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1. 发明授权

US07705174B2 Condensed polycyclic π-conjugated organic material, intermediate product therefor, and method of manufacturing condensed polycyclic π-conjugated organic material 有权
标题翻译：稠合多环和共轭有机材料，其中间产物和制备缩合多环和共轭有机材料的方法
公开(公告)号：US07705174B2
公开(公告)日：2010-04-27
申请号：US10525221
申请日：2003-08-20
申请人： Shigehiro Yamaguchi , Caihong Xu , Kohei Tamao
发明人： Shigehiro Yamaguchi , Caihong Xu , Kohei Tamao
IPC分类号： C07F7/08
CPC分类号： C07F7/0807 , C07F7/0812 , C08G61/123 , C08G77/60
摘要： The invention provides condensed polycyclic π-conjugated organic materials and manufacturing methods for the materials. A metal reducing agent is reacted with a straight-chain, triple bond-containing hydrocarbon (aryl acetylene compound, phenyl acetylene compound), the hydrocarbon being a benzene ring with an organic silicon as a substituent, so as to allow an intramolecular reductive cyclization reaction to proceed between the silicon and the triple-bond carbon. The reaction produces condensed polycyclic π-conjugated organic materials of the invention. The invention provides light-emitting materials applicable for organic electroluminescent devices, condensed polycyclic π-conjugated organic materials applicable for charge transport materials, their intermediate products, and a manufacture method for condensed polycyclic π-conjugated organic materials.
摘要翻译：本发明提供了缩合多环和共轭有机材料及其制备方法。使金属还原剂与直链，含三键的烃（芳基乙炔化合物，苯基乙炔化合物）反应，该烃为具有有机硅作为取代基的苯环，以使分子内还原环化反应在硅和三键碳之间进行。该反应产生本发明的缩合多环和共轭有机材料。本发明提供适用于有机电致发光器件，适用于电荷传输材料的冷凝多环和共轭有机材料及其中间产物以及冷凝多环和共轭有机材料的制造方法的发光材料。

2. 发明申请

US20060100433A1 n-conjugated organic material of polycyclic fused ring type,intermediate therefor, and process for producing n-conjugated organic material of polycyclic fused ring type 有权
标题翻译：多环稠环型的正共轭有机材料，其中间体，以及多环稠环类的共轭有机材料的制造方法
公开(公告)号：US20060100433A1
公开(公告)日：2006-05-11
申请号：US10525221
申请日：2003-08-20
申请人： Shigehiro Yamaguchi , Caihong Xu , Kohei Tamao
发明人： Shigehiro Yamaguchi , Caihong Xu , Kohei Tamao
IPC分类号： C07F7/02 , C07F9/02
CPC分类号： C07F7/0807 , C07F7/0812 , C08G61/123 , C08G77/60
摘要： The invention provides condensed polycyclic π-conjugated organic materials and manufacturing methods for the materials. A metal reducing agent is reacted with a straight-chain, triple bond-containing hydrocarbon (aryl acetylene compound, phenyl acetylene compound), the hydrocarbon being a benzene ring with an organic silicon as a substituent, so as to allow an intramolecular reductive cyclization reaction to proceed between the silicon and the triple-bond carbon. The reaction produces condensed polycyclic π-conjugated organic materials of the invention. The invention provides light-emitting materials applicable for organic electroluminescent devices, condensed polycyclic π-conjugated organic materials applicable for charge transport materials, their intermediate products, and a manufacture method for condensed polycyclic π-conjugated organic materials.
摘要翻译：本发明提供稠合多环式π共轭有机材料及其制备方法。使金属还原剂与直链，含三键的烃（芳基乙炔化合物，苯基乙炔化合物）反应，该烃为具有有机硅作为取代基的苯环，以使分子内还原环化反应在硅和三键碳之间进行。该反应产生本发明的稠合多环π-共轭有机材料。本发明提供适用于有机电致发光元件的发光材料，适用于电荷输送材料的缩合多环π共轭有机材料及其中间产物，以及冷凝多环π共轭有机材料的制造方法。

