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1. 发明申请

WO2004109825A2 CARBON MATERIAL FOR BATTERY ELECTRODE AND PRODUCTION METHOD AND USE THEREOF 审中-公开
标题翻译：用于电池电极的碳材料及其制造方法及其用途
公开(公告)号：WO2004109825A2
公开(公告)日：2004-12-16
申请号：PCT/JP2004/008157
申请日：2004-06-04
申请人： SHOWA DENKO K.K. , NANBA, Youichi , TAKEUCHI, Masataka , SUDOH, Akinori , IINOU, Satoshi
发明人： NANBA, Youichi , TAKEUCHI, Masataka , SUDOH, Akinori , IINOU, Satoshi
IPC分类号： H01M4/58
CPC分类号： H01M4/133 , H01M4/364 , H01M4/366 , H01M4/587 , H01M4/62 , H01M8/0213 , H01M8/0221 , H01M8/0226 , H01M10/052
摘要： The invention relates to a carbon material for forming a battery electrode, comprising carbon powder having a homogeneous structure which is produced by causing an organic compound, serving as a ra.w material of a polymer, to deposit onto and/or permeate into carbonaceous particles, and subsequently polymerizing the organic compound, followed by thermal treatment at a temperature of 1,800 to 3,300°C, which comprises a structure which is substantially uniform throughout the entirety of the particle from the surface to the central core where a graphite crystal structure region and an amorphous structure region are distributed. By using the material, a battery having high discharging capacity and low irreversible capacity, with excellent coulombic efficiency and excellent cycle characteristics can be fabricated.
摘要翻译：本发明涉及一种用于形成电池电极的碳材料，其包含具有均匀结构的碳粉末，其通过使作为聚合物的ra.w材料的有机化合物沉积到和/或渗透到碳质颗粒中而制备然后聚合该有机化合物，然后在1,800至3300℃的温度下进行热处理，该温度包括从表面到中心芯的整个颗粒基本均匀的结构，其中石墨晶体结构区域和分布非晶结构区域。通过使用该材料，可以制造具有高放电容量和低不可逆容量的电池，具有优异的库仑效率和优异的循环特性。

2. 发明申请

WO2010100764A1 COMPOSITE GRAPHITE PARTICLES AND LITHIUM SECONDARY BATTERY USING THE SAME 审中-公开
标题翻译：使用该复合石墨颗粒和锂二次电池
公开(公告)号：WO2010100764A1
公开(公告)日：2010-09-10
申请号：PCT/JP2009/054356
申请日：2009-03-02
申请人： SHOWA DENKO K.K. , LS MTRON Ltd. , SOTOWA, Chiaki , SUDOH, Akinori , TAKEUCHI, Masataka , HAN, Kyung-hee , HAN-Jung-min , OH, Jung-hun
发明人： SOTOWA, Chiaki , SUDOH, Akinori , TAKEUCHI, Masataka , HAN, Kyung-hee , HAN-Jung-min , OH, Jung-hun
IPC分类号： C01B31/04
CPC分类号： H01M4/587 , C01B32/20 , H01M4/133 , H01M4/1393 , H01M10/052
摘要： The present invention provides composite graphite particles, which are useful for a negative electrode in a secondary battery having high capacitance, good charge- discharge characteristics and good charge-discharge cycle characteristics; and a paste for negative electrode, a negative electrode and a lithium secondary battery which use the composite graphite particles. The composite graphite particles of the present invention comprises a core material consisting of graphite having a interlayer distance d(002) of 0.337 nm or less in which the intensity ratio I D /I G (R value) between the peak intensity (I D ) in a range of 1300 to 1400 cm -1 and the peak intensity ( I G ) in a range of 1580 to 1620 cm -1 as measured by Raman spectroscopy spectra is from 0.01 to 0.1 and a carbonaceous surface layer in which the intensity ratio I D /I G (R value) between the peak intensity (I D ) in a range of 1300 to 1400 cm -1 and the peak intensity ( I G ) in a range of 1580 to 1620 cm -1 as measured by Raman scattering spectroscopy is 0.2 or higher; wherein the peak intensity ratio I 110 /I 004 between the peak intensity (I 004 ) of face (110) and the peak intensity (I 004 ) of face (004) obtained by XRD measurement on the graphite crystal is 0.2 or higher when the particles are mixed with a binder and pressure-molded to a density of 1.55 to 1.65 g/cm 3 .
摘要翻译：本发明提供了复合石墨粒子，其可用于具有高电容，良好的充放电特性和良好的充放电循环特性的二次电池中的负极; 以及使用该复合石墨粒子的负极，负极和锂二次电池用糊料。本发明的复合石墨粒子包括由石墨构成的芯材，其中层间距离d（002）为0.337nm以下，其中峰强度（ID）在一定范围内的强度比ID / IG（R值）为1300〜1400cm -1，通过拉曼光谱测定的1580〜1620cm -1范围内的峰强度（IG）为0.01〜0.1，强度比ID / IG（R 通过拉曼散射光谱法测定的在1300〜1400cm -1范围内的峰强度（ID）与1580〜1620cm -1范围内的峰强度（IG）之差为0.2以上; 其中，当将所述颗粒与所述石墨晶体的XRD测量得到的在所述石墨晶体上通过XRD测量获得的面（110）的峰强度（I004）和所述面（004）的峰强度（I004）之间的峰强度比I110 / I004为0.2以上时，粘合剂，并以1.55-1.65g / cm3的密度进行压塑。

