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1. 发明专利

JP2004107318A Method for halogenating benzene and benzene derivative 审中-公开
公开(公告)号：JP2004107318A
公开(公告)日：2004-04-08
申请号：JP2003075145
申请日：2003-03-19
申请人： Toray Ind Inc , 東レ株式会社
发明人： UCHIYAMA NAOYUKI , YOSHIKAWA MASATO , KATO HAJIME , MINOMIYA HIDEKAZU
IPC分类号： C07C17/12 , C07B61/00 , C07C25/02 , C07C25/08 , C07C25/10 , C07C25/125
摘要： PROBLEM TO BE SOLVED: To provide a method for the selective production of a disubstituted halogenated benzene derivative having substituents at the para-sites or a trisubstituted halogenated benzene derivative having substituents at 1, 2, 4-sites by the halogenation of benzene or a benzene derivative. SOLUTION: Benzene or a benzene derivative is halogenated by using a zeolite as a catalyst. A zeolite such as a type-L zeolite containing fluorine as a catalyst is used in the production method. The reaction is preferably carried out in the presence of a solvent, preferably a halogen-containing compound. COPYRIGHT: (C)2004,JPO

2. 发明专利

JP2013010727A Production method of aromatic hydrocarbon having straight-chain alkyl group, and catalyst 审中-公开
标题翻译：具有直链烷基的芳族碳氢化合物的生产方法和催化剂
公开(公告)号：JP2013010727A
公开(公告)日：2013-01-17
申请号：JP2011145910
申请日：2011-06-30
申请人： Toray Ind Inc , 東レ株式会社
发明人： ARAKI YASUNORI , MINOMIYA HIDEKAZU
IPC分类号： C07C5/22 , B01J29/40 , C07B61/00 , C07C15/02
CPC分类号： Y02P20/52
摘要： PROBLEM TO BE SOLVED: To provide a production method of an aromatic hydrocarbon having a straight-chain alkyl group from an aromatic hydrocarbon having a branched alkyl group, the method suppressing a side reaction and economically excellent.SOLUTION: The production method of an aromatic hydrocarbon having a straight-chain alkyl group comprises bringing an aromatic hydrocarbon having a branched alkyl group into contact with an acid type zeolite catalyst, which is obtained by ion exchange between at least one kind of ion selected from the group consisting of alkali metal ions and alkaline earth metal ions and at least one kind of ion selected from the group consisting of proton and proton precursors.
摘要翻译：待解决的问题：提供具有支链烷基的芳族烃具有直链烷基的芳族烃的制备方法，抑制副反应的方法在经济上优异。解决方案：具有直链烷基的芳族烃的制备方法包括使具有支链烷基的芳族烃与酸型沸石催化剂接触，所述酸型沸石催化剂通过至少一种离子选自碱金属离子和碱土金属离子和选自质子和质子前体中的至少一种离子。版权所有（C）2013，JPO＆INPIT

3. 发明专利

JP2008238136A Bifunctional catalyst for dealkylating ethylbenzene and isomerizing xylene 有权
标题翻译：乙酰苯和二异氰酸酯二官能催化剂
公开(公告)号：JP2008238136A
公开(公告)日：2008-10-09
申请号：JP2007086459
申请日：2007-03-29
申请人： Toray Ind Inc , 東レ株式会社
发明人： ICHIOKA YOSHITSUGU , MINOMIYA HIDEKAZU , IMADA YUTAKA
IPC分类号： B01J29/48 , B01J35/10 , C07B61/00 , C07C4/18 , C07C5/27 , C07C15/04 , C07C15/08
CPC分类号： Y02P20/52
摘要： PROBLEM TO BE SOLVED: To provide a catalyst molding for dealkylating ethylbenzene in a raw material containing 8C aromatic hydrocarbons into benzene at a high conversion ratio and isomerizing xylene into paraxylene at a high isomerization ratio. SOLUTION: The bifunctional catalyst for dealkylating ethylbenzene and isomerizing xylene consists of a composition obtained by blending MFI-type zeolite with an inorganic oxide, is the catalyst molding having a group of pores each having 4-20 nm pore diameter and ≥0.45 mL/g pore volume and contains an alkaline earth metal. COPYRIGHT: (C)2009,JPO&INPIT
摘要翻译：要解决的问题：提供一种催化剂成型用于将含有8个芳香烃的原料中的乙苯脱氢烷基化成苯，并以高转化率将二甲苯以高异构化比例异构化成对二甲苯。解决方案：用于使乙苯和异构化二甲苯脱烷基化的双官能催化剂由通过将MFI型沸石与无机氧化物共混而获得的组合物组成，具有孔组的催化剂成型体具有孔径为4-20nm且≥0.45 mL / g孔体积，并含有碱土金属。版权所有（C）2009，JPO＆INPIT

