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1. 发明申请

US20070191212A1 Supported catalyst with a defined pore distribution in the mesopore range 审中-公开
标题翻译：在中孔范围内具有规定的孔分布的负载型催化剂
公开(公告)号：US20070191212A1
公开(公告)日：2007-08-16
申请号：US10590978
申请日：2005-02-24
申请人： Markus Schubert , Jurgen Stephan , Volker Bohm , Andreas Brodhagen , Frank Poplow , Christian Weichert , Holger Borchert
发明人： Markus Schubert , Jurgen Stephan , Volker Bohm , Andreas Brodhagen , Frank Poplow , Christian Weichert , Holger Borchert
IPC分类号： B01J35/08
CPC分类号： B01J35/10 , B01J21/04 , B01J23/36 , B01J35/1019 , B01J35/1042 , B01J35/1061 , B01J35/108 , B01J37/0018 , C07C5/333 , C07C11/02 , C07C11/08
摘要： Supported catalyst comprising a support (S) in which Al2O3 is present in a proportion of at least 75% by weight and rhenium compounds as active component (A), wherein the maximum of the distribution function of the pore diameters in the mesopore range is at from 0.008 to 0.050 μm.
摘要翻译：含有其中Al 2 O 3 N 3的载体（S）的负载型催化剂以至少75重量％的比例存在，铼化合物作为活性组分（A），其中中孔范围内孔径分布函数的最大值为0.008至0.050μm。

2. 发明申请

US20080254976A1 ACTIVATED METATHESIS CATALYSTS 失效
标题翻译：活化的METATHESIS催化剂
公开(公告)号：US20080254976A1
公开(公告)日：2008-10-16
申请号：US12098165
申请日：2008-04-04
申请人： Markus SCHUBERT , Michael Hesse , Jurgen Stephan , Volker Bohm , Andreas Brodhagen , Frank Poplow , Martina Sinner-Lang , Uwe Diehlmann , Gerhard Cox , Jochen Pfeifer
发明人： Markus SCHUBERT , Michael Hesse , Jurgen Stephan , Volker Bohm , Andreas Brodhagen , Frank Poplow , Martina Sinner-Lang , Uwe Diehlmann , Gerhard Cox , Jochen Pfeifer
IPC分类号： B01J21/08
CPC分类号： C07C6/04 , B01J21/08 , B01J23/28 , B01J23/30 , B01J23/36 , B01J27/22 , B01J37/0203 , B01J37/082 , C07C2523/28 , C07C2523/30 , C07C2523/36 , Y02P20/52 , C07C11/02 , C07C11/107 , C07C11/06
摘要： The present invention provides a process for preparing a supported catalyst (catalyst C) having a support (support S) selected from among oxides, phosphates, silicates, carbides, borides and nitrides of main group elements and elements of transition groups VI and II and mixtures of the abovementioned compounds and an active component (activator A) comprising one or more compounds containing one or more elements of transition groups V, VI and VII customary for the catalysis of metathesis reactions.
摘要翻译：本发明提供一种制备负载型催化剂（催化剂C）的方法，所述负载型催化剂（催化剂C）具有选自主要元素的氧化物，磷酸盐，硅酸盐，碳化物，硼化物和氮化物中的载体（载体S）和转变基团VI和II的元素以及混合物的上述化合物和包含一种或多种含有一种或多种通常用于复分解反应催化的过渡基团V，VI和VII元素的化合物（活化剂A）。