3. 发明申请

WO2005011027A2 HIGH DENSITY ELECTRODE AND BATTERY USING THE ELECTRODE 审中-公开
标题翻译：高密度电极和使用电极的电池
公开(公告)号：WO2005011027A2
公开(公告)日：2005-02-03
申请号：PCT/JP2004/011007
申请日：2004-07-27
申请人： SHOWA DENKO K.K. , OHKUBO, Takashi , SUDOH, Akinori , TAKEUCHI, Masataka
发明人： OHKUBO, Takashi , SUDOH, Akinori , TAKEUCHI, Masataka
IPC分类号： H01M4/02
CPC分类号： H01M4/40 , H01M4/13 , H01M4/131 , H01M4/133 , H01M4/134 , H01M4/136 , H01M4/382 , H01M4/405 , H01M4/483 , H01M4/485 , H01M4/505 , H01M4/525 , H01M4/58 , H01M4/581 , H01M4/5815 , H01M4/5825 , H01M4/583 , H01M4/587 , H01M4/625 , H01M10/052 , H01M10/0525 , H01M10/0565 , H01M10/0569 , H01M2004/021 , H01M2300/0082
摘要： The invention relates to a high-density electrode, obtained by impregnating a high-density electrode which comprises an electrode active substance and carbon fiber having a fiber filament diameter of 1 to 1,000 nm and has a porosity of 25% or less, with a solid polymer electrolyte; and to a battery including the resultant (high-density) electrode. According to the invention, electrolytic solution permeability and electrolytic solution retainability, which are matters of importance in realizing a high-density electrode for achieving a battery having a high energy density, can be improved.
摘要翻译：本发明涉及一种高密度电极，其通过浸渍包含电极活性物质和碳纤维的高密度电极而获得，所述碳纤维具有1至1,000nm的纤维丝直径并且具有 25％或更少，用固体聚合物电解质; 并涉及包括所得（高密度）电极的电池。根据本发明，可以改善对实现用于实现具有高能量密度的电池的高密度电极而言重要的电解液渗透性和电解液保持性。

