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1. 发明授权

US06794476B2 Propylene homopolymer and propylene copolymer 失效
标题翻译：丙烯均聚物和丙烯共聚物
公开(公告)号：US06794476B2
公开(公告)日：2004-09-21
申请号：US10070442
申请日：2002-03-19
申请人： Shuji Machida , Takashi Saeki , Tomio Tatsumi
发明人： Shuji Machida , Takashi Saeki , Tomio Tatsumi
IPC分类号： C08F11006
CPC分类号： C08F110/06 , C08F210/06 , C08L23/02 , C08L23/10 , C08L23/12 , C08L2666/04 , C08F2500/11 , C08F2500/12
摘要： Provided are a propylene homopolymer in which a melt tension (MT), a Z average molecular weight (Mz) and a melt index (MI) (g/10 minutes) are specifically related and in which a difference in eluting temperatures and a maximum eluting temperature in programmed temperature fractional chromatography and a propylene copolymer in which a comonomer is specific &agr;-olefin and a content thereof falls in a specific range and in which a melt tension (MT), a Z average molecular weight (Mz) and a melt index (MI) (g/10 minutes) are specifically related. The propylene homopolymer or the propylene copolymer of the present invention has physical properties equivalent to or not lower than those of conventional propylene polymers, and it can be controlled in a melt tension and is suited to foaming molding, sheet molding and blow molding. Further, it is excellent in melt-processing characteristics, molding stability and a recycling property and can be applied to molding methods which are restricted in use in conventional propylene polymers, for example, large size blow molding and extrusion foaming molding.
摘要翻译：提供了其中熔体张力（MT），Z平均分子量（Mz）和熔体指数（MI）（g / 10分钟）特别相关的丙烯均聚物，其中洗脱温度和最大洗脱程序温度分数色谱中的温度和丙烯共聚物，其中共聚单体是特定α-烯烃，其含量在特定范围内，其中熔体张力（MT），Z平均分子量（Mz）和熔体指数（MI）（g / 10分钟）具体相关。本发明的丙烯均聚物或丙烯共聚物具有与常规丙烯聚合物相同或不低于其特性的物理性质，并且可以以熔体张力控制，并且适于发泡成型，片状成型和吹塑。此外，其熔融加工特性，成型稳定性和再循环性优异，可用于常规丙烯聚合物中使用的成型方法，例如大型吹塑和挤出发泡成型。

2. 发明申请

US20070129490A1 PROPLYENE POLYMER COMPOSITION, MOLDED OBJECT, AND POLYOLEFIN COPOLYMER 审中-公开
标题翻译：丙烯聚合物组合物，成型对象和聚烯烃共聚物
公开(公告)号：US20070129490A1
公开(公告)日：2007-06-07
申请号：US11616633
申请日：2006-12-27
申请人： YASUHIRO GOTO , Masaru Nakagawa , Tomio Tatsumi , Shuji Machida
发明人： YASUHIRO GOTO , Masaru Nakagawa , Tomio Tatsumi , Shuji Machida
IPC分类号： C08L53/00
CPC分类号： C08L23/10 , C08F210/06 , C08F297/08 , C08F297/083 , C08L23/02 , C08L23/16 , C08L53/00 , C08L2666/06 , C08L2666/04 , C08L2666/24 , C08L2666/02 , C08F210/16 , C08F2500/03 , C08F2500/17
摘要： The present invention provides a propylene polymer composition containing a component (A) which is either a propylene block copolymer or a composition containing a propylene polymer and a rubber ingredient; and a component (B) which is a polyolefin copolymer that contains a fraction eluting at 101° C. or higher through temperature rising elution fractionation chromatography, the fraction exhibiting a 13C-NMR peak attributed to an ethylene chain, the polyolefin copolymer having an intrinsic viscosity falling within a range of 0.5 to 10.0 deciliter/g as measured at 135° C. in decalin; a molded product formed from the composition; and a polyolefin copolymer formed of the component (B) in which a propylene polymer segment and an ethylene copolymer segment are chemically linked. According to the invention, a propylene block copolymer or a composition containing a propylene polymer and a rubber ingredient that are excellent in impact strength and tensile strength, while maintaining high rigidity thereof can be produced.
摘要翻译：本发明提供一种丙烯聚合物组合物，其含有作为丙烯嵌段共聚物的组分（A）或含有丙烯聚合物和橡胶组分的组合物; 和含有通过升温洗脱分级分离法在101℃以上洗脱的级分的聚烯烃共聚物的组分（B），表现出由乙烯引起的13 C-NMR峰的级分链，所述聚烯烃共聚物的特性粘度在萘烷中在135℃下测得的范围为0.5-10.0分升/克; 由该组合物形成的模制品; 和由丙烯聚合物链段和乙烯共聚物链段化学连接的组分（B）形成的聚烯烃共聚物。根据本发明，可以制造出具有优异冲击强度和拉伸强度同时保持高刚性的丙烯嵌段共聚物或含有丙烯聚合物和橡胶成分的组合物。

