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1. 发明授权

US06306286B1 IM-5 phosphorus zeolite, catalytic composition, its preparation and its use in catalytic cracking 有权
标题翻译： IM-5磷沸石，催化剂组成，其制备及其在催化裂化中的应用
公开(公告)号：US06306286B1
公开(公告)日：2001-10-23
申请号：US09569303
申请日：2000-05-11
申请人： Samuel Mignard , Avelino Corma Canos , Joaquin Martinez Triguero , Eric Benazzi , Sylvie Lacombe , Gil Mabilon
发明人： Samuel Mignard , Avelino Corma Canos , Joaquin Martinez Triguero , Eric Benazzi , Sylvie Lacombe , Gil Mabilon
IPC分类号： C01G1105
CPC分类号： C10G11/05 , B01J29/005 , B01J29/084 , B01J29/70 , B01J29/85 , B01J2229/183 , B01J2229/26 , B01J2229/30 , B01J2229/36 , B01J2229/42 , C01B39/026 , C10G2400/20
摘要： An IM-5 zeolite that is modified by adding phosphorus that is optionally dealuminified, preferably in aluminosilicic form, and that contains at most 10% by weight of phosphorus, a composition that contains it, its processes for preparation and its application to catalytic cracking of hydrocarbon feedstocks are described.
摘要翻译：通过添加任选脱磷的铝，优选以铝硅酸盐形式，并且含有至多10重量％的磷的磷，含有它的组合物，其制备方法及其在催化裂化中的应用而改性的IM-5沸石描述了烃原料。

2. 发明授权

US5997725A Catalyst comprising a dioctahedral 2:1 phyllosilicate prepared in a fluoride medium and a process for the hydroconversion of petroleum feeds 失效
标题翻译：包含在氟化物介质中制备的二八面体2：1页硅酸盐的催化剂和用于石油进料加氢转化的方法
公开(公告)号：US5997725A
公开(公告)日：1999-12-07
申请号：US806672
申请日：1997-02-26
申请人： Eric Benazzi , Samuel Mignard
发明人： Eric Benazzi , Samuel Mignard
IPC分类号： B01J29/08 , C10G47/18
CPC分类号： B01J29/084
摘要： The invention concerns a catalyst comprising at least one catalytic element, and a support comprising 20-99% by weight of at least one matrix, 1-80% by weight of at least one 2:1 dioctahedral phyllosilicate containing fluorine and 0-30% by weight of at least one Y zeolite. The catalytic element is from groups VI and/or VIII. Phosphorous can be present. The invention also concerns a process for the hydroconversion of said catalyst.
摘要翻译：本发明涉及包含至少一种催化元素的催化剂和包含20-99重量％的至少一种基质，1-80重量％至少一种含氟二异丁基二甲硅烷基硅酸盐和0-30重量％的至少一种Y沸石。催化元素来自VI族和/或VIII族。可以存在磷。本发明还涉及所述催化剂的加氢转化方法。

3. 发明授权

US6045687A Catalyst containing at least two dealuminated Y zeolites and a conventional hydroconversion process for petroleum cuts using this catalyst 失效
标题翻译：含有至少两种脱铝Y沸石的催化剂和使用该催化剂的石油馏分的常规加氢转化方法
公开(公告)号：US6045687A
公开(公告)日：2000-04-04
申请号：US955626
申请日：1997-10-22
申请人： Samuel Mignard , Nathalie George-Marchal , Eric Benazzi , Slavik Kasztelan
发明人： Samuel Mignard , Nathalie George-Marchal , Eric Benazzi , Slavik Kasztelan
IPC分类号： B01J29/08 , B01J29/16 , B01J35/10 , C10G47/16 , C10G47/18 , C10G47/20
CPC分类号： C10G47/20 , B01J29/084 , C10G47/16 , B01J2229/26 , B01J2229/42
摘要： A catalyst support comprising at least one matrix, at least one Y zeolite with a lattice parameter which is in the range 24.15 .ANG. to 24.38 .ANG. (1 nm=10 .ANG.) and at least one Y zeolite with a lattice parameter of more than 24.38 .ANG. and less than or equal to 24.51 .ANG.. The invention also concerns a catalyst comprising said support and at least one hydro-dehydrogenating element, and a conventional hydroconversion process for petroleum cuts using said catalyst.
摘要翻译：一种催化剂载体，其包含至少一种基质，至少一种具有晶格参数的Y沸石，所述Y沸石的范围为24.15ng至24.38（1nm =10），和至少一个晶格参数大于24.38的Y沸石小于等于24.51安。本发明还涉及包含所述载体和至少一种氢脱氢元件的催化剂，以及使用所述催化剂进行石油切割的常规加氢转化方法。

