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1. 发明授权

US09224517B2 Paste composition for electrode and photovoltaic cell 有权
标题翻译：糊料组合物用于电极和光伏电池
公开(公告)号：US09224517B2
公开(公告)日：2015-12-29
申请号：US13439955
申请日：2012-04-05
申请人： Shuichiro Adachi , Masato Yoshida , Takeshi Nojiri , Mitsunori Iwamuro , Keiko Kizawa , Takuya Aoyagi , Hiroki Yamamoto , Takashi Naito , Takahiko Kato
发明人： Shuichiro Adachi , Masato Yoshida , Takeshi Nojiri , Mitsunori Iwamuro , Keiko Kizawa , Takuya Aoyagi , Hiroki Yamamoto , Takashi Naito , Takahiko Kato
IPC分类号： H01M4/88 , H01B1/22 , H01L31/0224
CPC分类号： H01B1/22 , H01L31/022425 , H01L31/02245 , Y02E10/50
摘要： A paste composition for an electrode, the paste composition comprising: phosphorous-containing copper alloy particles in which the content of phosphorous is from 6% by mass to 8% by mass; glass particles; a solvent; and a resin.
摘要翻译：一种电极用糊剂组合物，其特征在于，含有磷含量为6质量％〜8质量％的含磷铜合金粒子，玻璃颗粒; 溶剂; 和树脂。

2. 发明授权

US08790549B2 Electronic component provided with Cu—Al—Co-based alloy electrode or wiring 有权
标题翻译：电子元件配有Cu-Al-Co基合金电极或布线
公开(公告)号：US08790549B2
公开(公告)日：2014-07-29
申请号：US13263359
申请日：2010-04-08
申请人： Takahiko Kato , Takashi Naito , Hiroki Yamamoto , Takuya Aoyagi , Seiichi Watanabe , Seiji Miura , Norihito Sakaguchi , Kazuki Aoshima , Kenji Ohkubo
发明人： Takahiko Kato , Takashi Naito , Hiroki Yamamoto , Takuya Aoyagi , Seiichi Watanabe , Seiji Miura , Norihito Sakaguchi , Kazuki Aoshima , Kenji Ohkubo
IPC分类号： H01B1/02 , H05K1/09 , C22C9/00 , C22C9/02 , C22C9/01 , C22C9/06
CPC分类号： C22C9/01 , C22C9/06 , H01J1/02 , H01J2211/225 , H01L31/022425 , H05K1/092 , Y02E10/50
摘要： An object of the present invention is to provide an electronic component using a Cu-based conductive material that can suppress oxidization even in a heat treatment in an oxidizing atmosphere and that can suppress an increase in an electrical resistance. In an electronic component having an electrode or a wiring, a ternary alloy made from three elements consisting of Cu, Al, and Co is used as a Cu-based wiring material that can prevent oxidization of the electrode or the wiring. Specifically, part or the whole of the electrode or the wiring has a chemical composition in which an Al content is 10 at % to 25 at %, a Co content is 5 at % to 20 at %, and the balance is composed of Cu and unavoidable impurities, and the chemical composition represents a ternary alloy in which two phases of a Cu solid solution formed by Al and Co being dissolved into Cu and a CoAl intermetallic compound coexist together.
摘要翻译：本发明的目的是提供一种使用Cu基导电材料的电子部件，即使在氧化气氛中的热处理中也能够抑制氧化，并且能够抑制电阻的增加。在具有电极或布线的电子部件中，使用由Cu，Al和Co组成的三个元素制成的三元合金作为能够防止电极或布线的氧化的Cu系布线材料。具体地说，电极或布线的一部分或全部具有Al含量为10原子％至25原子％的Co化学组成，Co含量为5原子％至20原子％，余量由Cu和不可避免的杂质，化学组成表示三元合金，其中由Al和Co形成的Cu固溶体中的两相溶解于Cu和CoAl金属间化合物共存。

