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1. 发明授权

US06184173B2 Multimetal oxides 失效
标题翻译：多金属氧化物
公开(公告)号：US06184173B2
公开(公告)日：2001-02-06
申请号：US09492226
申请日：2000-01-27
申请人： Hartmut Hibst , Andreas Tenten , Laszlo Marosi
发明人： Hartmut Hibst , Andreas Tenten , Laszlo Marosi
IPC分类号： B01J2300
CPC分类号： C07C51/252 , B01J23/002 , B01J23/28 , B01J23/30 , B01J23/8877 , B01J23/888 , B01J23/8885 , B01J35/0006 , B01J2523/00 , C07C45/33 , C07C45/34 , C07C45/35 , C07C45/38 , C07C51/235 , C07C47/22 , B01J2523/55 , B01J2523/68 , B01J2523/17 , B01J2523/69 , C07C57/04
摘要： Multimetal oxides containing Mo, V and at least one of the elements W, Nb, Ti, Zr, Hf, Ta, Cr, Si and Ge and having a special three-dimensional atomic arrangement are used in catalysts for the catalytic gas-phase oxidation of organic compounds.
摘要翻译：含有Mo，V和元素W，Nb，Ti，Zr，Hf，Ta，Cr，Si和Ge中的至少一种的具有特殊三维原子排列的多金属氧化物用于催化气相氧化催化剂的有机化合物。

2. 发明授权

US5807531A Multimetal oxides 失效
标题翻译：多金属氧化物
公开(公告)号：US5807531A
公开(公告)日：1998-09-15
申请号：US744246
申请日：1996-11-05
申请人： Hartmut Hibst , Andreas Tenten , Laszlo Marosi
发明人： Hartmut Hibst , Andreas Tenten , Laszlo Marosi
IPC分类号： C01G1/00 , B01J23/00 , B01J23/20 , B01J23/28 , B01J23/30 , B01J23/88 , B01J23/887 , B01J23/888 , B01J35/00 , C01G31/00 , C01G39/00 , C01G41/00 , C07B61/00 , C07C45/33 , C07C45/34 , C07C45/35 , C07C45/38 , C07C51/235 , C07C51/25 , C07C57/05 , C07C57/055 , C04B35/495 , C01G31/02 , C01G39/02
CPC分类号： C07C51/252 , B01J23/002 , B01J23/28 , B01J23/30 , B01J23/8877 , B01J23/888 , B01J23/8885 , B01J35/0006 , C07C45/33 , C07C45/34 , C07C45/35 , C07C45/38 , C07C51/235 , B01J2523/00
摘要： Multimetal oxides containing Mo, V and at least one of the elements W, Nb, Ti, Zr, Hf, Ta, Cr, Si and Ge and having a special three-dimensional atomic arrangement are used in catalysts for the catalytic gas-phase oxidation of organic compounds.
摘要翻译：含有Mo，V和元素W，Nb，Ti，Zr，Hf，Ta，Cr，Si和Ge中的至少一种的具有特殊三维原子排列的多金属氧化物用于催化气相氧化催化剂的有机化合物。

3. 发明授权

US5885922A Multimetal oxide materials 失效
标题翻译：多金属氧化物材料
公开(公告)号：US5885922A
公开(公告)日：1999-03-23
申请号：US685490
申请日：1996-07-24
申请人： Hartmut Hibst , Andreas Tenten , Laszlo Marosi
发明人： Hartmut Hibst , Andreas Tenten , Laszlo Marosi
IPC分类号： B01J23/88 , B01J23/00 , B01J23/887 , B01J23/888 , B01J35/00 , C01G31/00 , C01G39/00 , C07B61/00 , C07C51/235 , C07C51/25 , C07C57/05 , C07C57/055 , B01J23/16
CPC分类号： C07C51/252 , B01J23/002 , B01J23/8877 , B01J23/8885 , B01J35/0006 , B01J2523/00
摘要： Multimetal oxide materials containing molybdenum, vanadium, copper and one or more of the elements tungsten, niobium, tantalum, chromium and cerium and having a multiphase structure, and their use for the preparation of acrylic acid from acrolein by gas-phase catalytic oxidation, and oxometallates of the HT Cu molybdate structure type which contain Cu, Mo and at least one of the elements W, V, Nb and Ta.
摘要翻译：含有钼，钒，铜以及钨，铌，钽，铬和铈中的一种或多种元素并具有多相结构的多金属氧化物材料及其用于通过气相催化氧化由丙烯醛制备丙烯酸的用途，以及包含Cu，Mo和元素W，V，Nb和Ta中的至少一种的HT Cu钼酸盐结构类型的氧化金属盐。