3. 发明申请

US20080045766A1 Supported Catalyst Comprising Delta- Or Theta-Modified Aluminium Oxide Supports 审中-公开
标题翻译：负载型催化剂包括三角形或者改性氧化铝载体
公开(公告)号：US20080045766A1
公开(公告)日：2008-02-21
申请号：US10590979
申请日：2005-02-24
申请人： Markus Schubert , Jurgen Stephan , Volker Bohn , Andreas Brodhagen , Frank Poplow
发明人： Markus Schubert , Jurgen Stephan , Volker Bohn , Andreas Brodhagen , Frank Poplow
IPC分类号： B01J21/04 , B01J23/36 , B01J32/00 , B01J37/08
CPC分类号： B01J21/04 , B01J23/36 , B01J35/002 , B01J35/1019 , B01J35/1042 , B01J35/1061 , B01J37/08 , C07C5/333 , C10G45/00 , C07C11/08 , C07C11/02
摘要： Process for producing a supported catalyst which comprises at least 75% by weight of Al2O3, whose proportion of Al2O3 in the delta or theta modification is, based on the proportion of Al2O3, at least 1% and which comprises a rhenium compound and, if appropriate, a promoter as active component (A), which comprises a) converting a customary support (S) which comprises at least 75% by weight of Al2O3 and to which a promoter may, if appropriate, have been applied is converted into a modified support (S) whose proportion of Al2O3 in the delta or theta modification is, based on the proportion of Al2O3, at least 1% by calcining the customary support (S) at a temperature of from 750 to 1100°C., b) producing a supported catalyst precursor from the modified support (S) by applying the active component (A) comprising the rhenium compound to the modified support (S) and c) calcining the supported catalyst precursor at a temperature of from 500 to 750° C.
摘要翻译：负载催化剂的制备方法，其包含至少75重量％的Al 2 O 3 O 3，其比例为Al 2 O 3 O 3， δ或θ改性中的3 N是基于Al 2 O 3 3 3％至少1％的比例，并且其包含铼化合物，如果合适的作为活性组分（A）的促进剂，其包括a）转化常规载体（S），其包含至少75重量％的Al 2 O 3 3和如果合适的话，启动子可以被施加到其上，转化成其在δ或θ改性中的Al 2 O 3 O 3比例为的改性载体（S）基于Al 2 O 3 3 3％的比例，通过在750至1100℃的温度下煅烧常规载体（S）至少1％，b）通过将包含铼化合物的活性组分（A）施加到改性载体（S）上，由改性载体（S）制备负载型催化剂前体，和c）在500-750℃的温度下煅烧负载的催化剂前体

4. 发明申请

US20080188696A1 Process For Preparing A C4-Olefin Mixture By Selective Hydrogenation And Metathesis Process For Using This Stream 有权
标题翻译：通过选择性氢化和复分解方法制备C4-烯烃混合物的方法
公开(公告)号：US20080188696A1
公开(公告)日：2008-08-07
申请号：US11665161
申请日：2005-10-13
申请人： Jurgen Stephan , Andreas Brodhagen , Markus Schubert , Frank Poplow , Michael Roper , Thomas Hill
发明人： Jurgen Stephan , Andreas Brodhagen , Markus Schubert , Frank Poplow , Michael Roper , Thomas Hill
IPC分类号： C07C11/00 , C07C5/02 , C07C6/02
CPC分类号： C07C11/08 , C07C6/04 , C07C2523/44 , C07C11/107 , C07C11/10
摘要： A C4-olefin mixture having a 1,3-butadiene content of from 100 to 500 ppm and a content of 1,2-dienes of less than 10 ppm is described. The present invention further provides a process for preparing this C4-olefin mixture and provides for its use in a metathesis reaction for preparing 2-pentene and/or 3-hexene.
摘要翻译：描述1,3-丁二烯含量为100-500ppm，1,2-二烯含量小于10ppm的C 4 - 烯烃混合物。本发明还提供了一种制备该C 4烯烃混合物的方法，并提供其在复分解反应中用于制备2-戊烯和/或3-己烯的用途。