3. 发明申请

US20110180137A1 PASTE COMPOSITION FOR ELECTRODE AND PHOTOVOLTAIC CELL 审中-公开
标题翻译：电极和光电池用糊剂组合物
公开(公告)号：US20110180137A1
公开(公告)日：2011-07-28
申请号：US13012920
申请日：2011-01-25
申请人： Mitsunori Iwamuro , Masato Yoshida , Takeshi Nojiri , Shuuichirou Adachi , Keiko Kizawa , Takuya Aoyagi , Hiroki Yamamoto , Takashi Naito , Takahiko Kato
发明人： Mitsunori Iwamuro , Masato Yoshida , Takeshi Nojiri , Shuuichirou Adachi , Keiko Kizawa , Takuya Aoyagi , Hiroki Yamamoto , Takashi Naito , Takahiko Kato
IPC分类号： H01L31/0224 , H01L31/0216 , H01B1/22
CPC分类号： H01B1/22 , H01L31/022425 , H01L31/02245 , H01L31/068 , Y02E10/547
摘要： The paste composition for an electrode are constituted with metal particles having copper as a main component, a phosphorous-containing compound, glass particles, a solvent, and a resin. Further, the photovoltaic cell has an electrode formed by using the paste composition for an electrode.
摘要翻译：用于电极的糊剂组合物由以铜为主要成分的金属颗粒，含磷化合物，玻璃颗粒，溶剂和树脂构成。此外，光伏电池具有通过使用电极用糊剂组合物形成的电极。

4. 发明授权

US08217274B2 Wiring member, method of manufacturing the wiring member and electronic element 失效
标题翻译：接线构件，配线构件和电子元件的制造方法
公开(公告)号：US08217274B2
公开(公告)日：2012-07-10
申请号：US12793335
申请日：2010-06-03
申请人： Hiroki Yamamoto , Takashi Naito , Takuya Aoyagi , Yuuichi Sawai , Takahiko Kato
发明人： Hiroki Yamamoto , Takashi Naito , Takuya Aoyagi , Yuuichi Sawai , Takahiko Kato
IPC分类号： H05K1/09
CPC分类号： H05K3/244 , H05K1/0306 , H05K3/388 , H05K2203/0315 , H05K2203/1105 , Y10T29/49142
摘要： A wiring member comprising a substrate, a copper wiring layer having an electrical resistivity of not larger than 4×10−6 Ωcm in directly or indirectly contact with the substrate, an aluminum diffusion layer, contiguous to the copper wiring layer, having an aluminum concentration gradient descending towards the inside, and an aluminum oxide layer contiguous to and covering the aluminum diffusion layer, wherein a ratio of a thickness of the copper wiring layer to a thickness of the aluminum diffusion layer is 1.5 to 5. The disclosure is also concerned with a method of manufacturing the wiring member and an electronic device.
摘要翻译：一种布线构件，包括基板，与基板直接或间接接触的电阻率不大于4×10-6＆OHgr; cm的铜布线层，与铜布线层邻接的铝扩散层，具有铝浓度梯度向内侧下降，以及与铝扩散层相邻并覆盖铝氧化物层，其中铜布线层的厚度与铝扩散层的厚度的比率为1.5〜5。还公开了涉及制造布线构件和电子装置的方法。

