml/g of from 80 to 20% of the total polymer and an isotactic sequence length of from 50 to 100.
摘要翻译：含有0至2.5重量％的C 2 -C 10烯烃共聚单体的丙烯聚合物的Mw为35万至1,000,000g / mol，Mw / Mn为4至10，聚合物部分的重量比为粘度 500至1400ml / g的总聚合物的20至80％，粘度为200至400ml / g的聚合物部分的重量比为总聚合物的80至20％和全同立构序列长度为50-100。

2. 发明授权

US06362298B1 High-molecular-weight polypropylene having a broad molecular-weight distribution 失效
公开(公告)号：US06362298B1
公开(公告)日：2002-03-26
申请号：US08804063
申请日：1997-02-21
申请人： Volker Dolle , Eduardo Chicote Carrion , Herbert Terwyen
发明人： Volker Dolle , Eduardo Chicote Carrion , Herbert Terwyen
IPC分类号： C08F21016
摘要： The invention relates to a high-molecular-weight copolymer comprising ethylene and propylene units which has an ethylene content in the range from 1 to 10% by weight, a melt flow rate MFR (230/5) of

3. 发明授权

US06218504B1 Method for deodorizing polyolefin granulates 失效
标题翻译：聚烯烃颗粒除臭方法
公开(公告)号：US06218504B1
公开(公告)日：2001-04-17
申请号：US09380404
申请日：1999-09-01
申请人： Volker Dolle , Eduardo Chicote Carrion , Paul-Richard Schöneborn , Herbert Terwyen
发明人： Volker Dolle , Eduardo Chicote Carrion , Paul-Richard Schöneborn , Herbert Terwyen
IPC分类号： C08F626
CPC分类号： B29B13/00 , B29C2071/0027 , B29K2023/00 , C08F6/005 , C08L23/00
摘要： A gaseous mixture of steam and air, a gaseous mixture of steam and nitrogen, or pure steam are passed around polyolefin granules in a deodorizing apparatus. The result is that the polyolefin granules have markedly improved properties with respect to odor and taste, and these are retained in moldings produced from the granules.
摘要翻译：蒸汽和空气的气体混合物，蒸气和氮气的气体混合物或纯蒸汽在除臭装置中通过聚烯烃颗粒。结果是聚烯烃颗粒在气味和味道方面具有显着改善的性能，并且这些颗粒保留在由颗粒制成的模制品中。

4. 发明授权

US07521104B2 Molding compositions made from a high-molecular-weight-propylene polymer 失效
标题翻译：由高分子量丙烯聚合物制成的成型组合物
公开(公告)号：US07521104B2
公开(公告)日：2009-04-21
申请号：US10539343
申请日：2003-12-19
申请人： Volker Dolle , Thomas Böhm , Herbert Terwyen
发明人： Volker Dolle , Thomas Böhm , Herbert Terwyen
IPC分类号： F16L9/12 , C08K5/3465 , C08L23/10 , B29D23/00
CPC分类号： F16L9/12 , C08F10/06 , C08F110/06 , C08F210/06 , C08K5/0083 , C08K5/3437 , C08L23/10 , C08L2205/02 , C08L2205/242 , D01F6/06 , Y10T428/139 , Y10T428/1397 , C08L2666/06 , C08F2500/03 , C08F2500/12 , C08F2500/01 , C08F210/16
摘要： Molding compositions made from a high-molecular-weight propylene polymer with a melt mass-flow rate MFR of from 0.3 to 1 g/10 min, to ISO 1133 at 230° C. and 5 kg, and with a proportion of β modification crystallites in the range from 2 to 20% by weight. The molding compositions of the invention preferably comprise a quinarcidone pigment as nucleating agent. The high-molecular-weight propylene polymer used preferably comprises a high-molecular-weight propylene copolymer with up to 30% by weight of other copolymerized olefins having up to 10 carbon atoms. One of the uses of the molding compositions of the invention is as materials for pipes.
摘要翻译：熔体质量流量MFR为0.3〜1g / 10分钟的高分子量丙烯聚合物，230℃，5kg的ISO 1133，以及β改性微晶比例的成型组合物在2至20重量％的范围内。本发明的成型组合物优选包含醌基酮颜料作为成核剂。所用的高分子量丙烯聚合物优选包含高达30重量％的具有至多10个碳原子的其它共聚烯烃的高分子量丙烯共聚物。本发明的成型组合物的用途之一是管道材料。

