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1. 发明授权

US4647625A Process for modifying conjugated diene polymers 失效
标题翻译：改性共轭二烯聚合物的方法
公开(公告)号：US4647625A
公开(公告)日：1987-03-03
申请号：US685234
申请日：1984-12-21
申请人： Mitsuyoshi Aonuma , Hiroyuki Watanabe , Haruki Kawada , Kohkichi Noguchi , Akio Ueda , Shuichi Akita , Tetsuo Ohyama , Toshio Kase
发明人： Mitsuyoshi Aonuma , Hiroyuki Watanabe , Haruki Kawada , Kohkichi Noguchi , Akio Ueda , Shuichi Akita , Tetsuo Ohyama , Toshio Kase
IPC分类号： C08C19/42 , C08F8/30 , C08F8/34
CPC分类号： C08C19/42
摘要： A process for modifying a polymer of a conjugated diene, which comprises reacting a polymer of a conjugated diene containing at least one metal selected from alkali metals and alkaline earth metals with a compound having a linkage of the following formula ##STR1## wherein X represents an oxygen or sulfur atom, in the molecule.
摘要翻译：一种改性共轭二烯的聚合物的方法，该方法包括使含有至少一种选自碱金属和碱土金属的金属的共轭二烯的聚合物与具有以下结构式的化合物反应，其中X表示氧或硫原子。

2. 发明授权

US4848511A Vibration insulating rubber 失效
标题翻译：隔振橡胶
公开(公告)号：US4848511A
公开(公告)日：1989-07-18
申请号：US219820
申请日：1988-07-15
申请人： Tetsuo Ohyama , Shuichi Akita , Hiroyuki Watanabe , Akio Ueda
发明人： Tetsuo Ohyama , Shuichi Akita , Hiroyuki Watanabe , Akio Ueda
IPC分类号： C08L15/00 , C08C19/42 , C08F8/30 , C08F8/34 , C08L7/00 , C08L21/00 , C08L23/00 , C08L33/00 , C08L33/02 , C08L101/00
CPC分类号： C08C19/42
摘要： A vibration insulating rubber having an improved balance between its loss tangent and dynamic-to-static modulus ratio is prepared by molding and curing a rubber compound comprising as a rubber component a modified rubbery polymer obtained by reacting (1) a rubbery polymer having at least one metal selected from alkali metals and alkaline earth metals bonded to its molecular chain with (2) at least one compound selected from organic compounds having a bond of the formula ##STR1## wherein X represents an oxygen or sulfur atom, in the molecule, benzophenones having at least one of unsubstituted and substituted amino groups, and thiobenzophenones having at least one of unsubstituted or substituted amino groups.
摘要翻译：通过将包含作为橡胶组分的橡胶化合物通过将（1）至少具有至少一种橡胶状聚合物的橡胶状聚合物反应而获得的改性橡胶状聚合物成型和固化，从而制备其损耗角正切和动静态模量比之间的平衡改善的隔振橡胶选自与其分子链结合的碱金属和碱土金属的一种金属（2）至少一种选自具有下式键的有机化合物的化合物，其中X表示氧或硫原子，在分子中，二苯甲酮具有至少一个未取代和取代的氨基，和具有至少一个未取代或取代的氨基的硫代二苯甲酮。

3. 发明授权

US4414363A Rubber composition 失效
标题翻译：橡胶组成
公开(公告)号：US4414363A
公开(公告)日：1983-11-08
申请号：US388973
申请日：1982-06-16
申请人： Shuichi Akita , Takeshi Chida , Hiroyuki Watanabe , Akio Ueda
发明人： Shuichi Akita , Takeshi Chida , Hiroyuki Watanabe , Akio Ueda
IPC分类号： C08L9/00 , C08L47/00
CPC分类号： C08L7/00 , C08L9/00
摘要： A rubber composition comprising as main components (1) at least one rubber having a glass transition temperature of from -45.degree. C. to 0.degree. C. and selected from the group consisting of an isoprene-butadiene copolymer rubber and polyisoprene rubber and (2) at least one rubber selected from the group consisting of natural rubber and cis-1,4-polyisoprene rubber having a cis-1,4-linkage content of at least 90 mole %, said composition having a value, defined by the following formula, of at least 10,[(R-53)+(S-100)]wherein R is a rebound (%) measured at 51.degree. C. by a Dunlop Tripso meter for a vulcanized product of said rubber composition, and S, as defined in the specification, is a wet skid resistance index on a road surface defined by ASTM E-303-74 which is determined at 19.degree. C. by a portable skid tester for a vulcanized product of said rubber composition.
摘要翻译：一种橡胶组合物，其包含主要组分（1）至少一种玻璃化转变温度为-45℃至0℃的橡胶，并且选自异戊二烯 - 丁二烯共聚物橡胶和聚异戊二烯橡胶和（2 ）至少一种选自顺式-1,4-键含量为至少90摩尔％的天然橡胶和顺式-1,4-聚异戊二烯橡胶的橡胶，所述组合物具有由下式定义的值至少10，[（R-53）+（S-100）]其中R是在51℃下用于所述橡胶组合物的硫化产品的Dunlop Tripso计测量的回弹率（％），如在说明书中所定义的，是由ASTM E-303-74限定的路面上的抗湿滑性指数，其通过用于所述橡胶组合物的硫化产品的便携式防滑测试仪在19℃下测定。

