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1. 发明授权

US09181147B2 Process for the production of xylenes and light olefins 有权
标题翻译：生产二甲苯和轻质烯烃的方法
公开(公告)号：US09181147B2
公开(公告)日：2015-11-10
申请号：US13465733
申请日：2012-05-07
申请人： Larry L. Iaccino , S. Mark Davis , John D. Y. Ou , Xiaobo Zheng
发明人： Larry L. Iaccino , S. Mark Davis , John D. Y. Ou , Xiaobo Zheng
IPC分类号： C07C1/24 , C07C2/86 , C10G29/20 , C10G35/00 , C10G57/00 , C10G9/00 , C10G9/36 , C10G11/00
CPC分类号： C07C2/864 , C10G9/005 , C10G9/36 , C10G11/00 , C10G29/205 , C10G35/00 , C10G57/005 , C10G2300/1092 , C10G2300/1096 , C10G2400/30 , C07C15/08
摘要： In a hydrocarbon upgrading process, a hydrocarbon feed is treated in at least one of a steam cracker, catalytic cracker, coker, hydrocracker, and reformer under suitable conditions to produce a first stream comprising olefinic and aromatic hydrocarbons. A second stream composed mainly of C4+ olefinic and aromatic hydrocarbons is recovered from the first stream and is fed together with a methylating agent to a reaction zone containing a catalyst under reaction conditions including a temperature of about 450° C. to about 700° C., such that aromatics components in the second stream undergo dealkylation, transalkylation and/or methylation and aliphatic components undergo cracking and aromatization to produce a third stream having an increased xylene content compared with said second stream and a C3− olefin by-product. The C3− olefin by-product is recovered and para-xylene is removed from at least part of said third stream.
摘要翻译：在烃改质方法中，在合适条件下，在蒸汽裂化器，催化裂化器，焦化器，加氢裂化器和重整器中的至少一种中处理烃进料以产生包含烯烃和芳族烃的第一流。从第一流回收主要由C4 +烯烃和芳烃组成的第二料流，并在包括约450℃至约700℃的温度的反应条件下与甲基化剂一起加入含有催化剂的反应区。使得第二流中的芳烃组分经历脱烷基化，烷基转移和/或甲基化，并且脂族组分经历裂化和芳构化以产生与所述第二料流和C3-烯烃副产物相比具有增加的二甲苯含量的第三料流。回收C3-烯烃副产物，并从至少部分所述第三料流中除去对二甲苯。

2. 发明申请

US20080051615A1 Process for the production of benzene, toluene, and xylenes 失效
标题翻译：生产苯，甲苯和二甲苯的方法
公开(公告)号：US20080051615A1
公开(公告)日：2008-02-28
申请号：US11509403
申请日：2006-08-24
申请人： Elizabeth L. Stavens , Stephen H. Brown , J. Scott Buchanan , Yun-feng Chang , Larry L. Iaccino , Paul F. Keusenkothen , John D. Y. Ou , Randall D. Partridge
发明人： Elizabeth L. Stavens , Stephen H. Brown , J. Scott Buchanan , Yun-feng Chang , Larry L. Iaccino , Paul F. Keusenkothen , John D. Y. Ou , Randall D. Partridge
IPC分类号： C07C5/10
CPC分类号： B01J29/126 , B01J29/22 , B01J29/44 , B01J29/74 , B01J29/7415 , B01J35/002 , B01J37/08 , B01J2229/42 , C10G45/64 , Y02P20/52
摘要： A hydrocarbon conversion process for producing an aromatics product containing of benzene, toluene, xylenes, or mixtures thereof. The process is carried out by converting precursors of benzene, toluene, and xylenes that are contained in a hydrocarbon feed (C6+ non-aromatic cyclic hydrocarbons, A8+ single-ring aromatic hydrocarbons having at least one alkyl group containing two or more carbon atoms; and A9+ single-ring aromatic hydrocarbons having at least three methyl groups) to produce a product that contains an increased amount of benzene, toluene, xylenes, or combinations thereof compared to said hydrocarbon feed.
摘要翻译：一种用于生产含苯，甲苯，二甲苯或其混合物的芳族化合物产物的烃转化方法。该方法通过将烃原料（C 6+非芳族环状烃，A 8+单体）中包含的苯，甲苯和二甲苯的前体转化具有至少一个含有两个或更多个碳原子的烷基的芳族烃;以及具有至少三个甲基的A 9 N +单环芳族烃），以产生含有增加量的苯，甲苯，二甲苯或其组合与所述烃进料相比。

