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1. 发明授权

US4532492A Temperature-compensated, oxygen-content gas sensor 失效
标题翻译：温度补偿，含氧气体传感器
公开(公告)号：US4532492A
公开(公告)日：1985-07-30
申请号：US620717
申请日：1984-06-14
申请人： Friedrich J. Esper , Hermann Fischer , Karl-Hermann Friese , Peter Scharner
发明人： Friedrich J. Esper , Hermann Fischer , Karl-Hermann Friese , Peter Scharner
IPC分类号： G01N27/12
CPC分类号： G01N27/12
摘要： To simplify manufacture and assembly of a temperature-compensated titanium dioxide oxygen sensor, the sensor (9, 9') is applied as a layer on the thermistor body (1), with an electrode (8) interposed; preferably, the thermistor body is densely sintered titanium dioxide, in the form of a closed tube (1, 1') which may have a central opening (FIG. 1: 2) therethrough, with the sensor body being porous titanium dioxide and located either on the inside (FIG. 1) surface of the thermistor body (1) or on the outside (FIG. 2) surface, and supported by the thermistor body, which forms the substrate and support surface for the sensor body.
摘要翻译：为了简化温度补偿二氧化钛氧传感器的制造和组装，将传感器（9,9'）作为层施加在热敏电阻体（1）上，其中插入电极（8）; 优选地，热敏电阻体是致密烧结的二氧化钛，其形式为密封管（1,1'），其可以具有穿过其的中心开口（图1：2），传感器体是多孔二氧化钛，并且位于在热敏电阻体（1）的内部（图1）表面或外部（图2）表面上，由形成基板的热敏电阻体和传感器体的支撑面支撑。

2. 发明授权

US4221650A Solid electrolyte oxygen sensors 失效
标题翻译：固体电解质氧传感器
公开(公告)号：US4221650A
公开(公告)日：1980-09-09
申请号：US910385
申请日：1978-05-30
申请人： Karl-Hermann Friese , Friedrich J. Esper , Heinz Geier
发明人： Karl-Hermann Friese , Friedrich J. Esper , Heinz Geier
IPC分类号： C04B35/48 , C04B14/32 , C04B35/119 , C04B35/488 , G01N27/12 , G01N27/407 , G01N27/409 , G01N27/413 , H01M8/1253 , G01N27/58
CPC分类号： G01N27/4073 , C04B35/119 , C04B35/4885 , H01M8/1253 , Y02E60/525 , Y02P70/56
摘要： Oxygen sensors having a fine-grained stabilized cubic zirconium dioxide electrolyte contact respective electrodes. The zirconium dioxide contains between 15% and 50% by volume of Al.sub.2 O.sub.3 in a crystalline state and has good mechanical and thermal properties. The oxygen sensor may have a composite zirconium dioxide solid electrolyte element. The invention also includes a wider range of related Al.sub.2 O.sub.3 - containing stabilized cubic zirconium dioxides containing between about 8% and 85% by volume Al.sub.2 O.sub.3. The invention further provides methods of manufacturing such Al.sub.2 O.sub.3 - containing zirconium dioxide and for manufacturing oxygen sensors.
摘要翻译：具有细粒度稳定的立方二氧化锆电解质的氧传感器与相应的电极接触。二氧化锆在结晶状态下含有15体积％至50体积％的Al 2 O 3，具有良好的机械和热性能。氧传感器可以具有复合二氧化锆固体电解质元件。本发明还包括含有约8％至85％（体积）Al 2 O 3的更广泛的相关的含Al 2 O 3的稳定的立方二氧化锆。本发明还提供制造这种含Al 2 O 3的二氧化锆和用于制造氧传感器的方法。

