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1. 发明申请

WO2017085229A1 CATALYST SYSTEM AND PROCESS FOR THE PRODUCTION OF GLYCOLS 审中-公开
标题翻译：催化剂体系和生产甘油的方法
公开(公告)号：WO2017085229A1
公开(公告)日：2017-05-26
申请号：PCT/EP2016/078079
申请日：2016-11-17
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , SHELL OIL COMPANY
发明人： GEYER, Reinhard , PREISING, Henri , DE VLIEGER, Dionysius, Jacobus, Maria , EDULJI, Smita , VAN DER HEIDE, Evert , LANGE, Jean Paul, Andre, Marie, Joseph, Ghislain
IPC分类号： B01J23/652 , B01J23/888 , B01J27/188 , C07C29/132 , C07C29/60
CPC分类号： B01J23/462 , B01J21/063 , B01J21/066 , B01J21/08 , B01J23/30 , B01J23/40 , B01J23/70 , B01J25/02 , B01J27/188 , B01J35/0006 , B01J2231/643 , C07C29/132 , Y02P20/52 , C07C31/202
摘要： The invention provides a catalyst system comprising: a) one or more Group 1 metal phosphotungstate- containing species; and b) one or more catalytic species suitable for hydrogenation; and a process for the preparation of monoethylene glycol from starting material comprising one or more saccharides, by contacting said starting material with hydrogen in a reactor in the presence of a solvent and said catalyst system.
摘要翻译：本发明提供了一种催化剂体系，其包含：a）一种或多种第1族金属含磷钨酸盐的物质; 和b）一种或多种适用于氢化的催化物质; 以及由包含一种或多种糖类的原料制备单乙二醇的方法，通过在反应器中在溶剂和所述催化剂体系的存在下使所述起始材料与氢气接触来进行。

2. 发明申请

WO2018024787A1 PROCESS FOR THE PRODUCTION OF GLYCOLS 审中-公开
标题翻译：生产甘油的方法
公开(公告)号：WO2018024787A1
公开(公告)日：2018-02-08
申请号：PCT/EP2017/069568
申请日：2017-08-02
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , SHELL OIL COMPANY
发明人： VAN DER HEIDE, Evert , HUIZENGA, Pieter , DE VLIEGER, Dionysius, Jacobus, Maria
IPC分类号： C07C29/132
摘要： The invention provides a process for the preparation of glycols from a saccharide-containing feedstock in a reactor system, said process comprising: i) providing a first feed stream comprising said saccharide-containing feedstock in a first solvent at a temperature of no more than 160°C; ii) providing a second feed stream comprising a tungsten- based retro-aldol catalytic species and an alkali metal containing species in a second solvent at a temperature in the range of from 150 to 250°C; iii) combining the first feed stream and the second feed stream, before they are provided to the reactor system, to form a combined feed stream; iv) providing the combined feed stream to the reactor system and operating the reactor at a temperature in the range of from 150°C to 250°C; and v) also contacting the combined feed stream with a hydrogenation catalytic species in the presence of hydrogen, wherein the molar ratio of alkali metal:tungsten in the combined feed stream is in the range of from 0.55 to 6.
摘要翻译：本发明提供了一种在反应器系统中由含糖原料制备二醇的方法，所述方法包括：i）提供包含所述含糖原料的第一进料流在第一溶剂在不超过160℃的温度下; ii）在150-250℃的温度下，在第二溶剂中提供包含钨基逆向醛Aldol催化物质和含碱金属物质的第二进料流; iii）在将第一原料流和第二原料流提供给反应器系统之前将第一原料流和第二原料流组合以形成合并的原料流; iv）将合并的进料流提供给反应器系统并在150℃至250℃的温度下操作反应器; 和v）还在氢气存在下使合并的进料物流与氢化催化物质接触，其中合并进料物流中碱金属：钨的摩尔比在0.55-6的范围内。

3. 发明申请

WO2017103009A2 HYDROGENATION OR HYDROGENOLYSIS OF AN OXYGENATE 审中-公开
标题翻译：一种氧化物的氢化或氢解
公开(公告)号：WO2017103009A2
公开(公告)日：2017-06-22
申请号：PCT/EP2016/081294
申请日：2016-12-15
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , SHELL OIL COMPANY
发明人： DE VLIEGER, Dionysius, Jacobus, Maria , LANGE, Jean Paul, Andre, Marie, Joseph, Ghislain , EDULJI, Smita , COLIJN, Hendrik, Albertus
IPC分类号： C07C29/149
CPC分类号： C07C29/141 , B01J23/462 , Y02P20/52 , C07C31/202
摘要： A process for the hydrogenation or hydrogenolysis of an oxygenate is disclosed. The process takes place in a reactor in the presence of a catalyst, hydrogen and liquid water and the catalyst comprises one or more elements from Groups 8 to 11 of the periodic table dispersed on a hydrothermally stable oxide support.
摘要翻译：公开了一种用于含氧化合物的氢化或氢解的方法。该方法在催化剂，氢和液态水存在下在反应器中进行，催化剂包含分散在水热稳定的氧化物载体上的周期表第8至11族的一种或多种元素。

