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1. 发明授权

US07658837B2 Process and device to optimize the yield of fluid catalytic cracking products 有权
标题翻译：流化床装置优化流化床催化裂化产物的产率
公开(公告)号：US07658837B2
公开(公告)日：2010-02-09
申请号：US11190863
申请日：2005-07-28
申请人： Henrique Soares Cerqueira , Claudia Maria de Lacerda Alvarenga Baptista , William Richard Gilbert , Oscar Rene Chamberlain Pravia
发明人： Henrique Soares Cerqueira , Claudia Maria de Lacerda Alvarenga Baptista , William Richard Gilbert , Oscar Rene Chamberlain Pravia
IPC分类号： C10G11/00 , B01J8/18
CPC分类号： B01J8/0055 , B01J8/1818 , B01J8/1872 , B01J2208/00707 , C10G11/182
摘要： A process and device to optimize the yield of fluid catalytic cracking products through a reactive stripping process are disclosed. One or more hydrocarbon streams (3) are introduced in an intermediary region of the stripper (1) of a fluid catalytic cracking unit (FCC), from a device that allows a homogeneous distribution with adequate dispersion. This/these stream(s) react(s) with the catalyst of FCC, although its activity is reduced due to the adsorption of hydrocarbons in the reaction zone, generating products that improve and/or change the global distribution of products, providing a refinery profile adequate to meet quality demands and requirements.
摘要翻译：公开了通过反应性汽提过程来优化流化催化裂化产物的产率的方法和装置。一种或多种烃流（3）从允许均匀分布且具有适当分散体的装置引入流化催化裂化装置（FCC）的汽提器（1）的中间区域。这些/这些流与FCC的催化剂反应，尽管其活性由于在反应区中的烃的吸附而减少，产生改善和/或改变产品的全球分布的产品，提供炼油厂外形足以满足质量要求和要求。

2. 发明授权

US07736491B2 Process for the fluid catalytic cracking of mixed feedstocks of hydrocarbons from different sources 有权
标题翻译：来自不同来源的烃混合原料流化催化裂化的方法
公开(公告)号：US07736491B2
公开(公告)日：2010-06-15
申请号：US10559528
申请日：2004-05-19
申请人： Claudia Maria de Lacerda Alvarenga Baptista , Henrique Soares Cerqueira , Emanuel Freire Sandes
发明人： Claudia Maria de Lacerda Alvarenga Baptista , Henrique Soares Cerqueira , Emanuel Freire Sandes
IPC分类号： C10G11/00 , C10G51/06 , C10G35/04 , F27B15/08 , B01J8/08
CPC分类号： C10G11/18 , C10G2400/28
摘要： A process for the fluid catalytic cracking of mixed hydrocarbon feeds from different sources is described, such as feeds A and B of different crackability, the process being especially directed to obtaining light fractions such as LPG and comprising injecting feed A in the base of the riser reactive section and feed B, of lower crackability, at a height between 10% and 80% of the riser, with feed B comprising between 5% and 50% of the total processed feed. The process requires that the feeds present differences in the contaminant content, improved dispersion of feeds A and B and feed B injection temperature same or higher than that of feed A.
摘要翻译：描述了用于来自不同来源的混合烃进料的流化催化裂化的方法，例如不同裂化性的进料A和B，该方法特别涉及获得轻馏分如LPG，并且包括将提取物A的基料中注入进料A 反应段和进料B在提升管的10％至80％之间的高度处具有较低的可裂性，进料B占加工进料总量的5％至50％。该方法要求进料存在污染物含量的差异，改善进料A和B的分散性，并将B进料温度与进料A相同或更高。

3. 发明授权

US08128806B2 Process and equipment for fluid catalytic cracking for the production of middle distillates of low aromaticity 有权
标题翻译：用于生产低芳烃中间馏分的流化催化裂化工艺和设备
公开(公告)号：US08128806B2
公开(公告)日：2012-03-06
申请号：US12358462
申请日：2009-01-23
申请人： Claudia Maria de Lacerda Alvarenga Baptista , Edisson Morgado Junior , William Richard Gilbert
发明人： Claudia Maria de Lacerda Alvarenga Baptista , Edisson Morgado Junior , William Richard Gilbert
IPC分类号： C10G11/04
CPC分类号： C10G11/18 , C10G11/02 , C10G11/04 , C10G2400/04
摘要： The present invention relates to a process and equipment for fluid catalytic cracking for the production of middle distillates of low aromaticity that comprises cracking a mixed feed consisting of heavy fractions of hydrocarbons, in the absence of added hydrogen and employing a catalyst of low activity and low acidity, in a dense-bed FCC reactor to produce an effluent constituted of fractions of middle distillates and naphtha of low aromaticity.
摘要翻译：本发明涉及一种用于生产低芳性中间馏分的流化催化裂化方法和设备，包括在没有加入氢气的情况下，裂解由重馏分的烃组成的混合进料，并使用低活性和低的催化剂酸性，在密床FCC反应器中，产生由中等馏出物和低芳烃度的石脑油组成的流出物。