3. 发明授权

US5412105A Thiophene-silole copolymer and its method of manufacture 失效
标题翻译：噻吩 - 噻咯共聚物及其制备方法
公开(公告)号：US5412105A
公开(公告)日：1995-05-02
申请号：US31980
申请日：1993-03-16
申请人： Yoshihiko Ito , Kohei Tamao , Shigehiro Yamaguchi , Yoshiki Nakagawa
发明人： Yoshihiko Ito , Kohei Tamao , Shigehiro Yamaguchi , Yoshiki Nakagawa
IPC分类号： C07F7/08 , C07F7/18 , C08G61/12 , C08G77/60 , C07D333/50 , C07D409/00 , C08G77/22
CPC分类号： C08G61/123 , C07F7/0812 , C07F7/1856 , C08G77/60
摘要： A thiophene-silole copolymer represented by the formula below and its method of manufacture are disclosed; ##STR1## wherein, R is a monofunctional hydrocarbon group having 1 to 20 carbon atoms or hydrogen, A and B are alkyl groups, aromatic groups, alkenyl groups, or represent an aliphatic group forming a ring wherein A is bonded to B, m and p are integers no less than 1, n is a natural number which can be 0, X is a hydrogen or halogen atom, and Y is a hydrogen atom, halogen atom or thiophene.
摘要翻译：公开了由下式表示的噻吩 - 噻咯共聚物及其制备方法：其中，R为碳原子数为1〜20的单官能烃基或氢原子，A和B为烷基，芳香族基团，链烯基，或代表形成环的脂族基团，其中A与B，m键合， p是不小于1的整数，n是可以为0的自然数，X是氢或卤素原子，Y是氢原子，卤素原子或噻吩。

4. 发明申请

US20050170202A1 Polymer and polymeric luminescent element comprising the same 有权
标题翻译：包含其的聚合物和聚合物发光元件
公开(公告)号：US20050170202A1
公开(公告)日：2005-08-04
申请号：US10518713
申请日：2003-06-25
申请人： Kohei Tamao , Shigehiro Yamaguchi , Makoto Kitano , Satoshi Kobayashi , Chizu Sekine
发明人： Kohei Tamao , Shigehiro Yamaguchi , Makoto Kitano , Satoshi Kobayashi , Chizu Sekine
IPC分类号： C08G61/12 , C09K11/06 , H01L51/30 , H01L51/50 , H05B33/14 , C08G79/08 , H01B1/12
CPC分类号： H01L51/0036 , C08G61/123 , C09K11/06 , C09K2211/1491 , H01L51/0035 , H01L51/0079 , H01L51/5012 , H05B33/14 , Y10S428/917 , Y10T428/10
摘要： A polymer characterized by comprising repeating units represented by the following formula (1) and having a number-average molecular weight, in terms of polystyrene, of 103 to 108. (In the formula, R1 represents hydrogen, alkyl, alkoxy, alkylthio, aryl, aryloxy, arylthio, arylalkyl, arylalkoxy, arylalkylthio, arylalkenyl, arylalkynyl, amino, substituted amino, silyl, substituted silyl, silyloxy, substituted silyloxy, monovalent heterocyclic group, or halogeno; and rings D and E each represents an optionally substituted aromatic ring.)
摘要翻译：一种聚合物，其特征在于包括由下式（1）表示的重复单元，其聚苯乙烯换算的数均分子量为10 -3至10 8。（式中，R 1表示氢，烷基，烷氧基，烷硫基，芳基，芳氧基，芳硫基，芳基烷基，芳基烷氧基，芳基烷硫基，芳基烯基，芳基炔基，氨基，取代的氨基，甲硅烷基，取代的甲硅烷基，取代的甲硅烷氧基，一价杂环基或卤素;环D和E各自表示任选取代的芳环）