4. 发明申请

WO2017178391A1 A PROCESS FOR THE PREPARATION OF A CATALYST AND A PROCESS FOR PRODUCING GLYCOLS USING THE CATALYST 审中-公开
标题翻译：一种催化剂的制备方法和使用该催化剂生产乙二醇的方法
公开(公告)号：WO2017178391A1
公开(公告)日：2017-10-19
申请号：PCT/EP2017/058465
申请日：2017-04-07
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , SHELL OIL COMPANY
发明人： COLIJN, Hendrik, Albertus , DE VLIEGER, Dionysius, Jacobus, Maria
IPC分类号： C07C29/157 , B01J37/18 , B01J23/46 , B01J37/02 , C07C29/141 , C07C29/132
摘要： A process for the preparation of a catalyst composition for catalysing hydrogenation and hydrogenolysis reactions wherein, (a) a carbon support is contacted with a catalyst precursor solution comprising at least one element from groups 7, 8, 9, 10 and 11 of 5 the periodic table to form a metal impregnated carbon; (b) the metal impregnated carbon is dried at a temperature of no greater than 400 o C and placed in a reactor vessel; (c) the reactor vessel is sealed; and (d) the metal impregnated carbon is treated in the reactor 10 vessel in an atmosphere comprising hydrogen at a temperature of from 25 o C to 350 o C.
摘要翻译：制备用于催化氢化和氢解反应的催化剂组合物的方法，其中，（a）使碳载体与包含至少一种来自7,8,9组的元素的催化剂前体溶液接触 5元素周期表中的10和11以形成金属浸渍碳; （b）将金属浸渍的碳在不高于400℃的温度下干燥并置于反应容器中; （c）反应器容器密封; 和（d）金属浸渍的碳在反应器10容器中在25℃至350℃的温度下在包含氢的气氛中处理。

5. 发明申请

WO2017137355A1 PROCESS FOR THE HYDROGENATION OF GLYCOLALDEHYDE 审中-公开
标题翻译：甘油醛的氢化方法
公开(公告)号：WO2017137355A1
公开(公告)日：2017-08-17
申请号：PCT/EP2017/052546
申请日：2017-02-06
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , SHELL OIL COMPANY
发明人： DE VLIEGER, Dionysius, Jacobus, Maria , HUIZENGA, Pieter , VAN DER HEIDE, Evert , EDULJI, Smita , LANGE, Jean Paul, Andre, Marie, Joseph, Ghislain
IPC分类号： C07C29/141 , C07C45/60 , C07C45/67 , C07C31/20 , C07C47/19 , C07H3/02
CPC分类号： C07C29/141 , C07C45/60 , Y02P20/582 , C07C31/202 , C07C47/19
摘要： The invention provides a process for the selective hydrogenation of glycolaldehyde in a process stream comprising glycolaldehyde and one or more monosaccharide in a solvent, said process comprising contacting the process stream with hydrogen in the presence of a hydrogenation catalyst composition at a temperature of no more than 150°C and for a residence time of no more than 90 minutes.
摘要翻译：本发明提供了用于在包含乙醇醛和一种或多种单糖的工艺物流中选择性氢化乙醇醛的方法，所述方法包括使工艺物流与氢在氢化催化剂在不超过150℃的温度和不超过90分钟的停留时间下进行组合。

6. 发明申请

WO2017102992A1 HYDROGENATION OR HYDROGENOLYSIS PROCESS 审中-公开
标题翻译：氢化或氢解过程
公开(公告)号：WO2017102992A1
公开(公告)日：2017-06-22
申请号：PCT/EP2016/081270
申请日：2016-12-15
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , SHELL OIL COMPANY
发明人： DE VLIEGER, Dionysius, Jacobus, Maria , LANGE, Jean Paul, Andre, Marie, Joseph, Ghislain , COLIJN, Hendrik, Albertus , EDULJI, Smita
IPC分类号： B01J21/06 , B01J23/46 , C07C29/141
CPC分类号： B01J23/462 , B01J21/063 , B01J21/066 , B01J21/08 , B01J37/10 , C07C29/141 , C07C31/20
摘要： A catalytic process for the hydrogenation or hydrogenolysis of a reactant in a reactor in the presence of hydrogen and liquid water is disclosed. The catalyst is stable under hydrothermal conditions.
摘要翻译：公开了在氢气和液态水存在下在反应器中对反应物进行氢化或氢解的催化方法。催化剂在水热条件下是稳定的。