4. 发明授权

US4555548A Rubber composition for tire treads 失效
标题翻译：轮胎胎面橡胶组合物
公开(公告)号：US4555548A
公开(公告)日：1985-11-26
申请号：US643420
申请日：1984-08-23
申请人： Akio Ueda , Shuichi Akita , Takeshi Chida
发明人： Akio Ueda , Shuichi Akita , Takeshi Chida
IPC分类号： B60C1/00 , C08C19/44 , C08L9/06 , C08L7/00 , C08L9/00
CPC分类号： C08L7/00 , B60C1/0016 , C08C19/44 , C08L21/00 , C08L9/06 , C08L9/00
摘要： A rubber composition for tire treads, comprising [I] 10 to 90% by weight of a styrene-butadiene copolymer rubber containing not more than 40% by weight of bound styrene and having bonded to a carbon atom of the rubber molecular chain at least 0.1 mole, per mole of the rubber molecular chain, of an atomic grouping represented by the following formula ##STR1## wherein: X represents O or S,R.sub.1 and R.sub.2 are identical or different and each represents an amino group or an alkyl-substituted amino group,R.sub.3 and R.sub.4 are identical or different and each represents a substituent other than the above-mentioned,m, p and q each represent O or an integer of at least 1,n represents an integer of at least 1, m+p=0-5, and n+q=1-5,and [II] 90 to 10% by weight of at least one rubber selected from the group consisting of styrene-butadiene copolymer rubber having a bound styrene content of not more than 40% by weight and polyisoprene rubber.
摘要翻译：一种用于轮胎胎面的橡胶组合物，其包含[I] 10至90重量％的含有不超过40重量％的结合苯乙烯并且与橡胶分子链的碳原子键合的苯乙烯 - 丁二烯共聚物橡胶至少为0.1 摩尔每摩尔橡胶分子链，由下式表示的原子组分其中：X表示O或S，R 1和R 2相同或不同，各自表示氨基或烷基取代的氨基，R 3和R 4相同或不同，各自表示除上述以外的取代基，m，p和q各自表示O或至少为1的整数，n表示至少为1的整数，m + p = 0 -5和n + q = 1-5，和[II] 90至10重量％的选自苯乙烯含量不大于40％的苯乙烯含量的苯乙烯 - 丁二烯共聚物橡胶中的至少一种橡胶由重量和聚异戊二烯橡胶。

5. 发明授权

US4555547A Rubber composition for tire treads 失效
标题翻译：轮胎胎面橡胶组合物
公开(公告)号：US4555547A
公开(公告)日：1985-11-26
申请号：US643421
申请日：1984-08-23
申请人： Akio Ueda , Shuichi Akita , Toshio Namizuka
发明人： Akio Ueda , Shuichi Akita , Toshio Namizuka
IPC分类号： B60C1/00 , C08C19/44 , C08L9/00 , C08L7/00 , C08L9/06
CPC分类号： C08L7/00 , B60C1/0016 , C08C19/44 , C08L9/00 , C08L9/06
摘要： A rubber composition for tire treads, comprising [I] 10 to 70% by weight of a polybutadiene rubber having bonded to a carbon atom of the rubber molecular chain at least 0.1 mole, per mole of the rubber molecular chain, of an atomic grouping represented by the following formula ##STR1## wherein X represents O or S, R.sub.1 and R.sub.2 are identical or different and each represents an amino group or an alkyl-substituted amino group, R.sub.3 and R.sub.4 are identical or different and each represents a substituent other than the above-mentioned, m, p and q each represent O or an integer of at least 1, n represents an integer of at least 1, m+p=0-5, and n+q=1-5,and [II] 90 to 30% by weight of at least one rubber selected from the group consisting of styrene-butadiene copolymer rubber having a bound stryene content of not more than 50% by weight and polyisoprene rubber.
摘要翻译：一种用于轮胎胎面的橡胶组合物，其包含10至70重量％的聚丁二烯橡胶，其每摩尔橡胶分子链与橡胶分子链的碳原子键合至少0.1摩尔，表示为原子组通过下式通过其中X表示O或S，R 1和R 2相同或不同，各自表示氨基或烷基取代的氨基，R 3和R 4相同或不同，并且各自表示除上述m，p和q各自表示O或至少为1的整数，n表示至少为1的整数，m + p = 0-5，n + q = 1-5，[II] 90〜30重量％的选自苯乙烯 - 丁二烯共聚物橡胶中的至少一种橡胶，其结合的苯乙烯含量不超过50重量％，聚异戊二烯橡胶。