5. 发明申请

US20080200745A1 Method For Producing Propene From 2-Butene And Isobutene-Rich Feeding Flows 审中-公开
标题翻译：从2-丁烯和异丁烯丰富的进料流中生产丙烯的方法
公开(公告)号：US20080200745A1
公开(公告)日：2008-08-21
申请号：US11817250
申请日：2006-02-24
申请人： Marcus Sigl , Markus Schubert , Jurgen Stephan , Frank Poplow
发明人： Marcus Sigl , Markus Schubert , Jurgen Stephan , Frank Poplow
IPC分类号： C07C2/00
CPC分类号： C07C11/02 , C07C6/04 , C07C2521/04 , C07C2523/30 , C07C2523/36 , Y02P30/464
摘要： Process for preparing a stream consisting essentially of ethene (stream C2=), a stream consisting essentially of propene (stream C3=), a stream consisting essentially of isobutene and possibly other olefins having 4 carbon atoms (stream C4=) and a stream consisting essentially of 2-methyl-2-butene and possibly 2-butene (stream C5=), and, if appropriate, a stream which comprises other hydrocarbons (stream Cx) and may consist of a plurality of separate substreams, which comprises a metathesis step in which a C4-hydrocarbon stream comprising at least 15% by weight of 2-butenes, at least 5% by weight of isobutene and not more than 5% by weight of 1-butene (feed stream) is brought into contact with ethene in the presence of a customary metathesis catalyst and the resulting hydrocarbon stream is fractionated to give the streams C2=, C3=, C4= and, if appropriate, Cx and all or part of the stream C5= is recirculated to the metathesis step.
摘要翻译：用于制备基本上由乙烯（料流C 2 H 2）组成的料流的方法，基本上由丙烯（料流C 3 H 3） =基本上由异丁烯和可能的具有4个碳原子的其它烯烃（流C 4 H 4）组成的料流）和基本上由2-甲基 -2-丁烯和可能的2-丁烯（流C 5 H 5），以及如果合适的话，包含其它烃（流C 1 H 2 O） SUB>），并且可以由多个单独的子流组成，其包括复分解步骤，其中包含至少15重量％的2-丁烯的C 4 - 烃烃流，至少5％的在常规复分解催化剂的存在下，异丁烯的重量和不超过5％（重量）的1-丁烯（进料流）与乙烯接触，并将所得烃流分馏，得到料流C 2， / SUB> ^{= ，C 3 = 并且如果合适的话，C＆gt; x＆gt;和全部或部分流C＆lt; 5＆gt;＆lt; / SUP>再循环到复分解步骤。}

6. 发明申请

US20090023882A1 PROCESS FOR PREPARATION OF POLYISOBUTYLENE WHOSE CONTENT OF TERMINAL DOUBLE BONDS IS MORE THAN 50% FROM AN INDUSTRIAL C4 HYDROCARBON STREAM COMPRISING 1-BUTENE, 2-BUTENE AND ISOBUTENE 审中-公开
标题翻译：用于制备聚异丁烯的方法包含1-BOTENE，2-BOTENE和ISOBUTENE的端子双重含量的含量超过了工业C4烃类流体的50％以上
公开(公告)号：US20090023882A1
公开(公告)日：2009-01-22
申请号：US12278590
申请日：2007-02-15
申请人： Phillip Hanefeld , Hans-Michael Walter , Matthias Kiefer , Helmut Mach , Thomas Wettling , Marcus Sigl , Markus Schubert , Jurgen Stephan , Rainer Papp , Frank Poplow
发明人： Phillip Hanefeld , Hans-Michael Walter , Matthias Kiefer , Helmut Mach , Thomas Wettling , Marcus Sigl , Markus Schubert , Jurgen Stephan , Rainer Papp , Frank Poplow
IPC分类号： C08F110/10
CPC分类号： C10G57/02 , C08F110/10 , C10G25/00 , C10G2300/1044 , C10G2300/1092 , C08F2/00
摘要： Preparation of polyisobutylene having a content of terminal double bonds of more than 50% by polymerizing isobutene using a polymerization catalyst customary therefor from a technical 1-butene-, 2-butene- and isobutene-containing C4 hydrocarbon stream which may comprise up to 3000 ppm by weight, of 1,3-butadiene, by reducing the content of oxygenates in the C4 hydrocarbon stream before the polymerization of the isobutene by contacting it with an inorganic adsorbent at a pressure of from 1 to 20 bar and a temperature of from 20 to 220° C.
摘要翻译：通过聚合催化剂制备具有大于50％的末端双键的聚异丁烯，所用的聚合催化剂通常来自可以包含高达3000ppm的1-丁烯，2-丁烯和异丁烷的C4烃流通过在异丁烯聚合之前通过将其与无机吸附剂在1至20巴的压力和20至20℃的温度下接触来降低C4烃流中的含氧化合物的含量，从而降低1,3-丁二烯的含量 220°C