3. 发明授权

US4183798A Stabilized zirconium dioxide compositions and oxygen sensors utilizing said compositions 失效
标题翻译：使用所述组合物的稳定二氧化锆组合物和氧传感器
公开(公告)号：US4183798A
公开(公告)日：1980-01-15
申请号：US888161
申请日：1978-03-20
申请人： Friedrich J. Esper , Karl-Hermann Friese
发明人： Friedrich J. Esper , Karl-Hermann Friese
IPC分类号： C04B35/48 , C04B35/486 , G01N27/58
CPC分类号： C04B35/486
摘要： Stabilized zirconium dioxide compositions sintered with a silicate flux and stabilized with (i) calcium oxide and (ii) magnesium oxide. The stabilized zirconium dioxide can be sintered at temperatures between 1460.degree. C. and 1480.degree. C. to form solids having high mechanical strength and a specific resistance of 1M.OMEGA.cm at a low temperature. The invention also provides oxygen sensors containing at least one measuring cell which is an oxygen concentration cell having two electrodes separated by and in ionic communication through a solid stabilized zirconium dioxide electrolyte which is prepared from the said compositions.
摘要翻译：稳定的二氧化锆组合物用硅酸盐助熔剂烧结并用（i）氧化钙和（ii）氧化镁稳定化。稳定的二氧化锆可以在1460℃和1480℃之间的温度下烧结，以在低温下形成具有高机械强度和1MΩEGAcm电阻率的固体。本发明还提供了含有至少一个测量池的氧传感器，该测量池是具有通过由所述组合物制备的固体稳定的二氧化锆电解质分离和离子连通的两个电极的氧浓度池。

4. 发明授权

US4347113A Oxygen content exhaust gas sensor, and method of its manufacture 失效
标题翻译：含氧废气传感器及其制造方法
公开(公告)号：US4347113A
公开(公告)日：1982-08-31
申请号：US133811
申请日：1980-03-25
申请人： Hermann Fischer , Karl-Hermann Friese , Hans-Ulrich Gruber , Wolfgang Heinemann , Gunter Knoll , Ernst Linder , Helmut Maurer , Rainer Noack , Leo Steinke , Lothar Weber , Helmut Weyl
发明人： Hermann Fischer , Karl-Hermann Friese , Hans-Ulrich Gruber , Wolfgang Heinemann , Gunter Knoll , Ernst Linder , Helmut Maurer , Rainer Noack , Leo Steinke , Lothar Weber , Helmut Weyl
IPC分类号： G01N27/409 , G01N27/407 , G01N27/413 , H01M4/88 , H01M8/12 , G01N27/58
CPC分类号： G01N27/4075 , G01N27/4078 , H01M4/881 , H01M4/8885 , H01M4/9066 , H01M8/1213 , H01M4/905 , Y02P70/56
摘要： To improve operation and output voltage, particularly at 400.degree. C. and less, an oxygen sensor, especially adapted to determine oxygen content of automotive exhaust gases, is constructed by utilizing two electrodes applied on a body of stabilized zirconium dioxide, for example a closed tube, by making an electrode exposed to the exhaust gases in form of a mixture of finely dispersed ceramic material and a platinum-rhodium alloy, the ceramic material being present at about 40% (by volume) and 60% (by volume) platinum-rhodium alloy of 50-94% platinum and 50-6% rhodium (by weight). The second electrode, exposed to a reference gas comprises an alloy of palladium and another noble metal in a ratio of about 19-90% (by weight) Pd and 81-10% (by weight) noble metal. This electrode may also contain up to 40% (by volume) finely dispersed ceramic material. The electrode exposed to the exhaust gases is covered with a porous coating. The electrodes can be applied as aqueous or organic solutions of soluble noble metal compounds or suspensions, colloidal suspensions, with organic solvents, and the like, and subsequent sintering.
摘要翻译：为了提高操作和输出电压，特别是在400℃以下，特别适用于测定汽车废气氧含量的氧气传感器是通过利用施加在稳定二氧化锆体上的两个电极构成的，例如封闭的通过使电极以细分散的陶瓷材料和铂 - 铑合金的混合物的形式暴露于废气，陶瓷材料以约40％（体积）和60％（体积）的铂 - 铑合金为50-94％铂和50-6％铑（重量）。暴露于参考气体的第二电极包括钯和另一贵金属的合金，其比例为约19-90％（重量）的Pd和81-10％（重量）的贵金属。该电极还可以含有高达40％（体积）的细分散的陶瓷材料。暴露于废气的电极被多孔涂层覆盖。电极可以作为可溶性贵金属化合物或悬浮液，胶体悬浮液，有机溶剂等的水溶液或有机溶液，以及随后的烧结。

