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1. 发明授权

US08979951B2 Additives for improving the cold properties of fuel oils 有权
标题翻译：用于改善燃油的冷特性的添加剂
公开(公告)号：US08979951B2
公开(公告)日：2015-03-17
申请号：US11879409
申请日：2007-07-17
申请人： Bettina Siggelkow , Werner Reimann , Matthias Krull , Markus Kupetz
发明人： Bettina Siggelkow , Werner Reimann , Matthias Krull , Markus Kupetz
IPC分类号： C10L1/196 , C10M145/10 , C10L1/14 , C10L1/197 , C10L10/14 , C10L1/195 , C10L1/198 , C10L1/224
CPC分类号： C10L1/143 , C10L1/195 , C10L1/1973 , C10L1/1981 , C10L1/1985 , C10L1/224 , C10L10/14
摘要： The invention provides terpolymers of ethylene, at least one ethylenically unsaturated ester and propene, which a) contain from 12.0 to 16.0 mol % of structural units derived from at least one ethylenically unsaturated ester, b) contain from 1.0 to 4.0 methyl groups derived from propene per 100 aliphatic carbon atoms, and c) have fewer than 6.5 methyl groups stemming from chain ends per 100 CH2 groups. and also their use as cold additives for middle distillates.
摘要翻译：本发明提供了乙烯，至少一种烯属不饱和酯和丙烯的三元共聚物，其中a）含有12.0至16.0mol％的衍生自至少一种烯属不饱和酯的结构单元，b）含有1.0-4.0个来自丙烯的甲基每100个脂族碳原子，和c）由每100个CH2基团的链端衍生的少于6.5个甲基。以及它们作为中间馏分的冷添加剂的用途。

2. 发明授权

US06281292B1 Mixtures of copolymers having an improved lubricating action 失效
标题翻译：具有改善的润滑作用的共聚物的混合物
公开(公告)号：US06281292B1
公开(公告)日：2001-08-28
申请号：US09320230
申请日：1999-05-26
申请人： Matthias Krull , Werner Reimann , Markus Kupetz
发明人： Matthias Krull , Werner Reimann , Markus Kupetz
IPC分类号： C08L3306
CPC分类号： C10L10/08 , C08L23/08 , C08L2203/40 , C08L2205/02 , C10L1/195 , C10L1/1955 , C10L1/1963 , C10L1/1973 , C08L2666/04
摘要： The invention relates to mixtures comprising A) from 10 to 90% by weight of at least one copolymer comprising structural units derived from ethylene and structural units derived from olefinically unsaturated, hydroxyl-containing compounds, and B) from 90 to 10% by weight of at least one copolymer comprising structural units derived from ethylene and structural units derived from vinyl esters, olefinically unsaturated ethers and/or acrylates.
摘要翻译：本发明涉及包含A）10至90重量％的至少一种共聚物，其包含衍生自乙烯的结构单元和衍生自烯属不饱和的含羟基化合物的结构单元，和B）至少90至10重量％一种共聚物，其包含衍生自乙烯的结构单元和衍生自乙烯基酯，烯属不饱和醚和/或丙烯酸酯的结构单元。

3. 发明授权

US06846338B2 Fuel oils based on middle distillates and copolymers of ethylene and unsaturated carboxylic esters 失效
标题翻译：基于中间馏分的燃料油和乙烯和不饱和羧酸酯的共聚物
公开(公告)号：US06846338B2
公开(公告)日：2005-01-25
申请号：US09788261
申请日：2001-02-19
申请人： Matthias Krull , Werner Reimann , Markus Kupetz , Waltraud Nagel , Raimund Wildfang
发明人： Matthias Krull , Werner Reimann , Markus Kupetz , Waltraud Nagel , Raimund Wildfang
IPC分类号： C10L1/195 , C10L1/196 , C10L1/197 , C10L1/236 , C10L1/18
CPC分类号： C10L1/1955 , C10L1/1963 , C10L1/1973 , C10L1/2364
摘要： A fuel oil comprising: A) a mineral oil having a cloud point of less than −8° C., a boiling range (90-20%) of less than 120° C. and a difference between CFPP and PP of less than 10° C., and B) one or more copolymers, wherein the copolymers comprise: a) bivalent structural unit (B1), wherein (B1) is a bivalent structural unit of formula (1) —CH2—CH2— (1) and b) one or more bivalent structural units (B2), wherein (B2) is either a bivalent structural unit of formula (2) —CH2—CR1R2— (2) in which R1 is hydrogen or methyl, R2 is COOR3, OR3 or OCOR3, and R3 is an alkyl radical having at least 4 and at most 30 carbon atoms, or (B2) is a bivalent structural unit of formula (2a) in which R3 is an alkyl radical having at least 4 and at most 30 carbon atoms.
摘要翻译：一种燃油，包括：A）浊点小于-8℃的矿物油，小于120℃的沸程（90-20％）和CFPP与PP之间的差异小于10 其中所述共聚物包括：a）二价结构单元（B1），其中（B1）是式（1）的二价结构单元，和b）一个或多个二价结构单元（B2）其中（B2）是式（2）的二价结构单元，其中R 1是氢或甲基，R 2是COOR 3，OR 3或OCOR 3，R 3是是具有至少4个且至多30个碳原子的烷基，或（B2）是式（2a）的二价结构单元，其中R 3是具有至少4个且至多30个碳原子的烷基。