4. 发明授权

US6124499A Preparation of organic acids such as acrylic acid by catalytic oxidation using a group V mixed metal oxide catalyst containing Cu, Mo, W, V, Nb and Ta 失效
标题翻译：使用含有Cu，Mo，W，V，Nb和Ta的V族混合金属氧化物催化剂通过催化氧化制备有机酸如丙烯酸
公开(公告)号：US6124499A
公开(公告)日：2000-09-26
申请号：US199487
申请日：1998-11-25
申请人： Hartmut Hibst , Andreas Tenten , Laszlo Marosi
发明人： Hartmut Hibst , Andreas Tenten , Laszlo Marosi
IPC分类号： B01J23/88 , B01J23/00 , B01J23/887 , B01J23/888 , B01J35/00 , C01G31/00 , C01G39/00 , C07B61/00 , C07C51/235 , C07C51/25 , C07C57/05 , C07C57/055 , C07C51/16
CPC分类号： C07C51/252 , B01J23/002 , B01J23/8877 , B01J23/8885 , B01J35/0006 , B01J2523/00
摘要： Multimetal oxide materials containing molybdenum, vanadium, copper and one or more of the elements tungsten, niobium, tantalum, chromium and cerium and having a multiphase structure, and their use for the preparation of acrylic acid from acrolein by gas-phase catalytic oxidation, and oxometallates of the HT Cu molybdate structure type which contain Cu, Mo and at least one of the elements W, V, Nb and Ta.
摘要翻译：含有钼，钒，铜以及钨，铌，钽，铬和铈中的一种或多种元素并具有多相结构的多金属氧化物材料及其用于通过气相催化氧化由丙烯醛制备丙烯酸的用途，以及包含Cu，Mo和元素W，V，Nb和Ta中的至少一种的HT Cu钼酸盐结构类型的氧化金属盐。

