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1. 发明申请

US20050233895A1 Crystalline intergrowth material, its synthesis and its use in the conversion of oxygenates to olefins 有权
标题翻译：结晶共生材料，其合成及其在含氧化合物转化为烯烃的应用
公开(公告)号：US20050233895A1
公开(公告)日：2005-10-20
申请号：US11072830
申请日：2005-03-04
申请人： Machteld Mertens , An Verberckmoes , Marcel Janssen , Yun-Feng Chang , Luc Martens , Stephen Vaughn , Kenneth Clem , Wilfried Mortier
发明人： Machteld Mertens , An Verberckmoes , Marcel Janssen , Yun-Feng Chang , Luc Martens , Stephen Vaughn , Kenneth Clem , Wilfried Mortier
IPC分类号： B01J27/14 , B01J29/85 , C01B39/54 , C07C1/20 , C10G3/00
CPC分类号： B01J29/85 , C01B39/54 , C07C1/20 , C07C2529/70 , C07C2529/85 , Y02P30/20 , Y02P30/42 , Y10S423/30 , Y10T428/2982 , C07C11/02
摘要： A silicoaluminophosphate molecular sieve is disclosed that comprises first and second intergrown phases of a CHA framework type and an AEI framework type, wherein said first intergrown phase has an AEI/CHA ratio of from about 5/95 to about 40/60 as determined by DIFFaX analysis, the second intergrown phase has an AEI/CHA ratio of about 30/70 to about 55/45 as determined by DIFFaX analysis and said molecular sieve has a silica to alumina molar ratio (Si/Al2) from about 0.13 to about 0.24.
摘要翻译：公开了一种硅铝磷酸盐分子筛，其包含CHA骨架型和AEI骨架型的第一和第二共生相，其中所述第一共生相的AEI / CHA比为约5/95至约40/60，如通过DIFFaX 分析，第二共生相具有通过DIFFaX分析确定的约30/70至约55/45的AEI / CHA比，并且所述分子筛具有二氧化硅与氧化铝的摩尔比（Si / Al 2 O 3 ）为约0.13至约0.24。

2. 发明申请

US20050256354A1 Molecular sieve catalyst composition, its making and use in conversion processes 有权
标题翻译：分子筛催化剂组成，其制备和用途在转化过程中
公开(公告)号：US20050256354A1
公开(公告)日：2005-11-17
申请号：US10844168
申请日：2004-05-12
申请人： Luc Martens , Marcel Janssen , Machteld Mertens , An Verberckmoes , Guang Cao
发明人： Luc Martens , Marcel Janssen , Machteld Mertens , An Verberckmoes , Guang Cao
IPC分类号： B01J29/85 , B01J37/00 , C07C1/20 , C10G3/00 , C07C1/00
CPC分类号： C07C1/20 , B01J29/85 , C10G3/49 , C10G3/56 , C10G3/62 , C10G2300/1022 , C10G2400/20 , Y02P30/20 , Y02P30/42 , Y10S423/30 , Y10S502/514 , C07C11/02
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock in the presence of a molecular sieve having been synthesized in the presence of a flocculant.
摘要翻译：本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。特别地，本发明涉及在存在已在絮凝剂存在下合成的分子筛的存在下从原料，优选含氧化合物原料生产烯烃，优选乙烯和/或丙烯的转化方法。

3. 发明申请

US20060079723A1 Catalyst and process for the conversion of oxygenates to olefins 审中-公开
公开(公告)号：US20060079723A1
公开(公告)日：2006-04-13
申请号：US11198655
申请日：2005-08-05
申请人： Machteld Mertens , Marcel Janssen , Luc Martens , Kenneth Clem
发明人： Machteld Mertens , Marcel Janssen , Luc Martens , Kenneth Clem
IPC分类号： B01J27/182 , C07C1/00
CPC分类号： B01J29/005 , B01J29/80 , B01J29/85 , C07C1/20 , Y02P30/42 , C07C11/02
摘要： A catalyst composition for use in the conversion of oxygenates to olefins comprises a first molecular sieve comprising a CHA framework type material and a second molecular sieve comprising an AFI framework type material, wherein said second molecular sieve is present in an amount up to 0.75% by weight of said first molecular sieve.