5. 发明授权

US5986121A Silacyclopentadiene derivatives and an organic electroluminescent element obtained by using the silacyclopentadiene derivative 失效
标题翻译：硅环戊二烯衍生物和通过使用硅环戊二烯衍生物获得的有机电致发光元件
公开(公告)号：US5986121A
公开(公告)日：1999-11-16
申请号：US678936
申请日：1996-07-12
申请人： Manabu Uchida , Takenori Izumizawa , Kenji Furukawa , Kohei Tamao , Shigehiro Yamaguchi
发明人： Manabu Uchida , Takenori Izumizawa , Kenji Furukawa , Kohei Tamao , Shigehiro Yamaguchi
IPC分类号： C07F7/08 , C09K11/06 , H01L51/00 , H01L51/30 , H01L51/50 , H05B33/14 , C07F9/02
CPC分类号： H05B33/14 , C07F7/0807 , C07F7/0812 , C07F7/0818 , C09K11/06 , H01L51/0094 , H01L51/0053 , H01L51/5012 , Y10S428/917
摘要： An electroluminescence element (EL) obtained by using a silacyclopentadiene. derivation expressed by the general formula (I) and the derivative are provided. ##STR1## (wherein X and Y are independently hydrocarbon radicals with from 1 to 6 atoms and R.sub.1 to R.sub.4 are hydrogen, halogens, alkyl radicals with from 1 to 6 carbon atoms, or a condensed (un)substituted ring if being adjacent).
摘要翻译：通过使用硅环戊二烯获得的电致发光元件（EL）。提供了由通式（I）表示的衍生物和衍生物。（其中X和Y独立地为具有1至6个原子的烃基和R 1至R 4为氢，卤素，具有1至6个碳原子的烷基或相邻的稠合（未）取代的环）。

6. 发明授权

US5498736A 2,5-reactive substituent group-containing siloles, silole polycondensates and preparation thereof 失效
标题翻译：含有2,5-反应性取代基的锡洛尔，silole缩聚物及其制备
公开(公告)号：US5498736A
公开(公告)日：1996-03-12
申请号：US360006
申请日：1994-12-20
申请人： Kohei Tamao , Shigehiro Yamaguchi
发明人： Kohei Tamao , Shigehiro Yamaguchi
IPC分类号： C07F7/08 , C07F7/22
CPC分类号： C07F7/0807 , C07F7/2212
摘要： 2,5-Reactive substituent group-containing siloles of the following general formula are provided ##STR1## wherein R.sup.1 to R.sup.4 may be the same or different and independently represent a monovalent hydrocarbon group having from 1 to 12 carbon atoms or a hydrogen atom, and R.sup.5 and R.sup.6 may be the same or different and independently represent a group selected from monovalent hydrocarbon-substituted sulfur, selenium, silicon, germanium, tin and phosphorus, or a halogen atom. Polycondensates of the siloles and processes for preparing the siloles and polycondensates are described.
摘要翻译：提供下列通式的2,5-反活性取代基的锡洛尔：（1）其中R 1至R 4可以相同或不同并且独立地表示具有1至12个碳原子的一价烃基或氢原子，R 5和R 6可以相同或不同，独立地表示选自一价烃取代的硫，硒，硅，锗，锡和磷或卤素原子的基团。叙述siloles的缩聚物和制备siloles和缩聚物的方法。

7. 发明授权

US07157154B2 Polymer and polymeric luminescent element comprising the same 有权
标题翻译：包含其的聚合物和聚合物发光元件
公开(公告)号：US07157154B2
公开(公告)日：2007-01-02
申请号：US10518713
申请日：2003-06-25
申请人： Kohei Tamao , Shigehiro Yamaguchi , Makoto Kitano , Satoshi Kobayashi , Chizu Sekine
发明人： Kohei Tamao , Shigehiro Yamaguchi , Makoto Kitano , Satoshi Kobayashi , Chizu Sekine
IPC分类号： C08G79/08 , H01L51/50 , C09K11/06 , H01B1/12 , H05B33/14
CPC分类号： H01L51/0036 , C08G61/123 , C09K11/06 , C09K2211/1491 , H01L51/0035 , H01L51/0079 , H01L51/5012 , H05B33/14 , Y10S428/917 , Y10T428/10
摘要： A polymer characterized by comprising repeating units represented by the following formula (1) and having a number-average molecular weight, in terms of polystyrene, of 103 to 108. (In the formula, R1 represents hydrogen, alkyl, alkoxy, alkylthio, aryl, aryloxy, arylthio, arylalkyl, arylalkoxy, arylalkylthio, arylalkenyl, arylalkynyl, amino, substituted amino, silyl, substituted silyl, silyloxy, substituted silyloxy, monovalent heterocyclic group, or halogeno; and rings D and E each represents an optionally substituted aromatic ring.)
摘要翻译：一种聚合物，其特征在于包括由下式（1）表示的重复单元，其聚苯乙烯换算的数均分子量为10 -3至10 8。（式中，R 1表示氢，烷基，烷氧基，烷硫基，芳基，芳氧基，芳硫基，芳基烷基，芳基烷氧基，芳基烷硫基，芳基烯基，芳基炔基，氨基，取代的氨基，甲硅烷基，取代的甲硅烷基，取代的甲硅烷氧基，一价杂环基或卤素;环D和E各自表示任选取代的芳环）

