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1. 发明授权

US06723794B2 Olefin thermoplastic elastomer composition comprising crystalline polyolefin resin and ethylene/&agr;-olefin/nonconjugated polyene copolymer rubber 有权
标题翻译：包含结晶聚烯烃树脂和乙烯/α-烯烃/非共轭多烯共聚物橡胶的烯烃热塑性弹性体组合物
公开(公告)号：US06723794B2
公开(公告)日：2004-04-20
申请号：US10066575
申请日：2002-02-06
申请人： Masaaki Kawasaki , Keiji Okada , Tetsuo Tojo , Kyoko Kobayashi , Yuichi Itoh , Akira Uchiyama , Toshiyuki Tsutsui , Toshihiro Sagane
发明人： Masaaki Kawasaki , Keiji Okada , Tetsuo Tojo , Kyoko Kobayashi , Yuichi Itoh , Akira Uchiyama , Toshiyuki Tsutsui , Toshihiro Sagane
IPC分类号： C08L2302
CPC分类号： C08L23/02 , A61J1/03 , B65D23/003 , B65D51/28 , C08K5/14 , C08L23/0815 , C08L23/10 , C08L23/142 , C08L23/16 , C08L23/22 , C08L91/00 , C08L2205/03 , C08L2207/04 , C08L2312/00 , C08L2666/04
摘要： An olefin thermoplastic elastomer composition comprises a crystalline polyolefin resin (A) and an ethylene/&agr;-olefin/nonconjugated polyene copolymer rubber (B), and optionally a softener (C) and/or an inorganic filler (D), in a specific ratio. The copolymer rubber (B) is prepared by the use of a metallocene catalyst and comprises ethylene, an &agr;-olefin of 3 to 20 carbon atoms and a nonconjugated polyene. This composition ca provide molded products of more excellent tensile strength, elongation at break, elastomeric properties (elongation set, permanent compression set, etc.), heat resistance and low-temperature properties than the conventional non-crosslinked olefin thermoplastic elastomers, even if the composition is in the non-crosslinked form. The composition in the partially or completely crosslinked form can provided molded products of more excellent low-temperature properties, tensile strength, elongation at break and elastomeric properties than the conventional vulcanized rubbers.
摘要翻译：烯烃热塑性弹性体组合物包含结晶聚烯烃树脂（A）和乙烯/α-烯烃/非共轭多烯共聚物橡胶（B）和任选的软化剂（C）和/或无机填料（D）。共聚物橡胶（B）通过使用茂金属催化剂制备，包括乙烯，3-20个碳原子的α-烯烃和非共轭多烯。该组合物提供比常规非交联烯烃热塑性弹性体更优异的拉伸强度，断裂伸长率，弹性体性能（伸长率设定，永久压缩变形等），耐热性和低温性能的成型产品，即使组合物为非交联形式。部分或完全交联形式的组合物可以提供比常规硫化橡胶更优异的低温性能，拉伸强度，断裂伸长率和弹性体性能的成型产品。