3. 发明申请

US20130066007A1 TERMINALLY UNSATURATED POLYOLEFIN AND METHOD FOR PRODUCING THE SAME 有权
标题翻译：终止不饱和聚烯烃及其制造方法
公开(公告)号：US20130066007A1
公开(公告)日：2013-03-14
申请号：US13700008
申请日：2011-05-17
申请人： Shuji Machida , Tomio Tatsumi , Takenori Fujimura
发明人： Shuji Machida , Tomio Tatsumi , Takenori Fujimura
IPC分类号： C08F8/50 , C08F110/08 , C08F210/06 , C09J151/06 , C08F255/10 , C08L51/06 , C09D151/06 , C08F210/08 , C08F255/02
CPC分类号： C08F10/06 , C08F8/00 , C08F8/50 , C08F110/06 , C08F210/06 , C08F290/042 , C08F2810/40 , C08L23/12 , C08L23/142 , C08L23/22 , C09D155/00 , C09J123/12 , C09J123/142 , C09J123/22 , C09J155/00 , C09K3/10 , C09K2200/0617 , C09K2200/0642 , C08F2500/15 , C08F2500/03 , C08F2500/17 , C08F210/08 , C08F210/16
摘要： A terminally unsaturated polyolefin satisfying the following (1) to (4): (1) the mesopentad fraction [mmmm] of propylene chain unit or butene-1 chain unit is 20 to 80 mol %; (2) the number of terminal vinylidene groups per molecule is 1.3 to 2.5; (3) the weight-average molecular weight Mw is 500 to 100,000; and (4) the molecular weight distribution Mw/Mn is 1.1 to 2.6.
摘要翻译：满足以下（1）〜（4）的末端不饱和的聚烯烃：（1）丙烯链单元或丁烯-1链单元的连翘组分[mmmm]为20〜80摩尔％（2）每分子末端亚乙烯基的数量为1.3〜2.5; （3）重均分子量Mw为500〜100,000; （4）分子量分布Mw / Mn为1.1〜2.6。

4. 发明授权

US06897261B1 Branched olefinic macromonomer, olefin graft copolymer, and olefin resin composition 失效
标题翻译：支链烯烃大分子单体，烯烃接枝共聚物和烯烃树脂组合物
公开(公告)号：US06897261B1
公开(公告)日：2005-05-24
申请号：US10019293
申请日：2000-07-18
申请人： Shuji Machida , Kazuo Sato , Tomio Tatsumi , Yasuhiro Goto
发明人： Shuji Machida , Kazuo Sato , Tomio Tatsumi , Yasuhiro Goto
IPC分类号： C08F290/04 , C08F290/14 , C08F297/08
CPC分类号： C08F290/04 , C08F290/042 , C08F290/14 , C08F290/141
摘要： The invention relates to olefin branched macromonomers, olefin graft copolymers and olefin resin compositions having the advantage of good compatibility with polyolefin resins and good moldability and workability. The olefin branched macromonomer satisfies the following (a) and (b): (a) its weight-average molecular weight (Mw) measured through gel permeation chromatography (GPC) falls between 400 and 200000; (b) its vinyl content is at least 70 mol % of all the unsaturated groups in the macromonomer.
摘要翻译：本发明涉及烯烃支链大分子单体，烯烃接枝共聚物和烯烃树脂组合物，其具有与聚烯烃树脂的良好相容性和良好的成型性和可加工性。烯烃支化大分子单体满足以下（a）和（b）：（a）通过凝胶渗透色谱法（GPC）测定的重均分子量（Mw）为400〜200000; （b）其乙烯基含量为大分子单体中所有不饱和基团的至少70摩尔％。

