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1. 发明授权

US08816043B2 Difluoro benzotriazolyl solar cell material, preparation method and use thereof 有权
标题翻译：二氟苯并三唑基太阳能电池材料及其制备方法及用途
公开(公告)号：US08816043B2
公开(公告)日：2014-08-26
申请号：US14126896
申请日：2011-09-23
申请人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Hui Huang
发明人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Hui Huang
IPC分类号： C08G75/00
CPC分类号： C08G75/06 , B82Y10/00 , C08G61/122 , C08G61/123 , C08G61/126 , C08G2261/146 , C08G2261/3223 , C08G2261/3241 , C08G2261/3246 , C08G2261/3327 , C08G2261/344 , C08G2261/364 , C08G2261/413 , C08G2261/91 , C09B21/00 , C09B23/105 , H01G9/2059 , H01L51/0036 , H01L51/0047 , H01L51/4253 , Y02E10/549 , Y02P70/521
摘要： The present invention relates to solar cells and discloses a difluoro benzotriazolyl solar cell material and preparation method and use thereof. The solar cell material is represented by formula (I), wherein both R1 and R2, are C1 to C20 alkyl, and n is an integer from 10 to 50. In the difluoro benzotriazolyl solar cell material, since the 1,2,3-benzotriazole solar cell material contains two fluorine atoms, the HOMO energy level is reduced by 0.11 eV, while the fluorine-substituted 1,2,3-benzotriazole has two imido groups with electron-withdrawing ability; the fluorine-substituted 1,2,3-benzotriazole is a heterocyclic compound with strong electron-withdrawing ability, and an alkyl chain can be easily introduced to the N-position of the N—H bond of the benzotriazole. The functional group of the alkyl chain can improve the solar energy conversion efficiency, thus solving the low efficiency problem of solar cells made of the solar cell material.
摘要翻译：本发明涉及太阳能电池，并公开了二氟苯并三唑基太阳能电池材料及其制备方法和用途。太阳能电池材料由式（I）表示，其中R1和R2均为C1至C20烷基，n为10至50的整数。在二氟苯并三唑基太阳能电池材料中，苯并三唑太阳能电池材料含有两个氟原子，HOMO能级降低0.11eV，而氟取代的1,2,3-苯并三唑具有两个具有吸电能力的亚氨基; 氟取代的1,2,3-苯并三唑是具有强吸电能力的杂环化合物，并且可以容易地将烷基链引入到苯并三唑的N-H键的N位上。烷基链的官能团可以提高太阳能转换效率，从而解决由太阳能电池材料制成的太阳能电池的低效率问题。

2. 发明申请

US20140230902A1 CO-POLYMER OF 2,7-FLUORENE AND BITHIAZOLE, METHOD FOR PREPARING SAME AND SOLAR BATTERY CONTAINING SAME 审中-公开
标题翻译： 2,7-氟和双嘧啶的聚合物，其制备方法和含有其的太阳能电池
公开(公告)号：US20140230902A1
公开(公告)日：2014-08-21
申请号：US14347510
申请日：2011-11-30
申请人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Hui Huang
发明人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Hui Huang
IPC分类号： H01L51/00
CPC分类号： H01L51/0043 , C08G61/123 , C08G2261/124 , C08G2261/1412 , C08G2261/3142 , C08G2261/3229 , C08G2261/411 , C08G2261/91 , H01L51/0036 , H01L51/0039 , Y02E10/549
摘要： Provided are a co-polymer of formula (I) of 2,7-fluorene and bithiazole, a method for preparing same, and a solar battery containing same. The structural formula of the copolymer of 2,7-fluorene and bithiazole is as shown by formula (I), wherein both R1 and R2 are C1-C20 alkyl groups, and n is an integer of 10-100. The co-polymer of the present invention has a novel structure, a good dissolving property, an excellent film-forming property, and a high power conversion efficiency, and can be used as the material for a solar battery. Also provided are the method for preparing the co-polymer and the solar battery containing same. The preparation method uses raw materials widely available and has a simple synthesis route.
摘要翻译：提供了2,7-芴和双噻唑的式（I）的共聚物，其制备方法和含有它的太阳能电池。 2,7-芴和双噻唑的共聚物的结构式如式（I）所示，其中R1和R2均为C1-C20烷基，n为10-100的整数。本发明的共聚物具有新颖的结构，良好的溶解性，优异的成膜性和高的功率转换效率，可用作太阳能电池的材料。还提供了制备共聚物和含有它的太阳能电池的方法。制备方法使用广泛使用的原料，具有简单的合成路线。