4. 发明授权

US08088274B2 Process for catalytic cracking of petroleum hydrocarbons in a fluidized bed with maximized production of light olefins 有权
标题翻译：在最大限度地生产轻质烯烃的流化床中对石油烃进行催化裂化的方法
公开(公告)号：US08088274B2
公开(公告)日：2012-01-03
申请号：US11957949
申请日：2007-12-17
申请人： William Richard Gilbert , Emanuel Freire Sandes , Andrea de Rezende Pinho , Claudia Maria de Lacerda Alvarenga Baptista
发明人： William Richard Gilbert , Emanuel Freire Sandes , Andrea de Rezende Pinho , Claudia Maria de Lacerda Alvarenga Baptista
IPC分类号： C10G11/18
CPC分类号： C10G11/18 , C10G2300/1044 , C10G2300/1055 , C10G2300/107 , C10G2300/4081 , C10G2300/805 , C10G2400/20
摘要： A process is described for catalytic cracking of hydrocarbon feedstocks from petroleum refining which increases substantially the yields of light olefins. The process limits the extreme conditions to a first reaction section and introduces a stream of cooling fluid above the feedstock injection point so as to maintain a second reaction section under cracking conditions which produce light olefins propene and ethene, and inhibits reactions undesirable for the process.
摘要翻译：描述了从石油精炼催化裂化烃原料的方法，其大大提高了轻质烯烃的产率。该方法将极端条件限制到第一反应段，并将冷却流体流引入原料注入点上方，以便在产生轻质烯烃丙烯和乙烯的裂化条件下保持第二反应段，并抑制对该方法不期望的反应。

5. 发明申请

US20080179219A1 PROCESS FOR CATALYTIC CRACKING OF PETROLEUM HYDROCARBONS IN A FLUIDIZED BED WITH MAXIMIZED PRODUCTION OF LIGHT OLEFINS 有权
标题翻译：在最大限度生产光油的流化床中催化裂化石油醚的方法
公开(公告)号：US20080179219A1
公开(公告)日：2008-07-31
申请号：US11957949
申请日：2007-12-17
申请人： William Richard GILBERT , Emanuel Freire Sandes , Andrea de Rezende Pinho , Claudia Maria de Lacerda Alvarenga Baptista
发明人： William Richard GILBERT , Emanuel Freire Sandes , Andrea de Rezende Pinho , Claudia Maria de Lacerda Alvarenga Baptista
IPC分类号： C10G11/05 , C10G11/00
CPC分类号： C10G11/18 , C10G2300/1044 , C10G2300/1055 , C10G2300/107 , C10G2300/4081 , C10G2300/805 , C10G2400/20
摘要： A process is described for catalytic cracking of hydrocarbon feedstocks from petroleum refining which increases substantially the yields of light olefins. The process limits the extreme conditions to a first reaction section and introduces a stream of cooling fluid above the feedstock injection point so as to maintain a second reaction section under cracking conditions which produce light olefins propene and ethene, and inhibits reactions undesirable for the process.
摘要翻译：描述了从石油精炼催化裂化烃原料的方法，其大大提高了轻质烯烃的产率。该方法将极端条件限制到第一反应段，并将冷却流体流引入原料注入点上方，以便在产生轻质烯烃丙烯和乙烯的裂化条件下保持第二反应段，并抑制对该方法不期望的反应。