5. 发明授权

US5608009A Olefin copolymer and process for preparing same 失效
标题翻译：烯烃共聚物及其制备方法
公开(公告)号：US5608009A
公开(公告)日：1997-03-04
申请号：US424384
申请日：1995-04-28
申请人： Shuji Machida , Haruo Shikuma , Toshinori Tazaki , Tomio Tatsumi , Shinichi Kurokawa
发明人： Shuji Machida , Haruo Shikuma , Toshinori Tazaki , Tomio Tatsumi , Shinichi Kurokawa
IPC分类号： C08F8/04 , C08F210/00 , C08F210/02 , C08F210/06 , C08F210/16 , C08F210/18 , C08F255/00 , C08F255/02 , C08F255/08 , C08F279/02
CPC分类号： C08F255/00 , C08F210/00 , C08F210/02 , C08F210/06 , C08F210/18 , C08F8/04 , C08F210/16
摘要： There are herein disclosed an olefin copolymer which comprises an olefin unit and a diolefin unit and in which a weight-average molecular weight is in the range of 200 to 800,000, the content of the diolefin unit is in the range of 0.002 to 30 mol%, and a ratio TUS/DOU between the total content of unsaturated groups observed in a molecular chain (TUS mol%) and the content of the diolefin unit (DOU mol%) is in the range of 0.001 to 200; an olefin graft copolymer obtained by the graft polymerization of this olefin copolymer and an olefin; a hydrogenated olefin copolymer and olefin graft copolymer thereof; and a process for preparing these copolymers.These olefin copolymers are excellent in molding/working properties and have a good thermal stability, transparency and uniformity. Therefore, they are useful as a high-performance VLDPE, LDPE, L-LDPE and HDPE, and further useful as a novel branched propylene polymer, a thermoplastic elastomer, a compatibilizing agent for other resins, and the like.
摘要翻译： PCT No.PCT / JP93 / 01556 Sec。 371日期：1995年4月28日 102（e）日期1995年4月28日PCT提交1993年10月28日PCT公布。公开号WO94 / 10216 PCT 日期1994年5月11日本文公开了一种烯烃共聚物，其包含烯烃单元和二烯烃单元，其中重均分子量在200至800,000的范围内，二烯烃单元的含量在0.002 至30摩尔％，在分子链中观察到的不饱和基团的总含量（TUS摩尔％）与二烯烃单元的含量（D摩尔％）之间的比TUS / DOU在0.001〜200的范围内; 通过该烯烃共聚物和烯烃的接枝聚合得到的烯烃接枝共聚物; 氢化烯烃共聚物及其烯烃接枝共聚物; 以及这些共聚物的制备方法。这些烯烃共聚物的成型/加工性能优异，并且具有良好的热稳定性，透明性和均匀性。因此，它们可用作高性能VLDPE，LDPE，L-LDPE和HDPE，并且还可用作新型支化丙烯聚合物，热塑性弹性体，其它树脂的相容剂等。

6. 发明授权

US08871855B2 Terminally unsaturated polyolefin and method for producing the same 有权
标题翻译：末端不饱和聚烯烃及其制造方法
公开(公告)号：US08871855B2
公开(公告)日：2014-10-28
申请号：US13700008
申请日：2011-05-17
申请人： Shuji Machida , Tomio Tatsumi , Takenori Fujimura
发明人： Shuji Machida , Tomio Tatsumi , Takenori Fujimura
IPC分类号： C08F290/14 , C08G63/91 , C08G63/48 , C08L33/02 , C08F20/08 , C08F22/40 , C09J123/14 , C09K3/10 , C08L23/22 , C08F290/04 , C09J123/22 , C09J123/12 , C08L23/12 , C08F10/06 , C08F110/06 , C08L23/14 , C08F210/06
CPC分类号： C08F10/06 , C08F8/00 , C08F8/50 , C08F110/06 , C08F210/06 , C08F290/042 , C08F2810/40 , C08L23/12 , C08L23/142 , C08L23/22 , C09D155/00 , C09J123/12 , C09J123/142 , C09J123/22 , C09J155/00 , C09K3/10 , C09K2200/0617 , C09K2200/0642 , C08F2500/15 , C08F2500/03 , C08F2500/17 , C08F210/08 , C08F210/16
摘要： A terminally unsaturated polyolefin satisfying the following (1) to (4): (1) the mesopentad fraction [mmmm] of propylene chain unit or butene-1 chain unit is 20 to 80 mol %; (2) the number of terminal vinylidene groups per molecule is 1.3 to 2.5; (3) the weight-average molecular weight Mw is 500 to 100,000; and (4) the molecular weight distribution Mw/Mn is 1.1 to 2.6.
摘要翻译：满足以下（1）〜（4）的末端不饱和的聚烯烃：（1）丙烯链单元或丁烯-1链单元的连翘组分[mmmm]为20〜80摩尔％（2）每分子末端亚乙烯基的数量为1.3〜2.5; （3）重均分子量Mw为500〜100,000; （4）分子量分布Mw / Mn为1.1〜2.6。