5. 发明授权

US06191223B1 Polymer blends 有权
标题翻译：聚合物共混物
公开(公告)号：US06191223B1
公开(公告)日：2001-02-20
申请号：US09336732
申请日：1999-06-21
申请人： Volker Dolle , Herbert Terwyen
发明人： Volker Dolle , Herbert Terwyen
IPC分类号： C08F800
CPC分类号： C08L23/14 , C08L23/06 , C08L23/16 , C08L2205/02 , C08L2666/04
摘要： a) from 50 to 85% by weight of a copolymer of propylene (A) with 1-alkenes comprising from 20 to 80% by weight of a high molecular weight copolymer of propylene (I) containing from 2.0 to 7.0% by weight of copolymerized 1-alkene and having a viscosity of from 500 to 1200 ml/g and from 20 to 80% by weight of a low molecular weight copolymer of propylene (II) containing from 4.0 to 10.0% by weight of copolymerized 1-alkene and having a viscosity of from 200 to 450 ml/g, b) from 5 to 10% by weight of a polymer of ethylene (B) and c) from 10 to 40% by weight of a rubber-like copolymer of propylene and a 1-alkene (C) containing from 30 to 70% by weight of copolymerized 1-alkene have a melt flow index (MFI) at 230° C. under a weight of 5 kg of from 0.1 to 5 g/10 min, a molecular weight distribution (Mw/Mn) of from 6 to 20 and a total 1-alkene content of from 4 to 15% by weight.
摘要翻译： a）50至85重量％的丙烯（A）与1-烯烃的共聚物，其包含20至80重量％的含有2.0至7.0重量％共聚合的丙烯（I）的高分子量共聚物并且具有500至1200ml / g的粘度和20至80重量％的含有4.0至10.0重量％的共聚1-烯烃的丙烯（II）的低分子量共聚物，并且具有粘度为200〜450ml / g，b）5〜10重量％的乙烯（B）和（c）的聚合物，c）10〜40重量％的丙烯与1-烯烃的橡胶状共聚物 C）含有30至70重量％的共聚1-烯烃，熔体流动指数（MFI）在230℃下以5kg的重量计0.1至5g / 10min，分子量分布（Mw / Mn）为6〜20，总1-烯烃含量为4〜15重量％。

6. 发明申请

US20060167141A1 Molding compositions made from high-molecular-weight-propylene polymer 失效
标题翻译：由高分子量丙烯聚合物制成的成型组合物
公开(公告)号：US20060167141A1
公开(公告)日：2006-07-27
申请号：US10539343
申请日：2003-12-19
申请人： Volker Dolle , Thomas Bohm , Herbert Terwyen
发明人： Volker Dolle , Thomas Bohm , Herbert Terwyen
IPC分类号： C08K5/34
CPC分类号： F16L9/12 , C08F10/06 , C08F110/06 , C08F210/06 , C08K5/0083 , C08K5/3437 , C08L23/10 , C08L2205/02 , C08L2205/242 , D01F6/06 , Y10T428/139 , Y10T428/1397 , C08L2666/06 , C08F2500/03 , C08F2500/12 , C08F2500/01 , C08F210/16
摘要： Molding compositions made from a high-molecular-weight propylene polymer with a melt mass-flow rate MFR of from 0.3 to 1 g/10 min, to ISO 1133 at 230° C. and 5 kg, and with a proportion of β modification crystallites in the range from 2 to 20% by weight. The molding compositions of the invention preferably comprise a quinacridone pigment as nucleating agent. The high-molecular-weight propylene polymer used preferably comprises a high-molecular-weight propylene copolymer with up to 30% by weight of other copolymerized olefins having up to 10 carbon atoms. One of the uses of the molding compositions of the invention is as materials for pipes.
摘要翻译：熔体质量流量MFR为0.3〜1g / 10分钟的高分子量丙烯聚合物，230℃，5kg的ISO 1133，以及β改性微晶比例的成型组合物在2至20重量％的范围内。本发明的成型组合物优选包含喹吖啶酮颜料作为成核剂。所用的高分子量丙烯聚合物优选包含高达30重量％的具有至多10个碳原子的其它共聚烯烃的高分子量丙烯共聚物。本发明的成型组合物的用途之一是管道材料。