4. 发明专利

JP2004107317A Method for halogenating benzene and benzene derivative 审中-公开
标题翻译：苯并苯和苯甲酸衍生物的方法
公开(公告)号：JP2004107317A
公开(公告)日：2004-04-08
申请号：JP2003075144
申请日：2003-03-19
申请人： Toray Ind Inc , 東レ株式会社
发明人： KATO HAJIME , MINOMIYA HIDEKAZU , UCHIYAMA NAOYUKI , YOSHIKAWA MASATO
IPC分类号： C07C25/125 , C07B61/00
摘要： PROBLEM TO BE SOLVED: To provide a method for the selective production of a disubstituted halogenated benzene derivative having substituents at the para-sites or a trisubstituted halogenated benzene derivative having substituents at 1,2,4-sites by the halogenation of benzene or a benzene derivative.
SOLUTION: Benzene or a benzene derivative is halogenated by using a zeolite as a catalyst. A zeolite such as a type-L zeolite having a crystallite diameter of ≤100 nm as a catalyst is used in the production method. The reaction is preferably carried out in the presence of a solvent, preferably a halogen-containing compound.
COPYRIGHT: (C)2004,JPO
摘要翻译：待解决的问题：提供选择性制备在对位具有取代基的二取代卤代苯衍生物或通过苯的卤化在1,2,4-位具有取代基的三取代卤代苯衍生物的方法或苯衍生物。解决方案：使用沸石作为催化剂将苯或苯衍生物卤化。在制造方法中使用沸石，例如微晶直径≤100nm的L型沸石作为催化剂。反应优选在溶剂，优选含卤素化合物的存在下进行。版权所有（C）2004，JPO

5. 发明专利

JP2004059447A Method for chlorinating disubstituted benzene derivative 审中-公开
公开(公告)号：JP2004059447A
公开(公告)日：2004-02-26
申请号：JP2002216453
申请日：2002-07-25
申请人： Toray Ind Inc , 東レ株式会社
发明人： MINOMIYA HIDEKAZU , KATO HAJIME , UCHIYAMA NAOYUKI , YOSHIKAWA MASATO
IPC分类号： C07C17/12 , C07B61/00 , C07C25/125
摘要： PROBLEM TO BE SOLVED: To provide a technique for selectively producing a 1,2,4-trisubstitution product in production of a trisubstituted chlorinated derivative by chlorinating a disubstituted benzene derivative having a substituent at the o- or the m-position.
SOLUTION: The disubstituted benzene derivative having the substituent at the o- or the p-position is chlorinated in the coexistence of a solvent using zeolite as a catalyst. In the process, a chlorinating reaction is carried out by using prediluted chlorine gas. The zeolite is preferably type L zeolite. The solvent is preferably a chloro-containing compound.
COPYRIGHT: (C)2004,JPO