4. 发明申请

US20060079397A1 Catalyst and process for the conversion of oxygenates to olefins 审中-公开
标题翻译：用于将含氧化合物转化为烯烃的催化剂和方法
公开(公告)号：US20060079397A1
公开(公告)日：2006-04-13
申请号：US10964172
申请日：2004-10-12
申请人： Machteld Mertens , Marcel Janssen , Luc Martens , Kenneth Clem
发明人： Machteld Mertens , Marcel Janssen , Luc Martens , Kenneth Clem
IPC分类号： B01J27/182
CPC分类号： B01J29/005 , B01J29/80 , B01J29/85 , C07C1/20 , Y02P30/42 , C07C11/02
摘要： A catalyst composition for use in the conversion of oxygenates to olefins comprises a first molecular sieve comprising a CHA framework type material and a second molecular sieve comprising an AFI framework type material, wherein said second molecular sieve is present in an amount up to 0.75% by weight of said first molecular sieve.
摘要翻译：用于将含氧化合物转化为烯烃的催化剂组合物包括包含CHA骨架型材料的第一分子筛和包含AFI骨架型材料的第二分子筛，其中所述第二分子筛以至多0.75％的量存在，所述第一分子筛的重量。

5. 发明申请

US20050245780A1 Attrition resistant molecular sieve catalyst, method of making and process for using 有权
标题翻译：耐磨分子筛催化剂，制备方法和使用方法
公开(公告)号：US20050245780A1
公开(公告)日：2005-11-03
申请号：US10833483
申请日：2004-04-28
申请人： Yun-Feng Chang , Stephen Vaughn , Kenneth Clem , Luc Martens , Alistair Westwood , Jeffery Sprinkle
发明人： Yun-Feng Chang , Stephen Vaughn , Kenneth Clem , Luc Martens , Alistair Westwood , Jeffery Sprinkle
IPC分类号： B01J29/85 , C07C1/20 , C07C1/00 , B01J27/14 , B01J27/186
CPC分类号： B01J29/85 , B01J2229/42 , C07C1/20 , C07C2529/85 , C07C11/02
摘要： This invention provides an attrition resistant metalloaluminophosphate molecular sieve catalyst composition, methods of making the catalyst composition and processes for using the catalyst composition. The metalloaluminophosphate molecular sieve catalyst composition is highly attrition resistant in dried as well as fully calcined forms.
摘要翻译：本发明提供了一种耐磨性金属铝磷酸盐分子筛催化剂组合物，制备催化剂组合物的方法和使用催化剂组合物的方法。金属铝磷酸盐分子筛催化剂组合物在干燥和完全煅烧形式中具有高度耐磨性。

6. 发明申请

US20050075525A1 Molecular sieve catalyst composition, its making and use in conversion processes 有权
标题翻译：分子筛催化剂组成，其制备和用途在转化过程中
公开(公告)号：US20050075525A1
公开(公告)日：2005-04-07
申请号：US10677654
申请日：2003-10-02
申请人： Yun-Feng Chang , Stephen Vaughn , Kenneth Clem , Luc Martens , Weiguo Hu
发明人： Yun-Feng Chang , Stephen Vaughn , Kenneth Clem , Luc Martens , Weiguo Hu
IPC分类号： B01J29/06 , B01J29/84 , B01J29/85 , B01J35/00 , B01J37/00 , C07C1/20 , B01J27/182
CPC分类号： B01J37/0045 , B01J29/06 , B01J29/84 , B01J29/85 , B01J35/002 , B01J37/0009 , C07C1/20 , C07C2521/04 , C07C2521/06 , C07C2521/16 , C07C2529/85 , Y02P30/20 , Y02P30/42 , Y10S502/504 , C07C11/02
摘要： This invention provides methods of making molecular sieve catalyst particles, molecular sieve slurries that can be used in such methods, molecular sieve catalyst compositions and their use in catalytic hydrocarbon conversion processes. In one of its aspects, the invention provides a method of making molecular sieve catalyst particles, the method comprising the steps of: a) providing a solution or suspension of an aluminum-containing inorganic oxide precursor in a liquid medium; b) combining the solution or suspension of aluminum-containing inorganic oxide precursor with a molecular sieve, and optionally other formulating agents, to form a catalyst formulation slurry; c) aging the catalyst formulation slurry to generate in said slurry a percentage, or increase in said slurry the existing percentage, of aluminum atoms of the aluminum-containing precursor in the form of oligomers having a sharp 27Al NMR peak at 62-63 ppm; and d) forming molecular sieve catalyst particles from the catalyst formulation slurry. The catalyst compositions obtained by the methods of the present invention have improved attrition resistance, and are particularly useful in hydrocarbon conversion processes.
摘要翻译：本发明提供制备分子筛催化剂颗粒，可用于这些方法的分子筛浆料，分子筛催化剂组合物及其在催化烃转化方法中的应用的方法。在其一个方面，本发明提供了制备分子筛催化剂颗粒的方法，该方法包括以下步骤：a）提供含铝无机氧化物前体在液体介质中的溶液或悬浮液; b）将含铝的无机氧化物前体的溶液或悬浮液与分子筛和任选的其它配制剂组合以形成催化剂配方浆料; c）使催化剂配方浆料老化，以在所述浆料中产生百分比，或增加所述浆料中现有百分比的含铝前体的铝原子具有在62℃具有尖锐的27 C NMR峰的低聚物形式， 63 ppm; 和d）从催化剂配方浆料形成分子筛催化剂颗粒。通过本发明的方法获得的催化剂组合物具有改善的耐磨耗性，并且在烃转化方法中特别有用。