4. 发明申请

WO2005043653A1 CARBON MATERIAL FOR BATTERY ELECTRODE AND PRODUCTION METHOD AND USE THEREOF 审中-公开
标题翻译：用于电池电极的碳材料及其制造方法及其用途
公开(公告)号：WO2005043653A1
公开(公告)日：2005-05-12
申请号：PCT/JP2004/016482
申请日：2004-10-29
申请人： SHOWA DENKO K.K. , SOTOWA, Chiaki , TAKEUCHI, Masataka , SUDOH, Akinori
发明人： SOTOWA, Chiaki , TAKEUCHI, Masataka , SUDOH, Akinori
IPC分类号： H01M4/58
CPC分类号： H01M4/133 , H01M4/1393 , H01M4/583 , H01M4/587 , H01M4/625 , H01M10/0525
摘要： The invention provides a carbon material for a battery electrode, which comprises a carbon powder material as a composite of carbonaceous particles and an a carbon material derived from an organic compound prepared by allowing the organic compound serving as a polymer source material to deposit onto and/or permeate into the carbonaceous particles to thereby polymerize the polymer material and then heating at 1,800 to 3,300°C, and which has an intensity ratio of 0.1 or more for peak intensity attributed to a (110) plane to peak intensity attributed to a (004) plane determined through X-ray diffraction spectroscopic analysis on a mixture of the carbon material and a binder resin when pressed at 10 3 kg/cm 2 or higher. The carbon material which undergoes less deformation/orientation due to application of pressure, has high discharge capacity and small irreversible capacity and exhibiting excellent coulombic efficiency, cycle characteristics and leakage-current load characteristics.
摘要翻译：本发明提供了一种用于电池电极的碳材料，其包括作为碳质颗粒的复合材料的碳粉末材料和通过使用作为聚合物源材料的有机化合物沉积到和/ 或渗透到碳质颗粒中，从而使聚合物材料聚合，然后在1,800〜3300℃下加热，对于（110）面归属于（004）面的峰强度，其强度比为0.1以上）平面，当以10 3 kg / cm 2或更高压力时，通过对碳材料和粘合剂树脂的混合物的X射线衍射光谱分析确定。由于施加压力而变形/取向较少的碳材料具有高放电容量和小的不可逆容量，并表现出优异的库仑效率，循环特性和漏电流负载特性。

5. 发明申请

WO2005011028A1 HIGH DENSITY ELECTRODE AND BATTERY USING THE ELECTRODE 审中-公开
标题翻译：高密度电极和使用电极的电池
公开(公告)号：WO2005011028A1
公开(公告)日：2005-02-03
申请号：PCT/JP2004/011028
申请日：2004-07-27
申请人： SHOWA DENKO K.K. , SUDOH, Akinori , TAKEUCHI, Masataka
发明人： SUDOH, Akinori , TAKEUCHI, Masataka
IPC分类号： H01M4/02
CPC分类号： H01M4/13 , H01M4/131 , H01M4/133 , H01M4/134 , H01M4/136 , H01M4/364 , H01M4/405 , H01M4/485 , H01M4/505 , H01M4/525 , H01M4/58 , H01M4/5815 , H01M4/5825 , H01M4/587 , H01M4/625 , H01M10/052 , H01M10/0525 , H01M10/0565 , H01M2004/021
摘要： The invention relates to a high-density electrode, comprising an electrode active substance and carbon fiber having a filament diameter of 1 to 1,000 nm, wherein the porosity of the electrode is 25% or less. According to the invention, electrolytic solution permeability and electrolytic solution retainability, which are matters of importance in realizing a high-density electrode for achieving a battery having a high energy density, can be improved.
摘要翻译：本发明涉及一种高密度电极，其包含电极活性物质和长丝直径为1〜1000nm的碳纤维，其中电极的孔隙率为25％以下。根据本发明，可以提高在实现用于实现具有高能量密度的电池的高密度电极中重要的电解液渗透性和电解液保持性。

