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1. 发明授权

US07915341B2 Ethylene-vinyl alcohol copolymer and molded article thereof 有权
标题翻译：乙烯 - 乙烯醇共聚物及其模制品
公开(公告)号：US07915341B2
公开(公告)日：2011-03-29
申请号：US11629051
申请日：2004-12-17
申请人： Mitsuo Shibutani , Takamasa Moriyama , Kaoru Inoue , Shinta Miyazumi , Ikko Matsui
发明人： Mitsuo Shibutani , Takamasa Moriyama , Kaoru Inoue , Shinta Miyazumi , Ikko Matsui
IPC分类号： C08F16/06
CPC分类号： B32B27/36 , B32B27/08 , B32B27/306 , B32B2307/518 , B32B2307/7242 , B32B2439/60 , C08F8/12 , C08F210/02 , C08F216/04 , C08F218/08 , C08F2800/10 , Y10T428/13 , Y10T428/1352 , Y10T428/31786 , Y10T428/31797 , C08F218/12
摘要： An ethylene-vinyl alcohol copolymer and a molded article thereof are disclosed. The ethylene-vinyl alcohol copolymer has improved stretching properties and provides the molded article with excellent gas barrier properties, appearance and strength. The ethylene-vinyl alcohol copolymer comprises the structural unit of formula (1): (wherein X represents any binding chain excluding an ether bond, each of R1 to R4 represents independently any substituent and n represents 0 or 1.).
摘要翻译：公开了一种乙烯 - 乙烯醇共聚物及其模制品。乙烯 - 乙烯醇共聚物具有改善的拉伸性能，并提供具有优异的阻气性，外观和强度的模塑制品。乙烯 - 乙烯醇共聚物包含式（1）的结构单元：（其中X表示不包括醚键的任何结合链，每个R 1至R 4独立地表示任何取代基，n表示0或1）。

2. 发明申请

US20070178268A1 Ethylene-vinyl alcohol copolymer and molded article thereof 有权
标题翻译：乙烯 - 乙烯醇共聚物及其模制品
公开(公告)号：US20070178268A1
公开(公告)日：2007-08-02
申请号：US11629051
申请日：2004-12-17
申请人： Ikko Matsui , Shinta Miyazumi , Takamasa Moriyama , Mitsuo Shibutani , Kaoru Inoue
发明人： Ikko Matsui , Shinta Miyazumi , Takamasa Moriyama , Mitsuo Shibutani , Kaoru Inoue
IPC分类号： B32B27/08
CPC分类号： B32B27/36 , B32B27/08 , B32B27/306 , B32B2307/518 , B32B2307/7242 , B32B2439/60 , C08F8/12 , C08F210/02 , C08F216/04 , C08F218/08 , C08F2800/10 , Y10T428/13 , Y10T428/1352 , Y10T428/31786 , Y10T428/31797 , C08F218/12
摘要： An ethylene-vinyl alcohol copolymer and a molded article thereof are disclosed. The ethylene-vinyl alcohol copolymer has improved stretching properties and provides the molded article with excellent gas barrier properties, appearance and strength. The ethylene-vinyl alcohol copolymer comprises the structural unit of formula (1): (wherein X represents any binding chain excluding an ether bond, each of R1 to R4 represents independently any substituent and n represents 0 or 1.).
摘要翻译：公开了一种乙烯 - 乙烯醇共聚物及其模制品。乙烯 - 乙烯醇共聚物具有改善的拉伸性能，并提供具有优异的阻气性，外观和强度的模塑制品。乙烯 - 乙烯醇共聚物包含式（1）的结构单元：（其中X表示除醚键之外的任何结合链，R 1至R 4各自表示独立地任何取代基，n表示0或1）。