5. 发明授权

US6084126A Oxidation using multimetal molybdenum and vanadium oxides 失效
标题翻译：使用多金属钼和氧化钒进行氧化
公开(公告)号：US6084126A
公开(公告)日：2000-07-04
申请号：US92181
申请日：1998-06-05
申请人： Hartmut Hibst , Andreas Tenten , Laszlo Marosi
发明人： Hartmut Hibst , Andreas Tenten , Laszlo Marosi
IPC分类号： C01G1/00 , B01J23/00 , B01J23/20 , B01J23/28 , B01J23/30 , B01J23/88 , B01J23/887 , B01J23/888 , B01J35/00 , C01G31/00 , C01G39/00 , C01G41/00 , C07B61/00 , C07C45/33 , C07C45/34 , C07C45/35 , C07C45/38 , C07C51/235 , C07C51/25 , C07C57/05 , C07C57/055 , C07C51/16
CPC分类号： C07C51/252 , B01J23/002 , B01J23/28 , B01J23/30 , B01J23/8877 , B01J23/888 , B01J23/8885 , B01J35/0006 , C07C45/33 , C07C45/34 , C07C45/35 , C07C45/38 , C07C51/235 , B01J2523/00
摘要： A method for gas-phase oxidation of an organic compound such as acrolein is provided, which includes oxidizing the organic compound with an oxidizing agent in the presence of a catalyst, to produce a product such as acrylic acid, wherein the catalyst includes a multimetal oxide material having at least two phases and of the formula III{A}.sub.p {B}.sub.q (III),wherein ##EQU1## M.sup.1, M.sup.2, a, b, c, x, M.sup.3, d, e, y, p and q are defined in the claims,which contains the moiety {A}.sub.p in the form of three-dimensional regions A which are delimited from their local environment owing to their chemical composition differing from their local environment and are of the chemical compositionA Mo.sub.12-a-b-c V.sub.a M.sub.b.sup.1 M.sub.c.sup.2 O.sub.xand the moiety {B}.sub.q in the form of three dimensional regions B which are delimited from their local environment owing to their chemical composition differing from their local environment and are of the chemical compositionB M.sub.12.sup.3 Cu.sub.d H.sub.e O.sub.ywhere the regions A and B are distributed relative to one another as in a mixture of finely divided A and finely divided B and, with the use of CuK.alpha. radiation (.lambda.=1.54178 .ANG.), the three-dimensional atomic arrangement of the regions A gives an X-ray powder diffraction spectrum (the intensity of the diffracted X-rays plotted as a function of twice the diffraction angle (2.sup..crclbar.)) which, in the 2.sup..crclbar. range from 5 to 50.degree., contains the diffraction lines A.sup.1, A.sup.3, A.sup.5, A.sup.9 and A.sup.10 but not more than diffraction lines A.sup.1 to A.sup.10 defined in the claims.
摘要翻译：提供了一种有机化合物如丙烯醛的气相氧化方法，其包括在催化剂存在下用氧化剂氧化有机化合物，以产生产物如丙烯酸，其中催化剂包括多金属氧化物具有至少两相和式III {A} p {B} q（III）的材料，其中M1，M2，a，b，c，x，M3，d，e，y，p和q定义在其包含三维区域A形式的部分{A} p，其由于其局部环境的化学组成不同而具有其局部环境，并且具有化学组成A Mo12-abc VaMb1Mc2Ox和部分{ B）以三维区域B的形式，由于其局部环境的化学组成不同于它们的局部环境而具有化学组成B M123CudHeOy，其中区域A和B相对于彼此分布，如混合物的细分的A和细分的B，并且使用CuKα辐射（λ= 1.54178 ANGSTROM），区域A的三维原子排列得到X射线粉末衍射光谱（衍射的X射线衍射的强度）在2〜（ - ）范围内，5〜50°的衍射角（2（ - ））的函数为2倍的折射线，分别为衍射线A1，A3，A5，A9，A10，但不超过衍射在权利要求中限定的线A1至A10。

6. 发明授权

US5686373A Polymetal oxide materials 失效
标题翻译：多金属氧化物材料
公开(公告)号：US5686373A
公开(公告)日：1997-11-11
申请号：US392322
申请日：1995-02-22
申请人： Andreas Tenten , Friedrich-Georg Martin , Hartmut Hibst , Laszlo Marosi , Veronika Kohl
发明人： Andreas Tenten , Friedrich-Georg Martin , Hartmut Hibst , Laszlo Marosi , Veronika Kohl
IPC分类号： C01G53/00 , B01J23/00 , B01J23/88 , B01J23/885 , B01J23/887 , B01J35/00 , C01G39/02 , C07B61/00 , C07C51/25 , C07C57/055
CPC分类号： C07C51/252 , B01J23/002 , B01J23/885 , B01J23/8876 , B01J35/0006 , B01J2523/00
摘要： Polymetal oxide materials of the general formula I �A!.sub.p �B!.sub.q (I), where ##STR1## X.sup.1 is W, Nb, Ta, Cr and/or Ce, X.sup.2 is Cu, Ni, Co, Fe, Mn and/or Zn, X.sup.3 is Sb and/or Bi, X.sup.4 is Li, Na, K, Rb, Cs and/or H, X.sup.5 is Mg, Ca, Sr and/or Ba, X.sup.6 is Si, Al, Ti and/or Zr, X.sup.7 is Mo, W, V, Nb and/or Ta, a is from 1 to 8, b is from 0.2 to 5, c is from 0 to 23, d is from 0 to 50, e is from 0 to 2, f is from 0 to 5, g is from 0 to 50, h is from 4 to 30, i is from 0 to 20, x and y are each a number which is determined by the valency and frequency of the elements other than oxygen in I and p and q are non-zero numbers whose ratio p/q is from 160:1 to 1:1, and their use as catalysts.
摘要翻译：通式I [A] p [B] q（I）的多金属氧化物材料，其中A为MO12VaX1bX2cX3dX4eX5fX6gOx（Co相），B为X712CuhHiOy（关键相），X1为W，Nb，Ta，Cr和/或Ce ，X2是Cu，Ni，Co，Fe，Mn和/或Zn，X3是Sb和/或Bi，X4是Li，Na，K，Rb，Cs和/或H，X5是Mg，Ca，Sr和/ 或Ba，X 6为Si，Al，Ti和/或Zr，X 7为Mo，W，V，Nb和/或Ta，a为1〜8，b为0.2〜5，c为0〜23， d为0〜50，e为0〜2，f为0〜5，g为0〜50，h为4〜30，i为0〜20，x和y分别为由I中除氧之外的元素的价态和频率确定，p和q是比值p / q为160:1至1:1的非零数，并且它们用作催化剂。

