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1. 发明授权

US08486246B2 Reference electrode coated with ionic liquid and electrochemical measurement system using the reference electrode 有权
标题翻译：参考电极涂有离子液体和电化学测量系统使用参比电极
公开(公告)号：US08486246B2
公开(公告)日：2013-07-16
申请号：US12441370
申请日：2007-09-13
申请人： Takashi Kakiuchi , Satoshi Nomura , Mikito Yamanuki , Yasukazu Iwamoto , Manabu Shibata
发明人： Takashi Kakiuchi , Satoshi Nomura , Mikito Yamanuki , Yasukazu Iwamoto , Manabu Shibata
IPC分类号： G01N27/26
CPC分类号： G01N27/401
摘要： This invention provides a reference electrode that can be downsized and stable in voltage. The reference electrode in accordance with this invention is a reference electrode that does not require an internal aqueous solution such as a KCl aqueous solution and comprises a metal body, a slightly soluble salt film that comprises a slightly soluble salt of the metal body and that coats the metal body and a hydrophobic ionic liquid that is arranged to make contact with both the slightly soluble salt film and a sample to be measured.
摘要翻译：本发明提供一种可以小型化并且电压稳定的参比电极。根据本发明的参考电极是不需要诸如KCl水溶液的内部水溶液的参考电极，并且包括金属体，包含金属体的微溶盐的薄溶性盐膜，所述金属体和疏水性离子液体被布置成与所述可溶性盐膜和待测样品接触。

2. 发明申请

US20080000771A1 Reference electrode, salt bridge and ionic concentration measuring device by the use of reference electrode and salt bridge 有权
标题翻译：参考电极，盐桥和离子浓度测量装置通过使用参比电极和盐桥
公开(公告)号：US20080000771A1
公开(公告)日：2008-01-03
申请号：US11432973
申请日：2006-05-12
申请人： Takashi Kakiuchi , Manabu Shibata , Satoshi Nomura , Yasukazu Iwamoto , Mikito Yamanuki
发明人： Takashi Kakiuchi , Manabu Shibata , Satoshi Nomura , Yasukazu Iwamoto , Mikito Yamanuki
IPC分类号： G01N27/30 , G01F1/64 , H01M6/16
CPC分类号： G01N27/301
摘要： The present claimed invention is to provide a reference electrode wherein variations of a potential difference at a liquid junction can be removed almost completely, contamination of a sample solution can be minimized, a frequency to supply and replace an internal solution is lessened, the liquid junction is prevented from being clogged, high durability for a long term can be maintained and a measurement with high accuracy can be conducted, and comprises an internal electrode 21, an internal solution 22 that makes a contact with the internal electrode 21 and a liquid junction 23 that continues into the internal solution 22, wherein the liquid junction 23 is made by the use of a gelled hydrophobic ionic liquid.
摘要翻译：本发明要提供一种参考电极，其中液体接头处的电位差的变化可以几乎完全去除，样品溶液的污染可以最小化，减少内部溶液的供应和更换频率，液体接点防止堵塞，可以保持长期的高耐久性并且可以进行高精度的测量，并且包括内部电极21，与内部电极21接触的内部溶液22和液体接合部23 其继续进入内部溶液22，其中液体接头23通过使用胶凝的疏水性离子液体制成。