3. 发明授权

US07563358B2 Process for the production of benzene, toluene, and xylenes 失效
标题翻译：生产苯，甲苯和二甲苯的方法
公开(公告)号：US07563358B2
公开(公告)日：2009-07-21
申请号：US11509403
申请日：2006-08-24
申请人： Elizabeth L. Stavens , Stephen H. Brown , J. Scott Buchanan , Yun-Feng Chang , Larry L. Iaccino , Paul F. Keusenkothen , John D. Y. Ou , Randall D. Partridge
发明人： Elizabeth L. Stavens , Stephen H. Brown , J. Scott Buchanan , Yun-Feng Chang , Larry L. Iaccino , Paul F. Keusenkothen , John D. Y. Ou , Randall D. Partridge
IPC分类号： C10G35/06 , C10G35/085 , C10G35/095
CPC分类号： B01J29/126 , B01J29/22 , B01J29/44 , B01J29/74 , B01J29/7415 , B01J35/002 , B01J37/08 , B01J2229/42 , C10G45/64 , Y02P20/52
摘要： A hydrocarbon conversion process for producing an aromatics product containing of benzene, toluene, xylenes, or mixtures thereof. The process is carried out by converting precursors of benzene, toluene, and xylenes that are contained in a hydrocarbon feed (C6+ non-aromatic cyclic hydrocarbons, A8+ single-ring aromatic hydrocarbons having at least one alkyl group containing two or more carbon atoms; and A9+ single-ring aromatic hydrocarbons having at least three methyl groups) to produce a product that contains an increased amount of benzene, toluene, xylenes, or combinations thereof compared to said hydrocarbon feed.
摘要翻译：一种用于生产含苯，甲苯，二甲苯或其混合物的芳族化合物产物的烃转化方法。该方法通过将烃原料（C6 +非芳族环状烃，具有至少一个含有两个以上碳原子的烷基的A8 +单环芳香族烃）所含有的苯，甲苯和二甲苯的前体具有至少三个甲基的A9 +单环芳烃）以产生与所述烃进料相比含有增加量的苯，甲苯，二甲苯或其组合的产物。

4. 发明申请

US20120083637A1 Regeneration of Metal-Containing Catalysts 有权
标题翻译：含金属催化剂的再生
公开(公告)号：US20120083637A1
公开(公告)日：2012-04-05
申请号：US13218520
申请日：2011-08-26
申请人： Kenneth R. Clem , Larry L. Iaccino , Mobae Afeworki , Juan D. Henao , Neeraj Sangar , Xiaobo Zheng , Lorenzo C. DeCaul
发明人： Kenneth R. Clem , Larry L. Iaccino , Mobae Afeworki , Juan D. Henao , Neeraj Sangar , Xiaobo Zheng , Lorenzo C. DeCaul
IPC分类号： C07C2/76 , B01J38/02
CPC分类号： C07C2/76 , B01J29/48 , B01J29/90 , B01J38/02 , B01J38/10 , C07C1/12 , C07C2/66 , C07C2/864 , C07C2/865 , C07C5/10 , C07C5/11 , C07C2521/06 , C07C2523/02 , C07C2523/06 , C07C2523/08 , C07C2523/10 , C07C2523/12 , C07C2523/14 , C07C2523/16 , C07C2523/18 , C07C2523/20 , C07C2523/26 , C07C2523/28 , C07C2523/30 , C07C2523/34 , C07C2523/36 , C07C2523/42 , C07C2523/44 , C07C2523/46 , C07C2523/50 , C07C2523/52 , C07C2523/72 , C07C2523/745 , C07C2523/75 , C07C2523/755 , C07C2527/22 , C07C2529/08 , C07C2529/18 , C07C2529/40 , C07C2529/60 , C07C2529/65 , C07C2529/70 , C07C2601/14 , C07C2601/16 , C07C2602/26 , C07C2602/28 , C10G50/00 , C10G2300/708 , C10G2400/30 , Y02P20/52 , Y02P20/584 , Y02P20/588 , C07C15/04 , C07C15/24 , C07C11/04 , C07C9/04 , C07C9/06 , C07C15/073 , C07C15/08 , C07C13/18 , C07C13/50 , C07C13/20 , C07C13/48
摘要： In a process for the regeneration of a coked metal-containing catalyst, the coked catalyst is contacted in a regeneration zone with an atmosphere which contains carbon dioxide and carbon monoxide at a temperature of at least 400° C.
摘要翻译：在含焦炭金属催化剂的再生方法中，焦化催化剂在再生区与含有二氧化碳和一氧化碳的气氛在至少400℃的温度下接触。