4. 发明授权

US08968428B2 Additives for improving the cold properties of fuel oils 有权
标题翻译：用于改善燃油的冷特性的添加剂
公开(公告)号：US08968428B2
公开(公告)日：2015-03-03
申请号：US11879431
申请日：2007-07-17
申请人： Bettina Siggelkow , Werner Reimann , Matthias Krull , Ulrike Neuhaus , Markus Kupetz , Andre Graf
发明人： Bettina Siggelkow , Werner Reimann , Matthias Krull , Ulrike Neuhaus , Markus Kupetz , Andre Graf
IPC分类号： C10L1/196 , C10M145/10 , C10L1/14 , C10L10/14 , C10L1/16 , C10L1/197 , C10L1/198 , C10L1/224 , C10L1/236
CPC分类号： C10L1/146 , C10L1/1641 , C10L1/165 , C10L1/1658 , C10L1/1966 , C10L1/1973 , C10L1/1981 , C10L1/1985 , C10L1/224 , C10L1/2364 , C10L10/14
摘要： The invention provides additive mixtures comprising A) at least one terpolymer of ethylene, propene and at least one ethylenically unsaturated ester, which i) contains from 6.0 to 12.0 mol % of structural units derived from at least one ethylenically unsaturated ester having a C1- to C3-alkyl radical, ii) contains from 0.5 to 4.0 methyl groups derived from propene per 100 aliphatic carbon atoms, iii) has fewer than 8.0 methyl groups stemming from chain ends per 100 CH2 groups, and B) from 0.5 to 20 parts by weight, based on A), of at least one further component which is effective as a cold additive for mineral oils and is selected from B1) copolymers of ethylene and ethylenically unsaturated compounds whose content of ethylenically unsaturated compounds is at least 2 mol % higher than the content of ethylenically unsaturated esters in the terpolymer defined under A), B2) comb polymers, and B3) mixtures of B1) and B2), and also their use as a cold additive for middle distillates.
摘要翻译：本发明提供添加剂混合物，其包括A）至少一种乙烯，丙烯和至少一种烯键式不饱和酯的三元共聚物，其i）含有6.0至12.0mol％的至少一种烯属不饱和酯的结构单元，其具有C1-至 C3-烷基，ii）含有每100个脂族碳原子衍生自丙烯的0.5至4.0个甲基，iii）由每100个CH 2基团的链端衍生的少于8.0个甲基，和B）0.5至20重量份基于A）的至少一种作为矿物油的冷添加剂有效的其它组分，并且选自B1）乙烯和烯属不饱和化合物的共聚物，其烯键式不饱和化合物的含量比所述烯属不饱和化合物的含量高至少2摩尔％在A），B2）梳状聚合物和B3）B1）和B2的混合物中定义的三元共聚物中的烯键式不饱和酯的含量，以及它们作为中间馏分的冷添加剂的用途。