5. 发明授权

US5474665A Measuring sensor for determining the oxygen content of gas mixtures 失效
标题翻译：用于测定气体混合物氧含量的测量传感器
公开(公告)号：US5474665A
公开(公告)日：1995-12-12
申请号：US306572
申请日：1994-09-15
申请人： Karl-Hermann Friese , Hermann Dietz , Hermann Fischer , Manfred Koeder , Werner Gruenwald , Ulrich Eisele
发明人： Karl-Hermann Friese , Hermann Dietz , Hermann Fischer , Manfred Koeder , Werner Gruenwald , Ulrich Eisele
IPC分类号： F02B1/04 , F02D41/14 , G01N27/409 , G01N27/419 , G01N27/407
CPC分类号： G01N27/419 , F02B1/04
摘要： The invention relates to a measuring sensor having pump reference for measuring the oxygen content of gas mixtures, particularly exhaust gases of internal combustion engines. The sensor includes a measuring cell (A) and a reference cell (B) each having a pair of electrodes, with one of each respective pairs of electrodes being common to the two cells, and having a fixed electrolyte. Reference cell (B) has defined therein an internal oxygen reference zone which is hermetically sealed from the gas mixture and which is connected to the atmosphere by way of a pressure-equalization line. The measuring cell (A) and the reference cell (B) can be heated by heating apparatus to a temperature at which the fixed electrolyte has an ionic conductivity which is sufficiently high. The heating apparatus and a porous insulation are advantageously disposed in the vicinity of the electrode of the reference cell which is not in common with the measuring cell and which is porous so that the porous insulation, together with the porous electrode, form the internal oxygen reference zone and, together with the porous electrode and its porous conductor track, form the pressure-equalization line.
摘要翻译：本发明涉及一种具有用于测量气体混合物，特别是内燃机废气的氧含量的泵参考的测量传感器。传感器包括测量单元（A）和参考单元（B），每个参考单元具有一对电极，每对电极中的每一对电极与两个单元共用，并具有固定的电解液。参考电池（B）在其中限定了内部氧参考区，其内部氧参考区与气体混合物气密密封，并通过压力平衡线连接到大气。测量单元（A）和参考单元（B）可以通过加热装置加热至固定电解质具有足够高的离子电导率的温度。加热装置和多孔绝缘体有利地设置在参比单元的电极附近，其与测量池不相同，并且是多孔的，使得多孔绝缘体与多孔电极一起形成内部氧参考并且与多孔电极及其多孔导体轨道一起形成压力平衡线。

6. 发明申请

US20080269043A1 Ceramic Insulating Material and Sensor Element Containing a Ceramic Insulating Material 审中-公开
标题翻译：陶瓷绝缘材料和包含陶瓷绝缘材料的传感器元件
公开(公告)号：US20080269043A1
公开(公告)日：2008-10-30
申请号：US11667867
申请日：2005-11-09
申请人： Thomas Wahl , Ulrich Eisele , Thomas Koehler , Bernd Schumann , Karl-Hermann Friese , Juergen Sindel , Stefan Nufer , Frank Buse
发明人： Thomas Wahl , Ulrich Eisele , Thomas Koehler , Bernd Schumann , Karl-Hermann Friese , Juergen Sindel , Stefan Nufer , Frank Buse
IPC分类号： C04B35/10
CPC分类号： G01N27/4071 , C04B35/117 , C04B2235/3205 , C04B2235/3215 , C04B2235/3222 , C04B2235/3239 , C04B2235/3244 , C04B2235/3248 , C04B2235/3418 , C04B2235/3472 , C04B2235/447 , C04B2235/80 , G01N27/4067
摘要： A ceramic insulating material, in particular for sensor elements for determining the concentration of gas components in gas mixtures, is based on an alkaline earth-containing ceramic. The insulating material contains a hexaaluminate of the alkaline earth metal and at least one mixed compound of the alkaline earth metal with an acid oxide, the molar ratio of hexaaluminate to the sum of mixed compounds in the insulating material being 1.3 to 4.0.
摘要翻译：特别是用于确定气体混合物中气体组分浓度的传感器元件的陶瓷绝缘材料是基于含碱土金属陶瓷的。绝缘材料包含碱土金属的六铝酸盐和碱土金属与酸性氧化物的至少一种混合化合物，六铝酸盐与绝缘材料中混合化合物的总和的摩尔比为1.3〜4.0。

