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1. 发明授权

US4403081A Method for producing .alpha.-olefin polymers 失效
标题翻译： α-烯烃聚合物的制备方法
公开(公告)号：US4403081A
公开(公告)日：1983-09-06
申请号：US13522
申请日：1979-02-21
申请人： Masato Harada , Akihiro Sato , Sadahiko Yamada , Kazutsune Kikuta , Atsushi Suzuki , Hiroshi Shimizu , Jun Masuda , Tadamitsu Hamasaki , Atsuyuki Kachi
发明人： Masato Harada , Akihiro Sato , Sadahiko Yamada , Kazutsune Kikuta , Atsushi Suzuki , Hiroshi Shimizu , Jun Masuda , Tadamitsu Hamasaki , Atsuyuki Kachi
IPC分类号： C08F4/62 , C08F4/64 , C08F10/00 , C08F4/02
CPC分类号： C08F10/00
摘要： A method for producing .alpha.-olefin polymers is provided. This method provides products having superior properties such as higher bulk density and uniform particle form which is close to sphere, with such an extremely higher catalyst efficiency that ash-removal step can be omitted without fear of coloring. The characteristic point of this method is in the improvement of conventional catalyst obtained by reacting a trivalent metal halide with a divalent metal hydroxide, oxide or carbonate or a double salt containing foregoing compounds or a hydrate of a compound containing a divalent metal to form a solid product (I), reacting an electron donor with said product (I), reacting the resulting product with a compound of transition metal of the 4th a or the 5th a group to form a final solid product and combining an organoaluminum compound with said final product,the improvement consisting in that said final product is obtained by reacting said solid product (I), said electron donor and said compound of transition metal, in the coexistence of said electron donor and said compound of transition metal.
摘要翻译：提供了一种生产α-烯烃聚合物的方法。该方法提供具有较高体积密度和接近球体的均匀颗粒形式的优异性能的产品，具有非常高的催化剂效率，可以省略除灰步骤而不用担心着色。该方法的特征在于改进通过使三价金属卤化物与二价金属氢氧化物，氧化物或碳酸盐或含有前述化合物的复盐或含有二价金属的化合物的水合物反应形成固体而获得的常规催化剂产物（I），使电子给体与所述产物（I）反应，使所得产物与第4或第5族的过渡金属的化合物反应以形成最终固体产物，并将有机铝化合物与所述最终产物所述最终产物的改进是通过所述固体产物（I），所述电子给体和所述过渡金属化合物在所述电子给体和所述过渡金属化合物的共存下反应而获得的。

2. 发明授权

US4103078A Method for producing polymers of alpha-olefin 失效
标题翻译： α-烯烃聚合物的制备方法
公开(公告)号：US4103078A
公开(公告)日：1978-07-25
申请号：US340854
申请日：1973-03-13
申请人： Akihiro Sato , Shiro Konotsune , Atsuyuki Kachi , Hiroshi Shimizu
发明人： Akihiro Sato , Shiro Konotsune , Atsuyuki Kachi , Hiroshi Shimizu
IPC分类号： C08F4/02 , C08F10/00
CPC分类号： C08F10/00 , C08F4/025 , C08F2410/04
摘要： Polymers of .alpha.-olefin such as polyethylene, polypropylene, copolymers of ethylene with propylene, butene-1 or styrene, are produced by the (co-) polymerization using a catalyst obtained by mill-mixing an oxide of a metal belonging to I, II, III, VII or VIII Group of the Periodic Table of Elements such as MgO or SiO.sub.2 or B.sub.2 O.sub.3, with a trivalent metal halide such as AlCl.sub.3, then reacting the resultant mixture with a transition metal compound such as TiCl.sub.4 in the presence of an aromatic compound such as xylene, and activating the resultant solid reaction product with an organoaluminum compound such as triethyl aluminum.In the preparation of the present catalyst, no dehydrochlorination occurs. The present catalyst has an excellent utilization efficiency of transition metal compound in the polymerization. Further, no polymer film forms on the wall surface of the polymerization vessel.
摘要翻译：通过（共）聚合，使用通过将属于I，II的金属的氧化物混合而获得的催化剂制备α-烯烃如聚乙烯，聚丙烯，乙烯与丙烯的共聚物，丁烯-1或苯乙烯的聚合物，III，VII或VIII族元素如MgO或SiO 2或B 2 O 3与三价金属卤化物如AlCl 3组合，然后使所得混合物与诸如TiCl 4的过渡金属化合物在芳族化合物的存在下反应例如二甲苯，并用有机铝化合物如三乙基铝活化所得的固体反应产物。

