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1. 发明授权

US07482075B2 Reforming apparatus for fuel cell, fuel cell and operation method of fuel cell 失效
标题翻译：燃料电池，燃料电池改造设备及燃料电池运行方法
公开(公告)号：US07482075B2
公开(公告)日：2009-01-27
申请号：US11008760
申请日：2004-12-09
申请人： Toru Kato , Masatsugu Amano , Ken Nozaki , Ken Kato , Akira Negishi
发明人： Toru Kato , Masatsugu Amano , Ken Nozaki , Ken Kato , Akira Negishi
IPC分类号： H01M8/06 , C01B3/24
CPC分类号： H01M8/0618 , C01B3/323 , C01B2203/0233 , C01B2203/0238 , C01B2203/066 , C01B2203/0816 , C01B2203/0822 , C01B2203/0827 , C01B2203/1211 , C01B2203/148 , H01M8/04231 , Y02P20/128 , Y02P20/142
摘要： In a reforming method for a high temperature type fuel cell in which dimethyl ether is used as fuel gas, and a gas containing hydrogen and carbon monoxide produced by reacting dimethyl ether with carbon dioxide is fed into the anode, the carbon deposition at the time of reforming is prevented. The feeding amounts of dimethyl ether and carbon dioxide from a pipe h1 into the reforming reactor are regulated in such a way that the relation between temperature inside the reforming reactor and the molar ratio of carbon dioxide to dimethyl ether in the reforming reactor falls within the region C.
摘要翻译：在其中使用二甲醚作为燃料气体的高温型燃料电池的重整方法中，将通过二甲醚与二氧化碳反应生成的含氢气和一氧化碳的气体进料到阳极中，防止重整。从管h1进入重整反应器的二甲醚和二氧化碳的进料量以重整反应器内的温度与重整反应器中的二氧化碳与二甲醚的摩尔比之间的关系落在区域内 C。

2. 发明申请

US20050129995A1 Reforming apparatus for fuel cell, fuel cell and operation method of fuel cell 失效
标题翻译：燃料电池，燃料电池改造设备及燃料电池运行方法
公开(公告)号：US20050129995A1
公开(公告)日：2005-06-16
申请号：US11008760
申请日：2004-12-09
申请人： Toru Kato , Masatsugu Amano , Ken Nozaki , Ken Kato , Akira Negishi
发明人： Toru Kato , Masatsugu Amano , Ken Nozaki , Ken Kato , Akira Negishi
IPC分类号： C01B3/32 , H01M8/04 , H01M8/06 , H01M8/12 , C01B3/24
CPC分类号： H01M8/0618 , C01B3/323 , C01B2203/0233 , C01B2203/0238 , C01B2203/066 , C01B2203/0816 , C01B2203/0822 , C01B2203/0827 , C01B2203/1211 , C01B2203/148 , H01M8/04231 , Y02P20/128 , Y02P20/142
摘要： In a reforming method for a high temperature type fuel cell in which dimethyl ether is used as fuel gas, and a gas containing hydrogen and carbon monoxide produced by reacting dimethyl ether with carbon dioxide is fed into the anode, the carbon deposition at the time of reforming is prevented. The feeding amounts of dimethyl ether and carbon dioxide from a pipe h1 into the reforming reactor are regulated in such a way that the relation between temperature inside the reforming reactor and the molar ratio of carbon dioxide to dimethyl ether in the reforming reactor falls within the region C.
摘要翻译：在其中使用二甲醚作为燃料气体的高温型燃料电池的重整方法中，将通过二甲醚与二氧化碳反应生成的含氢气和一氧化碳的气体进料到阳极中，防止重整。从管h 1进入重整反应器的二甲醚和二氧化碳的进料量以重整反应器内的温度与重整反应器中二氧化碳与二甲醚的摩尔比之间的关系落在内部地区C.