7. 发明申请

US20080194903A1 Metathesis Method for Purifying Starting Products 审中-公开
标题翻译：净化起始产品的复分解方法
公开(公告)号：US20080194903A1
公开(公告)日：2008-08-14
申请号：US11817237
申请日：2006-02-24
申请人： Markus Schubert , Jurgen Stephan , Frank Poplow , Thomas Heidemann , Uwe Diehlmann , Michaela Maltry
发明人： Markus Schubert , Jurgen Stephan , Frank Poplow , Thomas Heidemann , Uwe Diehlmann , Michaela Maltry
IPC分类号： C07C7/12
CPC分类号： C07B37/08 , C07C6/04 , C07C7/12 , C07C2521/04 , C07C2523/16 , Y02P30/464 , C07C11/02
摘要： Processes comprising: (a) providing a feed stream comprising a C4 compound having at least a nonaromatic C—C double bond or C—C triple bond; (b) contacting the feed stream with an adsorbent which has been activated at a temperature of 450 to 1000° C. comprising at least 3% by weight of aluminum oxide to remove one or more impurities from the feed stream; and (c) contacting the feed stream from which one or more impurities have been removed with a metathesis catalyst under metathesis reaction conditions to form a compound or a mixture of compounds having a nonaromatic C—C double bond or C—C triple bond.
摘要翻译：方法包括：（a）提供包含至少具有非芳族C-C双键或C-C三键的C 4+化合物的进料流; （b）使进料流与在450至1000℃的温度下活化的吸附剂接触，所述吸附剂包含至少3重量％的氧化铝以从进料流中除去一种或多种杂质; 和（c）在复分解反应条件下使已经除去一种或多种杂质的进料流与复分解催化剂接触，以形成具有非芳族C-C双键或C-C三键的化合物或混合物。

8. 发明申请

US20080033223A1 Method for the Production of C5 Aldehydes and Propene from a C4 Stream Containing 1-Butene and 2-Butene 有权
标题翻译：从含有1-丁烯和2-丁烯的C4流中制备C5醛和丙烯的方法
公开(公告)号：US20080033223A1
公开(公告)日：2008-02-07
申请号：US11661543
申请日：2005-08-06
申请人： Marcus Sigl , Markus Schubert , Jurgen Stephan , Rainer Papp , Frank Poplow
发明人： Marcus Sigl , Markus Schubert , Jurgen Stephan , Rainer Papp , Frank Poplow
IPC分类号： C07C6/04
CPC分类号： C07C6/04 , C07C7/13 , C07C45/50 , C07C11/06 , C07C11/08 , C07C47/02
摘要： Processes for preparing a C5 aldehyde and propene are disclosed, the processes comprising: (a) providing a feedstream, the feedstream comprising butane, 1-butene, 2-butene and 1,3-butadiene, the 1,3-butadiene present in the feedstream in an amount up to 1000 ppm; (b) contacting the feedstream with hydrogen and carbon monoxide in the presence of a hydroformylation catalsyt to form a 2-butene-rich butane stream and a C5 aldehyde; (c) separating the 2-butene-rich butane stream and the C5 aldehyde; and (d) contacting the 2-butene-rich butane stream with ethene in the presence of a metathesis catalyst to form a propene-containing hydrocarbon stream.
摘要翻译：公开了制备C 5 H 5醛和丙烯的方法，所述方法包括：（a）提供进料流，所述进料流包含丁烷，1-丁烯，2-丁烯和1,3-丁二烯，存在于进料流中的1,3-丁二烯以高达1000ppm的量存在; （b）在加氢甲酰化催化剂存在下使进料流与氢气和一氧化碳接触以形成富含2-丁烯的丁烷流和C 5 H 5醛; （c）分离富含2-丁烯的丁烷流和C 5 H 5醛; 和（d）在复分解催化剂存在下使富含2-丁烯的丁烷流与乙烯接触以形成含丙烯烃流。