3. 发明授权

US3987233A Method for producing ethylene polymers 失效
标题翻译：生产乙烯聚合物的方法
公开(公告)号：US3987233A
公开(公告)日：1976-10-19
申请号：US572818
申请日：1975-04-29
申请人： Akihiro Sato , Hiroshi Shimizu , Atsuyuki Kachi
发明人： Akihiro Sato , Hiroshi Shimizu , Atsuyuki Kachi
IPC分类号： C08F4/00 , C08F4/60 , C08F10/00 , C08F10/02 , C08F4/02
CPC分类号： C08F10/00 , C08F10/02 , C08F110/02 , C08F210/16 , C08F2410/04 , Y10S526/906
摘要： In a method for producing a polymer or a copolymer of ethylene carried out in the presence of a catalyst obtained by a combination of a solid product containing a transition metal of the fourth a or fifth a group and an organoaluminum compound, an improvement has been made to provide a catalyst having such an efficiency as being capable of omitting ash-removal step and providing a high production yield of polymer per unit volume of polymerization vessel per hour and a polymer having a high B.D. Said catalyst can be obtained by (1) reacting a halide of trivalent metal (A) with a divalent metal compound or its derivative (B) such as hydroxide, oxide or carbonate thereof, or hydrate of these, to produce a solid product (I); (2) reacting said solid product (I) with a chain or cyclic polysiloxane having a general formula of ##EQU1## WHEREIN R.sub.1 and R.sub.2 are same or different kinds, and each mean hydrogen atom, alkyl, aryl, halogen atom, alkoxy, aryloxy radical or a residual radical of an aliphatic carboxylic acid and n is a number in the range of 3-10,000 to produce a solid product (II), and (3) further reacting said solid product (II) with a liquid transition metal compound (D) to produce a solid product (III).

4. 发明授权

US4027087A Method for producing ethylene polymers 失效
标题翻译：生产乙烯聚合物的方法
公开(公告)号：US4027087A
公开(公告)日：1977-05-31
申请号：US301908
申请日：1972-10-30
申请人： Akihiro Satoh , Shiro Konotsune , Atsuyuki Kachi , Hiroshi Shimizu
发明人： Akihiro Satoh , Shiro Konotsune , Atsuyuki Kachi , Hiroshi Shimizu
IPC分类号： C08F10/00 , C08F4/02 , C08F10/02
CPC分类号： C08F10/00 , C08F2410/04 , Y10S526/903
摘要： Ethylene can be polymerized or copolymerized by the use of a catalyst prepared by mixing a trivalent metal halide with a metal carbonate or/and a metal hydrogen carbonate, reacting the resulting mixture with a transition metal compound in the presence of an aromatic compound, and activating the resulting solid product with an organoaluminum compound.By substituting said metal carbonate or/and metal hydrogen carbonate for metal salt hydrates, sulfide hydrates, hydroxides or hydroxide hydrates, or metal oxides in our prior art, drawbacks such as dehydrochlorination in the preparation of catalyst or difficulty in removal of catalyst residue from polymer can be overcome while various advantages in our prior art are still maintained.
摘要翻译：乙烯可以通过使用通过将三价金属卤化物与金属碳酸盐或/和金属碳酸氢盐混合制备的催化剂进行聚合或共聚，使所得混合物与过渡金属化合物在芳族化合物的存在下反应，并使活化得到的固体产物与有机铝化合物。