3. 发明授权

US5250158A Method for producing vanadium electrolytic solution 失效
标题翻译：钒电解液生产方法
公开(公告)号：US5250158A
公开(公告)日：1993-10-05
申请号：US772794
申请日：1991-10-08
申请人： Hiroko Kaneko , Akira Negishi , Ken Nozaki , Kenji Sato , Ichiro Nakahara
发明人： Hiroko Kaneko , Akira Negishi , Ken Nozaki , Kenji Sato , Ichiro Nakahara
IPC分类号： C01G31/00 , H01M8/18 , C25B1/00
CPC分类号： H01M8/188 , C01G31/00 , Y02E60/528
摘要： A vanadium electrolytic solution containing highly concentrated and dissolved vanadium is produced by a method wherein a vanadium compound selected from the group consisting of ammonium metavanadate and vanadium pentaoxide is subjected to a reduction operation in the presence of inorganic acids. At this time, by repeating the addition of the concentrated inorganic acids and the vanadium compound, a tetravalent and pentavalent vanadium solution of 3.4 mol/l is obtained.In addition, the resulting vanadium electrolytic solution is electrolyzed, whereby tetravalent vanadium is reduced to be trivalent on the negative electrode and is oxidized into pentavalent vanadium on the positive electrode, and then pentavalent vanadium is reduced into tetravalent vanadium by a reducing agent to form a discharged couple of trivalent and tetravalent vanadium, and an electrolytic solution is obtained which is capable of being charge-discharged.This electrolytic solution can be used as the electrolytic solution for redox batteries using vanadium as the active material in both positive and negative electrodes.
摘要翻译：通过一种方法制备含有高浓度和溶解的钒的钒电解液，其中选自偏钒酸铵和五氧化钒的钒化合物在无机酸的存在下进行还原操作。此时，通过重复添加浓缩的无机酸和钒化合物，得到3.4mol / l的四价和五价钒溶液。此外，所得到的钒电解液被电解，四价钒在负极上还原为三价，在正极上被氧化成五价钒，然后用还原剂将五价钒还原成四价钒，形成放出一对三价和四价钒，得到能够进行电荷放电的电解液。该电解液可以用作在正极和负极中使用钒作为活性材料的氧化还原电池的电解液。

4. 发明授权

US5704118A Method of making a carbon sensor electrode 失效
标题翻译：制作碳传感器电极的方法
公开(公告)号：US5704118A
公开(公告)日：1998-01-06
申请号：US411525
申请日：1995-03-28
申请人： Hiroko Kaneko , Akira Negishi , Ken Nozaki
发明人： Hiroko Kaneko , Akira Negishi , Ken Nozaki
IPC分类号： C12Q1/00 , G01N27/30 , H01R43/16
CPC分类号： G01N27/308 , C12Q1/001 , Y10T29/49204
摘要： A process for producing a carbon sensor for measuring a composition, includes (a) providing first and second carbon electrodes each comprised of a bundle of linear, thin carbon members; (b) surrounding the first carbon electrode by dipping the first carbon electrode in a solution comprised of a reactive substance which reacts chemically with the composition to be measured; (c) disposing the first carbon electrode and the solution in a cylindrical ion permeable membrane to hold the solution in the first carbon electrode as well as between the first carbon electrode and the cylindrical ion permeable membrane; (d) positioning the cylindrical ion permeable membrane including the first carbon electrode and the solution in an insulating tubular member; and (e) disposing the second carbon electrode between the insulating tubular member and the cylindrical ion permeable membrane. Alternatively, the solution may be poured into a cylindrical ion permeable membrane and the first carbon electrode may be inserted into the cylindrical ion permeable membrane to hold the solution between the first carbon electrode and the ion permeable membrane and thereby surround the bundle.
摘要翻译：一种用于测量组合物的碳传感器的制造方法，包括（a）提供第一和第二碳电极，每个碳电极由一系列线性，薄碳构件构成; （b）通过将第一碳电极浸入由与要测量的组合物化学反应的反应物质的溶液中来围绕第一碳电极; （c）将第一碳电极和溶液设置在圆柱形离子渗透膜中以将溶液保持在第一碳电极以及第一碳电极和圆柱形离子可渗透膜之间; （d）将包括第一碳电极和溶液的圆柱形离子可渗透膜定位在绝缘管状构件中; 和（e）将第二碳电极设置在绝缘管状构件和圆柱形离子可渗透膜之间。或者，将溶液倒入圆柱形离子渗透膜中，将第一碳电极插入到圆柱形离子可渗透膜中，以将溶液保持在第一碳电极和离子可渗透膜之间，从而包围束。

