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1. 发明授权

US07825287B2 Process for production of triptane and triptene 有权
标题翻译：生产曲坦和三肽的方法
公开(公告)号：US07825287B2
公开(公告)日：2010-11-02
申请号：US12058300
申请日：2008-03-28
申请人： John Ahn , Burcin Temel , Enrique Iglesia
发明人： John Ahn , Burcin Temel , Enrique Iglesia
IPC分类号： C07C1/00
CPC分类号： C07C1/20 , C07C9/16 , C07C11/107
摘要： High octane C7 hydrocarbons, particularly 2,2,3-trimethylbutane (“triptane”) and 2,2,3-trimethyl-but-1-ene (“triptene”) (collectively “triptyls”) are produced by homologation of a feed comprising dimethyl ether and/or methanol and optionally including one or more aliphatic hydrocarbons in the presence of certain acidic zeolite catalysts. The process can be carried out at temperatures lower than those previously used for conversion of dimethyl ether and/or methanol to higher alkanes, including C7 alkanes, and results in selective production of triptane and/or triptene with relatively little isomerization to or production of other C7 alkanes.
摘要翻译：高辛烷值的C7烃，特别是2,2,3-三甲基丁烷（“triptane”）和2,2,3-三甲基 - 丁-1-烯（“triptene”）（统称为“triptyl”）是通过进料包括二甲醚和/或甲醇，并且在某些酸性沸石催化剂的存在下任选地包括一种或多种脂族烃。该方法可以在比以前用于将二甲醚和/或甲醇转化为高级烷烃（包括C 7烷烃）的温度低的温度下进行，并且导致选择性生产具有相对较少的异构化或生产其它的三烷基和/或三丁烯 C7烷烃。

2. 发明申请

US20090247803A1 Process for Production of Triptane and Triptene 有权
标题翻译：三甲苯和三氯甲烷生产工艺
公开(公告)号：US20090247803A1
公开(公告)日：2009-10-01
申请号：US12058300
申请日：2008-03-28
申请人： John Ahn , Burcin Temel , Enrique Iglesia
发明人： John Ahn , Burcin Temel , Enrique Iglesia
IPC分类号： C07C1/00
CPC分类号： C07C1/20 , C07C9/16 , C07C11/107
摘要： High octane C7 hydrocarbons, particularly 2,2,3-trimethylbutane (“triptane”) and 2,2,3-trimethyl-but-1-ene (“triptene”) (collectively “triptyls”) are produced by homologation of a feed comprising dimethyl ether and/or methanol and optionally including one or more aliphatic hydrocarbons in the presence of certain acidic zeolite catalysts. The process can be carried out at temperatures lower than those previously used for conversion of dimethyl ether and/or methanol to higher alkanes, including C7 alkanes, and results in selective production of triptane and/or triptene with relatively little isomerization to or production of other C7 alkanes.
摘要翻译：高辛烷值的C7烃，特别是2,2,3-三甲基丁烷（“triptane”）和2,2,3-三甲基 - 丁-1-烯（“triptene”）（统称为“triptyl”）是通过进料包括二甲醚和/或甲醇，并且在某些酸性沸石催化剂的存在下任选地包括一种或多种脂族烃。该方法可以在比以前用于将二甲醚和/或甲醇转化为高级烷烃（包括C 7烷烃）的温度低的温度下进行，并且导致选择性生产具有相对较少的异构化或生产其它的三烷基和/或三丁烯 C7烷烃。

3. 发明授权

US08637580B2 Process for the preparation of ethanol and higher alcohols 有权
标题翻译：乙醇和高级醇的制备方法
公开(公告)号：US08637580B2
公开(公告)日：2014-01-28
申请号：US13808240
申请日：2011-05-17
申请人： Poul Erik Højlund Nielsen , Burcin Temel , Pablo Beato
发明人： Poul Erik Højlund Nielsen , Burcin Temel , Pablo Beato
IPC分类号： C07C27/00
CPC分类号： C07C29/1516 , C07C29/1512 , C07C29/32 , C07C31/08 , C07C31/10 , C07C31/12 , C07C31/125
摘要： Process for the preparation of ethanol and/or higher alcohols comprising the steps of: (a) providing an alcohol synthesis gas comprising carbon monoxide and hydrogen in a molar ratio of higher than 0.5; (c) adding an amount of methanol and/or higher alcohols to the synthesis gas to obtain a synthesis gas mixture. (d) converting the synthesis gas mixture from step (c) in presence of one or more catalysts catalysing the conversion of the synthesis gas mixture into a ethanol and/or higher alcohols containing product; and (e) withdrawing the product from step (d), wherein the synthesis gas is purified by removing iron and nickel carbonyl compounds prior or after the addition methanol and/or higher alcohols to the synthesis gas and optionally (I) cooling the withdrawn product in step (e); and (g) contacting the cooled product with a hydrogenation catalyst.
摘要翻译：制备乙醇和/或高级醇的方法包括以下步骤：（a）提供摩尔比高于0.5的一氧化碳和氢气的醇合成气; （c）向合成气中加入一定量的甲醇和/或高级醇以得到合成气体混合物。（d）在催化合成气混合物转化为乙醇和/或高级醇的产物的一种或多种催化剂的存在下，转化来自步骤（c）的合成气混合物; 和（e）从步骤（d）中取出产物，其中通过在向合成气中加入甲醇和/或高级醇之前或之后除去铁和镍羰基化合物来纯化合成气，并且任选地（I）冷却所提取的产物在步骤（e）中; 和（g）使冷却的产物与氢化催化剂接触。