6. 发明公开

EP2187468A1 NEGATIVE ELECTRODE FOR LITHIUM SECONDARY BATTERY, METHOD FOR PRODUCING CARBON-BASED NEGATIVE ELECTRODE ACTIVE MATERIAL, LITHIUM SECONDARY BATTERY AND USE THEREOF 有权
标题翻译：二次电池负极的锂，用于生产负极活性物质中碳系，锂二次电池及其用途
公开(公告)号：EP2187468A1
公开(公告)日：2010-05-19
申请号：EP08827284.4
申请日：2008-08-08
申请人： Showa Denko K.K.
发明人： SOTOWA, Chiaki , SUDOH, Akinori , TAKEUCHI, Masataka
IPC分类号： H01M4/58 , H01M4/02 , H01M4/62 , H01M10/40
CPC分类号： H01M4/133 , H01M4/0471 , H01M4/1393 , H01M4/587 , H01M2004/021 , Y02E60/122 , Y02P70/54 , Y10T29/49108
摘要： Disclosed are a negative electrode for lithium secondary batteries, containing an active material (A) capable of absorbing/desorbing lithium ions and a binder (B), wherein the active material (A) is a carbon-based material obtained from at least one starting material selected from a group consisting of petroleum cokes and coal cokes and having a mean particle size of from 1 to 30 µm and a true density of from 1.90 to 2.00 g/cm 3 and its use; and a method for producing a carbon-based negative electrode active material having a mean particle size of from 1 to 30 µm and a true density of from 1.90 to 2.00 g/cm 3 , the method comprising (a) a step of grinding at least one selected from a group consisting of petroleum cokes and coal cokes, (b) a step of controlling the particle size, and (c) a step of heat-treating in an inert gas atmosphere at 900 to 1900°C.

7. 发明授权

EP2187468B1 NEGATIVE ELECTRODE FOR LITHIUM SECONDARY BATTERY, METHOD FOR PRODUCING CARBON-BASED NEGATIVE ELECTRODE ACTIVE MATERIAL, LITHIUM SECONDARY BATTERY AND USE THEREOF 有权
标题翻译：锂二次电池用负极，碳系负极活性物质的制造方法，锂二次电池及其用途
公开(公告)号：EP2187468B1
公开(公告)日：2018-02-28
申请号：EP08827284.4
申请日：2008-08-08
申请人： Showa Denko K.K.
发明人： SOTOWA, Chiaki , SUDOH, Akinori , TAKEUCHI, Masataka
IPC分类号： H01M4/58 , H01M4/133 , H01M4/1393 , H01M4/139 , H01M4/04 , H01M4/587 , H01M4/02
CPC分类号： H01M4/133 , H01M4/0471 , H01M4/1393 , H01M4/587 , H01M2004/021 , Y02E60/122 , Y02P70/54 , Y10T29/49108
摘要： Disclosed are a negative electrode for lithium secondary batteries, containing an active material (A) capable of absorbing/desorbing lithium ions and a binder (B), wherein the active material (A) is a carbon-based material obtained from at least one starting material selected from a group consisting of petroleum cokes and coal cokes and having a mean particle size of from 1 to 30 µm and a true density of from 1.90 to 2.00 g/cm 3 and its use; and a method for producing a carbon-based negative electrode active material having a mean particle size of from 1 to 30 µm and a true density of from 1.90 to 2.00 g/cm 3 , the method comprising (a) a step of grinding at least one selected from a group consisting of petroleum cokes and coal cokes, (b) a step of controlling the particle size, and (c) a step of heat-treating in an inert gas atmosphere at 900 to 1900°C.