4. 发明授权

US5961816A Catalyst comprising a trioctahedral 2:1 phyllosilicate prepared in a fluoride medium and a process for the hydroconversion of petroleum feeds 失效
标题翻译：包含在氟化物介质中制备的三八面体2:1页硅酸盐和用于石油进料加氢转化的方法的催化剂
公开(公告)号：US5961816A
公开(公告)日：1999-10-05
申请号：US813587
申请日：1997-03-07
申请人： Eric Benazzi , Samuel Mignard
发明人： Eric Benazzi , Samuel Mignard
IPC分类号： B01J29/08 , C10G47/12 , C10G47/18 , B01J21/16
CPC分类号： B01J29/084 , C10G47/12 , B01J2229/42
摘要： A catalyst comprising at least one catalytic element, and a support comprising 20-99% by weight of at least one matrix, 1-80% by weight of at least one 2:1 trioctahedral phyllosilicate containing fluorine and 0-30% by weight of at least one Y zeolite, in which the catalytic element is from groups VI and/or VIII, and phosphorous can be present, as well as a process for the hydroconversion of petroleum with said catalyst.
摘要翻译：包含至少一种催化元素的催化剂和包含20-99重量％的至少一种基质，1-80重量％至少一种含氟的三氧八面体页硅酸盐的含量为1-30重量％的载体和0-30重量％至少一种Y沸石，其中催化元素来自基团VI和/或VIII，并且可以存在磷，以及用所述催化剂加氢转化石油的方法。

5. 发明授权

US5762902A Catalyst comprising a faujasite type zeolite and a ton type zeolite and a process for the hydroconversion of hydrocarbon petroleum feeds 失效
标题翻译：包含八面沸石型沸石和吨型沸石的催化剂以及烃石油原料的加氢转化方法
公开(公告)号：US5762902A
公开(公告)日：1998-06-09
申请号：US786646
申请日：1997-01-21
申请人： Eric Benazzi , Samuel Mignard , Nathalie George-Marchal , Slavik Kasztelan
发明人： Eric Benazzi , Samuel Mignard , Nathalie George-Marchal , Slavik Kasztelan
IPC分类号： B01J29/08 , B01J29/70 , B01J29/80 , C01B39/20 , C10G47/20 , C10G49/16 , C01B33/36 , B01J29/06
CPC分类号： C10G49/16 , B01J29/80 , B01J29/084 , B01J29/70 , Y10S423/21 , Y10S423/35
摘要： The invention concerns a composition comprising at least one matrix, at least one faujasite type zeolite and at least one TON type zeolite. The TON type zeolite can be Nu-10, THETA-1, KZ-2, or ISI-1. The catalyst also contains at least one hydrogenating element from groups VIII and VI. The catalyst is particularly for use for hydrocracking to maximize the yield of middle distillates (kerosine and gas oil).
摘要翻译：本发明涉及包含至少一种基质，至少一种八面沸石型沸石和至少一种TON型沸石的组合物。 TON型沸石可以是Nu-10，THETA-1，KZ-2或ISI-1。催化剂还含有至少一个来自VIII和VI族的氢化元素。催化剂特别用于加氢裂化以使中间馏分（煤油和瓦斯油）的产率最大化。