7. 发明申请

WO2017137440A1 PROCESS FOR THE PRODUCTION OF ALKYLENE GLYCOLS 审中-公开
标题翻译：生产亚乙基二醇的方法
公开(公告)号：WO2017137440A1
公开(公告)日：2017-08-17
申请号：PCT/EP2017/052759
申请日：2017-02-08
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , SHELL OIL COMPANY
发明人： VAN DER HEIDE, Evert , HUIZENGA, Pieter , DE VLIEGER, Dionysius, Jacobus, Maria
IPC分类号： C07C29/141 , C07C31/20
CPC分类号： C07C29/132 , C07C29/60 , Y02P20/582 , C07C31/202 , C07C31/205 , C07C31/207
摘要： The invention provides a process for the production of alkylene glycols, said process comprising providing a feed comprising at least 10wt% of lignocellulose and/or one or more saccharides, on the basis of the overall feed, in water to a reactor; also providing a feed comprising one or more hydrogen-donating organic solvent species to the reactor; contacting the lignocellulose and/or one or more saccharides in the reactor with a retro-aldol catalyst composition at a temperature in the range of from at least 160 to at most 270°C, wherein the combined solvent system within the reactor comprises in the range of from at least 5 to at most 95wt% of one or more hydrogen-donating organic solvent species and in the range of from at least 5 to at most 95wt% of water.
摘要翻译：本发明提供了生产亚烷基二醇的方法，所述方法包括提供包含至少10重量％木质纤维素和/或一种或多种糖的饲料，基于总饲料，在水加入反应器; 还向反应器提供包含一种或多种供氢有机溶剂物质的进料; 使反应器中的木质纤维素和/或一种或多种糖与逆醛醇催化剂组合物在至少160℃至最多270℃的温度范围内接触，其中反应器内的组合溶剂系统包含在范围的至少5重量％至最多95重量％的一种或多种供氢有机溶剂物质和至少5重量％至最多95重量％的水。

8. 发明申请

WO2017042125A1 PROCESS FOR RECOVERING A METALLIC COMPONENT 审中-公开
标题翻译：回收金属部件的方法
公开(公告)号：WO2017042125A1
公开(公告)日：2017-03-16
申请号：PCT/EP2016/070857
申请日：2016-09-05
申请人： SHELL INTERNATIONALE RESEARCH MAATSCHAPPIJ B.V. , SHELL OIL COMPANY
发明人： COLIJN, Hendrik, Albertus , DE VLIEGER, Dionysius, Jacobus, Maria
IPC分类号： C22B7/00 , C07C29/132
CPC分类号： C22B7/009 , C07C29/132 , Y02P10/214 , C07C31/202
摘要： A process for recovering a metallic component from a hydrocarbon product stream is disclosed. The hydrocarbon product stream is subjected to a thermal oxidation. A process for preparing glycols from a saccharide-containing feedstock is additionally disclosed.
摘要翻译：公开了一种从烃产物流中回收金属成分的方法。烃产物流经受热氧化。另外公开了一种从含糖原料制备二醇的方法。

9. 发明公开

EP3377218A1 CATALYST SYSTEM AND PROCESS FOR THE PRODUCTION OF GLYCOLS 有权
公开(公告)号：EP3377218A1
公开(公告)日：2018-09-26
申请号：EP16801412.4
申请日：2016-11-17
申请人： Shell Internationale Research Maatschappij B.V.
发明人： GEYER, Reinhard , PREISING, Henri , DE VLIEGER, Dionysius, Jacobus, Maria , EDULJI, Smita , VAN DER HEIDE, Evert , LANGE, Jean Paul, Andre, Marie, Joseph, Ghislain
IPC分类号： B01J23/652 , B01J23/888 , B01J27/188 , C07C29/132 , C07C29/60
CPC分类号： B01J27/188 , B01J21/063 , B01J21/066 , B01J21/08 , B01J23/30 , B01J23/40 , B01J23/462 , B01J23/70 , B01J25/02 , B01J35/0006 , B01J2231/643 , B01J2523/69 , C07C29/132 , C07C29/141 , C07C31/202 , Y02P20/52
摘要： The invention provides a catalyst system comprising: a) one or more Group 1 metal phosphotungstate-containing species; and b) one or more catalytic species suitable for hydrogenation; and a process for the preparation of monoethylene glycol from starting material comprising one or more saccharides, by contacting said starting material with hydrogen in a reactor in the presence of a solvent and said catalyst system.

10. 发明授权

EP3347499B1 PROCESS FOR RECOVERING OF METALLS 有权
公开(公告)号：EP3347499B1
公开(公告)日：2019-12-11
申请号：EP16766255.0
申请日：2016-09-05
申请人： Shell Internationale Research Maatschappij B.V.
发明人： COLIJN, Hendrik, Albertus , DE VLIEGER, Dionysius, Jacobus, Maria
IPC分类号： C22B7/00 , C07C29/132

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