7. 发明授权

US08569434B2 Ethylene copolymers, catalyst system and process for preparing the same 有权
标题翻译：乙烯共聚物，催化剂体系及其制备方法
公开(公告)号：US08569434B2
公开(公告)日：2013-10-29
申请号：US13148041
申请日：2010-02-16
申请人： Fabiana Fantinel , Shahram Mihan , Volker Dolle , Andreas Maus
发明人： Fabiana Fantinel , Shahram Mihan , Volker Dolle , Andreas Maus
IPC分类号： C08L23/08
CPC分类号： C08F210/16 , C08F4/63912 , C08F4/6392 , C08F2420/01 , C08L23/0815 , C08L2205/02 , C08L2308/00 , C08L2314/06 , C08L2666/06 , C08F210/14 , C08F2500/20 , C08F2500/17 , C08F2500/12 , C08F2500/03 , C08F2500/05 , C08F2500/08 , C08F4/63904
摘要： An ethylene copolymer, a catalyst system suitable to prepare the ethylene copolymer, and a process to prepare such ethylene copolymer are described. The use of the ethylene copolymer as impact modifier in polyethylene and as compatibilizer in a polymer blend are also described. The ethylene copolymer has a density from 0.855 g/cm3 to 0.910 g/cm3, a polydispersity Mw/Mn lower than 3.5, comprises at least one first ethylene polymer component and at least one second ethylene polymer component having different comonomer contents so as to show at least two predetermined CRYSTAF peak temperatures.
摘要翻译：描述了乙烯共聚物，适于制备乙烯共聚物的催化剂体系，以及制备这种乙烯共聚物的方法。还描述了在聚乙烯中使用乙烯共聚物作为抗冲改性剂和在聚合物共混物中作为增容剂。乙烯共聚物的密度为0.855g / cm 3至0.910g / cm 3，多分散性Mw / Mn低于3.5，包含至少一种第一乙烯聚合物组分和至少一种具有不同共聚单体含量的第二乙烯聚合物组分，以显示至少两个预定的CRYSTAF峰值温度。

8. 再颁专利

USRE39532E1 Metallocenes containing ligands of 2-substituted indenyl derivatives, process for their preparation, and their use as catalysts 失效
标题翻译：含有2-取代茚基衍生物配体的金属茂，其制备方法及其作为催化剂的用途
公开(公告)号：USRE39532E1
公开(公告)日：2007-03-27
申请号：US08895909
申请日：1997-07-17
申请人： Andreas Winter , Martin Antberg , Walter Spaleck , Jürgen Rohrmann , Volker Dolle
发明人： Andreas Winter , Martin Antberg , Walter Spaleck , Jürgen Rohrmann , Volker Dolle
IPC分类号： C07F7/28 , C07F9/00 , C07F11/00 , C07C13/465
CPC分类号： C07F17/00 , C07F7/0805 , C08F4/63912 , C08F4/63927 , C08F10/00 , C08F110/06 , C08F2500/03 , C08F2500/17 , C08F2500/15
摘要： The novel metallocenes of the formula I in which, preferably, M1 is Zr or Hf, R1 and R2 are alkyl or halogen, R3 and R4 are hydrogen, R5 and R6 are alkyl or haloalkyl, —(CR8R9)m—R7—(CR8R9)n— is a single- or multi-membered chain in which R7 may also be a (substituted) hetero atom, m+n is zero or 1, and R10 is hydrogen, form, together with aluminoxanes as cocatalysts, a very effective catalyst system for the preparation of polyolefins of high stereospecificity and high melting point.
摘要翻译：配方的新金属茂

