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1. 发明申请

US20110009555A1 FLUORINE-CONTAINING POLYMER AND SURFACE-MODIFYING AGENT CONTAINING THE SAME AS ACTIVE INGREDIENT 有权
标题翻译：含有含氟聚合物和表面改性剂，其含有活性成分
公开(公告)号：US20110009555A1
公开(公告)日：2011-01-13
申请号：US12677187
申请日：2008-07-16
申请人： Satoshi Kurihara , Seiichiro Murata , Katsuyuki Sato , Masayosi Horiuti , Sumiko Mouri , Hideki Abe , Ji-Shan Jin
发明人： Satoshi Kurihara , Seiichiro Murata , Katsuyuki Sato , Masayosi Horiuti , Sumiko Mouri , Hideki Abe , Ji-Shan Jin
IPC分类号： C08L27/12 , C08F114/18 , C08F214/18
CPC分类号： C09K3/18 , C08F220/18 , C08F220/24 , C08F220/26
摘要： A fluorine-containing polymer comprising a fluoroalkyl alcohol (meth)acrylic acid derivative represented by a general formula, CnF2n+1(CH2CF2)a(CF2CF2)b(CH2CH2)cOCOCR═CH2 (in the formula, R is a hydrogen atom or a methyl group, n is an integer of 1 to 6, preferably 2 to 4, a is an integer of 1 to 4, b is an integer of 0 to 3, and c is an integer of 1 to 3) containing in 5 to 100 wt % as a polymerization unit. A organic solvent solution or aqueous dispersion of the fluorine-containing polymer is effectively used as, for example, a surface-modifying agent such as a water- and oil-repellent or an oil barrier.
摘要翻译：包含由通式CnF2n + 1（CH2CF2）a（CF2CF2）b（CH2CH2）cOCOCR=CH2表示的氟烷基醇（甲基）丙烯酸衍生物的含氟聚合物（式中，R为氢原子或甲基，n为1〜6的整数，优选为2〜4，a为1〜4的整数，b为0〜3的整数，c为1〜3的整数），以5〜100 wt％作为聚合单元。含氟聚合物的有机溶剂溶液或水分散体有效地用作例如防水防油剂或油屏障的表面改性剂。

2. 发明授权

US08501888B2 Fluorine-containing polymer and surface-modifying agent containing the same as active ingredient 有权
标题翻译：含氟聚合物和含有活性成分的表面改性剂
公开(公告)号：US08501888B2
公开(公告)日：2013-08-06
申请号：US12677187
申请日：2008-07-16
申请人： Satoshi Kurihara , Seiichiro Murata , Katsuyuki Sato , Masayosi Horiuti , Sumiko Mouri , Hideki Abe , Ji-Shan Jin
发明人： Satoshi Kurihara , Seiichiro Murata , Katsuyuki Sato , Masayosi Horiuti , Sumiko Mouri , Hideki Abe , Ji-Shan Jin
IPC分类号： C08F18/20
CPC分类号： C09K3/18 , C08F220/18 , C08F220/24 , C08F220/26
摘要： A fluorine-containing polymer comprising a fluoroalkyl alcohol (meth)acrylic acid derivative represented by a general formula, CnF2n+1(CH2CF2)a(CF2CF2)b(CH2CH2)cOCOCR═CH2 (in the formula, R is a hydrogen atom or a methyl group, n is an integer of 1 to 6, preferably 2 to 4, a is an integer of 1 to 4, b is an integer of 0 to 3, and c is an integer of 1 to 3) containing in 5 to 100 wt % as a polymerization unit. A organic solvent solution or aqueous dispersion of the fluorine-containing polymer is effectively used as, for example, a surface-modifying agent such as a water- and oil-repellent or an oil barrier.
摘要翻译：包含由通式CnF2n + 1（CH2CF2）a（CF2CF2）b（CH2CH2）cOCOCR = CH2表示的氟烷基醇（甲基）丙烯酸衍生物的含氟聚合物（式中，R为氢原子或甲基，n为1〜6的整数，优选为2〜4，a为1〜4的整数，b为0〜3的整数，c为1〜3的整数），以5〜100 wt％作为聚合单元。含氟聚合物的有机溶剂溶液或水分散体有效地用作例如防水防油剂或油屏障的表面改性剂。

