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1. 发明授权

US4500417A Conversion of Fischer-Tropsch products 失效
标题翻译：费托产品的转化
公开(公告)号：US4500417A
公开(公告)日：1985-02-19
申请号：US453970
申请日：1982-12-28
申请人： Nai Y. Chen , Werner O. Haag , Tracy J. Huang , Stephen S. Wong
发明人： Nai Y. Chen , Werner O. Haag , Tracy J. Huang , Stephen S. Wong
IPC分类号： C10G45/64 , B01J29/00 , B01J29/74 , B01J29/78 , C07C1/00 , C07C1/04 , C07C9/00 , C07C67/00 , C10G47/16 , C10G49/08 , C10G47/20
CPC分类号： C10G47/16 , B01J2229/37 , B01J29/7415 , B01J29/7815 , Y10S208/95
摘要： The high boiling fraction of Fischer-Tropsch synthesis is upgraded by contact with a catalyst comprising a high-silica, large pore zeolite and a hydrogenation component. The products are a distillate fraction characterized by low sulfur and nitrogen content, high isoparaffin content and low pour point and a lube fraction characterized by its high viscosity index and low pour point.
摘要翻译：通过与包含高二氧化硅，大孔沸石和氢化组分的催化剂接触来提高费 - 托合成的高沸点馏分。该产品是以低硫和氮含量，高异链烷烃含量和低倾点为特征的馏出物部分，其特征在于其高粘度指数和低倾点。

2. 发明授权

US4260839A Ethane conversion process 失效
标题翻译：乙烷转化过程
公开(公告)号：US4260839A
公开(公告)日：1981-04-07
申请号：US57924
申请日：1979-07-16
申请人： Nai Y. Chen , Werner O. Haag , Tracy J. Huang
发明人： Nai Y. Chen , Werner O. Haag , Tracy J. Huang
IPC分类号： C07C2/00 , C07C4/00 , C07C9/04 , B01J29/30 , C07C2/12 , C07C6/10
CPC分类号： C07C2/00 , C07C4/00 , C07C2529/40 , C07C2529/50 , C07C2529/65 , C07C2529/70 , Y10S208/02
摘要： A process for effecting an endothermic and an exothermic reaction, under conversion conditions, in a single reaction zone wherein ethane is endothermically converted to C.sub.3 + hydrocarbons, and wherein an unconverted portion of ethane is simultaneously exothermically hydrogenated to methane in the presence of a catalyst system comprising a crystalline aluminosilicate zeolite having a uniform structure characterized by pores, the major dimension of which is less than 6 Angstroms and ZSM-5 type aluminosilicate zeolite, containing a minor amount of Zn in combination with a Group VIII noble metal or a Group IB metal, the exothermic reaction providing sufficient heat to maintain the reaction zone at a temperature capable of sustaining the endothermic reaction.
摘要翻译：在转化条件下在单一反应区中进行吸热和放热反应的方法，其中乙烷吸热转化为C 3+烃，并且其中未转化部分的乙烷在催化剂体系存在下同时放热氢化成甲烷，所述催化剂体系包含具有均匀结构的结晶硅铝酸盐沸石，其主要尺寸小于6埃，ZSM-5型硅铝酸盐沸石，其含有少量的Zn与VIII族贵金属或IB族金属组合，放热反应提供足够的热量以将反应区保持在能够维持吸热反应的温度。