5. 发明授权

US5503728A Carbon sensor electrode and process for producing the same 失效
标题翻译：碳传感器电极及其制造方法
公开(公告)号：US5503728A
公开(公告)日：1996-04-02
申请号：US317816
申请日：1994-10-04
申请人： Hiroko Kaneko , Akira Negishi , Ken Nozaki
发明人： Hiroko Kaneko , Akira Negishi , Ken Nozaki
IPC分类号： C12Q1/00 , G01N27/30 , G01N27/26 , C25B11/00
CPC分类号： G01N27/308 , C12Q1/001 , Y10T29/49204
摘要： A carbon electrode is dipped in a solution containing a reactive substance, and the carbon electrode impregnated with the solution is covered with an insulating tubular member; or a solution containing a reactant is poured into an insulating tube, and a carbon electrode is inserted into the tube; whereby the reactant is made coexistent in the periphery of the carbon electrode. Alternatively, a reactive substance such as an active enzyme and graphite particles or activated carbon particles are mixed with a liquid and dispersed therein to prepare a thoroughly wetted paste. The paste is introduced by means of an extruding mechanism such as a syringe into an insulating tubular member in which a bundle of many thin carbon rods as a lead is inserted. Thus, a carbon sensor electrode is produced. Alternatively, a first carbon electrode that has been dipped in an active enzyme or an enzyme-like reactive substance solution is disposed in a wet condition in a cylindrical ion permeable membrane. To prevent the enzyme or enzyme-like reactive substance in the electrode from becoming deactivated with the passage of time, a preliminary electrode is further inserted into the insulating tubular member, whereby the potential can be kept to be oxidation or reduction potential so as to ensure a constant sensor life. A fresh electrode surface having the active enzyme or enzyme-like reactive substance can be easily obtained by cutting or snapping off a tip portion of the sensor including the insulating tubular member.
摘要翻译：将碳电极浸渍在含有反应性物质的溶液中，浸渍有溶液的碳电极被绝缘管状部件覆盖; 或将包含反应物的溶液倒入绝缘管中，并将碳电极插入管中; 由此使反应物在碳电极的周围共存。或者，将活性物质和石墨颗粒或活性炭颗粒等反应性物质与液体混合并分散在其中以制备充分湿润的糊剂。通过诸如注射器的挤出机构将糊剂引入绝缘管状构件中，其中插入有许多薄碳棒作为引线。因此，生成碳传感器电极。或者，已经浸渍在活性酶或酶状反应物质溶液中的第一碳电极在湿式条件下设置在圆柱形离子渗透膜中。为了防止电极中的酶或酶状反应物质随时间变得失活，将预备电极进一步插入到绝缘管状部件中，由此可以将电位保持为氧化还原电位，以确保传感器寿命恒定。具有活性酶或酶状反应物质的新鲜电极表面可以通过切断或剥离包括绝缘管状构件的传感器的末端部分而容易地获得。