3. 发明授权

US08680223B2 Water-and oil-repellent 有权
标题翻译：防水防油
公开(公告)号：US08680223B2
公开(公告)日：2014-03-25
申请号：US12682617
申请日：2008-08-08
申请人： Ji-Shan Jin , Satoshi Kurihara , Sumiko Mouri , Katsuyuki Sato
发明人： Ji-Shan Jin , Satoshi Kurihara , Sumiko Mouri , Katsuyuki Sato
IPC分类号： C08F18/20
CPC分类号： D06M15/248 , C08F220/10 , C08F220/14 , C08F220/18 , C08F220/24 , C08F220/26 , C08F222/10 , C08F2220/286 , C09K3/18 , D06M15/263 , D06M15/277 , D06M15/285 , D06M15/29 , D06M2200/10 , D06M2200/11 , D06M2200/12
摘要： A water- and oil-repellent includes, as an active ingredient, a fluorine-containing copolymer including as a copolymer unit (A) at least one of perfluoroalkylalkyl acrylates and corresponding methacrylates, (B) benzyl acrylate or benzyl methacrylate represented by the general formula: CnF2n+1CmH2mOCOCR═CH2 (wherein R represents a hydrogen atom or a methyl group; n represents 4, 5, or 6; and m represents 1, 2, 3, or 4), (C) a fluorine-free polymerizable monomer other than benzyl acrylate and benzyl methacrylate, and (D) a cross-linkable group-containing polymerizable monomer.
摘要翻译：防水防油剂包括作为共聚物单元（A）的共聚物单元（A）中的至少一种全氟烷基烷基丙烯酸酯和相应的甲基丙烯酸酯的含氟共聚物，（B）丙烯酸苄酯或由通式：CnF2n + 1CmH2mOCOCR=CH2（其中R表示氢原子或甲基; n表示4,5或6; m表示1,2,3或4），（C）无氟可聚合单体其他丙烯酸苄酯和甲基丙烯酸苄酯，（D）可交联基团的可聚合单体。

4. 发明授权

US08916643B2 Water-and oil-repellent 有权
公开(公告)号：US08916643B2
公开(公告)日：2014-12-23
申请号：US13088697
申请日：2011-04-18
申请人： Ji-Shan Jin , Satoshi Kurihara , Sumiko Mouri , Katsuyuki Sato
发明人： Ji-Shan Jin , Satoshi Kurihara , Sumiko Mouri , Katsuyuki Sato
IPC分类号： D06M15/277 , D06M15/29 , D06M15/248 , D06M15/285 , D06M15/263 , C08F220/28 , C08F220/18 , C08F220/24 , C08F220/26
CPC分类号： D06M15/248 , C08F220/10 , C08F220/14 , C08F220/18 , C08F220/24 , C08F220/26 , C08F222/10 , C08F2220/286 , C09K3/18 , D06M15/263 , D06M15/277 , D06M15/285 , D06M15/29 , D06M2200/10 , D06M2200/11 , D06M2200/12
摘要： A water- and oil-repellent includes, as an active ingredient, a fluorine-containing copolymer including as a copolymer unit (A) at least one of perfluoroalkylalkyl acrylates and corresponding methacrylates, (B) benzyl acrylate or benzyl methacrylate represented by the general formula: CnF2n+1CmH2mOCOCR═CH2 (wherein R represents a hydrogen atom or a methyl group; n represents 4, 5, or 6; and m represents 1, 2, 3, or 4), (C) a fluorine-free polymerizable monomer other than benzyl acrylate and benzyl methacrylate, and (D) a cross-linkable group-containing polymerizable monomer.