5. 发明授权

US08859835B2 Regeneration of metal-containing catalysts 有权
标题翻译：含金属催化剂的再生
公开(公告)号：US08859835B2
公开(公告)日：2014-10-14
申请号：US13218520
申请日：2011-08-26
申请人： Kenneth R. Clem , Larry L. Iaccino , Mobae Afeworki , Juan D. Henao , Neeraj Sangar , Xiaobo Zheng , Lorenzo C. DeCaul
发明人： Kenneth R. Clem , Larry L. Iaccino , Mobae Afeworki , Juan D. Henao , Neeraj Sangar , Xiaobo Zheng , Lorenzo C. DeCaul
IPC分类号： C07C15/00
CPC分类号： C07C2/76 , B01J29/48 , B01J29/90 , B01J38/02 , B01J38/10 , C07C1/12 , C07C2/66 , C07C2/864 , C07C2/865 , C07C5/10 , C07C5/11 , C07C2521/06 , C07C2523/02 , C07C2523/06 , C07C2523/08 , C07C2523/10 , C07C2523/12 , C07C2523/14 , C07C2523/16 , C07C2523/18 , C07C2523/20 , C07C2523/26 , C07C2523/28 , C07C2523/30 , C07C2523/34 , C07C2523/36 , C07C2523/42 , C07C2523/44 , C07C2523/46 , C07C2523/50 , C07C2523/52 , C07C2523/72 , C07C2523/745 , C07C2523/75 , C07C2523/755 , C07C2527/22 , C07C2529/08 , C07C2529/18 , C07C2529/40 , C07C2529/60 , C07C2529/65 , C07C2529/70 , C07C2601/14 , C07C2601/16 , C07C2602/26 , C07C2602/28 , C10G50/00 , C10G2300/708 , C10G2400/30 , Y02P20/52 , Y02P20/584 , Y02P20/588 , C07C15/04 , C07C15/24 , C07C11/04 , C07C9/04 , C07C9/06 , C07C15/073 , C07C15/08 , C07C13/18 , C07C13/50 , C07C13/20 , C07C13/48
摘要： In a process for the regeneration of a coked metal-containing catalyst, the coked catalyst is contacted in a regeneration zone with an atmosphere which contains carbon dioxide and carbon monoxide at a temperature of at least 400° C.
摘要翻译：在含焦炭金属催化剂的再生方法中，焦化催化剂在再生区与含有二氧化碳和一氧化碳的气氛在至少400℃的温度下接触。

