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1. 发明授权

US4463072A Secondary batteries containing room-temperature molten 1,2,3-trialkylimidazolium halide non-aqueous electrolyte 失效
标题翻译：含有室温熔融的1,2,3-三烷基咪唑卤化物非水电解质的二次电池
公开(公告)号：US4463072A
公开(公告)日：1984-07-31
申请号：US556497
申请日：1983-11-30
申请人： Paul R. Gifford , James B. Palmisano , Lawrence W. Shacklette , Ronald R. Chance , James E. Toth
发明人： Paul R. Gifford , James B. Palmisano , Lawrence W. Shacklette , Ronald R. Chance , James E. Toth
IPC分类号： H01M4/36 , H01M4/60 , H01M4/62 , H01M6/14 , H01M10/36
CPC分类号： H01M4/36 , H01M10/36 , H01M4/60 , H01M4/621 , H01M6/14
摘要： Batteries and especially secondary batteries employing an anode comprising aluminum and a molten, non-aqueous electrolyte containing admixtures of aluminum halide and 1,2,3-trialkylimidazolium halides having the formula TimX: ##STR1## wherein R.sub.1, R.sub.2 and R.sub.3 are independently alkyl groups of 1 to 12 carbons and X is independently halide or mixtures of halides, e.g., chloride and/or bromide are disclosed. The molar ratio of aluminum hereinafter denoted by Al, to trialkylimidalozium, hereinafter denoted by Tim, in the electrolyte, may be varied over a wide range so as to make the molten electrolyte composition acidic and as such the electrolyte is useful in batteries, especially secondary batteries employing aluminum anodes and a variety of cathodes.
摘要翻译：电池，特别是使用包含铝的阳极和含有卤化铝和具有式TimX的1,2,3-三烷基咪唑卤化物的熔融非水电解质的二次电池：其中R1，R2和R3独立地为烷基 1至12个碳，X独立地为卤化物或卤化物的混合物，例如氯化物和/或溴化物。以下由Al表示的铝与三烷基酰亚胺的摩尔比（以下用Tim表示）在电解质中可以在宽范围内变化，以使熔融电解质组合物呈酸性，并且因此电解质可用于电池，特别是二次采用铝阳极和各种阴极的电池。

2. 发明授权

US4463071A Secondary batteries using room-temperature molten non-aqueous electrolytes containing 1,2,3-trialkylimidazolium halides or 1,3-dialkylimidazolium halide 失效
标题翻译：使用含有1,2,3-三烷基咪唑鎓卤化物或1,3-二烷基咪唑鎓卤化物的室温熔融非水电解质的二次电池
公开(公告)号：US4463071A
公开(公告)日：1984-07-31
申请号：US556496
申请日：1983-11-30
申请人： Paul R. Gifford , Lawrence W. Shacklette , James E. Toth , James F. Wolf
发明人： Paul R. Gifford , Lawrence W. Shacklette , James E. Toth , James F. Wolf
IPC分类号： H01M4/36 , H01M4/60 , H01M6/14 , H01M10/36
CPC分类号： H01M6/14 , H01M10/36 , H01M4/36 , H01M4/60
摘要： Batteries and especially secondary batteries employing selected anodes and cathodes such as conjugated backbone polymers and transition metal chalcogenides inserted with alkali metal cations (especially lithium) and molten, non-aqueous electrolyte compositions containing admixture of aluminum halide and at least one of 1,2,3-trialkylimidazolium halide and 1,3-dialkylimidazolium halide having the formulae TimX and DimX, respectively: ##STR1## wherein R.sub.1, R.sub.2, R.sub.3, R.sub.4, and R.sub.5 are independently alkyl groups of 1 to 12 carbons and X is independently halide, e.g., chloride and bromide and in some instances an alkali metal and/or tetraalkylammonium salt which may also be incorporated into the electrolyte composition are disclosed. The molar ratio of aluminum to trialkylimidazolium or to dialkylimidazolium in the electrolyte, may be varied over a wide range so as to make the molten electrolyte composition basic or neutral and as such the electrolyte is useful in batteries, especially secondary batteries comprising anodes of reduced conjugated backbone polymers or lithiated transition-metal chalcogenides such as Li.sub.x WO.sub.2 and a variety of cathodes such as oxidized conjugated backbone polymers or lithiated transition-metal chalcogenides such as Li.sub.x CoO.sub.2.
摘要翻译：电池，特别是使用插入有碱金属阳离子（特别是锂）的共轭主链聚合物和过渡金属硫族化合物的选定阳极和阴极以及阴极，其包含铝卤化物和至少一种1,2的混合物的熔融的非水电解质组合物， 3-三烷基咪唑鎓卤化物和具有式TimX和DimX的1,3-二烷基咪唑鎓卤化物：其中R 1，R 2，R 3，R 4和R 5独立地为1至12个碳的烷基，X独立地为卤素，例如，氯化物和溴化物，并且在一些情况下，还可以并入电解质组合物中的碱金属和/或四烷基铵盐。电解质中铝与三烷基咪唑或二烷基咪唑的摩尔比可以在很宽的范围内变化，以使熔融电解质组合物成为碱性或中性，因此电解质可用于电池，尤其是包含还原共轭阳极的二次电池骨架聚合物或锂化过渡金属硫族化物如LixWO2和各种阴极如氧化共轭主链聚合物或锂化过渡金属硫族化物如LixCoO2。