5. 发明申请

US20100224817A1 WATER-AND OIL-REPELLENT 有权
标题翻译：水和油
公开(公告)号：US20100224817A1
公开(公告)日：2010-09-09
申请号：US12682617
申请日：2008-08-08
申请人： Ji-Shan Jin , Satoshi Kurihara , Sumiko Mouri , Katsuyuki Sato
发明人： Ji-Shan Jin , Satoshi Kurihara , Sumiko Mouri , Katsuyuki Sato
IPC分类号： D06M15/263
CPC分类号： D06M15/248 , C08F220/10 , C08F220/14 , C08F220/18 , C08F220/24 , C08F220/26 , C08F222/10 , C08F2220/286 , C09K3/18 , D06M15/263 , D06M15/277 , D06M15/285 , D06M15/29 , D06M2200/10 , D06M2200/11 , D06M2200/12
摘要： A water- and oil-repellent includes, as an active ingredient, a fluorine-containing copolymer including as a copolymer unit (A) at least one of perfluoroalkylalkyl acrylates and corresponding methacrylates, (B) benzyl acrylate or benzyl methacrylate represented by the general formula: CnF2n+1CmH2mOCOCR═CH2 (wherein R represents a hydrogen atom or a methyl group; n represents 4, 5, or 6; and m represents 1, 2, 3, or 4), (C) a fluorine-free polymerizable monomer other than benzyl acrylate and benzyl methacrylate, and (D) a cross-linkable group-containing polymerizable monomer.
摘要翻译：防水防油剂包括作为共聚物单元（A）的共聚物单元（A）中的至少一种全氟烷基烷基丙烯酸酯和相应的甲基丙烯酸酯的含氟共聚物，（B）丙烯酸苄酯或由通式：CnF2n + 1CmH2mOCOCR=CH2（其中R表示氢原子或甲基; n表示4,5或6; m表示1,2,3或4），（C）无氟可聚合单体其他丙烯酸苄酯和甲基丙烯酸苄酯，（D）可交联基团的可聚合单体。

6. 发明授权

US08796368B2 Water-and oil-repellent 有权
标题翻译：防水防油
公开(公告)号：US08796368B2
公开(公告)日：2014-08-05
申请号：US12739028
申请日：2008-08-08
申请人： Ji-Shan Jin , Sumiko Mouri , Katsuyuki Sato
发明人： Ji-Shan Jin , Sumiko Mouri , Katsuyuki Sato
IPC分类号： C08F220/24 , C08F220/16 , C08F214/08 , C08K5/29
CPC分类号： D06M15/277 , C08F214/18 , C08F220/18 , C08F220/24 , C08F220/26 , C08F2220/286 , C08K5/205 , C09D133/16 , C09K3/18 , D06M15/227 , D06M15/256 , D06M15/273 , D06M15/576 , D06M2200/11 , D06M2200/12
摘要： A water- and oil-repellent comprising an aqueous dispersion of a fluorine-containing copolymer including as a copolymerization unit (a) a perfluoroalkylalkyl (meth)acrylate represented by the general formula CnF2n+1CmH2mOCOCR═CH2 (wherein R represents hydrogen atom or methyl group; n represents 4, 5, or 6; and m represents 1, 2, 3, or 4), (b) benzyl (meth)acrylate, (c) a fluorine-free polymerizable monomer other than benzyl (meth)acrylate, and (d) a cross-linkable group-containing polymerizable monomer; and a blocked isocyanate added to the aqueous dispersion in a weight ratio of 0.05 to 3.0 to the weight of the solid content of the aqueous dispersion.
摘要翻译： 1.一种拒水拒油剂，其特征在于，含有含氟共聚物的水分散体，其含有作为共聚单元（a）由通式CnF2n + 1CmH2mOCOCR=CH2表示的（甲基）丙烯酸全氟烷基烷基酯（其中，R表示氢原子或甲基（甲基）丙烯酸苄酯，（c）除（甲基）丙烯酸苄酯以外的无氟可聚合单体，和（d）可交联基团的可聚合单体; 和与水性分散体的固体成分的重量比为0.05〜3.0的嵌段异氰酸酯。