8. 发明授权

US6051319A Silacyclopentadiene derivatives and an organic electroluminescent element obtained by using the silacyclopentadiene derivative 有权
标题翻译：硅环戊二烯衍生物和通过使用硅环戊二烯衍生物获得的有机电致发光元件
公开(公告)号：US6051319A
公开(公告)日：2000-04-18
申请号：US265855
申请日：1999-03-11
申请人： Manabu Uchida , Takenori Izumizawa , Kenji Furukawa , Kohei Tamao , Shigehiro Yamaguchi
发明人： Manabu Uchida , Takenori Izumizawa , Kenji Furukawa , Kohei Tamao , Shigehiro Yamaguchi
IPC分类号： C07F7/08 , C09K11/06 , H01L51/00 , H01L51/30 , H01L51/50 , H05B33/14 , B32B9/04
CPC分类号： H05B33/14 , C07F7/0807 , C07F7/0812 , C07F7/0818 , C09K11/06 , H01L51/0094 , H01L51/0053 , H01L51/5012 , Y10S428/917
摘要： An electroluminescence element (EL) obtained by using a silacyclopentadiene derivation expressed by the general formula (I) and the derivative are provided. ##STR1## (wherein X and Y are independently hydrocarbon radicals with from 1 to 6 atoms and R.sub.1 to R.sub.4 are hydrogen, halogens, alkyl radicals with from 1 to 6 carbon atoms, or a condensed (un)substituted ring if being adjacent).
摘要翻译：提供通过使用由通式（I）表示的硅环戊二烯衍生物和衍生物获得的电致发光元件（EL）。（其中X和Y独立地为具有1至6个原子的烃基和R 1至R 4为氢，卤素，具有1至6个碳原子的烷基或相邻的稠合（未）取代的环）。

9. 发明授权

US6005128A Silacyclopentadiene derivative 失效
标题翻译：硅环戊二烯衍生物
公开(公告)号：US6005128A
公开(公告)日：1999-12-21
申请号：US37794
申请日：1998-03-10
申请人： Kohei Tamao , Shigehiro Yamaguchi , Manabu Uchida
发明人： Kohei Tamao , Shigehiro Yamaguchi , Manabu Uchida
IPC分类号： C07F7/10 , C07F7/12 , C07F7/18
CPC分类号： C07F7/10 , C07F7/12 , C07F7/18
摘要： The present invention provides a silacyclopentadiene derivative represented by the following Formula (1): ##STR1## wherein X.sub.1 and Y.sub.1 represent independently a halogen atom, an amino group, a hydroxyl group, or an amino group or a hydroxyl group each having a substituent; R.sub.1 to R.sub.4 represent independently a hydrogen atom, a halogen atom, an alkyl group, an amino group, a silyl group, an aryl group, a cyano group, or the respective groups describe above each having a substituent; out of the groups represented by R.sub.1 to R.sub.4, those adjacent may be combined with each other to form rings; when R.sub.1 and R.sub.4 are phenyl groups or when combined are R.sub.1 with R.sub.2 and R.sub.3 with R.sub.4 respectively to form benzene rings, X.sub.1 and Y.sub.1 are not a chlorine atom or a hydroxyl group; and when R.sub.1 and R.sub.4 are methyl groups, X.sub.1 and Y.sub.1 are not bromine atoms.
摘要翻译：本发明提供由下式（1）表示的硅环戊二烯衍生物：其中X1和Y1独立地表示卤素原子，氨基，羟基或氨基或各自具有取代基的羟基; R 1〜R 4分别独立地表示氢原子，卤素原子，烷基，氨基，甲硅烷基，芳基，氰基或各自具有取代基的各基团。在由R1至R4表示的基团中，相邻的基团可以彼此结合形成环; 当R 1和R 4为苯基时，或者当R 1与R 2和R 3与R 4分别形成苯环时，X 1和Y 1不是氯原子或羟基; 当R 1和R 4为甲基时，X 1和Y 1不是溴原子。

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