7. 发明申请

US20070238911A1 Molecular sieve catalyst composition, its making and use in conversion processes 有权
标题翻译：分子筛催化剂组成，其制备和用途在转化过程中
公开(公告)号：US20070238911A1
公开(公告)日：2007-10-11
申请号：US11805984
申请日：2007-05-25
申请人： Yun-feng Chang , Stephen Vaughn , Luc Martens , Kenneth Clem
发明人： Yun-feng Chang , Stephen Vaughn , Luc Martens , Kenneth Clem
IPC分类号： C07C4/02
CPC分类号： B01J37/0009 , B01J29/85 , B01J35/10 , B01J35/1019 , B01J35/1023 , B01J37/0045 , B01J2229/42 , C07C1/20 , C07C2529/85 , C10G3/48 , C10G3/49 , C10G3/62 , C10G2300/1022 , C10G2400/20 , Y02P20/52 , Y02P30/42 , C07C11/06 , C07C11/04
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to a molecular sieve catalyst composition of a molecular sieve, a binder and a matrix material, wherein the weight ratio of the binder to the molecular sieve is controlled to provide an improved attrition resistant catalyst composition, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译：本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。特别地，本发明涉及分子筛，粘合剂和基质材料的分子筛催化剂组合物，其中控制粘合剂与分子筛的重量比以提供改进的耐磨性催化剂组合物，特别适用于用于从原料，优选含氧化合物原料生产烯烃，优选乙烯和/或丙烯的转化方法。

8. 发明申请

US20050137080A1 Molecular sieve catalyst compositions, its making and use in conversion processes 有权
标题翻译：分子筛催化剂组合物，其制备和用于转化过程
公开(公告)号：US20050137080A1
公开(公告)日：2005-06-23
申请号：US11039294
申请日：2005-01-20
申请人： Yun-feng Chang , Stephen Vaughn , Luc Martens , Joseph Baumgartner , Stuart Soled , Kenneth Clem
发明人： Yun-feng Chang , Stephen Vaughn , Luc Martens , Joseph Baumgartner , Stuart Soled , Kenneth Clem
IPC分类号： B01J29/85 , B01J35/10 , B01J37/00 , B01J37/10 , C07C1/20 , C07C11/02 , C07C11/04 , C07C11/06 , C10G3/00 , B01J27/182
CPC分类号： B01J37/10 , B01J29/85 , B01J35/10 , B01J37/0009 , B01J37/0045 , B01J2229/36 , B01J2229/42 , C07C1/20 , C07C11/02 , C07C11/04 , C07C11/06 , C07C2529/00 , C07C2529/85 , C10G3/48 , C10G3/49 , C10G3/62 , C10G2300/1022 , C10G2400/20 , Y02P20/52 , Y02P30/42
摘要： The invention relates to a molecular sieve catalyst composition, to a method of making or forming the molecular sieve catalyst composition, and to a conversion process using the catalyst composition. In particular, the invention is directed to a making a molecular sieve catalyst composition by forming a slurry by combining a molecular sieve, a binder and a matrix material, wherein the slurry has a pH, above or below the isoelectric point of the molecular sieve. The catalyst composition has improved attrition resistance, particularly useful in a conversion process for producing olefin(s), preferably ethylene and/or propylene, from a feedstock, preferably an oxygenate containing feedstock.
摘要翻译：本发明涉及分子筛催化剂组合物，制备或形成分子筛催化剂组合物的方法，以及使用该催化剂组合物的转化方法。特别地，本发明涉及通过组合分子筛，粘合剂和基质材料形成浆料来制备分子筛催化剂组合物，其中所述浆料具有高于或低于分子筛等电点的pH。催化剂组合物具有改善的耐磨性，特别适用于从原料，优选含氧化合物原料生产烯烃，优选乙烯和/或丙烯的转化方法。

