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1. 发明授权

US4395519A Physically blended propylene polymer composition 失效
标题翻译：物理混合丙烯聚合物组成
公开(公告)号：US4395519A
公开(公告)日：1983-07-26
申请号：US196550
申请日：1980-10-14
申请人： Syuji Minami , Norio Kashiwa , Akifumi Kato , Junichi Watanabe
发明人： Syuji Minami , Norio Kashiwa , Akifumi Kato , Junichi Watanabe
IPC分类号： C08L23/10 , C08L23/16 , C08L23/06 , C08L23/12
CPC分类号： C08L23/10 , C08L23/16 , Y10S2/918
摘要： A physically blended propylene polymer composition composed of(A) 100 parts by weight of crystalline polypropylene containing 0 to 10 mole % of ethylene and/or another .alpha.-olefin,(B) 1 to 30 parts by weight of a propylene/ethylene random copolymer composed of 30 to 85 mole % of propylene, said copolymer containing 0 to 10 mole % of a diene component and having (i) a micro-isotacticity of at least 0.8 and (ii) a boiling n-cyclohexane insolubles content of 0 to 10% by weight, and(C) 0 to 30 parts by weight of polyethylene containing 0 to 15 mole % of an .alpha.-olefin,said components (A) and (B) having been physically mixed with each other.
摘要翻译：由（A）100重量份含有0-10摩尔％乙烯和/或另一个α-烯烃的结晶聚丙烯组成的物理混合丙烯聚合物组合物，（B）1至30重量份丙烯/乙烯无规共聚物由30至85摩尔％的丙烯组成，所述共聚物含有0至10摩尔％的二烯组分，并且具有（i）至少0.8的微全同立构规整度和（ii）沸点的n-环己烷不溶物含量为0至10 （C）0〜30重量份含有0〜15摩尔％α-烯烃的聚乙烯，所述成分（A）和（B）彼此物理混合。

2. 发明授权

US4490513A Process for producing polymers or copolymers of olefins containing at least three carbon atoms and catalysts therefor 失效
标题翻译：制备含有至少三个碳原子的烯烃的聚合物或共聚物的方法及其催化剂
公开(公告)号：US4490513A
公开(公告)日：1984-12-25
申请号：US836056
申请日：1977-09-23
申请人： Syuji Minami , Akinori Toyota , Norio Kashiwa
发明人： Syuji Minami , Akinori Toyota , Norio Kashiwa
IPC分类号： C08F4/00 , C08F4/60 , C08F4/64 , C08F10/00 , C08F10/04 , C08F4/02
CPC分类号： C08F10/00 , Y10S526/906
摘要： A process for producing a polymer or copolymer of an olefin containing at least 3 carbon atoms which comprises polymerizing or copolymerizing at least one olefin containing at least 3 carbon atoms, or copolymerizing the olefin with to 10 mole % of ethylene and/or a diolefin in the presence of a catalyst composed of (A) a magnesium-containing solid titanium catalyst component and (B) an organometallic compound of a metal of Groups I to III of the periodic table; wherein the solid titanium catalyst component (A) is a composition formed by contacting(i) a reaction product of an organic magnesium compound containing magnesium directly bonded to at least one carbon atom with an organic silicon-containing compound selected from the group consisting of organic silanols containing at least one hydroxyl group directly bonded to silicon and organopolysiloxanes,(ii) an organic acid ester, and(iii) a titanium compound.
摘要翻译：一种制备包含至少3个碳原子的烯烃的聚合物或共聚物的方法，其包括聚合或共聚至少一种含有至少3个碳原子的烯烃，或将烯烃与10摩尔％的乙烯和/或二烯烃共聚存在由（A）含镁固体钛催化剂组分和（B）元素周期表第I至III族金属的有机金属化合物组成的催化剂; 其中所述固体钛催化剂组分（A）是通过使（i）含有与至少一个碳原子直接键合的镁的有机镁化合物的反应产物与选自有机基团的有机含硅化合物含有至少一个与硅和有机聚硅氧烷直接结合的羟基的硅烷醇，（ii）有机酸酯，和（iii）钛化合物。