5. 发明申请

US20110315937A1 CONDUCTIVE PASTE AND ELECTRONIC PART EQUIPPED WITH ELECTRODE WIRING FORMED FROM SAME 有权
标题翻译：导电胶和电子部件配有电极从其形成的接线
公开(公告)号：US20110315937A1
公开(公告)日：2011-12-29
申请号：US13203876
申请日：2009-03-27
申请人： Takuya Aoyagi , Takashi Naito , Hiroki Yamamoto , Takahiko Kato
发明人： Takuya Aoyagi , Takashi Naito , Hiroki Yamamoto , Takahiko Kato
IPC分类号： H01B1/20 , H01B1/02
CPC分类号： H01L31/022425 , H01B1/16 , H01J11/22 , H01J2211/225 , H01L31/03529 , H01L31/068 , H01L31/0682 , Y02E10/547
摘要： Provided is a conductive paste which contains an inexpensive metal, such as copper or aluminum, as an electrode wiring material and has oxidation resistance that enables the paste to withstand a high-temperature process performed in an oxidizing atmosphere and an electronic part equipped with electrode wiring formed from the paste. The electronic part in accordance with the present invention is equipped with electrode wiring that comprises a conductive glass phase containing transition metals and phosphorus, metal particles, and none of the substances prohibited by the RoHS directive. The electronic part is characterized in that each of the transition metals contained in the conductive glass phase is present in the state of having a plurality of oxidation numbers and that the proportion of the atoms which have the largest oxidation number for each transition metal satisfies a given relationship.
摘要翻译：本发明提供一种导电性糊剂，其含有诸如铜或铝的廉价金属作为电极配线材料，并且具有能够使膏体经受在氧化气氛中进行的高温处理和具有电极配线的电子部件的抗氧化性由膏形成。根据本发明的电子部件配备有包含含有过渡金属和磷，金属颗粒以及RoHS指令禁止的物质的导电玻璃相的电极配线。电子部件的特征在于，导电性玻璃相中含有的过渡金属中的每一种以具有多个氧化数的状态存在，并且每个过渡金属具有最大氧化数的原子的比例满足给定的关系。

6. 发明申请

US20110180138A1 PASTE COMPOSITION FOR ELECTRODE AND PHOTOVOLTAIC CELL 审中-公开
标题翻译：电极和光电池用糊剂组合物
公开(公告)号：US20110180138A1
公开(公告)日：2011-07-28
申请号：US13012947
申请日：2011-01-25
申请人： Shuuichirou Adachi , Masato Yoshida , Takeshi Nojiri , Mitsunori Iwamuro , Keiko Kizawa , Takuya Aoyagi , Hiroki Yamamoto , Takashi Naito , Takahiko Kato
发明人： Shuuichirou Adachi , Masato Yoshida , Takeshi Nojiri , Mitsunori Iwamuro , Keiko Kizawa , Takuya Aoyagi , Hiroki Yamamoto , Takashi Naito , Takahiko Kato
IPC分类号： H01L31/0224 , H01L31/0216 , H01B1/22
CPC分类号： H01B1/22 , H01L31/022425 , H01L31/02245 , H01L31/068 , Y02E10/547
摘要： The paste composition for an electrode includes metal particles having copper as a main component, glass particles including diphosphorus pentoxide and divanadium pentoxide and having a content of divanadium pentoxide of 1% by mass or more, a solvent, and a resin. Further, the photovoltaic cell has an electrode formed by using the paste composition for an electrode.
摘要翻译：电极用糊料组合物包括以铜为主要成分的金属粒子，五氧化二磷和五氧化二钒的玻璃粒子，五氧化二钒的含量为1质量％以上，溶剂和树脂。此外，光伏电池具有通过使用电极用糊剂组合物形成的电极。