6. 发明授权

US4321168A Process for preparing rubber composition for tire treads 失效
标题翻译：制备轮胎胎面橡胶组合物的方法
公开(公告)号：US4321168A
公开(公告)日：1982-03-23
申请号：US116887
申请日：1980-01-30
申请人： Akio Ueda , Shuichi Akita , Hiroshi Hirakawa , Asahiro Ahagon
发明人： Akio Ueda , Shuichi Akita , Hiroshi Hirakawa , Asahiro Ahagon
IPC分类号： C08L7/00 , B60C1/00 , C08J3/20 , C08J3/22 , C08K3/04 , C08K3/18 , C08L21/00 , C08L47/00
CPC分类号： B60C1/0016 , C08L21/00 , Y10S152/905
摘要： A process for preparing a tire tread rubber composition having improved rolling resistance and wet skid resistance comprising [I] 100 parts by weight of a rubber material composed of 25 to 75% by weight of substantially amorphous polybutadiene having a 1,2-bond unit content of 65 to 90 mole % and a Mooney viscosity (ML.sub.1+4, 100.degree. C.) of 20 to 100 and 75 to 25% by weight of natural rubber and/or cis-1,4-polyisoprene, and [II] 40 to 70 parts by weight of carbon black, said process comprising (1) mechanically compounding 40 to 60 parts by weight of the rubber material [I] with 40 to 70 parts by weight of carbon black [II], and then (2) adding to the resulting mixture the rubber material [I] in an amount sufficient to adjust the amount of the carbon black [II] to 40 to 70 parts by weight per 100 parts by weight of the rubber material [I] and mechanically compounding them.
摘要翻译：一种制备具有改善的滚动阻力和耐湿滑性的轮胎胎面橡胶组合物的方法，其包括：[I] 100重量份由25-75重量％的具有1,2-键单元含量的基本无定形聚丁二烯组成的橡胶材料为65至90摩尔％，门尼粘度（ML1 + 4，100℃）为20至100和75至25重量％的天然橡胶和/或顺式-1,4-聚异戊二烯，和[II] 40 至70重量份的炭黑，所述方法包括（1）将40至60重量份的橡胶材料[I]与40至70重量份的炭黑[II]机械混合，然后（2）加入对于所得混合物，橡胶材料[I]的量足以将炭黑[II]的量调节至40至70重量份/ 100重量份的橡胶材料[I]并机械混合它们。

7. 发明授权

US4224197A Rubber composition for tire tread 失效
标题翻译：轮胎胎面橡胶组合物
公开(公告)号：US4224197A
公开(公告)日：1980-09-23
申请号：US55520
申请日：1979-07-09
申请人： Akio Ueda , Shuichi Akita
发明人： Akio Ueda , Shuichi Akita
IPC分类号： C08L47/00 , B60C1/00 , C08L7/00 , C08L9/00 , C08L21/00 , C08L45/00
CPC分类号： B60C1/0016 , C08L9/00 , C08L7/00 , C08L9/06 , Y10S152/905
摘要： A rubber composition for the tread of tire having reduced rolling resistance and increased wet skid resistance with the mechanical properties unimpaired, said rubber composition comprising 20 to 80% by weight of (I) essentially amorphous polybutadiene having a 1,2-bond units content of at least 70% and a Mooney viscosity (ML.sub.1+4, 100.degree. C.) of 10 to 100; 10 to 75% by weight of (II) polybutadiene rubber having a 1,2-bond units content of 20% or less and a Mooney viscosity (ML.sub.1+4, 100.degree. C.) of 20 to 130; and 3 to 35% by weight of (III) at least one rubber selected from styrene/butadiene copolymer rubber having a bound styrene content of 15 to 25% by weight, natural rubber, and polyisoprene rubber having a cis-1,4-bond units content of at least 90%.
摘要翻译：一种用于轮胎胎面的橡胶组合物，具有降低的滚动阻力和增加的耐湿滑性，机械性能未受损，所述橡胶组合物包含20至80重量％的（I）基本无定形聚丁二烯，其具有1,2-键单元含量至少70％，门尼粘度（ML1 + 4,100℃）为10〜100; 10〜75重量％的1,2-结构单元含量为20％以下，门尼粘度（ML1 + 4,100℃）为20〜130的（II）聚丁二烯橡胶; 和3〜35重量％的（III）选自苯乙烯含量为15〜25重量％的苯乙烯/丁二烯共聚物橡胶中的至少一种橡胶，天然橡胶和具有顺式-1,4-键的聚异戊二烯橡胶单位含量至少为90％。