3. 发明授权

US4370455A Process for polymerizing or copolymerizing olefins 失效
标题翻译：烯烃聚合或共聚方法
公开(公告)号：US4370455A
公开(公告)日：1983-01-25
申请号：US101470
申请日：1979-12-10
申请人： Takashi Ueda , Syuji Minami , Mamoru Kioka , Norio Kashiwa
发明人： Takashi Ueda , Syuji Minami , Mamoru Kioka , Norio Kashiwa
IPC分类号： C08F4/00 , C08F4/60 , C08F10/00 , C08F4/02
CPC分类号： C08F10/00
摘要： In a process for producing a polymer or copolymer of an alpha-olefin which comprises continuously polymerizing or copolymerizing the alpha-olefin or the alpha-olefin with up to 5 mole % of a diolefin in the presence of a catalyst comprising a transition metal catalyst component and an organoaluminum catalyst component, the improvement wherein:(I) said polymerization or copolymerization is carried out in the presence of a catalyst composed of (A) a solid magnesium compound obtained by reacting (i) an adduct between a magnesium halide and an electron donor, with (ii) an organometallic compound of a metal of Groups I to III of the Mendelejeff's periodic table, (B) a liquid transition metal compound, and (C) an organoaluminum compound, and(II) said continuous polymerization or copolymerization is carried out while feeding the compound (B) separately from the other compounds (A) and (C) into a polymerization or copolymerization zone.
摘要翻译：在制备α-烯烃的聚合物或共聚物的方法中，其包括在包含过渡金属催化剂组分的催化剂存在下，使α-烯烃或α-烯烃与至多5摩尔％的二烯烃连续聚合或共聚和有机铝催化剂组分的改进，其中：（I）所述聚合或共聚在催化剂存在下进行，所述催化剂由（A）通过（i）卤化镁和电子之间的加合物反应获得的固体镁化合物（ii）Mendelejeff周期表第I至III族金属的有机金属化合物，（B）液体过渡金属化合物和（C）有机铝化合物，和（II）所述连续聚合或共聚是在将化合物（B）与其它化合物（A）和（C）分开地进料到聚合或共聚区中的同时进行。

4. 发明授权

US4232139A Process for producing polymers or copolymers of olefins containing at least 3 carbon atoms 失效
标题翻译：制备含有至少3个碳原子的烯烃的聚合物或共聚物的方法
公开(公告)号：US4232139A
公开(公告)日：1980-11-04
申请号：US801234
申请日：1977-05-27
申请人： Syuji Minami , Norio Kashiwa
发明人： Syuji Minami , Norio Kashiwa
IPC分类号： C08F4/00 , C08F4/60 , C08F4/64 , C08F10/00 , C08F4/02 , C08F10/06
CPC分类号： C08F10/00
摘要： A process for producing a polymer or copolymer of an olefin containing at least 3 carbon atoms which comprises polymerizing or copolymerizing at least one olefin containing at least 3 carbon atoms, or copolymerizing the olefin with up to 10% mole of ethylene and/or a diolefin, in the presence of a catalyst composed of (A) a magnesium-containing solid titanium composition and (B) an organometallic compound of a metal of Groups I to III of the periodic table; characterized in that the solid titanium composition (A) is a composition formed by contacting (i) a halogen-containing magnesium organo-aromatic compound of the formula Mg(OR).sub.n X.sub.2-n wherein R represents an aryl or aralkyl group and n is a positive number of 0
摘要翻译：一种制备含有至少3个碳原子的烯烃的聚合物或共聚物的方法，其包括聚合或共聚至少一种含有至少3个碳原子的烯烃，或使烯烃与至多10％摩尔的乙烯和/或二烯烃共聚在（A）含镁固体钛组合物和（B）元素周期表中第I至III族金属的有机金属化合物的催化剂存在下，其特征在于，所述固体钛组合物（A）是通过使（i）式Mg（OR）n X 2-n的含卤素的镁有机芳族化合物（其中R表示芳基或芳烷基，n为正数为0