7. 发明申请

US20100249312A1 WATER-AND OIL-REPELLENT 有权
标题翻译：水和油
公开(公告)号：US20100249312A1
公开(公告)日：2010-09-30
申请号：US12739028
申请日：2008-08-08
申请人： Ji-Shan Jin , Sumiko Mouri , Katsuyuki Sato
发明人： Ji-Shan Jin , Sumiko Mouri , Katsuyuki Sato
IPC分类号： C08L53/00
CPC分类号： D06M15/277 , C08F214/18 , C08F220/18 , C08F220/24 , C08F220/26 , C08F2220/286 , C08K5/205 , C09D133/16 , C09K3/18 , D06M15/227 , D06M15/256 , D06M15/273 , D06M15/576 , D06M2200/11 , D06M2200/12
摘要： A water- and oil-repellent comprising an aqueous dispersion of a fluorine-containing copolymer including as a copolymerization unit (a) a perfluoroalkylalkyl (meth)acrylate represented by the general formula CnF2n+1CmH2mOCOCR═CH2 (wherein R represents hydrogen atom or methyl group; n represents 4, 5, or 6; and m represents 1, 2, 3, or 4), (b) benzyl (meth)acrylate, (c) a fluorine-free polymerizable monomer other than benzyl (meth)acrylate, and (d) a cross-linkable group-containing polymerizable monomer; and a blocked isocyanate added to the aqueous dispersion in a weight ratio of 0.05 to 3.0 to the weight of the solid content of the aqueous dispersion.
摘要翻译： 1.一种拒水拒油剂，其特征在于，含有含氟共聚物的水分散体，其含有作为共聚单元（a）由通式CnF2n + 1CmH2mOCOCR=CH2表示的（甲基）丙烯酸全氟烷基烷基酯（其中，R表示氢原子或甲基（甲基）丙烯酸苄酯，（c）除（甲基）丙烯酸苄酯以外的无氟可聚合单体，和（d）可交联基团的可聚合单体; 和与水性分散体的固体成分的重量比为0.05〜3.0的嵌段异氰酸酯。

8. 发明授权

US09096695B2 Method for producing an aqueous emulsion 有权
标题翻译：水乳液的制造方法
公开(公告)号：US09096695B2
公开(公告)日：2015-08-04
申请号：US12993569
申请日：2009-06-09
申请人： Yoshiyama Kaneumi , Sumiko Mouri , Katsuyuki Sato
发明人： Yoshiyama Kaneumi , Sumiko Mouri , Katsuyuki Sato
IPC分类号： C08L27/12 , C08F2/24 , C08F220/24 , C09K3/18 , C08F214/08 , C08F220/18 , C08F220/26 , C08F220/58
CPC分类号： C08F2/24 , C08F214/08 , C08F220/18 , C08F220/24 , C08F220/26 , C08F220/58 , C09K3/18
摘要： Disclosed is a method for producing an aqueous emulsion containing a fluorine-containing copolymer comprising, as copolymerizable monomers, (A) at least one of a perfluoroalkylalkyl acrylate and a corresponding methacrylate represented by the general formula: CnF2n+1CmH2mOCOCR═CH2, wherein R is hydrogen or methyl group, n is 4, 5, or 6, and m is 1, 2, 3, or 4; (B) benzyl acrylate or benzyl methacrylate; (C) a fluorine-free polymerizable monomer other than benzyl acrylate and benzyl methacrylate; and (D) a crosslinkable group-containing polymerizable monomer; the copolymer being produced by previously subjecting 10 to 80 wt. % of the total weight of component (A) and 0 to 60 wt. % of the total weight of component (B) to a first polymerization reaction using an emulsion polymerization method; and then subjecting the remaining components to a second polymerization reaction using an emulsion polymerization method; wherein an emulsifier is used in the emulsion polymerization reaction in an amount of 21 to 150 parts by weight based on 100 parts by weight of the total weight of polymerizable monomers (A) and (B) used in the first polymerization reaction.
摘要翻译：公开了含有含氟共聚物的水性乳液的方法，该含水共聚物包含作为可共聚单体的（A）丙烯酸全氟烷基烷基酯和由通式C n F 2n + 1C m H 2 mOCO CR = CH 2表示的相应甲基丙烯酸中的至少一种，其中R为氢或甲基，n为4,5或6，m为1,2,3或4; （B）丙烯酸苄酯或甲基丙烯酸苄酯; （C）丙烯酸苄酯和甲基丙烯酸苄酯以外的无氟可聚合单体; 和（D）含可交联基团的可聚合单体; 该共聚物通过预先使10〜80wt。组分（A）的总重量的％和0至60wt。使用乳液聚合法的组分（B）与第一聚合反应的总重量的％; 然后使用乳液聚合法对剩余的组分进行第二聚合反应; 其中基于在第一聚合反应中使用的可聚合单体（A）和（B）的总重量的100重量份，乳液聚合反应中使用的乳化剂的量为21〜150重量份。