7. 发明申请

US20060127287A1 Combinatorial preparation and testing of heterogeneous catalysts 审中-公开
标题翻译：组合制备和非均相催化剂的试验
公开(公告)号：US20060127287A1
公开(公告)日：2006-06-15
申请号：US11336843
申请日：2006-01-23
申请人： Hartmut Hibst , Andreas Tenten , Dirk Demuth , Ferdi Schueth , Stephan Schunk
发明人： Hartmut Hibst , Andreas Tenten , Dirk Demuth , Ferdi Schueth , Stephan Schunk
IPC分类号： D21C11/00
CPC分类号： B01J19/0046 , B01J37/0215 , B01J37/0217 , B01J2219/00286 , B01J2219/00306 , B01J2219/00511 , B01J2219/00585 , B01J2219/0059 , B01J2219/00599 , B01J2219/00747
摘要： The array of heterogeneous catalysts and/or their precursors, is made up of a body which has, preferably parallel, through-channels and in which at least n channels comprise n different heterogeneous catalysts and/or their precursors, where n is 2, preferably 10, particularly preferably 100, in particular 1000, especially 10,000. A process for preparing arrays comprising the following steps: a1) preparing solutions, emulsions and/or dispersions of elements and/or element compounds of the elements present in the catalyst and/or catalyst precursor and, if appropriate preparing dispersions of inorganic support materials, a2) if appropriate introducing adhesion promoters, binders, viscosity regulators, pH regulators and/or solid inorganic supports into the solutions, emulsions and/or dispersions, a3) simultaneously or successively coating the channels of the body with the solutions, emulsions and/or dispersions, a predetermined amount of the solutions, emulsions and/or dispersions being introduced into each channel to obtain a predetermined composition and a4) if appropriate heating the coated body in the presence or absence of inert gases or reactive gases to a temperature in the range from 20 to 1500° C. to dry, with or without sintering or calcining, the catalysts and/or catalyst precursors.
摘要翻译：非均相催化剂和/或其前体的阵列由具有优选平行的通道的主体组成，其中至少n个通道包含n个不同的非均相催化剂和/或其前体，其中n为2，优选为 10，特别优选100，特别是1000，特别是10,000。一种制备阵列的方法，包括以下步骤：a1）制备存在于催化剂和/或催化剂前体中的元素和/或元素化合物的溶液，乳液和/或分散体，以及如果合适的话，制备无机载体材料的分散体， a2）如果合适，将粘合促进剂，粘合剂，粘度调节剂，pH调节剂和/或固体无机载体引入溶液，乳液和/或分散体中，a3）用溶液，乳液和/或分散体同时或连续地涂覆身体的通道分散体，预定量的溶液，乳液和/或分散体被引入每个通道以获得预定的组合物和a）如果在存在或不存在惰性气体或反应气体的情况下适当地加热涂覆体到达该范围内的温度 20至1500℃，用或不用烧结或煅烧来干燥催化剂和/或催化剂前体。