5. 发明授权

US4328328A Continuous process for production of olefin polymers or copolymers 失效
标题翻译：用于生产烯烃聚合物或共聚物的连续方法
公开(公告)号：US4328328A
公开(公告)日：1982-05-04
申请号：US100098
申请日：1979-12-04
申请人： Syuji Minami , Takashi Ueda , Mamoru Kioka , Norio Kashiwa
发明人： Syuji Minami , Takashi Ueda , Mamoru Kioka , Norio Kashiwa
IPC分类号： C08F4/00 , C08F4/02 , C08F4/60 , C08F4/62 , C08F4/639 , C08F4/64 , C08F10/00 , C08F10/02
CPC分类号： C08F10/00 , C08F4/022
摘要： In a continuous process for producing a polymer or copolymer of an alpha-olefin in a hydrocarbon solvent in the presence of a catalyst comprising a transition metal compound and an organoaluminum compound, the improvement wherein[I] polymerization or copolymerization is carried out in the presence of a catalyst composed of(A) a magnesium compound in the liquid state which is soluble in said hydrocarbon solvent and is free from an organoaluminum compound and a transition metal compound, said magnesium compound being obtained from specific reactants,(B) a transition metal compound in the liquid state, and(C) an organoaluminum compound, and[II] said polymerization or copolymerization is carried out while feeding said compound (C) into a polymerization or copolymerization zone separately from said other compounds (A) and (B), or while adding a part or the whole of said compound (C) to a liquid mixture of said other compounds (A) and (B) and feeding the resulting mixture into said zone, or while feeding a mixture of the compounds (A), (B) and (C) into said zone.
摘要翻译：在包含过渡金属化合物和有机铝化合物的催化剂存在下，在烃溶剂中制备α-烯烃的聚合物或共聚物的连续方法中，其中[I]聚合或共聚在存在下进行由（A）液态的镁化合物（其可溶于所述烃溶剂并且不含有机铝化合物和过渡金属化合物）组成的催化剂，所述镁化合物由特定反应物获得，（B）过渡金属以及（C）有机铝化合物，和[II]在将所述化合物（C）与所述其它化合物（A）和（B）分开地进入聚合或共聚区的同时进行聚合或共聚，或者将所述化合物（C）的一部分或全部添加到所述其它化合物（A）和（B）的液体混合物中，并将所得混合物进料到所述区域或者将化合物（A），（B）和（C）的混合物进料到所述区域中。

6. 发明授权

US4221894A Process for polymerizing .alpha.-olefins containing at least 3 carbon atoms and catalyst therefor 失效
标题翻译：用于聚合含有至少3个碳原子的α-烯烃和其催化剂的方法
公开(公告)号：US4221894A
公开(公告)日：1980-09-09
申请号：US951973
申请日：1978-10-16
申请人： Yoshihisa Ushida , Kiyoshi Odawara , Norio Kashiwa , Akinori Toyota , Syuji Minami
发明人： Yoshihisa Ushida , Kiyoshi Odawara , Norio Kashiwa , Akinori Toyota , Syuji Minami
IPC分类号： C08F4/02 , C08F4/64 , C08F10/00 , C08F10/06
CPC分类号： C08F10/00 , C08F4/022 , Y10S526/906
摘要： A process for polymerizing or copolymerizing .alpha.-olefins having at least 3 carbon atoms or copolymerizing .alpha.-olefins having at least 3 carbon atoms with not more than 50 mole % of ethylene in the presence of a catalyst composed of an organometallic compound of a metal of Groups I to III of the periodic table and a titanium catalyst component supported on a halogen-containing magnesium compound, said titanium catalyst component being a solid reaction product obtained by treating (i) a mechanically copulverized product of a halogen-containing compound and an organic acid ester with (ii) an organo-metallic compound of a metal of Groups I to III of the periodic table, and then reacting the resulting solid product with (iii) a titanium compound in the absence of mechanical pulverization.
摘要翻译：在具有至少3个碳原子的α-烯烃或具有至少3个碳原子的α-烯烃与不超过50摩尔％的乙烯的聚合或共聚的催化剂的存在下，在由金属的有机金属化合物元素周期表的I至III族和负载在含卤素的镁化合物上的钛催化剂组分，所述钛催化剂组分是通过处理（i）含卤素化合物和有机物的机械共缩合产物得到的固体反应产物酸酯与（ⅱ）元素周期表第I至III族金属的有机金属化合物反应，然后在没有机械粉碎的情况下使得到的固体产物与（ⅲ）钛化合物反应。