9. 发明授权

US5328969A Process for the preparation of a high molecular weight olefin polymer 失效
标题翻译：制备高分子量烯烃聚合物的方法
公开(公告)号：US5328969A
公开(公告)日：1994-07-12
申请号：US980643
申请日：1992-11-24
申请人： Andreas Winter , Jurgen Rohrmann , Volker Dolle , Frank Kuber
发明人： Andreas Winter , Jurgen Rohrmann , Volker Dolle , Frank Kuber
IPC分类号： C07F7/00 , C07C13/465 , C07C45/46 , C07C45/67 , C07F17/00 , C08F4/60 , C08F4/639 , C08F4/6392 , C08F4/64 , C08F4/642 , C08F4/655 , C08F4/659 , C08F4/6592 , C08F10/00 , C08F10/06 , C08F110/06 , C08F210/06
CPC分类号： C08F10/06 , C07C13/465 , C07C45/46 , C07C45/67 , C07F17/00 , C08F10/00 , C07C2102/08 , C08F110/06 , C08F210/06 , C08F4/63912 , C08F4/63927 , C08F4/65908 , Y10S526/943
摘要： A very active catalyst system for olefin polymerization comprises a cocatalyst, preferably an aluminoxane, and a metallocene of the formula I ##STR1## in which, preferably, M.sup.1 is Zr or Hf, R.sup.1 and R.sup.2 are alkyl or halogen, R.sup.3 is hydrogen, R.sup.4 to R.sup.6 are alkyl or aryl, --(CR.sup.8 R.sup.9).sub.m --R.sup.7 --(CR.sup.8 R.sup.9).sub.n is a single- or multi-membered chain, in which R.sup.7 can also be a (substituted) hetero atom, and m+n is zero or 1.
摘要翻译：用于烯烃聚合的非常活泼的催化剂体系包括助催化剂，优选铝氧烷和式I（I）的茂金属，其中优选地，M1是Zr或Hf，R1和R2是烷基或卤素，R3是氢，R4至R6是烷基或芳基， - （CR8R9）m-R7-（CR8R9）n是单或多元链，其中R7也可以是（取代的）杂原子，m + n是零或1。

10. 发明授权

US5304614A Process for the preparation of an olefin polymer using metallocenes having specifically substituted indenyl ligands 失效
标题翻译：使用具有特异取代的茚基配体的金属茂制备烯烃聚合物的方法
公开(公告)号：US5304614A
公开(公告)日：1994-04-19
申请号：US960893
申请日：1992-10-14
申请人： Andreas Winter , Martin Antberg , Volker Dolle , Jurgen Rohrmann , Walter Spaleck
发明人： Andreas Winter , Martin Antberg , Volker Dolle , Jurgen Rohrmann , Walter Spaleck
IPC分类号： C08F4/622 , C08F4/60 , C08F4/64 , C08F4/642 , C08F4/659 , C08F4/6592 , C08F10/00 , C08F4/42
CPC分类号： C08F10/00 , C08F4/65912 , C08F4/65927 , Y10S526/943
摘要： A very active catalyst system for olefin polymerization comprises a cocatalyst, preferably an aluminoxane, and a metallocene of the formula I or Ia ##STR1## in which, preferably, M.sup.1 is Zr or Hf, R.sup.1 and R.sup.2 are alkyl or halogen, R.sup.3 and R.sup.4 are hydrogen or alkyl, R.sup.5 and R.sup.6 are alkyl, --(CR.sup.8 R.sup.9).sub.m --R.sup.7 --(CR.sup.8 R.sup.9).sub.n is a chain with one or more members, in which R.sup.7 can also be a (substituted) heteroatom, and m+n is zero or 1.
摘要翻译：用于烯烃聚合的非常活泼的催化剂体系包括助催化剂，优选铝氧烷和式I或Ia的茂金属（*化学结构*），其中优选地是M1是Zr或Hf，R1和R2是烷基或卤素， R3和R4是氢或烷基，R5和R6是烷基， - （CR8R9）m-R7-（CR8R9）n是具有一个或多个成员的链，其中R7也可以是（取代的）杂原子，并且m + n为零或1。

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