3. 发明授权

US4229608A Heat balanced cyclic process for manufacture of light olefins 失效
标题翻译：用于制造轻质烯烃的热平衡循环过程
公开(公告)号：US4229608A
公开(公告)日：1980-10-21
申请号：US970718
申请日：1978-12-18
申请人： Nai Y. Chen , Werner O. Haag , Rudolph M. Lago
发明人： Nai Y. Chen , Werner O. Haag , Rudolph M. Lago
IPC分类号： B01J8/38 , C07C1/20 , C07C1/00
CPC分类号： B01J8/388 , C07C1/20 , C07C2529/06 , C07C2529/50 , C07C2529/70 , Y02P20/584 , Y02P30/42
摘要： A catalytic heat balanced cyclic process is provided for converting a charge consisting essentially of methanol, dimethyl ether or mixtures thereof to a hydrocarbon product rich in ethylene and propylene by contact, under specified conditions of temperature and contact time, with a catalyst comprising a crystalline aluminosilicate zeolite characterized by pores, the major dimension of which is less than 6 Angstroms and the capability, under such conditions, of producing less than about 20 weight percent methane in said hydrocarbon product, regenerating the catalyst so employed at a temperature between about 1200.degree. and about 1400.degree. F. to remove accumulated carbonaceous deposit therefrom and provide a source of hot regenerated catalyst for further contact, under controlled temperature conditions, with said charge.
摘要翻译：提供催化热平衡循环方法，用于在基本上由甲醇，二甲醚或其混合物组成的电荷下，在特定的温度和接触时间条件下，与包含结晶硅铝酸盐的催化剂接触，将富含乙烯和丙烯的烃产物沸石的特征在于其主要尺寸小于6埃的孔，以及在这种条件下在所述烃产物中产生小于约20重量％的甲烷的能力，在约1200℃和约1400°F以从其中除去积聚的碳质沉积物，并提供热再生催化剂源，在受控的温度条件下与所述电荷进一步接触。

4. 发明授权

US4339606A Conversion of ketones over metal-containing zeolite catalysts 失效
标题翻译：酮与含金属的沸石催化剂的转化
公开(公告)号：US4339606A
公开(公告)日：1982-07-13
申请号：US232074
申请日：1981-02-06
申请人： Tracy J. Huang , Werner O. Haag
发明人： Tracy J. Huang , Werner O. Haag
IPC分类号： C07C45/73 , C07C45/45
CPC分类号： C07C45/73
摘要： Ketones are converted in one step to saturated dimeric ketones by passing them over a zeolite having a silica to alumina ratio of at least 12 and a Constraint Index of from 1 to 12 and containing a Group VIII metal.
摘要翻译：将酮通过使它们通过二氧化硅与氧化铝之比至少为12且约束指数为1至12并含有第Ⅷ族金属的沸石而在一个步骤中转化成饱和二聚酮。

5. 发明授权

US4157338A Conversion of synthesis gas to hydrocarbon mixtures 失效
标题翻译：将合成气转化为烃混合物
公开(公告)号：US4157338A
公开(公告)日：1979-06-05
申请号：US883970
申请日：1978-03-06
申请人： Werner O. Haag , Tracy J. Huang
发明人： Werner O. Haag , Tracy J. Huang
IPC分类号： C07C1/04
CPC分类号： C07C1/0455 , C07C2529/068
摘要： A mixture of carbon monoxide and hydrogen is contacted with a mixture comprising an element selected from the group consisting of ruthenium, rhodium and osmium carbon monoxide reduction catalyst and a crystalline alumino-silicate providing a pore dimension greater than about 5 Angstroms and a constraint index in the range of 1 to 12 to produce hydrocarbon mixtures useful in forming gasoline boiling range products, aromatic rich hydrocarbons, and chemical intermediates.
摘要翻译：将一氧化碳和氢气的混合物与包含选自钌，铑和锇一氧化碳还原催化剂的元素的混合物和提供孔尺寸大于约5埃的结晶铝硅酸盐接触，并且约束指数范围为1至12，以产生可用于形成汽油沸点产物，富含芳烃的化学中间体的烃混合物。