9. 发明申请

US20070083066A1 Method for the production of 1,7-octadiene and use thereof 审中-公开
标题翻译： 1,7-辛二烯的制备方法及其用途
公开(公告)号：US20070083066A1
公开(公告)日：2007-04-12
申请号：US10572077
申请日：2004-09-17
申请人： Volker Bohm , Michael Roper , Jurgen Stephan , Regina Benfer , Markus Schubert , Jorn Karl , Klaus Ebel , Oliver Lober , Martin Volland
发明人： Volker Bohm , Michael Roper , Jurgen Stephan , Regina Benfer , Markus Schubert , Jorn Karl , Klaus Ebel , Oliver Lober , Martin Volland
IPC分类号： C07C45/68 , C07C45/49 , C07C5/08
CPC分类号： C07C49/587 , C07C6/06 , C07C45/50 , C07C45/62 , C07C45/73 , C07C49/385 , C07C2521/04 , C07C2523/20 , C07C2523/28 , C07C2523/30 , C07C2523/36 , C07C2523/74 , C07C11/12 , C07C47/12 , C07C49/12
摘要： The invention relates to a method for the production of 1,7 octadiene by reacting metathesis of cyclohexene with ethylene. The invention also relates to the production of 1,10-decandiol by hydroformulating 1,7 octadiene produced according to said method. The invention further relates to a method for the production of muscone or olefinically unsaturated analogs thereof using 1,10 decandiol which is obtainable in said manner.
摘要翻译：本发明涉及通过使环己烯的复分解与乙烯反应制备1,7辛二烯的方法。本发明还涉及通过根据所述方法制备的1,7辛二烯加氢制备1,10-癸二醇。本发明还涉及使用可以所述方式获得的1,10-癸二醇生产肌醇或其烯属不饱和类似物的方法。

10. 发明申请

US20060183627A1 Method for regenerating re2o7 doped catalyst supports 审中-公开
标题翻译：再生Re2o7掺杂催化剂载体的方法
公开(公告)号：US20060183627A1
公开(公告)日：2006-08-17
申请号：US10547293
申请日：2004-02-16
申请人： Jurgen Stephan , Markus Schubert , Christian Weichert , Wilhelm Ruppel , Peter Resch , Soeren Zimdahl , Frank Mrzena , Andreas Molitor , Stefan Berg , Mathias Fohrmann
发明人： Jurgen Stephan , Markus Schubert , Christian Weichert , Wilhelm Ruppel , Peter Resch , Soeren Zimdahl , Frank Mrzena , Andreas Molitor , Stefan Berg , Mathias Fohrmann
IPC分类号： B01J38/12
CPC分类号： B01J23/92 , B01J23/36 , B01J38/12 , B01J38/14 , C07C6/04 , Y02P20/584
摘要： Method of regenerating an Re2O7-doped supported catalyst which has been deactivated by use in the metathesis of a hydrocarbon mixture comprising C2-C6-olefins (C2-6= feed) (deactivated catalyst), which comprises treating the deactivated catalyst with an inert gas (regeneration gas K1) at from 400 to 800° C. and subsequently treating the deactivated catalyst which has been pretreated with regeneration gas K1 with an oxygen-containing gas (regeneration gas K2).
摘要翻译：通过在包含C 2 -C 6烷基的烃混合物的复分解中使用已经失活的Re 2 O 2 O 7重掺合载体催化剂的再生方法， C 6 - 6 - 烯烃（C 2-6）进料）（失活催化剂），其包括用惰性气体处理失活的催化剂（再生气体K 1），然后用含氧气体（再生气体K 2）处理已经用再生气体K 1预处理的失活催化剂。

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