2. 发明授权

US06635705B2 Olefinic thermoplastic elastomer composition and method for producing the same 失效
标题翻译：烯烃类热塑性弹性体组合物及其制造方法
公开(公告)号：US06635705B2
公开(公告)日：2003-10-21
申请号：US09986477
申请日：2001-11-08
申请人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama , Masaaki Kawasaki
发明人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama , Masaaki Kawasaki
IPC分类号： C08L2316
CPC分类号： C08L23/02 , C08K5/01 , C08K5/02 , C08K5/14 , C08L23/0815 , C08L23/12 , C08L23/16 , C08L23/22 , C08L91/00 , C08L2205/02 , C08L2205/03 , C08L2207/04 , C08L2312/02 , C08L2314/06 , Y10S526/943 , C08L2666/04
摘要： The present invention relates to an olefinic thermoplastic elastomer composition which comprises a crystalline polyolefin resin (A), an ethylene-&agr;-olefin-non-conjugated polyene copolymer rubber (B) and at least on rubber (C) selected from polyisobutylene, butyl rubber and a propylene-ethylene copolymer rubber having a propylene content of 50 mol % or more or an ethylene-&agr;-olefin copolymer (D) having a density of 0.870 to 0.940 (g/cm3) and an ethylene content of 85 mol % or more, said ethylene-&agr;-olefin-non-conjugated polyene copolymer rubber (B) being crosslinked thermoplastic elastomer composition, being obtained by random copolymerization of ethylene, and &agr;-olefin having 3 to 20 carbon atoms and a non-conjugated polyene in the presence of a metallocene catalyst, (1) containing the unit (a) derived from the ethylene and the unit (b) derived from the &agr;-olefin in a molar ratio of 40/60 to 95/5 [(a)/(b)], (2) having an iodine value of 1 to 50 and (3) having an intrinsic viscosity [&eegr;] measured in decalin at 135° C. of 1.0 to 10 dl/g; and relates to a method for manufacturing the same.
摘要翻译：本发明涉及一种烯烃热塑性弹性体组合物，其包含结晶聚烯烃树脂（A），乙烯-α-烯烃 - 非共轭多烯共聚物橡胶（B）和至少在选自聚异丁烯，丁基橡胶丙烯含量为50摩尔％以上的丙烯 - 乙烯共聚物橡胶或密度为0.870〜0.940（g / cm 3），乙烯含量为85摩尔的乙烯-α-烯烃共聚物（D）％以上，所述乙烯-α-烯烃 - 非共轭多烯共聚物橡胶（B）为交联热塑性弹性体组合物，其通过乙烯的无规共聚和具有3-20个碳原子的α-烯烃和非共轭多烯在茂金属催化剂的存在下，（1）含有衍生自乙烯的单元（a）和衍生自α-烯烃的单元（b），摩尔比为40/60至95/5 [（a）/ （b）]，（2）碘值为1〜50，（3）具有内嵌在135℃萘烷中测得的粘度η为1.0-10dl / g; 涉及其制造方法。

3. 发明授权

US6146739A Glass run channel 失效
标题翻译：玻璃运行通道
公开(公告)号：US6146739A
公开(公告)日：2000-11-14
申请号：US27178
申请日：1998-02-20
申请人： Yuichi Itoh , Masato Karaiwa , Kyoko Kobayashi , Akira Uchiyama
发明人： Yuichi Itoh , Masato Karaiwa , Kyoko Kobayashi , Akira Uchiyama
IPC分类号： B60J10/00 , B60J10/04 , C08L23/06 , C08L23/12 , C08L23/16 , B32B27/08 , B32B27/32
CPC分类号： C08L23/06 , B60J10/17 , B60J10/27 , B60J10/74 , C08L23/12 , C08L23/16 , Y10T428/24198 , Y10T428/31917
摘要： A glass run channel comprising a glass run channel body composed of a bottom wall and side walls extending from two opposite edges of the bottom wall, the glass run channel body having a substantially U-shaped section and provided with a groove, and tonguelike draining parts protruding from vicinities of distal edges of the side walls toward the bottom wall of the glass run channel body so as to become proximate to each other. Each of the tonguelike draining parts has a window glass contact part composed of a surface to be brought into contact with a window glass, which comprises a layer of a thermoplastic elastomer and a layer of an ultrahigh molecular weight polyolefin composition. The layer of ultrahigh molecular weight polyolefin composition is arranged so as to contact a window glass. The ultrahigh molecular weight polyolefin composition comprises at least a polyolefin (composition) having a specified intrinsic viscosity and an olefinic thermoplastic elastomer. The glass run channel is excellent in the durability, tight contactability with a window glass exhibited when the window glass is held closed and supple slide exhibited when a window glass is closed or opened and, even when twisted or bent, is free from a creasing of the ultrahigh molecular weight polyolefin composition layer.
摘要翻译：一种玻璃导槽，包括由底壁和从底壁的两个相对边缘延伸的侧壁组成的玻璃导槽体，所述玻璃导槽体具有大致U形截面并设置有凹槽，并且舌状排液部分从侧壁的远侧边缘的附近向玻璃导槽体的底壁突出，以使彼此靠近。每个舌形排液部分具有由玻璃接触的表面组成的窗玻璃接触部分，其包括热塑性弹性体层和超高分子量聚烯烃组合物层。超高分子量聚烯烃组合物层布置成与窗玻璃接触。超高分子量聚烯烃组合物至少包含具有特定特性粘度的聚烯烃（组合物）和烯属热塑性弹性体。玻璃运行通道在窗玻璃闭合时呈现的窗玻璃的耐久性，与窗玻璃紧密接触的紧密接触性，并且当窗玻璃闭合或打开时呈现柔顺的滑动，并且即使扭曲或弯曲也不会起皱超高分子量聚烯烃组合物层。