3. 发明授权

US07628901B2 Reference electrode, salt bridge and ionic concentration measuring device by the use of reference electrode and salt bridge 有权
标题翻译：参考电极，盐桥和离子浓度测量装置通过使用参比电极和盐桥
公开(公告)号：US07628901B2
公开(公告)日：2009-12-08
申请号：US11432973
申请日：2006-05-12
申请人： Takashi Kakiuchi , Manabu Shibata , Satoshi Nomura , Yasukazu Iwamoto , Mikito Yamanuki
发明人： Takashi Kakiuchi , Manabu Shibata , Satoshi Nomura , Yasukazu Iwamoto , Mikito Yamanuki
IPC分类号： G01N27/26
CPC分类号： G01N27/301
摘要： The present claimed invention is to provide a reference electrode wherein variations of a potential difference at a liquid junction can be removed almost completely, contamination of a sample solution can be minimized, a frequency to supply and replace an internal solution is lessened, the liquid junction is prevented from being clogged, high durability for a long term can be maintained and a measurement with high accuracy can be conducted, and comprises an internal electrode 21, an internal solution 22 that makes a contact with the internal electrode 21 and a liquid junction 23 that continues into the internal solution 22, wherein the liquid junction 23 is made by the use of a gelled hydrophobic ionic liquid.
摘要翻译：本发明要提供一种参考电极，其中液体接头处的电位差的变化可以几乎完全去除，样品溶液的污染可以最小化，减少内部溶液的供应和更换频率，液体接点防止堵塞，可以保持长期的高耐久性并且可以进行高精度的测量，并且包括内部电极21，与内部电极21接触的内部溶液22和液体接合部23 其继续进入内部溶液22，其中液体接头23通过使用胶凝的疏水性离子液体制成。

4. 发明申请

US20090283404A1 Reference Electrode Coated with Ionic Liquid and Electrochemical Measurement System Using the Reference Electrode 有权
标题翻译：参考电极涂覆离子液体和电化学测量系统使用参考电极
公开(公告)号：US20090283404A1
公开(公告)日：2009-11-19
申请号：US12441370
申请日：2007-09-13
申请人： Takashi Kakiuchi , Satoshi Nomura , Mikito Yamanuki , Yasukazu Iwamoto , Manabu Shibata
发明人： Takashi Kakiuchi , Satoshi Nomura , Mikito Yamanuki , Yasukazu Iwamoto , Manabu Shibata
IPC分类号： G01N27/30
CPC分类号： G01N27/401
摘要： This invention provides a reference electrode (3) that can be downsized and stable in voltage. The reference electrode (3) in accordance with this invention is a reference electrode (3) that does not require an internal aqueous solution such as a KCl aqueous solution and comprises a metal body (31), a slightly soluble salt film (32) that comprises a slightly soluble salt of the metal body (31) and that coats the metal body (31) and a hydrophobic ionic liquid (33) that is arranged to make contact with both the slightly soluble salt film (32) and a sample to be measured.
摘要翻译：本发明提供一种可以小型化并且电压稳定的参比电极（3）。根据本发明的参考电极（3）是不需要诸如KCl水溶液的内部水溶液的参考电极（3），并且包括金属体（31），微溶性盐膜（32），其中包括金属体（31）的微溶盐，并且涂覆金属体（31）和疏水性离子液体（33），该疏水性离子液体被设置为与微溶盐膜（32）和样品接触测量。

5. 发明授权

US08608917B2 Reference electrode 有权
标题翻译：参考电极
公开(公告)号：US08608917B2
公开(公告)日：2013-12-17
申请号：US13819320
申请日：2011-08-25
申请人： Manabu Shibata , Yasukazu Iwamoto
发明人： Manabu Shibata , Yasukazu Iwamoto
IPC分类号： C25B11/04
CPC分类号： G01N27/302 , G01N27/301
摘要： A reference electrode for improving a product life cycle without using a gelled hydrophobic ionic liquid having a prescribed hardness or viscosity and without having a large thickness so as to be difficult to manufacture is provided. The reference electrode is provided with a housing for accommodating an internal electrode, a filler for electrically connecting the internal electrode, and a sample liquid. The filler is formed having a layer between the internal electrode and an opening formed in the housing for contacting the sample liquid and the filler. The filler includes a first layer including a water soluble electrolytic solution formed to be in contact with the internal electrode a second layer including a hydrophobic ionic liquid formed to be in contact with the first layer; and a third layer including a gelled hydrophobic ionic liquid formed in the opening so as to be in contact with the second layer.
摘要翻译：提供了一种用于改善产品寿命周期的参比电极，而不使用具有规定硬度或粘度并且不具有大厚度以致难以制造的凝胶状疏水性离子液体。参考电极设置有用于容纳内部电极的壳体，用于电连接内部电极的填充物和样品液体。填料形成在内部电极和形成在壳体中的开口之间的层，用于接触样品液体和填料。填料包括第一层，其包括形成为与内部电极接触的水溶性电解液，第二层包括形成为与第一层接触的疏水性离子液体; 以及第三层，其包括在所述开口中形成的与所述第二层接触的凝胶状疏水性离子液体。