3. 发明申请

US20140090711A1 DIFLUORO BENZOTRIAZOLYL SOLAR CELL MATERIAL, PREPARATION METHOD AND USE THEREOF 有权
标题翻译：二氟苯甲酸钠太阳能电池材料及其制备方法及用途
公开(公告)号：US20140090711A1
公开(公告)日：2014-04-03
申请号：US14126896
申请日：2011-09-22
申请人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Hui Huang
发明人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Hui Huang
IPC分类号： C08G75/06 , H01G9/20
CPC分类号： C08G75/06 , B82Y10/00 , C08G61/122 , C08G61/123 , C08G61/126 , C08G2261/146 , C08G2261/3223 , C08G2261/3241 , C08G2261/3246 , C08G2261/3327 , C08G2261/344 , C08G2261/364 , C08G2261/413 , C08G2261/91 , C09B21/00 , C09B23/105 , H01G9/2059 , H01L51/0036 , H01L51/0047 , H01L51/4253 , Y02E10/549 , Y02P70/521
摘要： The present invention relates to solar cells and discloses a difluoro benzotriazolyl solar cell material and preparation method and use thereof. The solar cell material is represented by formula (I), wherein both R1 and R2, are C1 to C20 alkyl, and n is an integer from 10 to 50. In the difluoro benzotriazolyl solar cell material, since the 1,2,3-benzotriazole solar cell material contains two fluorine atoms, the HOMO energy level is reduced by 0.11 eV, while the fluorine-substituted 1,2,3-benzotriazole has two imido groups with electron-withdrawing ability; the fluorine-substituted 1,2,3-benzotriazole is a heterocyclic compound with strong electron-withdrawing ability, and an alkyl chain can be easily introduced to the N-position of the N—H bond of the benzotriazole. The functional group of the alkyl chain can improve the solar energy conversion efficiency, thus solving the low efficiency problem of solar cells made of the solar cell material.
摘要翻译：本发明涉及太阳能电池，并公开了二氟苯并三唑基太阳能电池材料及其制备方法和用途。太阳能电池材料由式（I）表示，其中R1和R2均为C1至C20烷基，n为10至50的整数。在二氟苯并三唑基太阳能电池材料中，苯并三唑太阳能电池材料含有两个氟原子，HOMO能级降低0.11eV，而氟取代的1,2,3-苯并三唑具有两个具有吸电能力的亚氨基; 氟取代的1,2,3-苯并三唑是具有强吸电能力的杂环化合物，并且可以容易地将烷基链引入到苯并三唑的N-H键的N位上。烷基链的官能团可以提高太阳能转换效率，从而解决由太阳能电池材料制成的太阳能电池的低效率问题。

4. 发明申请

US20140128558A1 AMINE-CONTAINING DIFLUORO BENZOTRIAZOLYL POLYMER, PREPARATION METHOD AND USE THEREOF 有权
标题翻译：含氨基二烯基苯甲酰基聚合物，其制备方法及其用途
公开(公告)号：US20140128558A1
公开(公告)日：2014-05-08
申请号：US14128707
申请日：2011-09-23
申请人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Hui Huang
发明人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Hui Huang
IPC分类号： H01L51/00
CPC分类号： H01L51/0043 , B82Y10/00 , C08G61/12 , C08G61/123 , C08G61/126 , C08G2261/1424 , C08G2261/146 , C08G2261/3162 , C08G2261/3223 , C08G2261/3227 , C08G2261/3241 , C08G2261/3327 , C08G2261/344 , C08G2261/364 , C08G2261/413 , C08G2261/91 , C08G2261/94 , C09B57/008 , C09B69/105 , C09B69/109 , H01L51/0035 , H01L51/0036 , H01L51/0047 , H01L51/4253 , Y02E10/549 , Y02P70/521
摘要： The present disclosure relates to the field of solar cells. An amine-containing difluoro benzotriazolyl polymer, preparation method, and use thereof are provided; the polymer has a structure as represented by formula (I), both R1 and R2 are alkyls from C1 to C20, n is an integer from 10 to 50. In the polymer of the present disclosure, because the 1, 2, 3-benzotriazole solar cell material contains two fluorine atoms, the HOMO energy level is reduced by 0.11 eV, the fluorine-substituted 1, 2, 3-benzotriazole has two imido groups with strong electron-withdrawing property; the 1, 2, 3-benzotriazole is a heterocyclic compound with strong electron-withdrawing property, and an alkyl chain can be easily introduced to the N-position of the N—H bond of the benzotriazole; the functional group of the alkyl chain can improve solar energy conversion efficiency, thus solving the low efficiency problem of the solar cell made from the solar cell material.
摘要翻译：本公开涉及太阳能电池领域。提供含胺的二氟苯并三唑基聚合物，其制备方法和用途; 该聚合物具有由式（I）表示的结构，R 1和R 2均为C 1至C 20的烷基，n为10至50的整数。在本公开的聚合物中，由于1,2-苯并三唑太阳能电池材料含有两个氟原子，HOMO能级降低0.11eV，氟取代的1,2,3-苯并三唑具有强吸电性的两个亚氨基; 1,3-苯并三唑是具有强吸电性的杂环化合物，可以容易地将烷基链引入苯并三唑的N-H键的N位; 烷基链的官能团可以提高太阳能转换效率，从而解决由太阳能电池材料制成的太阳能电池的低效率问题。