3. 发明授权

US5322877A Ternary resin composition and production thereof 失效
标题翻译：三元树脂组合物及其制备方法
公开(公告)号：US5322877A
公开(公告)日：1994-06-21
申请号：US029408
申请日：1993-03-10
申请人： Takamasa Moriyama , Hiroki Masumoto , Kiniyasu Kato , Mitsuo Shibutani
发明人： Takamasa Moriyama , Hiroki Masumoto , Kiniyasu Kato , Mitsuo Shibutani
IPC分类号： C08J5/18 , C08K5/09 , C08L23/02 , C08L23/08 , C08L23/26 , C08L29/04 , C08L51/06
CPC分类号： C08L29/04 , B29C47/0877 , C08L51/06 , B29C47/0021 , C08L2205/08 , C08L23/02 , C08L23/08
摘要： A resin composition including (A) a saponified ethylene-vinyl acetate copolymer having an ethylene content of 20 to 60 mole percent and a saponification degree of not less than 90 mole percent, (B) a polyolefin resin, (C) a carboxylic acid-modified polyolefin resin and (D) a lower fatty acid alkaline earth metal salt, characterized in:that the proportion of (A) relative to the total amount of (A) plus (B) plus (C) is 0.3 to 0.7 on the weight basis;that the composition contains the carbonyl group in an amount of 0.002 to 0.05 equivalent per 100 grams of the total of (B) plus (C); andthat the equivalent ratio between (D) and the carbonyl group in (C) is 0.5 to 5,and a method of producing the resin composition are provided.
摘要翻译：一种树脂组合物，其包含（A）乙烯含量为20〜60摩尔％，皂化度为90摩尔％以上的皂化乙烯 - 乙酸乙烯酯共聚物，（B）聚烯烃树脂，（C）改性聚烯烃树脂和（D）低级脂肪酸碱土金属盐，其特征在于（A）相对于（A）加（B）加（C）的总量的比例为0.3〜0.7 基础; 该组合物含有每100克（B）加（C）总计0.002至0.05当量的羰基; （D）和（C）中的羰基的当量比为0.5〜5，提供了树脂组合物的制造方法。

4. 发明申请

US20130131270A1 RESIN COMPOSITION AND MOLDED ARTICLE THEREOF 有权
标题翻译：树脂组合物及其成型品
公开(公告)号：US20130131270A1
公开(公告)日：2013-05-23
申请号：US13813046
申请日：2011-07-28
申请人： Mitsuo Shibutani , Kaoru Inoue , Norihito Sakai
发明人： Mitsuo Shibutani , Kaoru Inoue , Norihito Sakai
IPC分类号： C08L29/04
CPC分类号： C08L29/04 , C08L51/08 , C08L53/02 , C08L2205/03 , C08L53/025 , C08L87/005 , C08L77/00
摘要： There is provided a resin composition affording a melt-molded article having excellent gas barrier properties and flex crack resistance. The present invention relates to a resin composition comprising a polyvinyl alcohol resin (A) having a 1,2-diol structural unit represented by the following general formula (1), a styrene-based thermoplastic elastomer (B), and a polyamide graft block copolymer (C) containing a polymer block of an aromatic vinyl compound and a polymer block of an olefinic compound in a main chain and having a graft chain composed of a polyamide: wherein each of R1, R2, and R3 independently represents a hydrogen atom or an organic group, X represents a single bond or a linking chain, and each of R4, R5, and R6 independently represents a hydrogen atom or an organic group.
摘要翻译：提供了提供具有优异的阻气性和抗开裂性的熔融模制品的树脂组合物。本发明涉及一种树脂组合物，其包含具有由以下通式（1）表示的1,2-二醇结构单元的聚乙烯醇树脂（A），苯乙烯类热塑性弹性体（B）和聚酰胺接枝嵌段共聚物（C），其包含芳族乙烯基化合物的聚合物嵌段和主链中的烯属化合物的聚合物嵌段，并且具有由聚酰胺构成的接枝链：其中R 1，R 2和R 3各自独立地表示氢原子或有机基团，X表示单键或连接链，R 4，R 5和R 6各自独立地表示氢原子或有机基团。