5. 发明授权

US4591577A Solid catalyst component for alpha-olefin polymerization and process for producing same 失效
标题翻译：用于α-烯烃聚合的固体催化剂组分及其制备方法
公开(公告)号：US4591577A
公开(公告)日：1986-05-27
申请号：US740999
申请日：1985-06-04
申请人： Akihiro Sato , Masami Tachibana , Hiroshi Shimizu , Toshihiro Uwai
发明人： Akihiro Sato , Masami Tachibana , Hiroshi Shimizu , Toshihiro Uwai
IPC分类号： C08F4/00 , C08F4/60 , C08F4/64 , C08F4/642 , C08F10/00
CPC分类号： C08F10/00 , Y10S526/908 , Y10S526/909
摘要： A solid catalyst component for .alpha.-olefin polymerization which, when produced, causes any troubles due to its small particle size and when used, yields a spherical polymer of a suitably less particle size and a high bulk density with a slightest quantity of atactic polymer and affording a very good dispersibility of powdery additives therein in spite of its narrow particle size distribution, and a process for producing the same, are provided, which solid catalyst component comprises Ti and Cl as active ingredients, having an average particle diameter of 2 to 10.mu., a specific surface area of 100 m.sup.2 /g or more and a diffraction line corresponding to a distance between lattices of 4.80 to 5.10 .ANG. by way of X-ray diffraction; and which process is characterized in that when TiCl.sub.4 is reduced with a reducing agent comprising an organoaluminum compound to produce a solid intermediate, there is employed an agitation intensity defined by definite values of agitation power and baffle ratio.
摘要翻译：一种用于α-烯烃聚合的固体催化剂组分，其在制备时由于其小粒径而引起任何故障，并且当使用时，产生具有适度较小粒径和高堆积密度的球形聚合物，其中最少量的无规立构聚合物和提供粉末状添加剂的分散性非常好，尽管其粒度分布窄，并且提供了其制备方法，该固体催化剂组分包含Ti和Cl作为活性成分，其平均粒径为2至10 mu，比表面积为100m 2 / g以上，通过X射线衍射对应于晶格之间的间距4.80〜5.10的衍射线; 并且该方法的特征在于，当用包含有机铝化合物的还原剂还原TiCl 4以产生固体中间体时，使用通过搅拌功率和挡板比的确定值定义的搅拌强度。

6. 发明授权

US4535069A Catalyst component for .alpha.-olefin polymerization 失效
标题翻译：用于α-烯烃聚合的催化剂组分
公开(公告)号：US4535069A
公开(公告)日：1985-08-13
申请号：US466971
申请日：1983-02-16
申请人： Hiroshi Shimizu , Masaki Abe , Akihiro Sato
发明人： Hiroshi Shimizu , Masaki Abe , Akihiro Sato
IPC分类号： C08F4/00 , C08F4/60 , C08F4/64 , C08F4/658 , C08F10/00
CPC分类号： C08F10/00
摘要： A supported type catalyst component for .alpha.-olefin polymerization, having a higher activity and capable of affording a highly stereoregular polymer is provided, which component comprises a solid product (II) obtained by reacting Mg compound(s) of formula MgR.sup.1 R.sup.2 (wherein R.sup.1 is alkyl, aryl, alkoxy or aryloxy and R.sup.2, alkyl, aryl, alkoxy, aryloxy or halogen), with a complex of compound(s) selected from Al halides and Al compounds of formula AlR.sub.n.sup.3 X.sub.3-n (wherein R.sub.3 is alkyl, aryl, alkoxy or aryloxy; X, halogen; 0.ltoreq.n
摘要翻译：提供了具有较高活性并且能够提供高度立构规整性聚合物的用于α-烯烃聚合的负载型催化剂组分，该组分包括通过使MgCl 2（其中R 1为与选自Al卤化物和式AlRn3X3-n（其中R3是烷基，芳基，烷氧基）的Al化合物的化合物的络合物与R 2，烷基，芳氧基，芳氧基，或芳氧基; X，卤素; 0 <= n <2）与有机酸酯反应; 并使得到的固体产物（I）（载体）与含液体含卤素的Ti化合物反应。固体产物（II）与有机铝化合物和α-烯烃的预活化提供了在储存稳定性和聚合重现性方面优异的催化剂组分。