5. 发明申请

US20080016753A1 Additives for improving the cold properties of fuel oils 有权
标题翻译：用于改善燃油的冷特性的添加剂
公开(公告)号：US20080016753A1
公开(公告)日：2008-01-24
申请号：US11879409
申请日：2007-07-17
申请人： Bettina Siggelkow , Werner Reimann , Matthias Krull , Markus Kupetz
发明人： Bettina Siggelkow , Werner Reimann , Matthias Krull , Markus Kupetz
IPC分类号： C10L1/195 , C08F220/10 , C08L33/02
CPC分类号： C10L1/143 , C10L1/195 , C10L1/1973 , C10L1/1981 , C10L1/1985 , C10L1/224 , C10L10/14
摘要： The invention provides terpolymers of ethylene, at least one ethylenically unsaturated ester and propene, which a) contain from 12.0 to 16.0 mol % of structural units derived from at least one ethylenically unsaturated ester, b) contain from 1.0 to 4.0 methyl groups derived from propene per 100 aliphatic carbon atoms, and c) have fewer than 6.5 methyl groups stemming from chain ends per 100 CH2 groups. and also their use as cold additives for middle distillates.
摘要翻译：本发明提供了乙烯，至少一种烯属不饱和酯和丙烯的三元共聚物，其中a）含有12.0至16.0mol％的衍生自至少一种烯属不饱和酯的结构单元，b）含有1.0-4.0个来自丙烯的甲基每100个脂族碳原子，和c）由每100个CH 2个基团的链端衍生的少于6.5个甲基。以及它们作为中间馏分的冷添加剂的用途。

6. 发明申请

US20080016754A1 Additives for improving the cold properties of fuel oils 有权
标题翻译：用于改善燃油的冷特性的添加剂
公开(公告)号：US20080016754A1
公开(公告)日：2008-01-24
申请号：US11879431
申请日：2007-07-17
申请人： Bettina Siggelkow , Werner Reimann , Matthias Krull , Ulrike Neuhaus , Markus Kupetz , Andre Graf
发明人： Bettina Siggelkow , Werner Reimann , Matthias Krull , Ulrike Neuhaus , Markus Kupetz , Andre Graf
IPC分类号： C10L1/195 , C08F220/10 , C08L33/02
CPC分类号： C10L1/146 , C10L1/1641 , C10L1/165 , C10L1/1658 , C10L1/1966 , C10L1/1973 , C10L1/1981 , C10L1/1985 , C10L1/224 , C10L1/2364 , C10L10/14
摘要： The invention provides additive mixtures comprising A) at least one terpolymer of ethylene, propene and at least one ethylenically unsaturated ester, which i) contains from 6.0 to 12.0 mol % of structural units derived from at least one ethylenically unsaturated ester having a C1- to C3-alkyl radical, ii) contains from 0.5 to 4.0 methyl groups derived from propene per 100 aliphatic carbon atoms, iii) has fewer than 8.0 methyl groups stemming from chain ends per 100 CH2 groups, and B) from 0.5 to 20 parts by weight, based on A), of at least one further component which is effective as a cold additive for mineral oils and is selected from B1) copolymers of ethylene and ethylenically unsaturated compounds whose content of ethylenically unsaturated compounds is at least 2 mol % higher than the content of ethylenically unsaturated esters in the terpolymer defined under A), B2) comb polymers, and B3) mixtures of B1) and B2), and also their use as a cold additive for middle distillates.
摘要翻译：本发明提供添加剂混合物，其包含A）至少一种乙烯，丙烯和至少一种烯键式不饱和酯的三元共聚物，i）含有6.0-12.0mol％的至少一种具有C 1〜C 3 - 烷基，ii）含有每100个脂肪族碳原子衍生自丙烯的0.5〜4.0个甲基，iii）由链中衍生的少于8.0个甲基至少一种作为矿物油的冷添加剂有效的至少一种另外的组分，并且B）基于A）的0.5至20重量份，并且选自： B1）乙烯和烯键式不饱和化合物的共聚物，其烯键式不饱和化合物的含量比A），B2）梳状聚合物中定义的三元共聚物中烯属不饱和酯的含量高至少2摩尔％，和B3）B1）和 B2），以及它们作为冷添加剂的用途对于中间馏分。