6. 发明授权

US5954947A Process for mild hydrocracking of petroleum cuts using a catalyst containing at least two dealuminated Y zeolites 失效
标题翻译：使用含有至少两种脱铝Y沸石的催化剂轻度加氢裂化石油馏分的方法
公开(公告)号：US5954947A
公开(公告)日：1999-09-21
申请号：US955623
申请日：1997-10-22
申请人： Samuel Mignard , Nathalie George-Marchal , Eric Benazzi , Slavik Kasztelan
发明人： Samuel Mignard , Nathalie George-Marchal , Eric Benazzi , Slavik Kasztelan
IPC分类号： B01J29/16 , B01J29/08 , B01J29/40 , B01J29/80 , B01J37/20 , C10G47/16 , C10G47/18 , C10G47/20
CPC分类号： B01J29/80 , C10G47/16 , C10G47/20 , B01J2229/16 , B01J2229/26 , B01J2229/42 , B01J29/084 , B01J29/40
摘要： A mild hydroconversion process for petroleum cuts using a catalyst comprising at least one matrix, at least one Y zeolite with a lattice parameter which is in the range 24.15 .ANG. to 24.38 .ANG. (1 nm--10 .ANG.), at least one Y zeolite with a lattice parameter of more than 24.38 .ANG. and less than or equal to 24.51 .ANG., and at least one hydro-dehydrogenating element.
摘要翻译：用于使用包含至少一种基质，至少一种晶格参数的Y沸石的催化剂进行石油切割的温和加氢转化方法，所述Y沸石的范围为24.15至24.38（1nm-10），至少一个具有晶格参数大于24.38安培，小于或等于24.51安培，以及至少一个氢脱氢元件。

7. 发明授权

US06332976B1 Catalyst containing phosphorous and a process hydrotreatment of petroleum feeds using the catalyst 有权
标题翻译：含有磷的催化剂和使用催化剂的石油进料的工艺加氢处理
公开(公告)号：US06332976B1
公开(公告)日：2001-12-25
申请号：US09310105
申请日：1999-05-12
申请人： Samuel Mignard , Nathalie George-Marchal , Virginie Harle , Slavik Kasztelan
发明人： Samuel Mignard , Nathalie George-Marchal , Virginie Harle , Slavik Kasztelan
IPC分类号： C10G4508
CPC分类号： B01J27/188 , B01J35/002 , B01J35/1019 , B01J35/1061 , B01J35/108 , C10G45/08 , C10G49/04
摘要： The invention concerns an alumina based catalyst containing, expressed as the oxide content by weight, 2-10% by weight of cobalt oxide CoO, 10-30% by weight of molybdenum oxide MoO3 and 4-10% of phosphorous oxide P2O5, with a BET surface area in the range 100-300 m2/g, a crushing strength CSH of more than 1.4 MPa, and an average pore diameter in the range 8-11 nm, the pore volume of pores with diameter of more than 14 nm being less than 0.08 ml/g, or less than 22% of total pore volume, the volume of pores with a diameter of less than 8 nm being at most 0.05 ml/g, or less than 10% of total pore volume, the volume of pores with diameter less than 10 nm being in the range of 20%-70%, the volume of pores with diameter between 10 nm and 13 nm being in the range of 20%-60%, and the volume of pores with a diameter which is in the range 8 to 14 nm being in the range 0.20 ml/g to 0.8 ml/g. The invention also concerns a hydrotreatment process using the catalyst, in particular hydrodesulphuration.
摘要翻译：本发明涉及一种氧化铝基催化剂，其含有氧化物含量为2-10重量％的氧化钴CoO，10-30重量％的氧化钼MoO 3和4-10重量％的氧化磷P2O5，其中a BET表面积在100-300m2 / g范围内，抗碎强度CSH大于1.4MPa，平均孔径在8-11nm范围内，孔径大于14nm的孔体积较小直径小于8nm的孔的体积至少为0.05ml / g，或小于总孔体积的10％，孔的体积小于0.08ml / g，或小于总细孔容积的22％直径小于10nm的范围在20％-70％的范围内，直径在10nm和13nm之间的孔的体积在20％-60％的范围内，直径的孔的体积是在8至14nm的范围内在0.20ml / g至0.8ml / g的范围内。本发明还涉及使用该催化剂，特别是加氢脱硫的加氢处理方法。