6. 发明授权

US09056297B2 Integrated vacuum resid to chemicals conversion process 有权
标题翻译：集成减压渣油到化学品转化过程中
公开(公告)号：US09056297B2
公开(公告)日：2015-06-16
申请号：US13723591
申请日：2012-12-21
申请人： S. Mark Davis , Larry L. Iaccino , Richard C. Stell , Steven E. Silverberg , Jiunn-Shyan Liou , Howard Freund
发明人： S. Mark Davis , Larry L. Iaccino , Richard C. Stell , Steven E. Silverberg , Jiunn-Shyan Liou , Howard Freund
IPC分类号： B01J19/00 , C10B55/10 , C10B57/04 , C10B57/06 , C10G11/18 , C10J3/48 , B01J19/24 , B01J8/18 , C10G9/34 , C10G9/36 , C10J3/46
CPC分类号： B01J19/0053 , C10B55/10 , C10B57/04 , C10B57/06 , C10G9/36 , C10G11/18 , C10G2300/1077 , C10G2300/203 , C10G2300/206 , C10G2300/301 , C10G2300/4006 , C10G2300/807 , C10G2400/20 , C10J3/463 , C10J3/482 , C10J2300/0943 , C10J2300/0956 , C10J2300/0973
摘要： A process and apparatus for cracking a hydrocarbon feed containing resid, comprising: heating a hydrocarbon feedstock containing resid; passing said heated hydrocarbon feedstock to a vapor/liquid separator; flashing said heated hydrocarbon feedstock in said vapor/liquid separator to form a vapor phase and a liquid phase containing said resid; passing at least a portion of said resid-containing liquid phase from said vapor/liquid separator to a thermal conversion reactor operating at 649° C. or more, wherein the thermal conversion reactor contains coke particles; and converting at least a portion of said resid into olefins.
摘要翻译：一种用于裂化含有渣油的烃进料的方法和装置，包括：加热含有残渣的烃原料; 将所述加热的烃原料通入气/液分离器; 在所述气/液分离器中闪蒸所述加热的烃原料以形成含有所述残渣的气相和液相; 将来自所述蒸汽/液体分离器的至少一部分所述残留液体相转移到在649℃或更高温度下操作的热转化反应器，其中所述热转化反应器含有焦炭颗粒; 以及将所述残留物的至少一部分转化为烯烃。

7. 发明授权

US07781636B2 Process for methane conversion 有权
标题翻译：甲烷转化工艺
公开(公告)号：US07781636B2
公开(公告)日：2010-08-24
申请号：US11732039
申请日：2007-04-02
申请人： Larry L. Iaccino , Neeraj Sangar , Elizabeth L. Stavens , Matthew J. Vincent
发明人： Larry L. Iaccino , Neeraj Sangar , Elizabeth L. Stavens , Matthew J. Vincent
IPC分类号： C07C2/78
CPC分类号： C07C2/76 , C10G50/00 , C10G2300/1025 , C10G2400/30 , Y02P20/52 , Y10S585/943 , C07C15/02 , C07C15/04
摘要： A process for converting methane to higher hydrocarbon(s) including aromatic hydrocarbon(s) in a reaction zone comprises providing to a hydrocarbon feedstock containing methane and a catalytic particulate material to the reaction zone and contacting the catalytic particulate material and the hydrocarbon feedstock in a substantially countercurrent fashion in the reaction zone, while operating the reaction zone under reaction conditions sufficient to convert at least a portion of said methane to a first effluent having said higher hydrocarbon(s).
摘要翻译：在反应区中将甲烷转化为高级烃（包括芳族烃）的方法包括向反应区提供含有甲烷和催化颗粒物质的烃原料，并使催化颗粒材料和烃原料接触同时在足以将至少一部分甲烷转化为具有所述较高烃的第一流出物的反应条件下操作反应区。

8. 发明授权

US07759535B2 Production of aromatic hydrocarbons from methane 有权
标题翻译：从甲烷生产芳烃
公开(公告)号：US07759535B2
公开(公告)日：2010-07-20
申请号：US11792359
申请日：2005-12-02
申请人： Larry L. Iaccino , Xiaobing Feng , Matthew J. Vincent , Elizabeth L. Stavens
发明人： Larry L. Iaccino , Xiaobing Feng , Matthew J. Vincent , Elizabeth L. Stavens
IPC分类号： C07C2/78
CPC分类号： C07C2/76 , Y10S585/943 , C07C15/02
摘要： In a process for converting methane to higher hydrocarbons including aromatic hydrocarbons, a feed containing methane is contacted with a dehydrocyclization catalyst under conditions effective to convert said methane to aromatic hydrocarbons and produce a first effluent stream comprising aromatic hydrocarbons and hydrogen, wherein said first effluent stream comprises at least 5 wt % more aromatic hydrocarbons than said feed. At least part of the hydrogen from said first effluent stream is then reacted with an oxygen-containing species, such as carbon dioxide, to produce a second effluent stream having a reduced hydrogen content compared with said first effluent stream.
摘要翻译：在将甲烷转化为包括芳烃的高级烃的方法中，含有甲烷的进料在有效地将所述甲烷转化为芳烃并产生包含芳族烃和氢的第一流出物流的条件下与脱氢环化催化剂接触，其中所述第一流出物流包含比所述进料多至少5重量％的芳烃。然后使来自所述第一流出物流的氢的至少一部分与含氧物质如二氧化碳反应，以产生与所述第一流出物流相比具有降低的氢含量的第二流出物流。