8. 发明授权

US4677165A Rubber composition for tire tread 失效
标题翻译：轮胎胎面橡胶组合物
公开(公告)号：US4677165A
公开(公告)日：1987-06-30
申请号：US920335
申请日：1986-10-17
申请人： Yasushi Kikuchi , Kazuyoski Kayama , Akinori Tokieda , Hiroyuki Watanabe , Shuichi Akita
发明人： Yasushi Kikuchi , Kazuyoski Kayama , Akinori Tokieda , Hiroyuki Watanabe , Shuichi Akita
IPC分类号： B60C1/00 , C08K3/04 , C08L9/06 , C08L21/00 , C08F236/10
CPC分类号： B60C1/0016 , C08L9/06 , C08L7/00 , C08L9/00 , C08L9/02
摘要： A rubber composition for a tire tread comprising a novel modified styrene-butadiene copolymer rubber, carbon black, and aromatic oil.
摘要翻译：一种用于轮胎胎面的橡胶组合物，包括新型改性苯乙烯 - 丁二烯共聚物橡胶，炭黑和芳香油。

9. 发明授权

US5218023A Rubber composition and process for preparing same 失效
标题翻译：橡胶组合物及其制备方法
公开(公告)号：US5218023A
公开(公告)日：1993-06-08
申请号：US677186
申请日：1991-03-29
申请人： Hiroyoshi Horikawa , Shuichi Akita , Hiroyuki Watanabe
发明人： Hiroyoshi Horikawa , Shuichi Akita , Hiroyuki Watanabe
IPC分类号： C08K3/04 , C08C19/44 , C08K5/00 , C08K5/56 , C08L21/00
CPC分类号： C08C19/44 , C08L21/00
摘要： A rubber composition comprising a rubbery polymer, carbon black and a processing aid is described wherein the processing aid is a liquid diene polymer having a weight average molecular weight of about 5,000 to 140,000 and having an atomic group having a bond represented by the formula:>C.dbd.N.sup..crclbar.
摘要翻译：描述了一种包含橡胶状聚合物，炭黑和加工助剂的橡胶组合物，其中加工助剂是重均分子量为约5,000至140,000且具有由下式表示的键的原子团的液态二烯聚合物： C = N（ - ），其结合到聚合物链的末端，液体二烯聚合物的量相对于每100重量份的橡胶状聚合物为1〜100重量份。液体二烯聚合物通常通过使阴离子活性液体二烯聚合物与分子中具有由下式表示的键的化合物反应来制备：其中M表示氧或硫原子。

10. 发明授权

US5001196A Process for preparation of diene type polymer rubber 失效
标题翻译：二烯型聚合物橡胶的制备方法
公开(公告)号：US5001196A
公开(公告)日：1991-03-19
申请号：US330025
申请日：1989-03-29
申请人： Takafumi Kawanaka , Hiroyuki Watanabe , Kohkichi Noguchi , Shuichi Akita
发明人： Takafumi Kawanaka , Hiroyuki Watanabe , Kohkichi Noguchi , Shuichi Akita
IPC分类号： C08L15/00 , C08C19/42 , C08F8/30 , C08L21/00
CPC分类号： C08C19/42
摘要： An improved diene type polymer rubber is prepared by reacting a diene type polymer rubber, to which an alkali metal and/or an alkaline earth metal has been added, with a compound represented by the formula: ##STR1## wherein M is oxygen or sulfur, R.sub.1 and R.sub.4 are a substituent having no hydrogen on the .alpha.-carbon atom, R.sub.2 and R.sub.3 are hydrogen or a hydrocarbon group, m is an integer of at least 2, and n is an integer of 2 to 4. The diene type polymer rubber is characterized in that, even after storage for a long time, the Mooney viscosity rises only to a very slight extent, and the rebound, wet skid resistance and other physical properties of the cured product thereof are not substantially changed.
摘要翻译：通过使已经加入碱金属和/或碱土金属的二烯类聚合物橡胶与下式表示的化合物反应来制备改进的二烯类聚合物橡胶：其中M是氧或硫， R1和R4是在α-碳原子上没有氢的取代基，R2和R3是氢或烃基，m是至少为2的整数，n是2至4的整数。二烯型聚合物橡胶其特征在于，即使长时间保存，门尼粘度仅上升到非常小的程度，其固化物的回弹，抗湿滑性等物理性质基本上不发生变化。

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