6. 发明申请

US20130153417A1 REFERENCE ELECTRODE 有权
标题翻译：参考电极
公开(公告)号：US20130153417A1
公开(公告)日：2013-06-20
申请号：US13819320
申请日：2011-08-25
申请人： Manabu Shibata , Yasukazu Iwamoto
发明人： Manabu Shibata , Yasukazu Iwamoto
IPC分类号： G01N27/30
CPC分类号： G01N27/302 , G01N27/301
摘要： A reference electrode for improving a product life cycle without using a gelled hydrophobic ionic liquid having a prescribed hardness or viscosity and without having a large thickness so as to be difficult to manufacture is provided. The reference electrode is provided with a housing for accommodating an internal electrode, a filler for electrically connecting the internal electrode, and a sample liquid. The filler is formed having a layer between the internal electrode and an opening formed in the housing for contacting the sample liquid and the filler. The filler includes a first layer including a water soluble electrolytic solution formed to be in contact with the internal electrode a second layer including a hydrophobic ionic liquid formed to be in contact with the first layer; and a third layer including a gelled hydrophobic ionic liquid formed in the opening so as to be in contact with the second layer.
摘要翻译：提供了一种用于改善产品寿命周期的参比电极，而不使用具有规定硬度或粘度并且不具有大厚度以致难以制造的凝胶状疏水性离子液体。参考电极设置有用于容纳内部电极的壳体，用于电连接内部电极的填充物和样品液体。填料形成在内部电极和形成在壳体中的开口之间的层，用于接触样品液体和填料。填料包括第一层，其包括形成为与内部电极接触的水溶性电解液，第二层包括形成为与第一层接触的疏水性离子液体; 以及第三层，其包括在所述开口中形成的与所述第二层接触的凝胶状疏水性离子液体。

7. 发明授权

US08197651B2 Ion-selective electrode 失效
标题翻译：离子选择电极
公开(公告)号：US08197651B2
公开(公告)日：2012-06-12
申请号：US12744649
申请日：2008-12-17
申请人： Yuji Nishio , Yasukazu Iwamoto
发明人： Yuji Nishio , Yasukazu Iwamoto
IPC分类号： G01N27/333
CPC分类号： G01N27/36 , C03C3/111 , C03C4/18
摘要： Disclosed is an ion-selective electrode having excellent mechanical strength, excellent durability, low membrane resistance and good ion response accuracy. This ion-selective electrode comprises a response glass membrane which has ion selectivity and is made of an oxynitride glass containing Li.
摘要翻译：公开了具有优异的机械强度，优异的耐久性，低膜电阻和良好的离子响应精度的离子选择性电极。该离子选择电极包括具有离子选择性并由含有Li的氧氮化物玻璃制成的响应玻璃膜。