6. 发明授权

US5318865A Redox battery 失效
标题翻译：氧化还原电池
公开(公告)号：US5318865A
公开(公告)日：1994-06-07
申请号：US892032
申请日：1992-06-02
申请人： Hiroko Kaneko , Akira Negishi , Ken Nozaki , Kanji Sato , Masato Nakajima
发明人： Hiroko Kaneko , Akira Negishi , Ken Nozaki , Kanji Sato , Masato Nakajima
IPC分类号： H01M8/18 , H01M6/18
CPC分类号： B60L11/1879 , B60L11/1868 , H01M8/18 , Y02E60/528 , Y02T10/7005 , Y02T10/7066
摘要： In a redox battery including an electrolytic cell which has a circulating type electrolytic solution and an intermittent circulating type electrolytic solution which has a membrane and which employs an electrolytic solution permeable porous electrode, a solution of vanadium (II/III) dissolved in sulfuric acid is used as an active material on the negative electrode of a redox couple, and an oxidizing substance in a gas (such as oxygen) or in electrolytic solution is used as an active material on the positive electrode of the redox couple. The redox battery of the invention shows high energy density, and has a small size and a high output, thus it can be used for an electric vehicle or as a portable battery.
摘要翻译：在包括具有循环型电解液的电解池和间隔循环型电解液的氧化还原电池中，其具有膜并且使用电解液渗透性多孔电极，溶解在硫酸中的钒（II / III）溶液为在氧化还原对的负极上用作活性物质，在氧化还原对的正极上使用气体（如氧气）或电解液中的氧化物质作为活性物质。本发明的氧化还原电池显示出高能量密度，并且具有小尺寸和高输出，因此可用于电动车辆或便携式电池。

7. 发明授权

US4465576A Method for surface treatment of carbon catalyst 失效
标题翻译：碳催化剂表面处理方法
公开(公告)号：US4465576A
公开(公告)日：1984-08-14
申请号：US475948
申请日：1983-03-16
申请人： Akira Negishi , Ken Nozaki
发明人： Akira Negishi , Ken Nozaki
IPC分类号： B01J21/18 , B01J37/34 , C01B31/08 , C04B41/53 , C04B41/91 , H01M4/96 , C23C15/00
CPC分类号： C04B41/009 , C04B41/5346 , C04B41/91 , H01M4/96
摘要： A carbon catalyst is activated by subjecting the carbon catalyst to a treatment of dry etching utilizing the activity of low-temperature plasma generated by electric discharge under vacuum.
摘要翻译：利用在真空下通过放电产生的低温等离子体的活性，对碳催化剂进行干法蚀刻处理来活化碳催化剂。

8. 发明授权

US5273639A Probe electrode 失效
标题翻译：探头电极
公开(公告)号：US5273639A
公开(公告)日：1993-12-28
申请号：US905238
申请日：1992-06-29
申请人： Hiroko Kaneko , Ken Nozaki , Akira Negishi
发明人： Hiroko Kaneko , Ken Nozaki , Akira Negishi
IPC分类号： G01N27/30
CPC分类号： G01N27/308
摘要： A method of making a probe electrode includes the steps of kneading a mixture of 75-80% by weight of a carbon material, 10-14% by weight of an organic binder and 7-9% by weight of mineral oil, forming the kneaded mixture into a predetermined shape, heating the shaped mixture in air the temperature of up to 300.degree. C. and raising the temperature in an atmosphere of inert gas up to 1000.degree. C.
摘要翻译：制造探针电极的方法包括以下步骤：将75-80重量％的碳材料，10-14重量％的有机粘合剂和7-9重量％的矿物油混合，形成捏合的混合物形成预定形状，在空气中将成形混合物加热至高达300℃，并将其在惰性气体气氛中升温至1000℃。