5. 发明授权

US08871897B2 Amine-containing difluoro benzotriazolyl polymer, preparation method and use thereof 有权
标题翻译：含胺二氟苯并三唑基聚合物，其制备方法和用途
公开(公告)号：US08871897B2
公开(公告)日：2014-10-28
申请号：US14128707
申请日：2011-09-23
申请人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Hui Huang
发明人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Hui Huang
IPC分类号： C08G75/00 , H01L51/00 , C08G61/12 , H01L51/42
CPC分类号： H01L51/0043 , B82Y10/00 , C08G61/12 , C08G61/123 , C08G61/126 , C08G2261/1424 , C08G2261/146 , C08G2261/3162 , C08G2261/3223 , C08G2261/3227 , C08G2261/3241 , C08G2261/3327 , C08G2261/344 , C08G2261/364 , C08G2261/413 , C08G2261/91 , C08G2261/94 , C09B57/008 , C09B69/105 , C09B69/109 , H01L51/0035 , H01L51/0036 , H01L51/0047 , H01L51/4253 , Y02E10/549 , Y02P70/521
摘要： An amine-containing difluoro benzotriazolyl polymer, preparation method, and use thereof are provided; the polymer has a structure as represented by formula (I), both R1 and R2 are alkyls from C1 to C20, n is an integer from 10 to 50. In the polymer of the present disclosure, because the 1,2,3-benzotriazole solar cell material contains two fluorine atoms, the HOMO energy level is reduced by 0.11 eV, the fluorine-substituted 1,2,3-benzotriazole has two imido groups with strong electron-withdrawing property; the 1,2,3-benzotriazole is a heterocyclic compound with strong electron-withdrawing property, and an alkyl chain can be easily introduced to the N-position of the N—H bond of the benzotriazole; the functional group of the alkyl chain can improve solar energy conversion efficiency, thus solving the low efficiency problem of the solar cell made from the solar cell material.
摘要翻译：提供含胺的二氟苯并三唑基聚合物，其制备方法和用途; 聚合物具有由式（I）表示的结构，R1和R2均为C1至C20的烷基，n为10至50的整数。在本公开的聚合物中，由于1,2,3-苯并三唑太阳能电池材料含有两个氟原子，HOMO能级降低0.11eV，氟取代的1,2,3-苯并三唑具有两个吸电子性强的亚氨基; 1,2,3-苯并三唑是具有强吸电性的杂环化合物，可以容易地将烷基链引入苯并三唑的N-H键的N位; 烷基链的官能团可以提高太阳能转换效率，从而解决由太阳能电池材料制成的太阳能电池的低效率问题。