8. 发明授权

US07005403B2 Catalyst comprising a support body and a catalytically active oxide material applied to the surface of the substrate 失效
标题翻译：催化剂包括施加到基材表面的载体和催化活性氧化物材料
公开(公告)号：US07005403B2
公开(公告)日：2006-02-28
申请号：US10399039
申请日：2001-10-16
申请人： Frieder Borgmeier , Andreas Tenten , Hartmut Hibst
发明人： Frieder Borgmeier , Andreas Tenten , Hartmut Hibst
IPC分类号： B01J23/22 , B01J23/28 , B01J27/057 , B01J35/02 , B01J37/02
CPC分类号： C07C45/33 , C07C45/35 , Y10S502/514 , C07C47/22
摘要： A coated catalyst whose coating of active composition is a multimetal oxide comprising the elements Mo, V and Te and/or Sb can be used for the gas-phase catalytic oxidation of propane to acrylic acid.
摘要翻译：包覆催化剂，其活性组合物的涂层是包含元素Mo，V和Te和/或Sb的多金属氧化物，可用于丙烷至丙烯酸的气相催化氧化。

9. 发明授权

US06730808B2 Oxidative reactions using membranes that selectively conduct oxygen 失效
标题翻译：使用选择性导电氧化膜的氧化反应
公开(公告)号：US06730808B2
公开(公告)日：2004-05-04
申请号：US10130822
申请日：2002-05-23
申请人： Stefan Bitterlich , Hartwig Voss , Hartmut Hibst , Andreas Tenten , Ingolf Voigt , Ute Pippardt
发明人： Stefan Bitterlich , Hartwig Voss , Hartmut Hibst , Andreas Tenten , Ingolf Voigt , Ute Pippardt
IPC分类号： C07C5116
CPC分类号： C07C51/265 , B01J23/002 , B01J23/34 , B01J35/065 , B01J2523/00 , C07B41/00 , C07C5/48 , C07C45/35 , C07C45/38 , C07C51/215 , C07C51/252 , C07C253/24 , C07C253/26 , C07C253/28 , C07C2521/02 , C07C2521/10 , C07C2523/02 , C07C2523/04 , C07C2523/08 , C07C2523/10 , C07C2523/14 , C07C2523/34 , Y02P20/52 , C07C11/02 , C07C47/22 , C07C47/04 , C07C57/145 , C07C57/04 , C07C63/16 , B01J2523/23 , B01J2523/24 , B01J2523/72 , C07C255/51 , C07C255/08
摘要： Reactor membranes for used in oxidation reactions of hydrocarbons involving oxygen comprising a selective oxidation catalyst on a mixed conducting, oxide ion selective ceramic membrane of the composition (Sr1-xCax)1-yAyMn1-zBzO3-&dgr;, where A is Ba, Pb, Na, K, Y, an element of the lanthanide group or a combination thereof, B is Mg, Al, Ga, In, Sn, an element of the 3d or 4d period or a combination thereof, x is from 0.2 to 0.8, y is from 0 to 0.4, z is from 0 to 0.6, and &dgr; is a number, dependent on x, y and z, that renders the composition charge neutral.
摘要翻译：用于包含氧的烃的氧化反应的反应器膜包括选择性氧化催化剂在组合物（Sr1-xCax）1-yAyMn1-zBzO3-δ的混合导电氧化物离子选择性陶瓷膜上，其中A是Ba，Pb，Na， K，Y是镧系元素的元素或其组合，B为Mg，Al，Ga，In，Sn，3d或4d的元素或其组合，x为0.2〜0.8，y为 0至0.4，z为0至0.6，并且delta是取决于x，y和z的数字，其使组成电荷为中性。

10. 发明授权

US07214822B2 Catalyst comprising a support and a catalytically active oxide material applied to the surface of the substrate 有权
标题翻译：催化剂包括施加到基材表面的载体和催化活性氧化物材料
公开(公告)号：US07214822B2
公开(公告)日：2007-05-08
申请号：US11228285
申请日：2005-09-19
申请人： Frieder Borgmeier , Andreas Tenten , Hartmut Hibst
发明人： Frieder Borgmeier , Andreas Tenten , Hartmut Hibst
IPC分类号： B01J23/00
CPC分类号： C07C45/33 , C07C45/35 , Y10S502/514 , C07C47/22
摘要： A coated catalyst whose coating of active composition is a multimetal oxide comprising the elements Mo, V and Te and/or Sb can be used for the gas-phase catalytic oxidation of propane to acrylic acid.
摘要翻译：包覆催化剂，其活性组合物的涂层是包含元素Mo，V和Te和/或Sb的多金属氧化物，可用于丙烷至丙烯酸的气相催化氧化。

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