4. 发明授权

US5856399A Thermoplastic elastomer composition 失效
标题翻译：热塑性弹性体组合物
公开(公告)号：US5856399A
公开(公告)日：1999-01-05
申请号：US635319
申请日：1996-04-19
申请人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama
发明人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama
IPC分类号： C08K5/00 , C08L23/00 , C08L23/02 , C08L23/10 , C08L23/16 , C08L25/00 , C08L53/00 , C08L53/02 , C08L91/00
CPC分类号： C08L23/02 , C08L23/16 , C08L2207/04 , C08L23/10 , C08L2312/00 , C08L53/02 , C08L91/00
摘要： The thermoplastic elastomer composition of the invention comprises a crystalline polyolefin resin (A), an olefin rubber (B), a hydrogenated styrene block copolymer (C), a softener (D), and optionally, a peroxide non-crosslinked type hydrocarbon rubber (E) in a specific amount of each, and has a gel content of not less than 97%. This composition may be mixed with a crystalline polyolefin resin. The thermoplastic elastomer composition has excellent moldability and is able to provide a molded product having excellent elastomeric properties, high resistance to permanent compression set and good appearance. In particular, a composition obtained by mixing this thermoplastic elastomer composition and a crystalline polyolefin resin shows excellent moldability.
摘要翻译：本发明的热塑性弹性体组合物包含结晶聚烯烃树脂（A），烯烃橡胶（B），氢化苯乙烯嵌段共聚物（C），软化剂（D）和任选的过氧化物非交联型烃橡胶 E），其凝胶含量不低于97％。该组合物可以与结晶聚烯烃树脂混合。热塑性弹性体组合物具有优异的成型性，能够提供具有优异的弹性性能，高耐永久压缩永久变形和良好外观的成型体。特别地，通过混合该热塑性弹性体组合物和结晶聚烯烃树脂获得的组合物显示出优异的成型性。

5. 发明授权

US5702827A Olefin thermoplastic elastomer and laminate thereof 失效
公开(公告)号：US5702827A
公开(公告)日：1997-12-30
申请号：US459804
申请日：1995-06-02
申请人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama , Toru Takehara
发明人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama , Toru Takehara
IPC分类号： B32B27/32 , C08L23/02 , C08L23/10 , C08L23/16 , C08L53/00 , C08L53/02 , B32B23/08
CPC分类号： C08L23/16 , B32B27/32 , C08L23/02 , C08L23/10 , C08L53/02 , C08L53/025 , C08L53/00 , Y10T428/31917 , Y10T428/31924 , Y10T428/31931 , Y10T428/31938
摘要： Olefin thermoplastic elastomers which comprise a partially crosslinked thermoplastic elastomer comprising a crystalline polyolefin resin (A), a block copolymer (B) which is composed of a polymer block of styrene or its derivative and a specific isoprene polymer block, and an olefin rubber (C), and thermoplastic elastomer laminates, having a substrate formed from a specific olefin thermoplastic elastomer or a crystalline polyolefin resin and a skin layer formed from the above-mentioned olefin thermoplastic elastomer, which are excellent in mechanical strength, heat resistance, heat aging resistance, weathering resistance and scratch resistance have been provided by the present invention.