9. 发明申请

US20070249885A1 Molecular sieve catalyst composition, its making and use in conversion processes 有权
标题翻译：分子筛催化剂组成，其制备和用途在转化过程中
公开(公告)号：US20070249885A1
公开(公告)日：2007-10-25
申请号：US11818495
申请日：2007-06-14
申请人： Yun-Feng Chang , Stephen Vaughn , Kenneth Clem , Luc Martens , Weiguo Hu
发明人： Yun-Feng Chang , Stephen Vaughn , Kenneth Clem , Luc Martens , Weiguo Hu
IPC分类号： C07C1/00
CPC分类号： B01J37/0045 , B01J29/06 , B01J29/84 , B01J29/85 , B01J35/002 , B01J37/0009 , C07C1/20 , C07C2521/04 , C07C2521/06 , C07C2521/16 , C07C2529/85 , Y02P30/20 , Y02P30/42 , Y10S502/504 , C07C11/02
摘要： This invention provides methods of making molecular sieve catalyst particles, molecular sieve slurries that can be used in such methods, molecular sieve catalyst compositions and their use in catalytic hydrocarbon conversion processes. In one of its aspects, the invention provides a method of making molecular sieve catalyst particles, the method comprising the steps of: a) providing a solution or suspension of an aluminum-containing inorganic oxide precursor in a liquid medium; b) combining the solution or suspension of aluminum-containing inorganic oxide precursor with a molecular sieve, and optionally other formulating agents, to form a catalyst formulation slurry; c) aging the catalyst formulation slurry to generate in said slurry a percentage, or increase in said slurry the existing percentage, of aluminum atoms of the aluminum-containing precursor in the form of oligomers having a sharp 27Al NMR peak at 62-63 ppm; and d) forming molecular sieve catalyst particles from the catalyst formulation slurry. The catalyst compositions obtained by the methods of the present invention have improved attrition resistance, and are particularly useful in hydrocarbon conversion processes.
摘要翻译：本发明提供制备分子筛催化剂颗粒，可用于这些方法的分子筛浆料，分子筛催化剂组合物及其在催化烃转化方法中的应用的方法。在其一个方面，本发明提供了制备分子筛催化剂颗粒的方法，该方法包括以下步骤：a）提供含铝无机氧化物前体在液体介质中的溶液或悬浮液; b）将含铝的无机氧化物前体的溶液或悬浮液与分子筛和任选的其它配制剂组合以形成催化剂配方浆料; c）使所述催化剂配方浆料老化以在所述浆料中产生一种百分比，或增加所述浆料中含铝前体的铝原子的现有百分比，其具有尖锐的Al 2 O 3 在62-63ppm的NMR峰; 和d）从催化剂配方浆料形成分子筛催化剂颗粒。通过本发明的方法获得的催化剂组合物具有改善的耐磨耗性，并且在烃转化方法中特别有用。

10. 发明申请

US20060205587A1 Attrition resistant molecular sieve catalysts 有权
标题翻译：耐磨分子筛催化剂
公开(公告)号：US20060205587A1
公开(公告)日：2006-09-14
申请号：US11434013
申请日：2006-05-15
申请人： Yun-Feng Chang , Stephen Vaughn , Luc Martens , Kenneth Clem
发明人： Yun-Feng Chang , Stephen Vaughn , Luc Martens , Kenneth Clem
IPC分类号： B01J29/06
CPC分类号： B01J37/0045 , B01J29/06 , B01J29/85 , C07C1/20 , C07C2529/83 , C07C2529/85 , C10G2400/20 , Y02P30/20 , Y02P30/42 , C07C11/02
摘要： This invention is directed to a hardened molecular sieve catalyst composition, a method of making the composition and a method of using the composition. The catalyst composition is made by mixing together molecular sieve, liquid, and an effective hardening amount of a dried molecular sieve catalyst to form a slurry. The slurry is dried, and then calcined to form the hardened molecular sieve catalyst composition. The hardened molecular sieve catalyst is highly attrition resistant.
摘要翻译：本发明涉及硬化分子筛催化剂组合物，制备组合物的方法和使用该组合物的方法。催化剂组合物通过将分子筛，液体和有效硬化量的干燥的分子筛催化剂混合在一起而形成浆料而制成。将浆料干燥，然后煅烧以形成硬化的分子筛催化剂组合物。硬化分子筛催化剂具有高耐磨性。

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