9. 发明授权

US4814241A Electrolytes for redox flow batteries 失效
标题翻译：电解液用于氧化还原电池
公开(公告)号：US4814241A
公开(公告)日：1989-03-21
申请号：US025990
申请日：1987-03-16
申请人： Ikuo Nagashima , Jun Fukui , Hiroshi Gotoh , Hiroko Kaneko , Ken Nozaki , Takeo Ozawa
发明人： Ikuo Nagashima , Jun Fukui , Hiroshi Gotoh , Hiroko Kaneko , Ken Nozaki , Takeo Ozawa
IPC分类号： H01M8/18 , H01M8/08
CPC分类号： H01M8/188 , Y02E60/528
摘要： An electrolyte for a Redox flow battery contains from 1 to 4 normal hydrochloric acid and at least 0.5 mole/liter of an active material, and further contains from 0.1 to 4 normalities of an acid comprising an anion which does not inhibit the electrode reactions in addition to the hydrochloric acid. This electrolyte reduces the cell resistivity and improves the solubility of active materials.
摘要翻译：用于氧化还原液流电池的电解液包含1至4个常规盐酸和至少0.5摩尔/升活性物质，并且还包含0.1至4个正常的包含不抑制电极反应的阴离子的酸到盐酸。该电解质降低电池电阻率并改善活性材料的溶解度。

10. 发明申请

US20070163889A1 Method and apparatus for producing hydrogen 审中-公开
标题翻译：生产氢气的方法和装置
公开(公告)号：US20070163889A1
公开(公告)日：2007-07-19
申请号：US10589815
申请日：2005-02-17
申请人： Tohru Kato , Ken Nozaki , Hiroshi Yokota , Chi Matsumura , Hiroyuki Yamada
发明人： Tohru Kato , Ken Nozaki , Hiroshi Yokota , Chi Matsumura , Hiroyuki Yamada
IPC分类号： C25B1/02
CPC分类号： C25B1/04 , C25B9/08 , C25B15/08 , Y02E60/366
摘要： An electrolyzer structure is provided that is suitable for use in a method that produces hydrogen by steam electrolysis by feeding reducing gas to an anode side and feeding steam to a cathode side of an electrolyzer that is partitioned into the anode side and the cathode side by a diaphragm of solid oxide electrolyte, and feeding power to the anode and cathode of the electrolyzer. One embodiment of the present invention relates to an apparatus that produces hydrogen by high temperature steam electrolysis and that comprises an electrolyzer partitioned into an anode side and a cathode side by a solid oxide electrolyte diaphragm, a conduit that feeds reducing gas to the anode side of the electrolyzer, and a conduit that feeds steam to the cathode of the electrolyzer, in which a metal cermet stable in a reducing atmosphere is used as the material of the anode and the cathode. Another embodiment of the present invention relates to a method of producing hydrogen by high temperature steam electrolysis for reducing electrolysis voltage by feeding steam to a cathode side and feeding hydrocarbon-containing gas to an anode side for reaction with oxygen ion, the cathode side and the anode side being provided in a high temperature steam electrolytic apparatus in which an electrolyzer is partitioned into the anode side and the cathode side using a solid oxide electrolyte as the diaphragm, wherein offgas discharged from the anode side of the electrolytic apparatus is admixed into the hydrocarbon-containing gas that is fed to the anode side of the electrolytic apparatus.
摘要翻译：提供一种适用于通过蒸汽电解产生氢气的方法的电解器结构，其通过将还原气体供给到阳极侧并将蒸汽供给到分隔成阳极侧和阴极侧的电解槽的阴极侧，由固体氧化物电解质膜片，并向电解槽的阳极和阴极供电。本发明的一个实施例涉及一种通过高温蒸汽电解产生氢的装置，其包括通过固体氧化物电解质隔膜分隔成阳极侧和阴极侧的电解槽，将还原气体供给到阳极侧的导管电解槽以及向蒸发器的阴极供给蒸汽的导管，其中使用在还原气氛中稳定的金属陶瓷作为阳极和阴极的材料。本发明的另一个实施方案涉及一种通过高温蒸汽电解生产氢气的方法，用于通过向阴极侧供给蒸汽并将含烃气体供给到阳极侧以与氧离子，阴极侧和阳极侧设置在高温蒸汽电解装置中，其中使用固体氧化物电解质作为隔膜将电解器分隔成阳极侧和阴极侧，其中从电解装置的阳极侧排出的废气被混合到烃中供给到电解设备的阳极侧的气体。

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