7. 发明授权

US4157435A Process for preparing highly stereoregular polyolefins and catalyst used therefor 失效
标题翻译：制备高立体规则聚烯烃的方法和用于其的催化剂
公开(公告)号：US4157435A
公开(公告)日：1979-06-05
申请号：US710658
申请日：1976-08-02
申请人： Akinori Toyota , Norio Kashiwa , Syuji Minami
发明人： Akinori Toyota , Norio Kashiwa , Syuji Minami
IPC分类号： C08F4/02 , C08F10/00 , C08F10/06
CPC分类号： C08F4/022 , C08F10/00 , Y10S526/904 , Y10S526/906
摘要： A process for preparing highly stereoregular polyolefins in the presence of a catalyst comprising (A) a titanium-containing solid catalyst component composed of an organic complex derived from(i) a magnesium halide(ii) an organopolysiloxane selected from the group consisting of compounds of the formulaQ(Q.sub.2 SiO).sub.n SiQ.sub.3, (Q.sub.2 SiO).sub.n and X(Q.sub.2 SiO).sub.n SiQ.sub.2 X,(iii) an organic carboxylic acid ester, and(iv) a titanium compound of the formulaTi(OR).sub.l X.sub.4-l, and(B) an organoaluminum catalyst component of the formulaR'mAl(OR').sub.3-m,said organic complex being derived by bringing the component (i) into contact with a combination of the components (ii) and (iii) or a combination of the components (ii), (iii) and (iv) under mechanical pulverisation conditions and then treating the resulting pulverized composition with the component (iv) in the absence of mechanical pulverization.
摘要翻译：一种在催化剂存在下制备高立体规则聚烯烃的方法，包括（A）含钛固体催化剂组分，其由衍生自（I）选自由化合物组成的组中选择的一种有机金属氧化物（II）的有机络合物组成的含钛固体催化剂组分式（QSiO）nSiQ3，（Q2SiO）n和X（Q2SiO）nSiQ2X，（iii）有机羧酸酯和（Ⅳ）式（Ⅺ）Ⅺ4-Ⅳ的钛化合物和（B）一种式R'mAl（OR'）3-m的有机铝催化剂组分，通过使组分（I）与组分（II）和（III）的组合接触得到的有机复合物或其组合组件（II），（III）和（IV）在机械搅拌条件下，然后在组织（IV）的机械搅拌条件下处理结晶粉化组合物。

8. 发明授权

US4250285A Process for polymerizing olefins and catalysts therefor 失效
标题翻译：聚合烯烃及其催化剂的方法
公开(公告)号：US4250285A
公开(公告)日：1981-02-10
申请号：US902946
申请日：1978-05-04
申请人： Syuji Minami , Akinori Toyota , Norio Kashiwa
发明人： Syuji Minami , Akinori Toyota , Norio Kashiwa
IPC分类号： C08F4/00 , C08F4/02 , C08F4/60 , C08F4/64 , C08F10/04 , C08F10/06
CPC分类号： C08F10/04 , C08F4/022 , Y10S526/906
摘要： A process for preparing a polymer or copolymer of an olefin having at least 3 carbon atoms which comprises polymerizing or copolymerizing an olefin having at least 3 carbon atoms and containing 0 to 10 mole % of another olefin or diolefin in the presence of a catalyst composed of (i) a solid titanium catalyst component and (ii) an organoaluminum compound; wherein the solid titanium catalyst component is obtained by contacting(1) a magnesium containing copulverization product comprising (A) an aluminum or germanium compound selected from the group consisting of aluminum compounds of the formula AlR.sub.n X.sub.3-n wherein R is a hydrogen atom, or an alkyl, alkenyl, aryl, alkoxy, aryloxy or acyloxy group optionally having a substituent, X is a halogen atom, and O
摘要翻译：一种制备具有至少3个碳原子的烯烃的聚合物或共聚物的方法，该方法包括使聚合或共聚含有至少3个碳原子的烯烃并含有0-10摩尔％的另一种烯烃或二烯烃，催化剂由（i）固体钛催化剂组分和（ii）有机铝化合物; 其中所述固体钛催化剂组分是通过使（1）含镁共混物与（A）铝或锗化合物（其中R为氢原子的AlRnX3-n的铝化合物）或烷基，烯基，芳基，烷氧基，芳氧基或任选具有取代基的酰氧基，X是卤素原子，O