7. 发明授权

US06573352B1 Olefinic polymer 失效
标题翻译：烯烃聚合物
公开(公告)号：US06573352B1
公开(公告)日：2003-06-03
申请号：US09424985
申请日：1999-12-03
申请人： Tomio Tatsumi , Shuji Machida , Mitsugu Kanzawa , Yutaka Minami , Yasuhiro Goto , Masato Kijima
发明人： Tomio Tatsumi , Shuji Machida , Mitsugu Kanzawa , Yutaka Minami , Yasuhiro Goto , Masato Kijima
IPC分类号： C08F11006
CPC分类号： C08F10/06 , C08F110/06 , C08F210/06 , C08F290/042 , C08L2205/08 , C08F2500/03 , C08F2500/17 , C08F2500/11 , C08F2500/12 , C08F2500/09 , C08F210/14 , C08F210/16
摘要： Long-chain, branched, propylene-based polymers, of which the melt index and the molecular weight distribution and the melt tension and the limiting viscosity both satisfy specific requirements, have good physical properties that are comparable to or better than those of conventional propylene-based polymers. They have good melt workability and are favorable to large-size blow molding and extrusion foaming. They are favorably used as miscibility improvers for propylene homopolymers and propylene-based copolymers.
摘要翻译：长链，支链，丙烯基聚合物，其熔体指数和分子量分布以及熔体张力和极限粘度都满足特定要求，具有与常规丙烯类聚合物相当或更好的物理性能，基聚合物。它们具有良好的熔融加工性，有利于大型吹塑和挤出发泡。它们有利地用作丙烯均聚物和丙烯基共聚物的混溶性改进剂。

8. 发明授权

US06800711B2 Olefin-based polymer 失效
标题翻译：烯烃类聚合物
公开(公告)号：US06800711B2
公开(公告)日：2004-10-05
申请号：US10417155
申请日：2003-04-17
申请人： Tomio Tatsumi , Shuji Machida , Mitsugu Kanzawa , Yutaka Minami , Yasuhiro Goto , Masato Kijima
发明人： Tomio Tatsumi , Shuji Machida , Mitsugu Kanzawa , Yutaka Minami , Yasuhiro Goto , Masato Kijima
IPC分类号： C08F21014
CPC分类号： C08F10/06 , C08F110/06 , C08F210/06 , C08F290/042 , C08L2205/08 , C08F2500/03 , C08F2500/17 , C08F2500/11 , C08F2500/12 , C08F2500/09 , C08F210/14 , C08F210/16
摘要： Long-chain, branched, propylene-based polymers, of which the melt index and the molecular weight distribution and the melt tension and the limiting viscosity both satisfy specific requirements, have good physical properties that are comparable to or better than those of conventional propylene-based polymers. They have good melt workability and are favorable to large-size blow molding and extrusion foaming. They are favorably used as miscibility improvers for propylene homopolymers and propylene-based copolymers.
摘要翻译：长链，支链，丙烯基聚合物，其熔体指数和分子量分布以及熔体张力和极限粘度都满足特定要求，具有与常规丙烯类聚合物相当或更好的物理性能，基聚合物。它们具有良好的熔融加工性，有利于大型吹塑和挤出发泡。它们有利地用作丙烯均聚物和丙烯基共聚物的混溶性改进剂。