8. 发明授权

US06187708B1 Process for activation of catalysts with a nitrogenous compound and excess thionic compound the catalysts that is obtained and it use in hydroconversion 有权
标题翻译：用含氮化合物和过量的硫辛酸化合物活化催化剂的方法，所得催化剂及其在加氢转化中的应用
公开(公告)号：US06187708B1
公开(公告)日：2001-02-13
申请号：US09305285
申请日：1999-05-05
申请人： Samuel Mignard , Virginie Harle , Slavik Kasztelan , Nathalie Marchal-George
发明人： Samuel Mignard , Virginie Harle , Slavik Kasztelan , Nathalie Marchal-George
IPC分类号： B01J3720
CPC分类号： B01J37/20 , C10G47/12
摘要： The invention relates to a process for the sulfurization of hydroconversion catalysts, whereby said catalyst contains at least one element of group VIII of the periodic table and optionally an element of group VI, whereby said metal is present in the oxide state. Said process comprises at least one stage that is carried out in a hydrotreatment zone in the presence of at least one thionic compound and at least one nitrogenous compound. This process is carried out in such a way that before the final sulfurization temperature is reached, at least 130% of the stoichiometric amount of sulfur that is necessary for complete sulfurization of the catalyst is injected in said catalyst.
摘要翻译：本发明涉及一种加氢转化催化剂硫化方法，其中所述催化剂含有至少一种元素周期表第Ⅷ族元素和任选的第Ⅵ族元素，其中所述金属以氧化态存在。所述方法包括在至少一种硫辛酸化合物和至少一种含氮化合物的存在下在加氢处理区中进行的至少一个阶段。该方法是在达到最终硫化温度之前进行的，在催化剂中注入催化剂完全硫化所需的化学计量量的至少130％的硫。

9. 发明授权

US5789637A Process for the hydrogenation of aromatic compounds comprising chlorine injection, using catalysts based on a noble metal 失效
公开(公告)号：US5789637A
公开(公告)日：1998-08-04
申请号：US671501
申请日：1996-06-27
申请人： Samuel Mignard , Virginie France Harle , Slavik Kasztelan , Nathalie Marchal-George
发明人： Samuel Mignard , Virginie France Harle , Slavik Kasztelan , Nathalie Marchal-George
IPC分类号： B01J27/13 , C07B61/00 , C07C5/10 , C07C13/28 , C10G45/52
CPC分类号： C10G45/52
摘要： The invention concerns a process for the hydrogenation of aromatic compounds contained in feeds with an initial boiling point of more than 100.degree. C. and which contain at least 10% by weight of aromatic compounds. It consists of introducing chlorine in a concentration of 0.5-500 ppm by weight with respect to the feed at a temperature of between 200.degree. C. and 450.degree. C., a pressure in the range 1 MPa to 25 MPa, an HSV of between 0.1 h.sup.-1 and 10 h.sup.-1 and a volume ratio of hydrogen to feed of 100-2000. The catalyst used is a noble metal type and contains less than 1% of at least one halogen. Preferably, the catalyst is fluorinated or chlorinated.

10. 发明授权

US06174429B1 Catalyst and process for hydrocracking fractions that contain hydrocarbon 有权
$Catalyst and process for hydrocracking fractions that contain hydrocarbon$
标题翻译：含有烃的加氢裂化馏分的催化剂和方法
公开(公告)号：US06174429B1
公开(公告)日：2001-01-16
申请号：US09175468
申请日：1998-10-20
申请人： Nathalie George-Marchal , Samuel Mignard , Slavik Kasztelan
发明人： Nathalie George-Marchal , Samuel Mignard , Slavik Kasztelan
IPC分类号： C10G4700
CPC分类号： C10G47/20 , B01J29/166 , B01J35/108 , B01J2229/42
摘要： The invention relates to a hydrocracking catalyst that contains at least one metal of group VIB, and/or at least one metal of group VIII of the periodic table, an alumina matrix, phosphorus, optionally at least one element from group VIIA (fluorine), and a zeolite Y that is not fully dealuminificated, with a crystalline parameter that is greater than 2,438 nm, an overall SiO2/Al2O3 ratio that is less than 8, and a framework SiO2/Al2O3 ratio that is less than 21 and greater than the overall SiO2/Al2O3 ratio. The invention also relates to a process for hydrocracking with this catalyst, in particular at low pressure of 7.5 to 11 MPa.
摘要翻译：本发明涉及加氢裂化催化剂，其含有至少一种VIB族金属和/或至少一种周期表第VIII族金属，氧化铝基质，磷，任选地至少一种来自VIIA族（氟）的元素，和未完全脱沥青的沸石Y，其结晶参数大于2,438nm，SiO 2 / Al 2 O 3的总体比小于8，骨架SiO 2 / Al 2 O 3比小于21且大于总体 SiO2 / Al2O3比例。本发明还涉及一种用该催化剂进行加氢裂化的方法，特别是在7.5至11MPa的低压下。

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