9. 发明授权

US07754930B2 Use of isotopic analysis for determination of aromatic hydrocarbons produced from methane 有权
标题翻译：使用同位素分析测定甲烷产生的芳烃
公开(公告)号：US07754930B2
公开(公告)日：2010-07-13
申请号：US11805868
申请日：2007-05-24
申请人： Larry L. Iaccino
发明人： Larry L. Iaccino
IPC分类号： C07C13/00
CPC分类号： C07C2/66 , C07C2/76 , Y10S585/941 , C07C15/08 , C07C15/04
摘要： Benzene and xylene are described having a unique distribution of deuterium and 13C such that δ(deuterium) for each of the benzene and xylene is less than −250 and δ(13C) for the benzene is greater than −36 and for xylene is less than −24, wherein δ(deuterium)=(R′sample/R′standard−1)×1000 where R′sample is the ratio of deuterium to hydrogen in the benzene/xylene; and R′standard is the ratio of the natural abundance of deuterium to the natural abundance of hydrogen; and wherein δ(13C)=(R″sample/R″standard−1)×1000 where R″sample is the ratio of 13C to 12C in the benzene/xylene; and R″standard is the ratio of the natural abundance of 13C to the natural abundance of 12C.
摘要翻译：描述苯和二甲苯具有氘和13C的独特分布，使得苯和二甲苯中的每一个的δ（氘）小于-250，苯的δ（13℃）大于-36，并且对于二甲苯小于 -24，其中δ（氘）=（R'sample / R'standard-1）×1000其中R'示例是苯/二甲苯中氘与氢的比例; R'standard是氘的天然丰度与氢的天然丰度之比; 其中δ（13C）=（R“样品/ R”标准-1）×1000其中R“样品是苯/二甲苯中13C至12C的比例; 而R“标准是13C的天然丰度与12C的天然丰度之比。

10. 发明授权

US07615143B2 Hydrothermally stable catalyst and its use in catalytic cracking 失效
标题翻译：水热稳定催化剂及其在催化裂化中的应用
公开(公告)号：US07615143B2
公开(公告)日：2009-11-10
申请号：US10903152
申请日：2004-07-30
申请人： Tan-Jen Chen , Paul F. Keusenkothen , J. Jason Wu , John Scott Buchanan , Guang Cao , Larry L. Iaccino , David L. Stern , Matthew J. Vincent
发明人： Tan-Jen Chen , Paul F. Keusenkothen , J. Jason Wu , John Scott Buchanan , Guang Cao , Larry L. Iaccino , David L. Stern , Matthew J. Vincent
IPC分类号： C10G11/05
CPC分类号： C10G11/05 , C10G2400/20
摘要： There is provided a catalyst composition having improved hydrothermal stability for the catalytic cracking of a hydrocarbon feedstock to selectively produce propylene. The catalyst composition comprises a first crystalline molecular sieve selected from the group consisting of IM-5, MWW, ITH, FER, MFS, AEL, and AFO and an effective amount of a stabilization metal (copper, zirconium, or mixtures thereof) exchanged into the molecular sieve. The catalyst finds application in the cracking of naphtha and heavy hydrocarbon feedstocks. When used in the catalytic cracking of heavier hydrocarbon feedstocks, the catalyst composition preferably comprises a second molecular sieve having a pore size that is greater than the pore size of the first molecular sieve. The process is carried out by contacting a feedstock containing hydrocarbons having at least 4 carbon atoms is contacted, under catalytic cracking conditions, with the catalyst composition.
摘要翻译：提供了一种具有改进的水热稳定性用于烃原料的催化裂化以选择性地生产丙烯的催化剂组合物。催化剂组合物包含选自由IM-5，MWW，ITH，FER，MFS，AEL和AFO组成的组的第一结晶分子筛和有效量的稳定金属（铜，锆或其混合物）交换成分子筛。该催化剂可用于石脑油和重质烃原料的裂解。当用于较重烃原料的催化裂化时，催化剂组合物优选包含具有大于第一分子筛孔径的孔径的第二分子筛。该方法通过使含有至少4个碳原子的烃的原料在催化裂化条件下与催化剂组合物接触来进行。

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