6. 发明申请

US20070095724A1 FCC process for the maximization of medium distillates 审中-公开
标题翻译： FCC工艺可以使中等馏出物达到最大化
公开(公告)号：US20070095724A1
公开(公告)日：2007-05-03
申请号：US11545443
申请日：2006-10-11
申请人： Claudia Maria de Lacerda Alvarenga Baptista , William Richard Gilbert
发明人： Claudia Maria de Lacerda Alvarenga Baptista , William Richard Gilbert
IPC分类号： C10G11/00
CPC分类号： C10G11/18
摘要： A FCC process for the maximization of medium distillates from feedstocks of different sources, by the contact of the feedstock which circulates in a riser reactor together with a fine particulate catalyst from a regenerator (6), under FCC conditions of maximum LCO, at temperatures between about 480° C. and about 520° C., in the absence of added hydrogen, and with injection of coolant or quench to a riser ascendant R, and where the process consists of the injection of a coolant proportion between about 200 and about 50 kg/m3 of feedstock, preferably between about 100 and about 50 kg/m3 of feedstock, in a zone (3) of the riser ascendant R in a position located between about 25% and about 50% of the height of said riser R above the feedstock inlet mouths (2), the injection in this position resulting in the increase of the catalyst circulation and the temperature increase in the starting segment of the riser, yielding the production of medium distillates with low aromatic compounds content and bottoms conversion lower than when the coolant injection is employed in the base of the riser R as it is handled in the prior art processes.
摘要翻译： FCC方法，通过在最高LCO的FCC条件下，通过在提升管反应器中循环的原料与来自再生器（6）的细颗粒催化剂的原料的接触在不同来源的原料中最大化中间馏分，约480℃和约520℃，在没有加入氢气的情况下，并且注入冷却剂或骤冷至提升管上升R，并且其中该方法包括注入冷却剂比例为约200至约50 kg / m 3的原料，优选在约100至约50kg / m 3原料之间，在提升器上升R的区域（3）中位于在原料入口（2）上方的所述提升管R的高度的约25％至约50％之间，在该位置的注入导致催化剂循环的增加和提升管的起始段中的温度升高，产生中间馏分的生产低芳族化合物含量和底部转化率比在现有技术方法处理时在提升管R的基底中使用冷却剂注入时低。

7. 发明授权

US07691768B2 Additive to maximize GLP and propene suitable for use in low-severity operations of a fluid catalytic cracking unit and its preparatory process 有权
标题翻译：最大化GLP和丙烯的添加剂，适用于流化催化裂化装置的低强度操作及其制备过程
公开(公告)号：US07691768B2
公开(公告)日：2010-04-06
申请号：US11714117
申请日：2007-03-06
申请人： Lam Yiu Lau , Raquel Bastiani , Claudia Maria de Lacerda Alvarenga Baptista
发明人： Lam Yiu Lau , Raquel Bastiani , Claudia Maria de Lacerda Alvarenga Baptista
IPC分类号： B01J29/06
CPC分类号： B01J29/405 , B01J37/0045 , B01J37/06 , B01J37/08 , B01J2229/20 , B01J2229/40 , B01J2229/42 , C10G11/05 , C10G11/18
摘要： A process for the preparation and modification of additives, with a zeolite base and a high silica alumina ratio (SAR) like the ZSM-5, to increase the yield of propene and LPG in low severity FCC operations, that seeks to maximize the production of medium-distillates with low aromaticity and to minimize molecular cracking in the LCO range. The additives involved guarantee an increase in light olefin yields without altering the yield or the quality of the LCO produced. The innovative process includes surprising actions from rare earths (RE) on the active sites of zeolite, that at once partially block their pores and, in this way, make molecular cracking in the medium-distillate range difficult, which preferably occur at low reaction temperatures and keeps the remaining sites quite active. These sites are sufficiently active to crack smaller molecules in the gasoline range, guaranteeing an overall increase in light olefins and allowing the additive involved to be used industrially in operations to maximize medium-distillates in an FCC unit. This new additive may be obtained by modifying any commercial ZSM-5 zeolite additive.
摘要翻译：一种用于制备和改性添加剂的方法，具有沸石基质和高ZSM-5的高二氧化硅氧化铝比（SAR），以提高低浓度FCC操作中丙烯和LPG的产率，从而最大限度地提高生产具有低芳香度的中等馏出物，并使LCO范围内的分子裂解最小化。所涉及的添加剂保证轻烯烃产量的增加，而不改变生产的LCO的产率或质量。创新的方法包括来自稀土（RE）对沸石活性位点的惊人的作用，其一度部分阻断其孔，并且以这种方式使中等馏出物范围内的分子裂解困难，优选在低反应温度下发生并保持其余的网站相当活跃。这些位点具有足够的活性以在汽油范围内裂解较小的分子，保证轻质烯烃的总体增加，并允许所涉及的添加剂在工业上用于FCC装置中的中等馏出物的最大化。这种新添加剂可以通过改变任何商业的ZSM-5沸石添加剂来获得。