5. 发明授权

US09109104B2 Resin composition and molded article thereof 有权
标题翻译：树脂组合物及其成型品
公开(公告)号：US09109104B2
公开(公告)日：2015-08-18
申请号：US13813046
申请日：2011-07-28
申请人： Mitsuo Shibutani , Kaoru Inoue , Norihito Sakai
发明人： Mitsuo Shibutani , Kaoru Inoue , Norihito Sakai
IPC分类号： C08L29/02 , C08L29/04 , C08L53/00 , C08L53/02 , C08L51/08
CPC分类号： C08L29/04 , C08L51/08 , C08L53/02 , C08L2205/03 , C08L53/025 , C08L87/005 , C08L77/00
摘要： There is provided a resin composition affording a melt-molded article having excellent gas barrier properties and flex crack resistance. The present invention relates to a resin composition comprising a polyvinyl alcohol resin (A) having a 1,2-diol structural unit represented by the following general formula (1), a styrene-based thermoplastic elastomer (B), and a polyamide graft block copolymer (C) containing a polymer block of an aromatic vinyl compound and a polymer block of an olefinic compound in a main chain and having a graft chain composed of a polyamide: wherein each of R1, R2, and R3 independently represents a hydrogen atom or an organic group, X represents a single bond or a linking chain, and each of R4, R5, and R6 independently represents a hydrogen atom or an organic group.
摘要翻译：提供了提供具有优异的阻气性和抗开裂性的熔融模制品的树脂组合物。本发明涉及一种树脂组合物，其包含具有由以下通式（1）表示的1,2-二醇结构单元的聚乙烯醇树脂（A），苯乙烯类热塑性弹性体（B）和聚酰胺接枝嵌段共聚物（C），其包含芳族乙烯基化合物的聚合物嵌段和主链中的烯属化合物的聚合物嵌段，并且具有由聚酰胺构成的接枝链：其中R 1，R 2和R 3各自独立地表示氢原子或有机基团，X表示单键或连接链，R 4，R 5和R 6各自独立地表示氢原子或有机基团。

6. 发明申请

US20120156513A1 MULTILAYER STRUCTURE 审中-公开
标题翻译：多层结构
公开(公告)号：US20120156513A1
公开(公告)日：2012-06-21
申请号：US13392743
申请日：2010-08-18
申请人： Masayuki Kawabe , Mitsuo Shibutani , Kaoru Inoue , Norihito Sakai
发明人： Masayuki Kawabe , Mitsuo Shibutani , Kaoru Inoue , Norihito Sakai
IPC分类号： B32B27/08
CPC分类号： B32B27/08 , B32B27/18 , B32B27/285 , B32B27/306 , B32B27/36 , B32B2250/42 , B32B2307/50 , B32B2307/7166 , B32B2307/748 , B32B2439/00 , B32B2439/70 , B32B2439/80 , B32B2553/00 , Y10T428/31797
摘要： A multilayer structure includes (A) a layer consisting primarily of a polyethylene terephthalate resin which includes a dicarboxylic acid component unit including terephthalic acid and a diol component unit primarily including ethylene glycol, the dicarboxylic acid component including a non-terephthalic-acid dicarboxylic acid in a copolymerization ratio of 15 to 40 mol % based on the overall amount of the dicarboxylic acid component; and (B) a layer provided in stacked adjacent relation to the layer (A) and consisting primarily of a polyvinyl alcohol resin having a structural unit represented by the following general formula (1):
摘要翻译：多层结构体包括（A）主要由聚对苯二甲酸乙二醇酯树脂组成的层，该层包括主要包含乙二醇的二羧酸成分单元和主要包含乙二醇的二醇成分单元，二羧酸成分含有非对苯二甲酸二羧酸基于二羧酸成分的总量的共聚比为15〜40摩尔％和（B）与层（A）堆叠相邻的层并且主要由具有由以下通式（1）表示的结构单元的聚乙烯醇树脂组成的层：