9. 发明授权

US4143223A Process for polymerizing alpha-olefins and catalyst therefor 失效
标题翻译：用于聚合α-烯烃及其催化剂的方法
公开(公告)号：US4143223A
公开(公告)日：1979-03-06
申请号：US773266
申请日：1977-03-01
申请人： Akinori Toyota , Syuji Minami , Norio Kashiwa
发明人： Akinori Toyota , Syuji Minami , Norio Kashiwa
IPC分类号： C08F4/00 , C08F4/16 , C08F4/60 , C08F4/64 , C08F10/00 , C08F4/02 , C08F10/06
CPC分类号： C08F10/00 , Y10S526/906
摘要： A process for polymerizing or copolymerizing .alpha.-olefins in the presence of a catalyst composed of (A) a mechanically pulverized solid titanium-containing catalyst component and (B) an organometallic compound of a metal of Groups I to III of the periodic table, wherein said titanium-containing component is a solid halogen-containing titanium catalyst component obtained by reacting a mechanically copulverized solid product in the absence of mechanical pulverization with a titanium compound which is liquid under the reaction conditions, said mechanically copulverized product being derived from (1) a magnesium compound, (2) an organic acid ester, and (3) an active hydrogen-containing compound selected from the group of alcohols and phenols; and a catalyst composition used therefor.

10. 发明申请

US20090280318A1 OLEFIN POLYMER, COMPOSITION THEREOF AND ADHESIVE RESIN COMPRISING THE COMPOSITION 审中-公开
标题翻译： OLEFIN聚合物，其组合物和包含组合物的粘合树脂
公开(公告)号：US20090280318A1
公开(公告)日：2009-11-12
申请号：US12096655
申请日：2006-12-08
申请人： Tomoaki Matsugi , Junji Saito , Hideyuki Kaneko , Norio Kashiwa , Shin-ichi Kojoh , Takayuki Onogi , Motoaki Isokawa , Seiji Ota , Shigeyuki Yasui
发明人： Tomoaki Matsugi , Junji Saito , Hideyuki Kaneko , Norio Kashiwa , Shin-ichi Kojoh , Takayuki Onogi , Motoaki Isokawa , Seiji Ota , Shigeyuki Yasui
IPC分类号： B32B27/32 , C08F8/00 , C09J131/02
CPC分类号： C08L53/00 , C08F8/00 , C08F8/08 , C08F8/12 , C08F8/18 , C08F8/20 , C08F8/42 , C08F255/00 , C08F255/02 , C08F293/00 , C08F293/005 , C08F2810/50 , C08L23/0846 , C08L23/0884 , C08L23/0892 , C08L51/06 , C08L2205/02 , C08L2666/02 , C08L2666/14 , C09J123/02 , C09J123/0846 , C09J151/06 , C09J153/00 , Y10T428/263 , C08L2666/06 , C08F210/02 , C08F110/06 , C08F255/023 , C08F110/14 , C08F210/12
摘要： Provided is a new adhesive polyolefin resin composition, containing 1 to 100% by weight of a high polymer structure, that has good heat resistance and excellent adhesion performance to polyolefins and various polar materials, wherein a polyolefin segment (A) is bonded with an addition polymer segment (B) of a non-olefinic vinyl monomer and a reactive group is introduced into the addition polymer segment (B) and an adhesive or dispersion obtained therefrom.
摘要翻译：提供了一种新的粘合剂聚烯烃树脂组合物，其含有1至100重量％的高聚物结构，其具有良好的耐热性和对聚烯烃和各种极性材料的优异粘合性能，其中聚烯烃链段（A）与添加剂将非烯烃类乙烯基单体和反应性基团的聚合物链段（B）导入到加成聚合物链段（B）中，并由其获得粘合剂或分散体。

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