8. 发明申请

US20080015105A1 Additive to maximize GLP and propene suitable for use in low-severity operations of a fluid catalytic cracking unit and its preparatory process 有权
标题翻译：最大化GLP和丙烯的添加剂，适用于流化催化裂化装置的低强度操作及其制备过程
公开(公告)号：US20080015105A1
公开(公告)日：2008-01-17
申请号：US11714117
申请日：2007-03-06
申请人： Lam Yiu Lau , Raquel Bastiani , Claudia Maria de Lacerda Alvarenga Baptista
发明人： Lam Yiu Lau , Raquel Bastiani , Claudia Maria de Lacerda Alvarenga Baptista
IPC分类号： B01J29/04
CPC分类号： B01J29/405 , B01J37/0045 , B01J37/06 , B01J37/08 , B01J2229/20 , B01J2229/40 , B01J2229/42 , C10G11/05 , C10G11/18
摘要： A process for the preparation and modification of additives, with a zeolite base and a high silica alumina ratio (SAR) like the ZSM-5, to increase the yield of propene and LPG in low severity FCC operations, that seeks to maximize the production of medium-distillates with low aromaticity and to minimize molecular cracking in the LCO range. The additives involved guarantee an increase in light olefin yields without altering the yield or the quality of the LCO produced. The innovative process includes surprising actions from rare earths (RE) on the active sites of zeolite, that at once partially block their pores and, in this way, make molecular cracking in the medium-distillate range difficult, which preferably occur at low reaction temperatures and keeps the remaining sites quite active. These sites are sufficiently active to crack smaller molecules in the gasoline range, guaranteeing an overall increase in light olefins and allowing the additive involved to be used industrially in operations to maximize medium-distillates in an FCC unit. This new additive may be obtained by modifying any commercial ZSM-5 zeolite additive.
摘要翻译：一种用于制备和改性添加剂的方法，具有沸石基质和高ZSM-5的高二氧化硅氧化铝比（SAR），以提高低浓度FCC操作中丙烯和LPG的产率，从而最大限度地提高生产具有低芳香度的中等馏出物，并使LCO范围内的分子裂解最小化。所涉及的添加剂保证轻烯烃产量的增加，而不改变生产的LCO的产率或质量。创新的方法包括来自稀土（RE）对沸石活性位点的惊人的作用，其一度部分阻断其孔，并且以这种方式使中等馏出物范围内的分子裂解困难，优选在低反应温度下发生并保持其余的网站相当活跃。这些位点具有足够的活性以在汽油范围内裂解较小的分子，保证轻质烯烃的总体增加，并允许所涉及的添加剂在工业上用于FCC装置中的中等馏出物的最大化。这种新添加剂可以通过改变任何商业的ZSM-5沸石添加剂来获得。

9. 发明申请

US20090107885A1 CATALYTIC SYSTEM AND ADDITIVE FOR MAXIMISATION OF LIGHT OLEFINS IN FLUID CATALYTIC CRACKING UNITS IN OPERATIONS OF LOW SEVERITY 审中-公开
标题翻译：催化体系和添加剂在液体催化裂化装置中在低严重运行中最大化烯烃
公开(公告)号：US20090107885A1
公开(公告)日：2009-04-30
申请号：US12260181
申请日：2008-10-29
申请人： Raquel Bastiani , Lam Yiu Lam , Claudia Maria de Lacerda Alvarenga Baptista
发明人： Raquel Bastiani , Lam Yiu Lam , Claudia Maria de Lacerda Alvarenga Baptista
IPC分类号： C10G11/00 , B01J8/18 , C01B39/02 , B01J29/06
CPC分类号： C10G11/05 , B01J29/40 , B01J29/65 , B01J29/80 , C10G11/18
摘要： The present invention concerns the field of fluid catalytic cracking (FCC) processes. The invention provides a process increasing production of LPG and propene in FCC units operating under conditions of maximisation of middle distillates of low aromaticity, such that they may be incorporated into the diesel oil pool. The invention also relates to the preparation and employment of additives based on zeolites having small pores, such as ferrierite (FER), in catalytic systems for FCC units, wherein conditions of low severity are adopted with a view to increasing yields of LPG and light olefins whilst improving stability of petrol. The invention also provides an original catalytic system, being more efficient than catalytic systems known in the state of the art, to increase the yield of LPG and propene without prejudicing the yield and quality of LCO. Furthermore it provides a method of preparation of an additive for said process employing the zeolite ferrierite.
摘要翻译：本发明涉及流化催化裂化（FCC）方法领域。本发明提供一种加工生产液化石油气和丙烯的方法，其中FCC装置在低芳烃中间馏分最大化的条件下运行，使得它们可以并入柴油池中。本发明还涉及在FCC单元的催化体系中制备和使用基于具有小孔的沸石的添加剂，例如镁碱沸石（FER），其中采用低严重性的条件以提高LPG和轻质烯烃的产率同时提高汽油的稳定性。本发明还提供了比现有技术中已知的催化体系更有效的原始催化体系，以增加LPG和丙烯的产率而不损害LCO的产率和质量。此外，它提供了使用沸石镁碱沸石的所述方法的添加剂的制备方法。

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