7. 发明授权

US09822387B2 Microorganism having carbon dioxide fixation pathway introduced thereinto 有权
公开(公告)号：US09822387B2
公开(公告)日：2017-11-21
申请号：US14235756
申请日：2012-07-27
申请人： Ryota Fujii , Tomokazu Shirai , Tadashi Araki , Koh Amano , Yoshiko Matsumoto , Toshihiro Tateno , Nozomi Takebayashi , Takashi Morishige , Hitoshi Takahashi , Mitsufumi Wada , Hiroshi Shimizu , Chikara Furusawa , Takashi Hirasawa , Tomonori Hidesaki , Ayako Endo , Dominik Lukas Jürgen-Lohmann , Anjali Madhavan , Su Sun Chong
发明人： Ryota Fujii , Tomokazu Shirai , Tadashi Araki , Koh Amano , Yoshiko Matsumoto , Toshihiro Tateno , Nozomi Takebayashi , Takashi Morishige , Hitoshi Takahashi , Mitsufumi Wada , Hiroshi Shimizu , Chikara Furusawa , Takashi Hirasawa , Tomonori Hidesaki , Ayako Endo , Dominik Lukas Jürgen-Lohmann , Anjali Madhavan , Su Sun Chong
IPC分类号： C12N1/20 , C12N15/00 , C12N9/00 , C12N9/88 , C12N9/02 , C07H21/04 , C12P19/40 , C12P13/14 , C12N9/04 , C12P7/04 , C12P7/28 , C12P19/32
CPC分类号： C12P19/40 , C12N1/20 , C12N9/0006 , C12N9/88 , C12N9/93 , C12P7/04 , C12P7/28 , C12P13/14 , C12P19/32 , C12Y101/0106 , C12Y101/01081 , C12Y401/01047 , C12Y401/03024 , C12Y602/01009
摘要： An acetyl-CoA-producing microorganism, which is capable of efficiently synthesizing acetyl-CoA using carbon dioxide, and a substance production method using the same are provided. An acetyl-CoA-producing microorganism including an acetyl-CoA production cycle obtained by imparting at least one type of enzymatic activity selected from the group consisting of malate thiokinase, malyl-CoA lyase, glyoxylate carboligase, 2-hydroxy-3-oxopropionate reductase, and hydroxypyruvate reductase, to a microorganism.

8. 发明授权

US09640144B2 Projector, figure input/display apparatus, portable terminal, and program 有权
公开(公告)号：US09640144B2
公开(公告)日：2017-05-02
申请号：US14377245
申请日：2012-02-13
申请人： Hiroshi Shimizu , Kazuhiko Yoshizawa , Motoyuki Suzuki , Hideo Nishijima , Nobuo Masuoka
发明人： Hiroshi Shimizu , Kazuhiko Yoshizawa , Motoyuki Suzuki , Hideo Nishijima , Nobuo Masuoka
IPC分类号： G06F3/14 , G09G5/12 , G06F3/0488 , G06K9/22 , H04M3/56 , H04N9/31 , G06F3/041 , G06Q10/10 , H04N7/15
CPC分类号： G09G5/12 , G06F3/0416 , G06F3/04883 , G06F3/1423 , G06F3/1454 , G06K9/222 , G06Q10/101 , G09G2354/00 , G09G2360/04 , G09G2370/16 , H04M3/567 , H04N7/15 , H04N9/3179
摘要： Blocking a view of a whiteboard by a position of an attendee writing thereon is prevented, and writing records made by all attendees are stored to use the writing records including a course of the written records later. Each terminal of the attendees has a touch-panel-equipped terminal can divide any input line drawing on the terminal into line segment data, successively transmit the line segment data to the controller, and display line drawing information on the display of the touch-panel-equipped terminal. A liquid crystal projector having a controller that can be embedded therein or connected thereto is provided, the controller can sequentially record line drawing information transmitted from each touch-panel-equipped terminal in a data base, add the line drawing information to a video image memory of the whiteboard, and project the video image memory contents onto a wall surface while transmitting information of the data base to each touch-panel-equipped terminal.

9. 发明授权

US09548140B2 Nuclear reactor vessel support structure and construction method of nuclear reactor vessel support structure 有权
标题翻译：核反应堆船舶支撑结构和核反应堆船舶支撑结构施工方法
公开(公告)号：US09548140B2
公开(公告)日：2017-01-17
申请号：US13992999
申请日：2011-12-06
申请人： Hiroshi Shimizu , Ryo Fujimoto , Kentaro Mori , Hiromu Okamoto , Hisashi Sekimoto , Hiroyuki Iseki
发明人： Hiroshi Shimizu , Ryo Fujimoto , Kentaro Mori , Hiromu Okamoto , Hisashi Sekimoto , Hiroyuki Iseki
IPC分类号： G21C13/00 , G21C13/024 , F22B37/24 , E04B1/16
CPC分类号： G21C13/024 , E04B1/16 , F22B37/248 , Y02E30/40
摘要： A nuclear reactor vessel structure includes an inner peripheral tube-shaped steel plate, an outer peripheral tube-shaped steel plate, and an intermediate tube-shaped steel plate disposed between the inner and outer peripheral tube-shaped steel plates, and is configured to support a nuclear reactor vessel on the inner peripheral side of a tube-shaped structure with concrete placed between the steel plates. The nuclear reactor vessel structure includes a support having a tube-shaped plate disposed on the inner peripheral side of the intermediate tube-shaped steel plate, and an annular plate which protrudes to the inner peripheral side of the tube-shaped plate and to which a connection section is affixed. The support is affixed to the concrete, which is placed between the inner peripheral and the intermediate tube-shaped steel plates, by first bar members, and the support is also affixed to the inner peripheral tube-shaped steel plate by second bar members.
摘要翻译：核反应堆容器结构包括内周管状钢板，外周管状钢板和设置在内外管状钢板之间的中间管状钢板，构成为支承在管状结构的内周侧具有放置在钢板之间的混凝土的核反应堆容器。核反应堆容器结构包括具有设置在中间管状钢板的内周侧的管状板的支撑体和向管状板的内周侧突出的环状板，连接部分被贴上。支撑体通过第一杆构件固定在内周和中间管状钢板之间的混凝土上，并且支撑体也通过第二杆构件固定到内周管状钢板。