7. 发明申请

US20100151323A1 ELECTRODE, ELECTRODE PASTE AND ELECTRONIC PARTS USING THE SAME 审中-公开
标题翻译：电极，电极浆料和使用该电极的电子部件
公开(公告)号：US20100151323A1
公开(公告)日：2010-06-17
申请号：US12635731
申请日：2009-12-11
申请人： Takashi Naito , Takahiko Kato , Takuya Aoyagi , Hiroki Yamamoto
发明人： Takashi Naito , Takahiko Kato , Takuya Aoyagi , Hiroki Yamamoto
IPC分类号： H01M4/54 , H01M4/02
CPC分类号： H01L21/4867 , H01J2211/225 , H01L23/49883 , H01L2924/0002 , H01L2924/00
摘要： The objects of the present invention are to provide a copper-base electrode which can be calcined in an oxidative atmosphere, e.g., in air, like a silver electrode, and is less expensive than a silver electrode; an electrode paste; and electronic parts using it. The other objects of the present invention are to provide a copper-base electrode which can be calcined in an inert gas atmosphere, e.g., in nitrogen, at low temperature; an electrode paste; and electronic parts using it.The electrode of the present invention contains at least metallic particles and an oxide phase, wherein the metallic particles contain copper and aluminum, and the oxide phase contains phosphorus. The oxide phase is preferably present as a phosphate glass phase in grain boundaries of the metallic particles. The electrode preferably contains the metallic particles and oxide phase at respective 75 to 95% and 5 to 25%, all percentages by volume. The metallic particles contain copper and aluminum at respective 80% or more and 3% or more for the calcination in an oxidative atmosphere, and 97% or more and 3% or less for the calcination in an inert gas atmosphere, all percentages by mass.
摘要翻译：本发明的目的是提供一种铜基电极，其可以在诸如银电极的空气中的氧化气氛中煅烧，并且比银电极便宜; 电极膏; 和使用它的电子部件。本发明的另一个目的是提供一种可在惰性气体气氛例如氮气中在低温下煅烧的铜基电极; 电极膏; 和使用它的电子部件。本发明的电极至少含有金属颗粒和氧化物相，其中金属颗粒含有铜和铝，氧化物相含有磷。氧化物相优选以金属颗粒的晶界中的磷酸盐玻璃相存在。所述电极优选含有75-95％和5〜25％的金属颗粒和氧化物相，所有的体积百分数。金属颗粒含有在氧化性气氛中煅烧时分别为80％以上且3％以上的铜和铝，并且在惰性气体气氛中，所有的质量百分比均为97％以上且3％以下。

8. 发明申请

US20120125670A1 Cu-Al ALLOY POWDER, ALLOY PASTE UTILIZING SAME, AND ELECTRONIC COMPONENT 审中-公开
标题翻译：铜铝合金粉，合金粉及其电子元件
公开(公告)号：US20120125670A1
公开(公告)日：2012-05-24
申请号：US13388316
申请日：2010-08-02
申请人： Takahiko Kato , Takashi Naito , Takuya Aoyagi , Hiroki Yamamoto , Masato Yoshida , Mitsuo Katayose , Shinji Takeda , Naotaka Tanaka , Shuichiro Adachi
发明人： Takahiko Kato , Takashi Naito , Takuya Aoyagi , Hiroki Yamamoto , Masato Yoshida , Mitsuo Katayose , Shinji Takeda , Naotaka Tanaka , Shuichiro Adachi
IPC分类号： H01B1/02 , B22F9/06 , H05K1/09
CPC分类号： H01L23/49883 , B22F1/0055 , B22F1/0074 , B22F1/02 , C22C1/0425 , C22C1/05 , H01B1/026 , H01J11/12 , H01J11/22 , H01J2211/225 , H01L21/4867 , H01L31/022425 , H01L2924/0002 , H01L2924/09701 , H05K1/092 , H05K3/4629 , H05K2201/0224 , H05K2203/0315 , Y02E10/50 , H01L2924/00
摘要： In an electronic component having a wiring and/or an electrode prepared through firing of a paste or in an electronic component having a wiring in contact with a glass or glass ceramic member, provided is an electronic component using a Cu-based wiring material which less suffers from increase in electric resistance due to oxidation, which less causes bubbles in the glass or glass ceramic, and has satisfactory migration resistance. The Cu—Al alloy powder includes a Cu—Al alloy powder including Cu and, preferably, 50 percent by weight or less of Al; and an aluminum oxide film having a thickness of 80 nm or less and being present on the surface of the Cu—Al alloy powder. The powder, when compounded with a glass or glass ceramic material to give a paste, can be used to form wiring (interconnections), electrodes, and/or contact members.
摘要翻译：在具有布线和/或通过烧制制成的电极的电子部件或具有与玻璃或玻璃陶瓷部件接触的布线的电子部件中的电子部件中，提供了使用Cu基布线材料的电子部件由于氧化而导致的电阻增加，玻璃或玻璃陶瓷中的气泡较少，具有良好的耐迁移性。 Cu-Al合金粉末包括Cu-Cu合金粉末，优选为50重量％以下的Al; 以及Cu-Al合金粉末的表面上存在厚度为80nm以下的氧化铝膜。当与玻璃或玻璃陶瓷材料混合以得到糊剂时，该粉末可用于形成布线（互连），电极和/或接触构件。