3. 发明授权

US4695521A Conjugated polymer as substrate for the plating of alkali metal in a nonaqueous secondary battery 失效
标题翻译：共轭聚合物作为非水二次电池中碱金属电镀的底物
公开(公告)号：US4695521A
公开(公告)日：1987-09-22
申请号：US749325
申请日：1985-06-27
申请人： Lawrence W. Shacklette , James E. Toth , Ronald L. Elsenbaumer
发明人： Lawrence W. Shacklette , James E. Toth , Ronald L. Elsenbaumer
IPC分类号： H01M4/137 , H01M4/36 , H01M4/60 , H01M10/05 , H01M10/40
CPC分类号： H01M4/137 , H01M10/05 , H01M4/36 , H01M4/60
摘要： This invention relates to a novel anode for use in batteries, and to batteries containing the anode, which anode comprises of an electronically conductive n-doped conjugated backbone polymer having finely divided elemental alkali metal particles dispersed therein.
摘要翻译：本发明涉及一种用于电池的新型阳极，以及含有该阳极的电池，该阳极由其中分散有细分的元素碱金属颗粒的电子导电n掺杂共轭主链聚合物组成。

4. 发明授权

US4668596A Negative electrodes for non-aqueous secondary batteries composed on conjugated polymer and alkali metal alloying or inserting material 失效
标题翻译：由共轭聚合物和碱金属合金化或插入材料组成的非水二次电池的负极
公开(公告)号：US4668596A
公开(公告)日：1987-05-26
申请号：US875526
申请日：1986-06-20
申请人： Lawrence W. Shacklette , Taiguang R. Jow , James E. Toth , MacRae Maxfield
发明人： Lawrence W. Shacklette , Taiguang R. Jow , James E. Toth , MacRae Maxfield
IPC分类号： H01M4/02 , H01M4/04 , H01M4/36 , H01M4/40 , H01M4/48 , H01M4/60 , H01M4/62 , H01M4/66 , H01M4/74 , H01M6/14 , H01M10/36 , H01M6/16
CPC分类号： H01M10/05 , H01M10/36 , H01M4/0461 , H01M4/13 , H01M4/36 , H01M4/364 , H01M4/602 , H01M4/621 , H01M4/622 , H01M4/661 , H01M4/745 , H01M6/14 , H01M2004/027 , H01M2300/0025 , H01M4/40 , H01M4/485
摘要： This invention relates to a novel anode for use in batteries, and to batteries containing the anode, which anode comprises a mixture of a conjugated backbone polymer and another electroactive material selected from the group consisting of metals which alloy with alkali metals and alkali metal cation inserting materials as for example transition metal chalcogenides.
摘要翻译：本发明涉及一种用于电池的新型阳极和含阳极的电池，所述阳极包括共轭骨架聚合物和另一种电活性材料的混合物，该电极活性材料选自与碱金属和碱金属阳离子插入材料例如过渡金属硫族化物。

5. 发明授权

US4526708A Irreversible donor doping of conjugated backbone polymers 失效
标题翻译：共轭主链聚合物的不可逆施主掺杂
公开(公告)号：US4526708A
公开(公告)日：1985-07-02
申请号：US556718
申请日：1983-11-30
申请人： Ronald L. Elsenbaumer , Granville G. Miller , James E. Toth
发明人： Ronald L. Elsenbaumer , Granville G. Miller , James E. Toth
IPC分类号： C08K5/56 , C08F8/42 , C08J5/18 , C08L49/00 , H01B1/12 , H01L51/30 , H01M4/60 , H01M10/05 , H01B1/06
CPC分类号： H01M10/05 , H01L51/0041 , H01M4/60
摘要： Conjugated backbone polymers (e.g., polyacetylene), especially formed into a battery electrode, are contacted with a compound MR where M is an alkali metal and R is alkyl of 1-12 carbons, phenyl or alkylphenyl of 7-12 carbons. The method is particularly suited to treatment of battery electrodes to avoid a high initial internal resistance.
摘要翻译：特别是形成电池电极的共轭主链聚合物（例如聚乙炔）与化合物MR接触，其中M是碱金属，R是1-12个碳的烷基，苯基或7-12个碳的烷基苯基。该方法特别适用于处理电池电极以避免高的初始内阻。

6. 发明授权

US4640006A Method of forming battery electrode by irreversible donor doping of conjugated backbone polymers 失效
标题翻译：通过共轭主链聚合物的不可逆施主掺杂形成电池电极的方法
公开(公告)号：US4640006A
公开(公告)日：1987-02-03
申请号：US745099
申请日：1985-06-17
申请人： Ronald L. Elsenbaumer , Granville G. Miller , James E. Toth
发明人： Ronald L. Elsenbaumer , Granville G. Miller , James E. Toth
IPC分类号： H01L51/30 , H01M4/60 , H01M10/05 , H01M10/38 , H01B1/06
CPC分类号： H01M4/60 , H01L51/0041 , H01M10/05 , Y10T29/49108
摘要： Conjugated backbone polymers (e.g., polyacetylene), especially formed into a battery electrode, are contacted with a compound MR where M is an alkali metal and R is alkyl of 1-12 carbons, phenyl or alkylphenyl of 7-12 carbons. The method is particularly suited to treatment of battery electrodes to avoid a high initial internal resistance.
摘要翻译：特别是形成电池电极的共轭主链聚合物（例如聚乙炔）与化合物MR接触，其中M是碱金属，R是1-12个碳的烷基，苯基或7-12个碳的烷基苯基。该方法特别适用于处理电池电极以避免高的初始内阻。

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