7. 发明申请

US20120041118A1 POLYVINYL ALCOHOL-BASED RESIN COMPOSITION 有权
标题翻译：聚乙烯醇基树脂组合物
公开(公告)号：US20120041118A1
公开(公告)日：2012-02-16
申请号：US13266546
申请日：2010-04-27
申请人： Mitsuo Shibutani , Kaoru Inoue , Yuichi Takahashi
发明人： Mitsuo Shibutani , Kaoru Inoue , Yuichi Takahashi
IPC分类号： C08K5/09
CPC分类号： C08J5/18 , C08F216/02 , C08J2329/04 , C08K5/098 , C08L29/04
摘要： The present invention provides a polyvinyl alcohol-based resin (PVOH-based resin) composition having less coloration from melt processing and having high aging stability of the melt viscosity. The present invention relates to a polyvinyl alcohol-based resin composition comprising a polyvinyl alcohol-based rein having a structural unit represented by the following formula (1) and having an absorbance of 0.1 to 0.3 of 280 nm in an ultraviolet absorbance spectrum as a 4 mass % aqueous solution, a carboxylic acid and an alkaline (earth) metal salt, wherein when an aqueous solution of the polyvinyl alcohol-based resin composition is prepared so as to have a content of the polyvinyl alcohol-based resin of 4 mass %, the pH of the aqueous solution at 20° C. is from 5.5 to 7: [wherein R1, R2 and R3 independently represent a hydrogen atom or an organic group, X represents a single bond or a bonding chain, and R4, R5 and R6 independently represent a hydrogen atom or an organic group].
摘要翻译：本发明提供一种熔融加工着色少，熔融粘度老化稳定性高的聚乙烯醇系树脂（PVOH系树脂）组合物。本发明涉及一种聚乙烯醇类树脂组合物，其包含具有由下式（1）表示的结构单元并且在紫外吸收光谱中具有280nm的吸光度为0.1至0.3的吸光度为4的聚乙烯醇系树脂作为4 质量％水溶液，羧酸和碱土金属盐，其中当制备聚乙烯醇类树脂组合物的水溶液以使聚乙烯醇类树脂的含量为4质量％时， 20℃时的水溶液的pH为5.5〜7 [式中，R 1，R 2和R 3独立地表示氢原子或有机基团，X表示单键或键合链，R4，R5，R6 独立地表示氢原子或有机基团]。

8. 发明授权

US08569414B2 Polyvinyl alcohol resin composition and molded article thereof 有权
标题翻译：聚乙烯醇树脂组合物及其模制品
公开(公告)号：US08569414B2
公开(公告)日：2013-10-29
申请号：US13407278
申请日：2012-02-28
申请人： Mitsuo Shibutani , Kazutoshi Tsuji , Kaoru Inoue , Norihito Sakai
发明人： Mitsuo Shibutani , Kazutoshi Tsuji , Kaoru Inoue , Norihito Sakai
IPC分类号： C08G63/48 , C08L29/04
CPC分类号： C08L29/04 , C08L53/02 , C08L53/025 , C08L2205/02 , C08L2205/03
摘要： Disclosed is a polyvinyl alcohol resin composition capable of providing a melt-molded article with superior gas barrier properties and flex crack resistance. The resin composition comprises (A) a PVA resin having 1,2-diol unit in side chain thereof; and (B) a mixture of block copolymers each having an aromatic vinyl polymer block, and a conjugated diene polymer block and/or hydrogenated thereof, wherein the (B) mixture of block copolymers includes (B1) a block copolymer having no carboxyl group and (B2) a block copolymer modified with a carboxyl group-containing compound.
摘要翻译：公开了一种聚乙烯醇树脂组合物，其能够提供具有优异的阻气性和抗起裂性的熔融模制品。树脂组合物包含（A）其侧链上具有1,2-二醇单元的PVA树脂; 和（B）各自具有芳族乙烯基聚合物嵌段和共轭二烯聚合物嵌段和/或氢化的嵌段共聚物的混合物，其中嵌段共聚物的（B）混合物包括（B1）不具有羧基的嵌段共聚物和（B2）用含羧基的化合物改性的嵌段共聚物。