6. 发明授权

US07094828B2 Olefin thermoplastic elastomer composition 有权
标题翻译：烯烃热塑性弹性体组合物
公开(公告)号：US07094828B2
公开(公告)日：2006-08-22
申请号：US10199066
申请日：2002-07-22
申请人： Kyoko Kobayashi , Hiroyasu Yamaoka , Yuichi Itoh , Akira Uchiyama
发明人： Kyoko Kobayashi , Hiroyasu Yamaoka , Yuichi Itoh , Akira Uchiyama
IPC分类号： C08J3/22
CPC分类号： C08L53/00 , C08L23/10 , C08L23/12 , C08L23/16 , C08L53/02 , C08L91/00 , C08L2207/04 , C08L2312/00 , C08L2666/24 , C08L2666/04 , C08L2666/02
摘要： An olefin thermoplastic elastomer composition which is superior in the resistance to oils, heat resistance, formability and flexibility is provided, said elestomer composition comprising the components(A) 40–90 parts by weight of a polypropylene resin having a melt flow rate (determined at 230 ° C. under a load of 2.16 kg according to ASTM D 1238) of 0.1–5 g/10 minutes,(B) 10–60 parts by weight of a copolymer rubber based on olefin, the contents of the components (A) and (B) summing up to 100 parts by weight, and(C) 20–150 parts by weight of a softener,wherein the composition is in such a cross-linked state that the gel content thereof amounts to 97% by weight or higher.
摘要翻译：提供了耐油性，耐热性，成形性和柔软性优异的烯烃热塑性弹性体组合物，所述组分（A）包含40-90重量份的具有熔体流动速率的聚丙烯树脂（在 230℃，根据ASTM D 1238的2.16kg负荷）为0.1-5g / 10分钟，（B）10-60重量份基于烯烃的共聚物橡胶，组分（A）的含量和（B）总计100重量份，和（C）20-150重量份的软化剂，其中组合物处于交联状态，其凝胶含量为97重量％以上。

7. 发明授权

US5596042A Olefin thermoplastic elastomer and laminate thereof 失效
标题翻译：烯烃热塑性弹性体及其层压材料
公开(公告)号：US5596042A
公开(公告)日：1997-01-21
申请号：US626900
申请日：1996-04-04
申请人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama , Toru Takehara
发明人： Yuichi Itoh , Kyoko Kobayashi , Akira Uchiyama , Toru Takehara
IPC分类号： B32B27/32 , C08L23/02 , C08L23/10 , C08L23/16 , C08L53/00 , C08L53/02 , C08L25/08
CPC分类号： C08L23/16 , B32B27/32 , C08L23/02 , C08L23/10 , C08L53/02 , C08L53/025 , C08L53/00 , Y10T428/31917 , Y10T428/31924 , Y10T428/31931 , Y10T428/31938
摘要： Olefin thermoplastic elastomers which comprise a partially crosslinked thermoplastic elastomer comprising a crystalline polyolefin resin (A), a block copolymer (B) which is composed of a polymer block of styrene or its derivative and a specific isoprene polymer block, and an olefin rubber (C), and thermoplastic elastomer laminates, having a substrate formed from a specific olefin thermoplastic elastomer or a crystalline polyolefin resin and a skin layer formed from the above-mentioned olefin thermoplastic elastomer, which are excellent in mechanical strength, heat resistance, heat aging resistance, weathering resistance and scratch resistance have been provided by the present invention.
摘要翻译：包含部分交联的热塑性弹性体的烯烃热塑性弹性体包括结晶聚烯烃树脂（A），由苯乙烯或其衍生物的聚合物嵌段和特定的异戊二烯聚合物嵌段组成的嵌段共聚物（B）和烯烃橡胶（C ）和热塑性弹性体层压体，其具有由特定烯烃热塑性弹性体或结晶聚烯烃树脂形成的基材和由上述烯烃热塑性弹性体形成的表层，其机械强度，耐热性，耐热老化性优异，本发明提供了耐候性和耐划伤性。

8. 发明授权

US06610786B1 Thermoplastic elastomer and process for producing it 有权
标题翻译：热塑性弹性体及其生产方法
公开(公告)号：US06610786B1
公开(公告)日：2003-08-26
申请号：US09162168
申请日：1998-09-29
申请人： Yuichi Itoh , Akira Uchiyama
发明人： Yuichi Itoh , Akira Uchiyama
IPC分类号： C08F800
CPC分类号： C08L21/00 , C08L23/02 , C08L23/16 , C08L2207/04 , C08L2666/06 , C08L2666/04
摘要： A thermoplastic elastomer exhibiting scarce tendency of depositing gummy crust around the extrusion die upon extrusion molding articles therefrom and a superior oil-resistance, which comprises (A) a crystalline polyolefin resin and (B) a cross-linked rubber component produced by a specific melt-kneading technique and which has a certain high level of gel content, a high oil-resistance and a certain reduced rate of deposition of gummy crust on the extrusion die.
摘要翻译：一种热塑性弹性体，其表现出在挤压成形制品周围的挤出模头周围存在粘性外壳的难易的倾向，并具有优异的耐油性，其包括（A）结晶聚烯烃树脂和（B）通过特定熔体制备的交联橡胶组分该技术具有一定的高水平凝胶含量，高耐油性和一定降低挤出模头上胶粘层沉积速率。