4. 发明申请

US20130225879A1 PROCESS FOR THE SELECTIVE PREPARATION OF 1-PROPANOL, ISO-BUTANOL AND OTHER C3+ ALCOHOLS FROM SYNTHESIS GAS AND METHANOL 审中-公开
标题翻译：从合成气和甲醇中选择性制备1-丙醇，ISO-丁醇和其他C 3+醇的方法
公开(公告)号：US20130225879A1
公开(公告)日：2013-08-29
申请号：US13883059
申请日：2010-11-08
申请人： Burcin Temel , Poul Erik Højlund Nielsen , Pablo Beato
发明人： Burcin Temel , Poul Erik Højlund Nielsen , Pablo Beato
IPC分类号： C07C29/32
CPC分类号： C07C29/32 , C07C31/08 , C07C31/10 , C07C31/12
摘要： Process for the preparation of a product alcohol mixture comprising the steps of: (a) providing a synthesis gas comprising carbon monoxide and hydrogen (b) providing an amount of methanol and a second source alcohol Rn—CH2—CH2—OH comprising n+2 carbon atoms (Rn═CnH2n+1, n≧O) to the synthesis gas to obtain a selective alcohol synthesis mixture (c) converting the selective synthesis mixture in presence of one or more catalysts catalysing the conversion of the synthesis gas mixture into a product alcohol mixture in which the initially dominating alcohol is a preferred Cn+3 alcohol having the structure Rn—CH(CH3)—CH2—OH (d) withdrawing the product alcohol mixture of step (c).
摘要翻译：制备产物醇混合物的方法，包括以下步骤：（a）提供包含一氧化碳和氢气的合成气（b）提供一定量的甲醇和包含n + 2的第二源醇Rn-CH2-CH2-OH 碳原子（Rn = CnH2n + 1，n> = 0），以获得选择性醇合成混合物（c）在一种或多种催化剂将催化合成气混合物转化为产物醇混合物，其中最初占优势的醇是具有结构Rn-CH（CH3）-CH2-OH（d）的优选C n + 3醇（d）取出步骤（c）的产物醇混合物。

5. 发明授权

US08765019B2 Process for the preparation of synthesis gas 有权
标题翻译：合成气的制备方法
公开(公告)号：US08765019B2
公开(公告)日：2014-07-01
申请号：US13701488
申请日：2011-05-13
申请人： Kim Aasberg-Petersen , Poul Erik Højlund Nielsen , Peter Seier Christensen , Charlotte Stub Nielsen , Burcin Temel
发明人： Kim Aasberg-Petersen , Poul Erik Højlund Nielsen , Peter Seier Christensen , Charlotte Stub Nielsen , Burcin Temel
IPC分类号： C01B3/48
CPC分类号： C01B3/48 , C01B3/16 , C01B3/36 , C01B3/382 , C01B3/386 , C01B2203/0244 , C01B2203/0255 , C01B2203/0261 , C01B2203/0283 , C01B2203/062 , C01B2203/1264 , C10G2/32 , C10G2300/1022 , C10G2300/807 , C10G2400/02
摘要： Process for the preparation of synthesis gas from an essentially dry hydrocarbon feedstock (1) comprising olefins, hydrogen and carbon monoxide, the process comprising the steps: (a) selectively hydrogenating the olefins in the hydrocarbon feedstock at a temperature between 60 to 190° C. (2) to obtain a hydrogenated hydrocarbon feedstock comprising hydrogen, carbon monoxide and saturated hydrocarbons (3; (b) adding steam (4) to the hydrogenated hydrocarbon feedstock; (c) performing a water gas shift reaction in the presence of steam on the hydrogenated hydrocarbon feedstock (6) to obtain a shifted, hydrogenated hydrocarbon mixture; (d) converting the shifted, hydrogenated hydrocarbon mixture (8) to obtain a synthesis gas.
摘要翻译：用于从包含烯烃，氢气和一氧化碳的基本上干的烃原料（1）制备合成气的方法，该方法包括以下步骤：（a）在60至190℃的温度下选择性氢化烃原料中的烯烃（2）获得包含氢气，一氧化碳和饱和烃的氢化烃原料（3;（b）向氢化烃原料中加入蒸汽（4）;（c）在蒸汽存在下进行水煤气变换反应氢化烃原料（6）以获得偏移的氢化烃混合物;（d）转化转移的氢化烃混合物（8）以获得合成气。