9. 发明申请

US20110209751A1 PASTE COMPOSITION FOR ELECTRODE AND PHOTOVOLTAIC CELL 审中-公开
标题翻译：电极和光电池用糊剂组合物
公开(公告)号：US20110209751A1
公开(公告)日：2011-09-01
申请号：US13013293
申请日：2011-01-25
申请人： Takeshi Nojiri , Masato Yoshida , Mitsunori Iwamuro , Shuuichirou Adachi , Keiko Kizawa , Takuya Aoyagi , Hiroki Yamamoto , Takashi Naito , Takahiko Kato
发明人： Takeshi Nojiri , Masato Yoshida , Mitsunori Iwamuro , Shuuichirou Adachi , Keiko Kizawa , Takuya Aoyagi , Hiroki Yamamoto , Takashi Naito , Takahiko Kato
IPC分类号： H01L31/0224 , H01B1/22
CPC分类号： H01B1/22 , H01L31/022425 , H01L31/02245 , Y02E10/50
摘要： The paste composition for an electrode according to the present invention includes metal particles containing copper as a main component, a flux, glass particles, a solvent, and a resin. Further, a photovoltaic cell according to the present invention has an electrode formed by using the paste composition for an electrode.
摘要翻译：本发明的电极用糊剂组合物含有以铜为主要成分的金属粒子，助熔剂，玻璃粒子，溶剂和树脂。此外，根据本发明的光伏电池具有通过使用电极用糊剂组合物形成的电极。

10. 发明授权

US08945436B2 Conductive paste and electronic part equipped with electrode wiring formed from same 有权
标题翻译：导电膏和电子部件配备有由其形成的电极布线
公开(公告)号：US08945436B2
公开(公告)日：2015-02-03
申请号：US13203876
申请日：2009-03-27
申请人： Takuya Aoyagi , Takashi Naito , Hiroki Yamamoto , Takahiko Kato
发明人： Takuya Aoyagi , Takashi Naito , Hiroki Yamamoto , Takahiko Kato
IPC分类号： H01B1/22 , H01L31/0224 , H01B1/16 , H01J11/22 , H01L31/0352 , H01L31/068
CPC分类号： H01L31/022425 , H01B1/16 , H01J11/22 , H01J2211/225 , H01L31/03529 , H01L31/068 , H01L31/0682 , Y02E10/547
摘要： Provided is a conductive paste which contains an inexpensive metal, such as copper or aluminum, as an electrode wiring material and has oxidation resistance that enables the paste to withstand a high-temperature process performed in an oxidizing atmosphere and an electronic part equipped with electrode wiring formed from the paste. The electronic part in accordance with the present invention is equipped with electrode wiring that comprises a conductive glass phase containing transition metals and phosphorus, metal particles, and none of the substances prohibited by the RoHS directive. The electronic part is characterized in that each of the transition metals contained in the conductive glass phase is present in the state of having a plurality of oxidation numbers and that the proportion of the atoms which have the largest oxidation number for each transition metal satisfies a given relationship.
摘要翻译：本发明提供一种导电性糊剂，其含有诸如铜或铝的廉价金属作为电极配线材料，并且具有能够使膏体经受在氧化气氛中进行的高温处理和具有电极配线的电子部件的抗氧化性由膏形成。根据本发明的电子部件配备有包含含有过渡金属和磷，金属颗粒以及RoHS指令禁止的物质的导电玻璃相的电极配线。电子部件的特征在于，导电性玻璃相中含有的过渡金属中的每一种以具有多个氧化数的状态存在，并且每个过渡金属具有最大氧化数的原子的比例满足给定的关系。

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