9. 发明授权

US07049356B2 Low fogging thermoplastic elastomer composition and manufacturing method and use of same composition 有权
标题翻译：低雾热塑性弹性体组合物及其制造方法和用途相同
公开(公告)号：US07049356B2
公开(公告)日：2006-05-23
申请号：US09779558
申请日：2001-02-09
申请人： Yuichi Itoh , Kunihiko Mizumoto , Hiroyasu Yamaoka , Akira Uchiyama
发明人： Yuichi Itoh , Kunihiko Mizumoto , Hiroyasu Yamaoka , Akira Uchiyama
IPC分类号： C08L91/00 , C08L9/00 , C08J3/24
CPC分类号： C08L23/04 , C08L23/0815 , C08L23/10 , C08L23/16 , C08L2207/04 , C08L2312/00 , C08L2666/04
摘要： This invention relates to a perfectly or partially crosslinked olefinic thermoplastic elastomer composition which comprises 10 to 90 parts by weight of a crystalline polyolefin (a), 90 to 10 parts by weight of an olefin-based copolymer rubber (b) (the total amount of the components (a) and (b) being 100 parts by weight) and 3 to 100 parts by weight of a paraffinic mineral oil softening agent (c) having an evaporation loss of 0.4% by weight or less at a condition of 200° C., atmospheric pressure and 1 hour and having a kinetic viscosity (40° C.) of 50 to 250 cSt; an olefinic thermoplastic elastomer composition which is obtainable by subjecting a mixture including 40 to 85 parts by weight of an ethylene-based copolymer rubber (A), 60 to 15 parts by weight of an olefinic resin (B) and 45 parts by weight or less of a softening agent (C) [the total amount of the components (A), (B) and (C) being 100 parts by weight] to dynamic heat treatment in the presence of a crossliking agent and which has a gloss value of 80% or more and a haze value of 10% or less on glass plate when subjected to the fogging test at a condition of 100° C. and 3 hours according to the prescription of A method of DIN 75201; and a manufacturing method and use of the compositions.
摘要翻译：本发明涉及一种完全或部分交联的烯烃热塑性弹性体组合物，其包含10至90重量份的结晶聚烯烃（a），90至10重量份的烯烃基共聚物橡胶（b）（总计组分（a）和（b）为100重量份）和3至100重量份在200℃条件下蒸发损失为0.4重量％以下的石蜡矿物油软化剂（c）大气压和1小时，动力粘度（40℃）为50〜250cSt; 烯烃类热塑性弹性体组合物，其通过使含有乙烯系共聚物橡胶（A）40〜85重量份，烯烃系树脂（B）60〜15重量份和45重量份以下的混合物的软化剂（C）[组分（A），（B）和（C）的总量为100重量份]在光泽剂存在下进行动态热处理，其光泽值为80 ％以上，雾度值为10％以下时，在100℃，3小时的条件下进行雾化试验时，根据DIN75201A法的处方，以及组合物的制造方法和用途。

10. 发明授权

US06599981B2 Method for manufacturing olefinic thermoplastic elastomer composition 有权
标题翻译：烯烃类热塑性弹性体组合物的制造方法
公开(公告)号：US06599981B2
公开(公告)日：2003-07-29
申请号：US09988058
申请日：2001-11-16
申请人： Yuichi Itoh , Akira Uchiyama
发明人： Yuichi Itoh , Akira Uchiyama
IPC分类号： C08L2704
CPC分类号： B29C47/60 , B29C47/0009 , B29C47/38 , B29C47/402
摘要： This invention relates to a method for manufacturing an olefinic thermoplastic elastomer composition, characterized by disposing specific kneading segment at least at one place of the screw on the occasion of manufacturing an olefinic thermoplastic elastomer composition comprising a polyolefin resin and a crosslinked rubber by dynamic crosslinking with a twin screw extruder.
摘要翻译：烯烃类热塑性弹性体组合物的制造方法技术领域本发明涉及烯烃类热塑性弹性体组合物的制造方法，其特征在于，在制造含有聚烯烃树脂和交联橡胶的烯烃类热塑性弹性体组合物的情况下，至少在螺杆的一个位置配置特定的混炼段，双螺杆挤出机。

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