7. 发明申请

US20080178522A1 Pour point improvers for vegetable or animal fuel oils 审中-公开
公开(公告)号：US20080178522A1
公开(公告)日：2008-07-31
申请号：US11980292
申请日：2007-10-30
申请人： Bettina Siggelkow , Werner Reimann , Ulrike Neuhaus , Markus Kupetz
发明人： Bettina Siggelkow , Werner Reimann , Ulrike Neuhaus , Markus Kupetz
IPC分类号： C10L1/00 , G01N1/00
CPC分类号： C10L10/14 , C10L1/146 , C10L1/1955 , C10L1/1963 , C10L1/1966 , C10L1/1973 , C10L1/1985 , C10L1/2675 , C10L10/16
摘要： The invention provides a fuel oil composition comprising a fuel oil of animal or vegetable origin, in which a total of more than 6% by weight of palmitic acid methyl ester and stearic acid methyl ester are present, and, as an additive, A) at least one copolymer which contains 10-20 mol % of structural units of at least one vinyl ester and 80-90 mol % of structural units of ethylene, and B) at least one comb polymer containing structural units formed from B1) at least one olefin as monomer 1, which bears at least one C8-C18-alkyl radical on the olefinic double bond, and B2) at least one ethylenically unsaturated dicarboxylic acid as monomer 2, which bears at least one C8-C16-alkyl radical bonded via an amide and/or imide group, in which the parameter Q Q = ∑ i   w 1  i · n 1  i + ∑ j   w 2  j · n 2  j in which w1 is the molar proportion of the individual chain lengths n1 in the alkyl radicals of monomer 1, w2 is the molar proportion of the individual chain lengths n2 in the alkyl radicals of the amide and/or imide groups of monomer 2, n1 are the individual chain lengths in the alkyl radicals of monomer 1, n2 are the individual chain lengths in the alkyl radicals of the amide and/or imide groups of monomer 2, i is the serial variable for the chain lengths in the alkyl radicals of monomer 1, and j is the serial variable for the chain lengths in the alkyl radicals of the amide and/or imide groups of monomer 2, assumes values of from 23 to 27.

8. 发明授权

US06596037B2 Fatty acid mixtures of improved low-temperature stability which comprise comb polymers, and their use in fuel oils 有权
标题翻译：包含梳状聚合物的改进的低温稳定性的脂肪酸混合物及其在燃料油中的应用
公开(公告)号：US06596037B2
公开(公告)日：2003-07-22
申请号：US09993847
申请日：2001-11-16
申请人： Matthias Krull , Werner Reimann
发明人： Matthias Krull , Werner Reimann
IPC分类号： C10L118
CPC分类号： C10L10/08 , C10L1/143
摘要： The invention relates to low-temperature-stabilized fatty acid mixtures comprising A) from 10 to 99.99% by weight of fatty acid mixtures comprising: A1) from 1 to 99% by weight of at least one saturated mono- or dicarboxylic acid having 6 to 50 carbon atoms, A2) from 1 to 99% by weight of at least one unsaturated mono- or dicarboxylic acid having 6 to 50 carbon atoms, and B) from 0.01 to 90% by weight of copolymers comprising: B1) from 40 to 60 mol % of bivalent structural units of the formula where X═O or N—R1, in which a and b=0 or 1 and a+b=1, and B2) from 60 to 40 mol % of bivalent structural units of the formula —H2C—CR2R3— B2 and, if desired, B3) from 0 to 20 mol % of bivalent structural units derived from polyolefins, where the polyolefins can be derived from monoolefins having 3 to 5 carbon atoms, and in which a) R1 is an alkyl or alkenyl radical having from 10 to 40 carbon atoms or an alkoxyalkyl radical having from 1 to 100 alkoxy units and from 1 to 30 carbon atoms in the alkyl radical, and b) R3 is a radical of the formula OCOR4 or COOR4, in which R4 is C1-C24-alkyl, and c) the number of carbon atoms in the polyolefin molecules on which the structural units B3) are based is from 35 to 350, and d) R2 is hydrogen or methyl, and to the use of these mixtures for improving the lubrication properties of low-sulfur middle distillates.
摘要翻译：本发明涉及低温稳定的脂肪酸混合物，其包含A）10至99.99重量％的脂肪酸混合物，其包含：A1）1至99重量％的至少一种具有6至50个的饱和单羧酸或二羧酸碳原子，A2）1至99重量％的至少一种具有6至50个碳原子的不饱和单羧酸或二羧酸，和B）0.01至90重量％的共聚物，其包含：B1）40至60摩尔％其中X = O或N-R1的二价结构单元，其中a和b = 0或1和a + b = 1，B2）为60至40摩尔％的二价结构单元，如果所需的B3）0至20摩尔％的衍生自聚烯烃的二价结构单元，其中聚烯烃可以衍生自具有3至5个碳原子的单烯烃，并且其中a）R 1是具有10至40个的烷基或烯基碳原子或烷基中具有1至100个烷氧基单元和1至30个碳原子的烷氧基烷基，b ）R3是式OCOR4或COOR4的基团，其中R4是C1-C24-烷基，c）结构单元B3）所基于的聚烯烃分子中的碳原子数为35〜350，以及 d）R2是氢或甲基，以及使用这些混合物来改善低硫中间馏分的润滑性能。