8. 发明授权

US08080315B2 Responsive glass membrane and glass electrode 有权
标题翻译：响应玻璃膜和玻璃电极
公开(公告)号：US08080315B2
公开(公告)日：2011-12-20
申请号：US12037751
申请日：2008-02-26
申请人： Yuji Nishio , Yasukazu Iwamoto , Tadanori Hashimoto
发明人： Yuji Nishio , Yasukazu Iwamoto , Tadanori Hashimoto
IPC分类号： B32B3/26 , B32B17/06
CPC分类号： G01N27/36 , Y10T428/24999
摘要： An ion-selective electrode has a responsive glass membrane with an exterior thin film containing titanium dioxide of an anatase type that is continuously formed as an integrated body. The thin film, of several hundred nm in numbers, is electrically connected by an amount of titanium dioxide that will form a continuity in the thin film structure. The thin film can be porous and contain at least one metal selected from cobalt, nickel, tungsten, copper, platinum, gold, silver and iron. Additionally, significantly larger titanium dioxide particles of 0.02 μm in diameter can be further mixed into the thin film.
摘要翻译：离子选择性电极具有响应性玻璃膜，其具有外部薄膜，该外部薄膜包含连续形成为整体的锐钛矿型二氧化钛。数百nm的薄膜通过一定量的二氧化钛电连接，这将形成薄膜结构的连续性。薄膜可以是多孔的并且含有选自钴，镍，钨，铜，铂，金，银和铁中的至少一种金属。另外，直径0.02μm的显着更大的二氧化钛颗粒可以进一步混入薄膜中。

9. 发明申请

US20080206547A1 RESPONSIVE GLASS MEMBRANE AND GLASS ELECTRODE 有权
标题翻译：响应玻璃膜和玻璃电极
公开(公告)号：US20080206547A1
公开(公告)日：2008-08-28
申请号：US12037751
申请日：2008-02-26
申请人： Yuji Nishio , Yasukazu Iwamoto , Tadanori Hashimoto
发明人： Yuji Nishio , Yasukazu Iwamoto , Tadanori Hashimoto
IPC分类号： B32B3/26 , B32B17/06
CPC分类号： G01N27/36 , Y10T428/24999
摘要： This invention intends to provide a responsive glass membrane and a glass electrode comprising the responsive glass membrane to which taint is hardly attached and easily detached without hindering a function of measuring the ionic concentration. A thin film containing titanium dioxide of an anatase type is formed on a surface of the responsive glass membrane and whole of the thin film is continuously formed to be an integrated body.
摘要翻译：本发明旨在提供一种响应性玻璃膜和玻璃电极，其包含难以附着和容易分离的响应性玻璃膜，而不会妨碍测量离子浓度的功能。在响应性玻璃膜的表面上形成含有锐钛矿型二氧化钛的薄膜，并且将整个薄膜连续地形成为一体。

10. 发明申请

US20080011607A1 REFERENCE ELECTRODE WITH NON-BLOCKING LIQUID JUNCTION 失效
标题翻译：具有非阻塞液体接头的参考电极
公开(公告)号：US20080011607A1
公开(公告)日：2008-01-17
申请号：US11832537
申请日：2007-08-01
申请人： Yasukazu Iwamoto , Naomi Kitaoka
发明人： Yasukazu Iwamoto , Naomi Kitaoka
IPC分类号： G01N27/403
CPC分类号： G01N27/301
摘要： A reference electrode traps silver ions and chloro complex ions leaching to an internal filling solution so that the blocking of the liquid junction can be prevented. A silver/silver chloride electrode can be provided as an internal electrode in an internal filling solution; and a tube which houses, in order from top to bottom, the internal electrode, an inorganic cation exchanger for trapping silver ions and/or chloro complex ions from leaching from the internal electrode, and a ceramic member for preventing the diffusion of the silver ions and/or the chloro complex ions to the internal filling solution.
摘要翻译：参考电极捕获银离子和氯络合离子浸出到内部填充溶液中，从而可以防止液体结的阻塞。可以在内部填充溶液中提供银/氯化银电极作为内部电极; 以及从顶部到底部依次容纳内部电极的管，用于捕获银离子和/或氯配合物离子从内部电极浸出的无机阳离子交换器和用于防止银离子扩散的陶瓷构件和/或氯配合物离子到内部填充溶液。

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