6. 发明专利

JP2004043449A Method for producing halogenated benzene derivative 审中-公开
公开(公告)号：JP2004043449A
公开(公告)日：2004-02-12
申请号：JP2003135661
申请日：2003-05-14
申请人： Toray Ind Inc , 東レ株式会社
发明人： YOSHIKAWA MASATO , MINOMIYA HIDEKAZU , KATO HAJIME , UCHIYAMA NAOYUKI
IPC分类号： C07C17/12 , C07B61/00 , C07C25/02 , C07C25/125
摘要： PROBLEM TO BE SOLVED: To provide a method for producing a halogenated benzene derivative by the halogenation of a benzene derivative to selectively form a p-substituted halogenated benzene derivative while reducing the by-production of o-substituted halogenated benzene derivative, m-substituted halogenated benzene derivative, and the like in a disubstituted halogenated benzene derivative or to form a 1,2,4-trisubstituted derivative while reducing the by-production of a 1,2,3-trisubstituted benzene derivative, and the like, in a trisubstituted halogenated derivative.
SOLUTION: The halogenated benzene derivative is produced by halogenating the benzene derivative. In the process, the halogenation product is further halogenated after the 100% conversion of the benzene derivative.
COPYRIGHT: (C)2004,JPO

7. 发明专利

JP2012139618A Catalyst for conversion of mixed raw material comprising ethylbenzene and xylene, and conversion method using the same 审中-公开
标题翻译：用于转化包含乙烯和二甲苯的混合原料的催化剂和使用其的转化方法
公开(公告)号：JP2012139618A
公开(公告)日：2012-07-26
申请号：JP2010292448
申请日：2010-12-28
申请人： Toray Ind Inc , 東レ株式会社
发明人： YOSHIKAWA TAKAHIRO , WATANABE MASATOSHI , MINOMIYA HIDEKAZU
IPC分类号： B01J29/48 , C07B61/00 , C07C5/27 , C07C6/12 , C07C15/04 , C07C15/08
CPC分类号： Y02P20/52
摘要： PROBLEM TO BE SOLVED: To provide a catalyst for the conversion of a mixed raw material comprising ethylbenzene and xylenes, capable of attaining high conversion of xylenes to p-xylene with a small xylene loss and of exhibiting high ethylbenzene conversion performance at a low reaction temperature, upon causing a mixed raw material comprising ethylbenzene and xylenes to contact the catalyst to convert ethylbenzene present therein primarily to benzene and to isomerize xylenes present therein, and a conversion method using the same.SOLUTION: The catalyst obtained by subjecting a sodium-type MFI zeolite and a chemical liquid comprising a sodium ion and at least one cation other than the sodium ion to an ion exchange treatment is used in the method.
摘要翻译：要解决的问题：提供一种用于转化包含乙苯和二甲苯的混合原料的催化剂，其能够以较小的二甲苯损失获得二甲苯向对二甲苯的高转化率，并且在在使含有乙苯和二甲苯的混合原料与催化剂接触以将其中存在的乙苯转化为苯并使其中存在的二甲苯异构化的反应温度低的反应温度下，以及使用其的转化方法。解决方案：在该方法中使用通过使钠型MFI沸石和包含钠离子和至少一种阳离子以外的钠离子的化学液进行离子交换处理而获得的催化剂。版权所有（C）2012，JPO＆INPIT

8. 发明专利

JP2008106031A Method for conversion of ethylbenzene and method for production of para-xylene 有权
标题翻译：乙烯苯的转化方法及其制备方法
公开(公告)号：JP2008106031A
公开(公告)日：2008-05-08
申请号：JP2007018818
申请日：2007-01-30
申请人： Toray Ind Inc , 東レ株式会社
发明人： ICHIOKA YOSHITSUGU , MINOMIYA HIDEKAZU , YAMAKAWA SHINOBU
IPC分类号： C07C4/18 , C07B61/00 , C07C5/27 , C07C6/12 , C07C15/04 , C07C15/06 , C07C15/08
CPC分类号： Y02P20/52
摘要： PROBLEM TO BE SOLVED: To provide an ethylbenzene conversion method for converting ethylbenzene in a raw material containing an 8C aromatic hydrocarbon to benzene in a high conversion rate. SOLUTION: The ethylbenzene conversion method comprises bringing a mixed raw material of an 8C aromatic hydrocarbon containing ethylbenzene into contact with an acid type catalyst containing at least one metal selected from the metals of the groups VII and VIII in the presence of H 2 , to convert ethylbenzene to benzene. The raw material comprises an ethyltoluene-containing 9-10C aromatic hydrocarbon and the ethyltoluene is converted to toluene with the conversion of the ethylbenzene. COPYRIGHT: (C)2008,JPO&INPIT
摘要翻译：要解决的问题：提供一种乙苯改性方法，用于将含有8芳香烃的原料中的乙苯以高转化率转化为苯。解决方案：乙苯转化方法包括使含有乙苯的8C芳族烃的混合原料与含有选自第Ⅶ和Ⅷ族金属的至少一种金属的酸式催化剂在H 2存在下接触， SB> 2 ，将乙苯转化为苯。该原料包括含有甲基甲苯的9-10C芳烃，乙基甲苯转化为甲苯，转化为乙苯。版权所有（C）2008，JPO＆INPIT