6. 发明申请

US20140251430A1 POLYMER SOLAR CELL AND METHOD FOR PREPARING SAME 审中-公开
标题翻译：聚合物太阳能电池及其制备方法
公开(公告)号：US20140251430A1
公开(公告)日：2014-09-11
申请号：US14355004
申请日：2011-11-28
申请人： Mingjie Zhou , Ping Wang , Hui Huang , Zhenhua Zhang
发明人： Mingjie Zhou , Ping Wang , Hui Huang , Zhenhua Zhang
IPC分类号： H01L51/44 , H01L51/00
CPC分类号： H01L51/441 , H01L51/0035 , H01L51/0036 , H01L51/0038 , H01L51/4246 , H01L51/4253 , H01L2251/301 , Y02E10/549 , Y02P70/521
摘要： The present invention relates to a polymer solar cell and a method for preparing the same. The cell comprises a conductive anode substrate, a hole buffer layer, an active polymer layer, an electron buffer layer and a cathode laminated in succession, wherein the hole buffer layer comprises a metal compound host and a guest doped in the metal compound host, the metal compound host being one selected from ZnO, ZnS and CdS and the doped gust being one selected from Li2CO3, Li2O, LiF, LiCl and LiBr. By doping a lithium compound with few electrons as a dopant into the metal compound host, a p-type doped layer facilitating the hole transportation is formed in the polymer solar cell. The dopant and the metal compound host have stable properties and would not corrode the conductive anode substrate, facilitating industrial production in the future and effectively improving the energy conversion efficiency of the polymer solar cell.
摘要翻译：聚合物太阳能电池及其制备方法技术领域本发明涉及聚合物太阳能电池及其制备方法。电池包括导电阳极基板，空穴缓冲层，活性聚合物层，电子缓冲层和阴极层叠，其中空穴缓冲层包含金属化合物主体和掺杂在金属化合物主体中的客体，金属化合物主体为选自ZnO，ZnS和CdS，掺杂阵风为选自Li2CO3，Li2O，LiF，LiCl和LiBr中的一种。通过将少量电子的锂化合物掺杂到金属化合物主体中，在聚合物太阳能电池中形成有助于空穴传输的p型掺杂层。掺杂剂和金属化合物主体具有稳定的性能，不会腐蚀导电阳极基板，有利于将来的工业生产，并有效提高聚合物太阳能电池的能量转换效率。

7. 发明申请

US20140163166A1 FLUORENE-CONTAINING DIFLUORO BENZOTRIAZOLYL COPOLYMER AND PREPARATION METHOD AND USE THEREOF 审中-公开
标题翻译：含氟二烯基苯并噻唑共聚物及其制备方法及其应用
公开(公告)号：US20140163166A1
公开(公告)日：2014-06-12
申请号：US14234333
申请日：2011-09-23
申请人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Lusheng Liang
发明人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Lusheng Liang
IPC分类号： H01L31/0216
CPC分类号： H01L31/02167 , C08G61/123 , C08G61/126 , C08G2261/146 , C08G2261/3142 , C08G2261/3241 , C08G2261/344 , C08G2261/411 , C08G2261/91 , H01L51/0035 , H01L51/0036 , H01L51/0039 , H01L51/0043 , H01L51/42 , Y02E10/549
摘要： The present invention relates to solar cells. Disclosed are a fluorene-containing difluoro benzotriazolyl copolymer and preparation method and use thereof; the copolymer has a structure as represented by formula (I), wherein both R1 and R2 are alkyls from C1 to C20, and n is an integer from 10 to 100. In the fluorene-containing difluoro benzotriazolyl copolymer of the present invention, because the 1,2,3-benzotriazole copolymer contains two fluorine atoms, the HOMO energy level will be reduced by 0.11 eV while the fluorine-substituted 1,2,3-benzotriazole has two imido groups with strong electron-withdrawing property; the difluoro benzotriazole is a heterocyclic compound with strong electron-withdrawing property, and an alkyl chain can be easily introduced to the N-position of the N—H bond of the benzotriazole; the functional group of the alkyl chain can improve solar energy conversion efficiency, thus solving the low efficiency problem of polymer solar cells.
摘要翻译：本发明涉及太阳能电池。公开了含芴二氟苯并三唑共聚物及其制备方法和用途; 该共聚物具有由式（I）表示的结构，其中R1和R2均为C1至C20的烷基，n为10-100的整数。在本发明的含芴二氟苯并三唑共聚物中，由于 1,2,3-苯并三唑共聚物含有两个氟原子，HOMO能级将降低0.11eV，而氟取代的1,2,3-苯并三唑具有强吸电性的两个亚氨基; 二氟苯并三唑是具有强吸电性的杂环化合物，烷基链可以容易地引入到苯并三唑的N-H键的N位上; 烷基链的官能团可以提高太阳能转换效率，从而解决聚合物太阳能电池的低效问题。