9. 发明申请

US20110086962A1 METHOD FOR PRODUCING AN AQUEOUS EMULSION 有权
标题翻译：生产水性乳液的方法
公开(公告)号：US20110086962A1
公开(公告)日：2011-04-14
申请号：US12993569
申请日：2009-06-09
申请人： Yoshiyama Kaneumi , Sumiko Mouri , Katsuyuki Sato
发明人： Yoshiyama Kaneumi , Sumiko Mouri , Katsuyuki Sato
IPC分类号： C08L33/16 , C08K5/06
CPC分类号： C08F2/24 , C08F214/08 , C08F220/18 , C08F220/24 , C08F220/26 , C08F220/58 , C09K3/18
摘要： Disclosed is a method for producing an aqueous emulsion containing a fluorine-containing copolymer comprising, as copolymerizable monomers, (A) at least one of a perfluoroalkylalkyl acrylate and a corresponding methacrylate represented by the general formula: CnF2n+1CmH2mOCOCR═CH2, wherein R is hydrogen or methyl group, n is 4, 5, or 6, and m is 1, 2, 3, or 4; (B) benzyl acrylate or benzyl methacrylate; (C) a fluorine-free polymerizable monomer other than benzyl acrylate and benzyl methacrylate; and (D) a crosslinkable group-containing polymerizable monomer; the copolymer being produced by previously subjecting 10 to 80 wt. % of the total weight of component (A) and 0 to 60 wt. % of the total weight of component (B) to a first polymerization reaction using an emulsion polymerization method; and then subjecting the remaining components to a second polymerization reaction using an emulsion polymerization method; wherein an emulsifier is used in the emulsion polymerization reaction in an amount of 21 to 150 parts by weight based on 100 parts by weight of the total weight of polymerizable monomers (A) and (B) used in the first polymerization reaction.
摘要翻译：公开了含有含氟共聚物的水性乳液的方法，该含水共聚物包含作为可共聚单体的（A）丙烯酸全氟烷基烷基酯和由通式C n F 2n + 1C m H 2 mOCO CR = CH 2表示的相应甲基丙烯酸中的至少一种，其中R为氢或甲基，n为4,5或6，m为1,2,3或4; （B）丙烯酸苄酯或甲基丙烯酸苄酯; （C）丙烯酸苄酯和甲基丙烯酸苄酯以外的无氟可聚合单体; 和（D）含可交联基团的可聚合单体; 该共聚物通过预先使10〜80wt。组分（A）的总重量的％和0至60wt。使用乳液聚合法的组分（B）与第一聚合反应的总重量的％; 然后使用乳液聚合法对剩余的组分进行第二聚合反应; 其中基于在第一聚合反应中使用的可聚合单体（A）和（B）的总重量的100重量份，乳液聚合反应中使用的乳化剂的量为21〜150重量份。

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