9. 发明专利

JP2003342205A METHOD FOR PRODUCING 4-CHLORO-o-XYLENE 审中-公开
标题翻译：生产4-氯代邻苯二甲酸的方法
公开(公告)号：JP2003342205A
公开(公告)日：2003-12-03
申请号：JP2002152459
申请日：2002-05-27
申请人： Toray Ind Inc , 東レ株式会社
发明人： UCHIYAMA NAOYUKI , YOSHIKAWA MASATO , MINOMIYA HIDEKAZU , KATO HAJIME
IPC分类号： B01J29/60 , C07B61/00 , C07C17/12 , C07C25/125
CPC分类号： Y02P20/52
摘要： PROBLEM TO BE SOLVED: To provide a technique of a method for suppressing the formation of 3-chloro-o-xylene and selectively synthesizing 4-chloro-o-xylene with a high activity in a method for chlorinating o-xylene and affording the 4-chloro-o- xylene. SOLUTION: This method for producing the 4-chloro-o-xylene comprises using the following zeolite as a catalyst. The zeolite contains Rb and/or Cs, has ≤0.1 wt.% of Na content or contains ≥0.1 and ≤5 wt.% of a transition metal. Zeolite L is preferably used as the zeolite. COPYRIGHT: (C)2004,JPO

10. 发明专利

JP2008161738A Activity restoring method of zeolite catalyst 审中-公开
标题翻译：沸石催化剂的活性恢复方法
公开(公告)号：JP2008161738A
公开(公告)日：2008-07-17
申请号：JP2006350794
申请日：2006-12-27
申请人： Toray Ind Inc , 東レ株式会社
发明人： YOSHIKAWA TAKAHIRO , MINOMIYA HIDEKAZU
IPC分类号： B01J29/90 , B01J29/40 , B01J38/48
摘要： PROBLEM TO BE SOLVED: To provide a method for restoring the activity of a zeolite catalyst by simple treatment when an aromatic compound is reacted in a liquid phase using the zeolite catalyst, and a method for facilitating the control of activity restoring operation without performing exothermic operation such as combustion or the like and avoiding the destruction of the crystal structure of zeolite caused by heat, steaming, etc.
SOLUTION: In the activity restoring method of the zeolite catalyst used in the reaction of the aromatic compound in the liquid phase, water is adsorbed in the zeolite catalyst at 50°C or lower before the zeolite catalyst is subjected to ageing operation at a reaction temperature or below.
COPYRIGHT: (C)2008,JPO&INPIT
摘要翻译：待解决的问题：提供一种通过使用沸石催化剂在液相中使芳族化合物反应时通过简单的处理来恢复沸石催化剂的活性的方法，以及用于有助于控制活性恢复操作的方法而没有进行放热操作，如燃烧等，避免由热，蒸汽等引起的沸石的晶体结构的破坏。解决方案：在芳族化合物的反应中使用的沸石催化剂的活性还原方法在沸石催化剂在反应温度以下进行老化操作之前，液相中的水吸附在沸石催化剂中，在50℃以下。版权所有（C）2008，JPO＆INPIT

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