6. 发明授权

US4252736A Conversion of synthesis gas to hydrocarbon mixtures utilizing dual reactors 失效
标题翻译：使用双重反应器将合成气转化为烃混合物
公开(公告)号：US4252736A
公开(公告)日：1981-02-24
申请号：US44873
申请日：1979-06-01
申请人： Werner O. Haag , Tracy J. Huang , James W. Kuo , Reuel Shinnar
发明人： Werner O. Haag , Tracy J. Huang , James W. Kuo , Reuel Shinnar
IPC分类号： C01B3/16 , C07C1/04 , C07C1/06 , C10G3/00 , C10L1/06
CPC分类号： C07C1/066 , C01B3/16 , C07C1/0485 , C10G3/49 , C10L1/06 , C10G2300/1022 , C10G2300/805 , C10G2300/807 , C10G2400/02 , C10G2400/04 , C10G2400/28 , C10J2300/093 , C10J2300/0959 , C10J2300/0973 , C10J2300/1659 , C10J2300/1662 , Y02P20/52 , Y02P30/20 , Y10S208/95
摘要： In the conversion of coal to gaseous and liquid products, the heat value of the coal is more completely retained by the products through the selective high efficiency conversion of coal to a low ratio syngas utilizing a portion of the Fischer-Tropsch generated heat recovered as steam, conversion of the low ratio syngas with a water gas shift F-T catalyst to a product comprising C.sub.1 to C.sub.50 hydrocarbons and oxygenates, converting the F-T product to premium gas and increased liquid fuels comprising gasoline and distillate with a special zeolite catalyst and recovering the SNG and LPG products of the selective steps to provide an improved product slate. A portion of the produced fuel gas is used in lieu of coal to provide some of the heat energy requirements of the combination process.
摘要翻译：在将煤转化为气态和液态产物时，煤的热值通过煤的选择性高效转化为低比合成气而更完全地保留，利用一部分费 - 托产生的作为蒸汽回收的热量将低比例合成气与水煤气变换FT催化剂转化为包含C1至C50烃和含氧化合物的产物，将FT产物转化为优质气体，并用特殊的沸石催化剂将含有汽油和馏出物的液体燃料转化为回收SNG和石油气产品的选择性步骤提供了改进的产品板岩。使用生产的燃料气体的一部分代替煤以提供组合过程的一些热能需求。

7. 发明授权

US4159995A Conversion of synthesis gas to hydrocarbon mixtures utilizing dual reactors 失效
标题翻译：使用双重反应器将合成气转化为烃混合物
公开(公告)号：US4159995A
公开(公告)日：1979-07-03
申请号：US826487
申请日：1977-08-22
申请人： Werner O. Haag , Tracy J. Huang
发明人： Werner O. Haag , Tracy J. Huang
IPC分类号： C07C1/04
CPC分类号： C07C1/0485 , C07C2523/04 , C07C2523/745 , C07C2523/78 , Y10S585/943
摘要： A gaseous mixture of carbon monoxide and hydrogen is contacted in a first reactor with an iron Fischer-Tropsch catalyst such as potassium promoted iron under special conditions and the total products from said contact are then converted in a second reactor containing HZSM-5 to obtain either a highly olefinic or highly aromatic product depending on reaction conditions.
摘要翻译：一氧化碳和氢气的气体混合物在特殊条件下在第一反应器中与铁费 - 托催化剂如促进铁的铁接触，然后将所述接触物的总产物在含有HZSM-5的第二反应器中转化，以获得高度烯烃或高度芳族的产物，这取决于反应条件。

8. 发明授权

US4097367A Conversion of olefinic naphtha 失效
标题翻译：烯烃石脑油的转化
公开(公告)号：US4097367A
公开(公告)日：1978-06-27
申请号：US818632
申请日：1977-07-25
申请人： Werner O. Haag , Tracy J. Huang
发明人： Werner O. Haag , Tracy J. Huang
IPC分类号： C07C5/373 , B01J29/00 , B01J29/70 , B01J29/74 , C07B61/00 , C07C1/00 , C07C2/76 , C07C15/02 , C07C67/00 , C10G35/06 , C10G35/095 , C10G45/04 , C10G45/10 , C10G45/54
CPC分类号： C10G35/095 , B01J29/7049 , B01J29/74
摘要： High severity catalytic conversion of olefinic naphthas which contain diolefins is conducted over special catalysts to yield a product stream which contains little or no non-aromatics boiling in the range of benzene, toluene and xylene. The catalysts are combinations of zinc and a metal of Groups I B and VIII of the Periodic Table with a crystalline aluminosilicate zeolite having a silica/alumina ratio greater than 12 and a constraint index not less than one nor greater than 12.
摘要翻译：含有二烯烃的烯烃石脑油的高度苛刻度催化转化是通过特殊的催化剂进行的，以产生在苯，甲苯和二甲苯范围内很少或没有非芳族化合物沸腾的产物流。催化剂是锌和元素周期表ⅠB和Ⅷ族金属与二氧化硅/氧化铝比大于12的结晶硅铝酸盐沸石和约束指数不小于1或不超过12的组合。