9. 发明授权

US08722782B2 Polyvinyl alcohol-based resin composition 有权
标题翻译：聚乙烯醇类树脂组合物
公开(公告)号：US08722782B2
公开(公告)日：2014-05-13
申请号：US13266546
申请日：2010-04-27
申请人： Mitsuo Shibutani , Kaoru Inoue , Yuichi Takahashi
发明人： Mitsuo Shibutani , Kaoru Inoue , Yuichi Takahashi
IPC分类号： C08K5/04 , C08K5/00
CPC分类号： C08J5/18 , C08F216/02 , C08J2329/04 , C08K5/098 , C08L29/04
摘要： The present invention provides a polyvinyl alcohol-based resin composition having less coloration from melt processing and having high aging stability of the melt viscosity comprising a polyvinyl alcohol-based rein having a structural unit represented by the following formula (1) and having an absorbance of 0.1 to 0.3 of 280 nm in an ultraviolet absorbance spectrum as a 4 mass % aqueous solution, a carboxylic acid and an alkaline (earth) metal salt, wherein when an aqueous solution of the polyvinyl alcohol-based resin composition is prepared so as to have a content of the polyvinyl alcohol-based resin of 4 mass %, the pH of the aqueous solution at 20° C. is from 5.5 to 7: wherein R1, R2 and R3 independently represent a hydrogen atom or an organic group, X represents a single bond or a bonding chain, and R4, R5 and R6 independently represent a hydrogen atom or an organic group.
摘要翻译：本发明提供一种聚乙烯醇类树脂组合物，其熔融加工着色度较低，熔融粘度的老化稳定性高，具有下述式（1）表示的结构单元的聚乙烯醇系树脂，其吸光度为作为4质量％水溶液，羧酸和碱土金属盐的紫外吸收光谱中的280nm的0.1〜0.3，其中，当制备聚乙烯醇系树脂组合物的水溶液以具有聚乙烯醇系树脂的含量为4质量％，水溶液在20℃下的pH为5.5〜7，式中R1，R2和R3独立地表示氢原子或有机基团，X表示单键或键合链，R4，R5和R6独立地表示氢原子或有机基团。

10. 发明申请

US20140107275A1 COATING AGENT COMPOSITION FOR BATTERY ELECTRODE OR SEPARATOR 审中-公开
标题翻译：电池电极或分离器用涂料组合物
公开(公告)号：US20140107275A1
公开(公告)日：2014-04-17
申请号：US14123486
申请日：2012-05-31
申请人： Taichi Uemura , Satoshi Yamazaki , Mitsuo Shibutani , Kazuo Aiba
发明人： Taichi Uemura , Satoshi Yamazaki , Mitsuo Shibutani , Kazuo Aiba
IPC分类号： H01M4/62
CPC分类号： H01M4/62 , C09D5/022 , C09D5/027 , C09D133/04 , C09D133/12 , C09D151/00 , C09D153/00 , H01M2/145 , H01M2/1653 , H01M2/166 , H01M2/1686 , H01M4/0409 , H01M4/366 , H01M4/628 , H01M10/0525 , H01M10/4235 , H01M2220/20 , H01M2220/30 , C09D129/04 , C08L53/02 , C08L29/04
摘要： A coating agent composition for battery electrode or separator, comprises a vinyl alcohol copolymer having a structural unit represented by the general formula (1), and an aqueous emulsion of a synthetic resin obtained by polymerizing a copolymerizable monomer having an acrylic monomer as a main component, or an aqueous emulsion of a styrene thermoplastic elastomer.
摘要翻译：用于电池电极或隔膜的涂料组合物包括具有由通式（1）表示的结构单元的乙烯醇共聚物和通过聚合具有丙烯酸类单体作为主要成分的可共聚单体得到的合成树脂的水性乳液，或苯乙烯热塑性弹性体的水性乳液。

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