8. 发明公开

EP2282367A1 NEGATIVE ELECTRODE ACTIVE MATERIAL FOR LITHIUM SECONDARY BATTERY, PREPARATION METHOD OF THE SAME, AND LITHIUM SECONDARY BATTERY CONTAINING THE SAME 审中-公开
标题翻译：二次电池用负极活性材料的锂，工艺用于生产和锂二次电池
公开(公告)号：EP2282367A1
公开(公告)日：2011-02-09
申请号：EP09738953.0
申请日：2009-04-28
申请人： Ls Mtron Ltd. , SHOWA DENKO K.K.
发明人： HAN, Jung-Min , OH, Jeong-Hun , KIM, Jong-Sung , YOUM, Chul , HAN, Kyung-Hee , TAKEUCHI, Masataka , SUDOH, Akinori , SOTOWA, Chiaki
IPC分类号： H01M4/58
CPC分类号： H01M4/587 , H01M4/362 , H01M4/364 , H01M10/052
摘要： The present invention relates to a negative electrode active material for a lithium secondary battery, a preparation method thereof, and a lithium secondary battery containing the negative electrode active material. The negative electrode active material for the lithium secondary battery according to the present invention is formed by mixing: a carbon material coated with vapor growth carbon fiber (VGCF) and amorphous graphite; and one or more kinds of other carbon material selected from natural graphite, artificial graphite, amorphous-coated graphite, resin-coated graphite and amorphous carbon. According to the present invention, when the negative electrode active material is prepared, the carbon fiber is uniformly dispersed-throughout the carbon material, and the carbon material is coated with the amorphous graphite and then mixed with other carbon materials, and thus, a high electrode density can be achieved. Accordingly, even with high electrode density, the invention can provide the negative electrode active material with excellent electrochemical properties such as charge/discharge efficiency and cycle characteristics.
摘要翻译：本发明涉及一种负极活性物质的锂二次电池，其制备方法，以及含有该负极活性物质的锂二次电池。用于锂二次电池gemäß到本发明的负极活性材料通过混合而形成：涂布有气相生长碳纤维（VGCF）和非晶质石墨的碳材料; 和其他的碳材料的一种或多种选自天然石墨，人造石墨，非晶质被覆石墨，树脂被覆石墨和无定形碳中选择。。根据本发明，当制备负电极活性材料，碳纤维均匀地分散，在整个碳材料，并且该碳材料涂覆有非晶质石墨，然后与其他碳材料混合，因此，高电极密度就可以实现。如充电/放电效率和循环特性：因此，即使以高电极密度，本发明能够具有优良的电化学性能提供负电极活性材料。

9. 发明公开

EP2282366A1 CARBON NEGATIVE ELECTRODE MATERIAL FOR LITHIUM SECONDARY BATTERY, PRODUCTION METHOD THEREOF AND LITHIUM SECONDARY BATTERY USING THE SAME 有权
标题翻译：碳负极材料用于锂二次电池，工艺用于生产和锂二次电池
公开(公告)号：EP2282366A1
公开(公告)日：2011-02-09
申请号：EP09734880.9
申请日：2009-04-16
申请人： Ls Mtron Ltd. , Showa Denko K.K.
发明人： HAN, Kyung-Hee , OH, Jeong-Hun , KIM, Jong-Sung , YOUM, Chul , HAN, Jung-Min , TAKEUCHI, Masataka , SUDOH, Akinori , SOTOWA, Chiaki
IPC分类号： H01M4/36
CPC分类号： H01M4/587 , H01M4/133 , H01M4/362 , H01M10/052 , Y02E60/122 , Y02P70/54
摘要： A carbon negative electrode material for a lithium secondary battery includes: a core carbon material; and a coated layer covering the core carbon material and comprising a carbon coating material and carbon fiber.
摘要翻译：用于锂二次电池用碳阴极材料，包括：芯碳材料; 和涂布层，覆盖上述芯碳材料并包含被覆用碳材料和碳纤维。

10. 发明授权

EP1961700B1 METHOD FOR PRODUCING GRAPHITE MATERIAL 有权转让
公开(公告)号：EP1961700B1
公开(公告)日：2019-06-26
申请号：EP06834048.8
申请日：2006-12-05
申请人： SHOWA DENKO K.K.
发明人： SUDOH, Akinori , TAKEUCHI, Masataka
IPC分类号： C01B32/205 , H01M4/587 , H01M10/0525

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