9. 发明授权

US4409412A Process for producing alkyl aromatic compounds 失效
标题翻译：烷基芳族化合物的制备方法
公开(公告)号：US4409412A
公开(公告)日：1983-10-11
申请号：US423337
申请日：1982-09-24
申请人： Werner O. Haag , Tracy J. Huang
发明人： Werner O. Haag , Tracy J. Huang
IPC分类号： C07C2/86
CPC分类号： C07C2/862 , C07C2529/40 , C07C2529/44 , C07C2529/46
摘要： A process for alkylating aromatic compounds wherein the product aromatics are provided with one or more alkyl groups possessing at least two carbon atoms is disclosed wherein starting aromatic compound(s) and an alkylating atent which is a mixture of hydrogen and/or a hydrogen-containing substance which provides hydrogen under process conditions and a carbon oxide, e.g., a mixture of syngas (hydrogen and carbon monoxide) are reacted at elevated temperature in the presence of an activated catalyst containing metal values selected from the group consisting of iron, cobalt, ruthenium, manganese, rhodium and osmium, and a zeolite having a constraint index of 12 or less, e.g., ZSM-5. The alkylated aromatics can be dealkylated by known and conventional means to provide olefin and the dealkylated aromatics can be recycled to the alkylation zone.
摘要翻译：公开了一种芳族化合物的烷基化方法，其中产物芳族化合物具有一个或多个具有至少两个碳原子的烷基，其中起始芳族化合物和烷基化剂是氢和/或含氢的混合物在工艺条件下提供氢的物质和碳氧化物，例如合成气（氢气和一氧化碳）的混合物在升高的温度下在活性催化剂存在下反应，所述催化剂含有选自铁，钴，钌的金属值，锰，铑和锇以及具有12或更小约束指数的沸石，例如ZSM-5。烷基化芳族化合物可以通过已知和常规方法脱烷基化以提供烯烃，并且脱烷基化的芳族化合物可以再循环到烷基化区。

10. 发明授权

US4279830A Conversion of synthesis gas to hydrocarbon mixtures utilizing dual reactors 失效
标题翻译：使用双重反应器将合成气转化为烃混合物
公开(公告)号：US4279830A
公开(公告)日：1981-07-21
申请号：US44872
申请日：1979-06-01
申请人： Werner O. Haag , Tracy J. Huang
发明人： Werner O. Haag , Tracy J. Huang
IPC分类号： C07C1/04 , C10G3/00 , C10L1/06
CPC分类号： C07C1/046 , C07C1/0485 , C10G3/49 , C10G3/54 , C10L1/06 , C07C2523/04 , C07C2523/745 , C07C2523/78 , C10G2300/1022 , C10G2300/4006 , C10G2300/4012 , C10G2300/4018 , C10G2300/805 , C10G2400/02 , Y02P30/20 , Y10S208/95
摘要： The conversion of less than 1 H.sub.2 /CO ratio syngas to high yield of C.sub.3 plus product is accomplished with a CO reducing catalyst comprising shift characteristics and the product of Fischer-Tropsch synthesis is converted to premium gasoline and distillate fuels by contact with acidic ZSM-5 zeolite.The syngas conversion may be accomplished in any catalyst system permitting a very close temperature control on the exotherm encountered and the gasoline-distillate yield relationship may be varied as a function of temperature and pressure.
摘要翻译：通过包含转移特性的CO还原催化剂实现小于1 H 2 / CO比合成气转化为高产率的C3加产物，并且通过与酸性ZSM-3接触将费 - 托合成的产物转化为优质汽油和馏出燃料， 5沸石。合成气转化可以在任何催化剂体系中完成，允许对所遇到的放热进行非常接近的温度控制，并且汽油馏出物收率关系可以随着温度和压力的变化而变化。

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