6. 发明申请

US20130123377A1 PROCESS FOR THE PREPARATION OF ETHANOL AND HIGHER ALCOHOLS 有权
标题翻译：制备乙醇和高级醇的方法
公开(公告)号：US20130123377A1
公开(公告)日：2013-05-16
申请号：US13808240
申请日：2011-05-17
申请人： Poul Erik Højlund Nielsen , Burcin Temel , Pablo Beato
发明人： Poul Erik Højlund Nielsen , Burcin Temel , Pablo Beato
IPC分类号： C07C29/151
CPC分类号： C07C29/1516 , C07C29/1512 , C07C29/32 , C07C31/08 , C07C31/10 , C07C31/12 , C07C31/125
摘要： Process for the preparation of ethanol and/or higher alcohols comprising the steps of: (a) providing an alcohol synthesis gas comprising carbon monoxide and hydrogen in a molar ratio of higher than 0.5; (c) adding an amount of methanol and/or higher alcohols to the synthesis gas to obtain a synthesis gas mixture. (d) converting the synthesis gas mixture from step (c) in presence of one or more catalysts catalysing the conversion of the synthesis gas mixture into a ethanol and/or higher alcohols containing product; and (e) withdrawing the product from step (d), wherein the synthesis gas is purified by removing iron and nickel carbonyl compounds prior or after the addition methanol and/or higher alcohols to the synthesis gas and optionally (I) cooling the withdrawn product in step (e); and (g) contacting the cooled product with a hydrogenation catalyst.
摘要翻译：制备乙醇和/或高级醇的方法包括以下步骤：（a）提供摩尔比高于0.5的一氧化碳和氢气的醇合成气; （c）向合成气中加入一定量的甲醇和/或高级醇以得到合成气体混合物。（d）在催化合成气混合物转化为乙醇和/或高级醇的产物的一种或多种催化剂的存在下，转化来自步骤（c）的合成气混合物; 和（e）从步骤（d）中取出产物，其中通过在向合成气中加入甲醇和/或高级醇之前或之后除去铁和镍羰基化合物来纯化合成气，并且任选地（I）冷却所提取的产物在步骤（e）中; 和（g）使冷却的产物与氢化催化剂接触。

7. 发明申请

US20130082211A1 PROCESS FOR THE PREPARATION OF SYNTHESIS GAS 有权
标题翻译：制备合成气的方法
公开(公告)号：US20130082211A1
公开(公告)日：2013-04-04
申请号：US13701488
申请日：2011-05-13
申请人： Kim Aasberg-Petersen , Poul Erik Højlund Nielsen , Peter Seier Christensen , Charlotte Stub Nielsen , Burcin Temel
发明人： Kim Aasberg-Petersen , Poul Erik Højlund Nielsen , Peter Seier Christensen , Charlotte Stub Nielsen , Burcin Temel
IPC分类号： C01B3/48
CPC分类号： C01B3/48 , C01B3/16 , C01B3/36 , C01B3/382 , C01B3/386 , C01B2203/0244 , C01B2203/0255 , C01B2203/0261 , C01B2203/0283 , C01B2203/062 , C01B2203/1264 , C10G2/32 , C10G2300/1022 , C10G2300/807 , C10G2400/02
摘要： Process for the preparation of synthesis gas from an essentially dry hydrocarbon feedstock (1) comprising olefins, hydrogen and carbon monoxide, the process comprising the steps: (a) selectively hydrogenating the olefins in the hydrocarbon feedstock at a temperature between 60 to 190° C. (2) to obtain a hydrogenated hydrocarbon feedstock comprising hydrogen, carbon monoxide and saturated hydrocarbons (3; (b) adding steam (4) to the hydrogenated hydrocarbon feedstock; (c) performing a water gas shift reaction in the presence of steam on the hydrogenated hydrocarbon feedstock (6) to obtain a shifted, hydrogenated hydrocarbon mixture; (d) converting the shifted, hydrogenated hydrocarbon mixture (8) to obtain a synthesis gas.
摘要翻译：用于从包含烯烃，氢气和一氧化碳的基本上干的烃原料（1）制备合成气的方法，该方法包括以下步骤：（a）在60至190℃的温度下选择性氢化烃原料中的烯烃（2）获得包含氢气，一氧化碳和饱和烃的氢化烃原料（3;（b）向氢化烃原料中加入蒸汽（4）;（c）在蒸汽存在下进行水煤气变换反应氢化烃原料（6）以获得偏移的氢化烃混合物;（d）转化转移的氢化烃混合物（8）以获得合成气。

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