10. 发明授权

US09051333B2 6,7-dihydroimidazo [2,1-b] [1,3]oxazine bactericides 有权
标题翻译： 6,7-二氢咪唑并[2,1-b] [1,3]恶嗪类杀菌剂
公开(公告)号：US09051333B2
公开(公告)日：2015-06-09
申请号：US14111262
申请日：2012-04-13
申请人： Yoshikazu Kawano , Yoshikazu Haraguchi , Hirofumi Sasaki , Yukitaka Uematsu , Hidetsugu Tsubouchi , Hiromi Yata , Hiroshi Shimizu , Kazuho Kohashi , Motohiro Itotani , Kuninori Tai , Isao Takemura , Mikayo Hayashi , Hiroyuki Hashizume , Miki Matsuba , Izuru Nakamura , Xiuhao Chen , Makoto Matsumoto
发明人： Yoshikazu Kawano , Yoshikazu Haraguchi , Hirofumi Sasaki , Yukitaka Uematsu , Hidetsugu Tsubouchi , Hiromi Yata , Hiroshi Shimizu , Kazuho Kohashi , Motohiro Itotani , Kuninori Tai , Isao Takemura , Mikayo Hayashi , Hiroyuki Hashizume , Miki Matsuba , Izuru Nakamura , Xiuhao Chen , Makoto Matsumoto
IPC分类号： C07D498/04 , A61K31/5383
CPC分类号： C07D498/04
摘要： The present invention provides a novel 6,7-dihydroimidazo[2,1-b][1,3]oxazine compound that has excellent bactericidal action against tubercle bacilli, multidrug-resistant tubercle bacilli, and atypical acid-fast bacilli. Specifically, the present invention provides a compound represented by Formula (1): or a salt thereof, wherein R1 represents tetrahydroisoquinolyl, tetrahydroquinolyl, tetrahydrobenzoazepinyl, benzoxazolyl, benzothiazolyl, indolyl, isoindolinyl, naphthyl, quinolyl, phenyl, biphenylyl, or pyridyl, these groups being optionally substituted, the phenyl, biphenylyl, and pyridyl represented by R1 each being substituted directly or via a linker with at least one group selected from the group consisting of tetrahydropyridyl, diazepanyl, diazabicycloheptanyl, tetrahydrotriazolopyrazinyl, tetrahydroimidazopyrazinyl, azabicyclooctanyl, oxazolyl, piperazinyl, piperidyl, thiazolyl, and the like, each of these groups being optionally substituted; and R2 represents hydrogen or lower alkyl. The present invention further provides a pharmaceutical composition containing the above.
摘要翻译：本发明提供了对结核杆菌，多重耐药性结核杆菌和非典型抗酸杆菌具有优异的杀菌作用的新型6,7-二氢咪唑并[2,1-b] [1,3]恶嗪化合物。具体地说，本发明提供由式（1）表示的化合物或其盐，其中R1表示四氢异喹啉基，四氢喹啉基，四氢苯并氮杂基，苯并恶唑基，苯并噻唑基，吲哚基，异吲哚啉基，萘基，喹啉基，苯基，联苯基或吡啶基。任选被取代的苯基，联苯基和吡啶基，其各自被直接取代或经由具有至少一个选自四氢吡啶基，二氮杂环庚烷基，二氮杂双环庚烷基，四氢三唑并吡嗪基，四氢咪唑并吡嗪基，氮杂双环辛基，恶唑基，哌嗪基，哌啶基，噻唑基等，这些基团各自任选被取代; 并且R 2表示氢或低级烷基。本发明还提供含有上述物质的药物组合物。

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