8. 发明申请

US20130267657A1 PHOTOVOLTAIC POLYMER MATERIAL, PREPARATION METHOD AND USE THEREOF 有权
标题翻译：光伏聚合物材料，制备方法及其用途
公开(公告)号：US20130267657A1
公开(公告)日：2013-10-10
申请号：US13992166
申请日：2010-12-30
申请人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Lusheng Liang
发明人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Lusheng Liang
IPC分类号： H01L31/0256
CPC分类号： H01L31/0256 , C08G61/123 , C08G61/126 , C08G2261/3241 , C08G2261/3243 , C08G2261/3246 , C08G2261/344 , C08G2261/91 , H01L51/0036 , H01L51/0043 , H01L51/4253 , Y02E10/549 , Y02P70/521
摘要： A photovoltaic polymer material, preparation method and use thereof are provided. Said photovoltaic polymer material has the following formula (I). The photovoltaic polymer material has the thiophene-phenylene-thiophene (TPT) derivative as the basic structure unit, and by the introduction of D1 and D2 structures to modify the TPT, and the photovoltaic polymer material has the characters of higher hole mobility, narrower band gap and broader absorption region.
摘要翻译：提供光伏聚合物材料，其制备方法和用途。所述光伏聚合物材料具有下式（I）。光伏聚合物材料具有噻吩 - 亚苯基噻吩（TPT）衍生物作为基本结构单元，通过引入D1和D2结构来改性TPT，光伏聚合物材料具有较高的空穴迁移率，较窄的带间隙和更广泛的吸收区域。

9. 发明授权

US08802812B2 Photovoltaic polymer material, preparation method and use thereof 有权
标题翻译：光伏聚合物材料，其制备方法和用途
公开(公告)号：US08802812B2
公开(公告)日：2014-08-12
申请号：US13992166
申请日：2010-12-30
申请人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Lusheng Liang
发明人： Mingjie Zhou , Ping Wang , Zhenhua Zhang , Lusheng Liang
IPC分类号： C08G75/00 , H01L51/00 , C08G61/12 , H01L31/0256 , H01L51/42
CPC分类号： H01L31/0256 , C08G61/123 , C08G61/126 , C08G2261/3241 , C08G2261/3243 , C08G2261/3246 , C08G2261/344 , C08G2261/91 , H01L51/0036 , H01L51/0043 , H01L51/4253 , Y02E10/549 , Y02P70/521
摘要： A photovoltaic polymer material, preparation method and use thereof are provided. Said photovoltaic polymer material has the following formula (I). The photovoltaic polymer material has the thiophene-phenylene-thiophene (TPT) derivative as the basic structure unit, and by the introduction of D1 and D2 structures to modify the TPT, and the photovoltaic polymer material has the characters of higher hole mobility, narrower band gap and broader absorption region.
摘要翻译：提供光伏聚合物材料，其制备方法和用途。所述光伏聚合物材料具有下式（I）。光伏聚合物材料具有噻吩 - 亚苯基噻吩（TPT）衍生物作为基本结构单元，通过引入D1和D2结构来改性TPT，光伏聚合物材料具有较高的空穴迁移率，较窄的带间隙和更广泛的吸收区域。

10. 发明申请

US20140142310A1 ORGANIC ELECTROLUMINESCENT COMPOUND CONTAINING IRIDIUM, PREPARATION METHOD THEREOF AND ORGANIC ELECTROLUMINESCENT DEVICE 有权
标题翻译：含有IRI的有机电致发光体化合物，其制备方法及有机电致发光器件
公开(公告)号：US20140142310A1
公开(公告)日：2014-05-22
申请号：US14130183
申请日：2011-06-30
申请人： Mingjie Zhou , Ping Wang , Juanjuan Zhang , Zhenhua Zhang
发明人： Mingjie Zhou , Ping Wang , Juanjuan Zhang , Zhenhua Zhang
IPC分类号： H01L51/00
CPC分类号： H04W72/04 , C07F15/0033 , H04W16/10
摘要： An organic electroluminescent compound containing Iridium, preparation method thereof and an organic electroluminescent device are disclosed. The compound is represented by the structure (2), wherein, R is C1˜C4 alkyl. The structure of the compound contains bipyridine ligand, also carries alkoxy group and fluorine atom, which improves its carrier injection and transfer ability, and increases its internal quantum efficiency and electroluminescent efficiency. Furthermore, the compound uses strong field ligand 2-pyridine carboxylic acid as assistant ligand, which causes an effective blue shift of its emission spectrum and increases light-emitting efficiency of blue light phosphorescence greatly.
摘要翻译：公开了含有铱的有机电致发光化合物及其制备方法和有机电致发光器件。化合物由结构（2）表示，其中R是C 1 -C 4烷基。该化合物的结构含有联吡啶配位体，也带有烷氧基和氟原子，提高其载流子注入和转移能力，提高其内部量子效率和电致发光效率。此外，该化合物使用强场配体2-吡啶羧酸作为辅助配体，导致其发射光谱的有效蓝移，并大大提高蓝光磷光的发光效率。

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