9. 发明授权

US06592638B2 Mixtures of carboxylic acids, their derivatives and hydroxyl-containing polymers and their use for improving the lubricating effect of oils 失效
标题翻译：羧酸，其衍生物和含羟基聚合物的混合物及其用于改善油的润滑效果的用途
公开(公告)号：US06592638B2
公开(公告)日：2003-07-15
申请号：US09811307
申请日：2001-03-16
申请人： Matthias Krull , Werner Reimann
发明人： Matthias Krull , Werner Reimann
IPC分类号： C10L118
CPC分类号： C10L10/08 , C10L1/143 , C10L1/18
摘要： The invention relates to additives for improving lubricating properties of fuel oils, comprising A) 10-95% by weight of at least one oil-soluble amphiphile which comprises nitrogen- or oxygen-containing groups substituted by alkyl, alkenyl, hydroxyalkyl or aromatic radicals, and B) 5-90% by weight of at least one copolymer which contains B1) from 0.5 to 15 mol % of structural units which are derived from olefinically unsaturated compounds which have at least one free hydroxyl group, and B2) from 85 to 99.5 mol % of structural units which are derived from ethylene, and, if required, B3) from 0 to 20 mol % of further structural units selected from the group consisting of (meth)acrylic acid, (meth)acrylates, vinyl esters, vinyl ethers and alkenes, and the copolymer has an average molar mass Mw of from 500 to 100,000 g/mol and an OH number of from 5 to 500 mg KOH/g.
摘要翻译：本发明涉及用于改善燃料油的润滑性能的添加剂，其包括：A）10-95重量％的至少一种油溶性两亲物，其包含被烷基，链烯基，羟烷基或芳族基团取代的含氮或含氧基团，和B ）5-90重量％的至少一种共聚物，其含有B 1）0.5至15摩尔％的衍生自具有至少一个游离羟基的烯属不饱和化合物的结构单元，和B 2）85-99.5摩尔％的结构衍生自乙烯的单元，如果需要，B3）0至20摩尔％的选自（甲基）丙烯酸，（甲基）丙烯酸酯，乙烯基酯，乙烯基醚和烯烃的其它结构单元，以及共聚物的平均摩尔质量Mw为500〜100,000g / mol，OH值为5〜500mgKOH / g。

10. 发明授权

US6110238A Process for improving the cold-flow properties of fuel oils 有权
标题翻译：改进燃油的冷流特性的方法
公开(公告)号：US6110238A
公开(公告)日：2000-08-29
申请号：US235723
申请日：1999-01-22
申请人： Matthias Krull , Werner Reimann
发明人： Matthias Krull , Werner Reimann
IPC分类号： C10L1/192 , C10L1/14 , C10L1/195 , C10L1/196 , C10L1/197 , C10L10/18 , C10L1/18
CPC分类号： C10L1/195 , C10L1/143 , C10L1/1973
摘要： A process for improving the cold flow properties of fuel oils comprising the addition to fuel oil of an additive comprising copolymers of lower olefins and vinyl esters and a terpolymer of 4-methylpentene-1 and an additive composition comprising copolymers of lower olefins and vinyl esters and a terpolymer of 4-methylpentene-1.
摘要翻译：一种用于改进燃料油的冷流动性能的方法，其包括添加到包含低级烯烃和乙烯基酯的共聚物的添加剂的燃料油和4-甲基戊烯-1的三元共聚物和包含低级烯烃和乙烯基酯的共聚物的添加剂组合物的方法，以及 4-甲基戊烯-1的三元共聚物。

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