9. 发明申请

US20050245710A1 Process for producing modified butene-1 polymer and modified butene-1 polymer obtained by the process 失效
标题翻译：通过该方法制备改性丁烯-1聚合物和改性丁烯-1聚合物的方法
公开(公告)号：US20050245710A1
公开(公告)日：2005-11-03
申请号：US10504141
申请日：2003-02-19
申请人： Masami Kanamaru , Yutaka Minami , Ryo Aburatani , Tomio Tatsumi
发明人： Masami Kanamaru , Yutaka Minami , Ryo Aburatani , Tomio Tatsumi
IPC分类号： C08F8/00 , C08F8/46 , C08F255/00 , C08F255/10 , C08F257/02 , C08L23/20 , C08L51/00 , C08L51/06 , C09J123/20 , C09J151/00 , C09J151/06 , C08F34/02
CPC分类号： C09J151/003 , C08F255/00 , C08F255/10 , C08F257/02 , C08L23/20 , C08L51/003 , C08L51/06 , C08L2666/02 , C08L2666/24 , C09J123/20 , C09J151/06 , Y10S526/943 , C08F222/06 , C08F220/06 , C08F212/08
摘要： The present invention relates to a process for producing a buten-1-based polymer satisfying the following requirements (a), (b) and (c): (a) a crystalline resin having a melting point (Tm-D) of 0 to 100° C., the melting point being defined as a top of a peak observed on a highest-temperature side in a melting endothermic curve obtained by a differential scanning calorimeter (DSC) when a sample is held in a nitrogen atmosphere at −10° C. for 5 min and then heated at a temperature rise rate of 10° C./min; (b) a stereoregularity index represented by (mmmm)/(mmrr+rmmr) of 20 or less; and (c) a weight-average molecular weight (Mw) of 10,000 to 1,000,000 and a ratio (Mw/Mn) of weight-average molecular weight to number-average molecular weight of 4.0 or less; a modified buten-1-based polymer produced by modifying the buten-1-based polymer with a radical polymerization initiator and an organic acid; and an adhesive composition containing the modified buten-1-based polymer. The modified buten-1-based polymer of the present invention is capable of imparting a high adhesiveness, a high strength and a good softness to polyolefins, and providing sealants having a high adhesiveness, or polyolefins having an improved compatibility to inorganic fillers, etc., in particular, is useful as resins for hot-melt adhesives.
摘要翻译：本发明涉及一种满足以下要求（a），（b）和（c）的丁烯-1系聚合物的制造方法：（a）熔点（Tm-D）为0〜在将样品保持在-10℃的氮气气氛下，通过差示扫描量热计（DSC）获得的熔融吸热曲线中，熔点定义为在最高温度侧观察到的峰的顶部 C. 5分钟，然后以10℃/ min的升温速率加热; （b）由（mmmm）/（mmrr + rmmr）表示的立构规整性指数为20以下; 和（c）重均分子量（Mw）为10,000〜1,000,000，重均分子量与数均分子量的比（Mw / Mn）为4.0以下; 通过用自由基聚合引发剂和有机酸改性丁烯-1-基聚合物制备的改性丁烯-1基聚合物; 和含有改性丁烯-1-基聚合物的粘合剂组合物。本发明的改性丁烯-1类聚合物能够赋予聚烯烃高粘合性，高强度和良好的柔软性，并且提供具有高粘合性的密封剂，或具有改善的与无机填料相容性的聚烯烃等。特别是用作热熔粘合剂的树脂。

10. 发明申请

US20050171295A1 Process for production of modified propylene polymers and modifies propylene polymers produced by the process 失效
标题翻译：制备改性丙烯聚合物的方法，并改性由该方法生产的丙烯聚合物
公开(公告)号：US20050171295A1
公开(公告)日：2005-08-04
申请号：US10509329
申请日：2003-04-11
申请人： Masami Kanamaru , Yutaka Minami , Ryo Aburatani , Tomio Tatsumi , Takenori Fujimura
发明人： Masami Kanamaru , Yutaka Minami , Ryo Aburatani , Tomio Tatsumi , Takenori Fujimura
IPC分类号： C08F8/00 , C08F255/02 , C09J123/10 , C09J123/12 , C08F8/14
CPC分类号： C09J123/12 , C08L2023/42 , C08L2666/02 , C09J123/10
摘要： The present invention relates to a method for producing a modified propylene-based polymer containing modifying a propylene-based polymer by a radical initiator and an organic acid, a modified propylene-based polymer obtained by the method, and an adhesive composition containing the modified propylene-based polymer. The propylene-based polymer is a propylene homopolymer satisfying the conditions of (a) mmmm=20 to 60 mol %, (b) [rrrr/(1-mmmm)]≦0.1, (c) rmrm>2.5 mol %, (d) mmxrr/(mr)2=
摘要翻译：本发明涉及通过自由基引发剂和有机酸改性丙烯类聚合物的改性丙烯类聚合物的制造方法，该方法得到的改性丙烯类聚合物和含有改性丙烯的粘合剂组合物基聚合物。丙烯类聚合物是满足（a）mmmm = 20〜60mol％，（b）[rrrr /（1-mmmm）] <= 0.1，（c）rmrm> 2.5mol％的条件的丙烯均聚物， d）mmxrr /（mr）2≤2.0，（e）在温度程序化色谱法中在25℃以下洗脱的组分的重量比（W25）为20〜100％重量或满足条件（h）通过13 C-NMR测定获得的立构规整度指数（P）的丙烯共聚物为55〜90摩尔％。本发明的改性丙烯类聚合物可以使聚烯烃等具有更好的粘合性，更强或柔性，可用于具有增加与无机填料等的相容性的高粘合密封剂或聚烯烃，特别是作为用于热熔胶的树脂。

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