7. 发明授权

US6018982A Gas-permeable connecting lead for a probe 失效
标题翻译：用于探头的透气连接导线
公开(公告)号：US6018982A
公开(公告)日：2000-02-01
申请号：US51099
申请日：1998-05-26
申请人： Karl-Hermann Friese , Helmut Weyl , Anton Hans
发明人： Karl-Hermann Friese , Helmut Weyl , Anton Hans
IPC分类号： G01N27/409 , G01N27/407 , G01N27/26
CPC分类号： G01N27/407 , G01N27/4076
摘要： A Lambda probe type gas sensor for use in determining the oxygen content of exhaust gases produced by an internal combustion engine includes a sensor element of the electrochemical, solid electrolyte, metallic oxide semiconductor or Lambda air-fuel ratio variety, which sensor element is arranged in a metallic housing and is contacted by connecting cables that are brought out of the metallic housing. These connecting cables are each surrounded by cable insulation that is made of PTFE (Polytetra-fluoroethylene). The surface of the cable insulation has, at least in certain areas, a gas-permeable section that allows a reference atmosphere to arrive inside the cable insulation and, from there, in the metallic housing. The gas-permeable section, on the other hand, prevents ingress of liquids such as fuel, condensed water, etc., This is achieved, for example, by an additionally applied, PTFE film that is placed over the gas-permeable section.
摘要翻译： PCT No.PCT / DE97 / 01562 Sec。 371日期：1998年5月26日 102（e）日期1998年5月26日PCT提交1997年7月24日PCT公布。第WO98 / 05951号公报日期1998年2月12日用于确定由内燃机产生的废气的氧含量的λ探针型气体传感器包括电化学，固体电解质，金属氧化物半导体或λ空气燃料比品种的传感器元件，其中传感器元件布置在金属壳体中并且通过连接从金属壳体外出的电缆而接触。这些连接电缆各自被由PTFE（聚四氟乙烯）制成的电缆绝缘体包围。电缆绝缘体的表面至少在某些区域中具有允许参考气氛到达电缆绝缘体内部并且从那里到达金属外壳的透气部分。另一方面，透气部防止了诸如燃料，冷凝水等的液体的进入，例如通过设置在透气部上的附加的PTFE膜来实现。

8. 发明授权

US5846391A Seal for a sensor element of a gas sensor 失效
标题翻译：气体传感器传感器元件的密封
公开(公告)号：US5846391A
公开(公告)日：1998-12-08
申请号：US836425
申请日：1997-04-29
申请人： Karl-Hermann Friese , Helmut Weyl , Hans-Martin Wiedenmann , Anton Hans
发明人： Karl-Hermann Friese , Helmut Weyl , Hans-Martin Wiedenmann , Anton Hans
IPC分类号： G01N27/409 , G01N27/407
CPC分类号： G01N27/4078
摘要： A seal for a sensor element for a gas sensor for determining the oxygen content in a gas to be measured including exhaust gases of internal combustion engines, the seal including a metallic housing having defined therein a longitudinal bore; a sensor element inserted into the longitudinal bore; and a sealing arrangement provided in the longitudinal bore, surrounding at least a portion of the sensor element, and comprised of at least one seal element comprised of steatite and an additional seal element comprised of boron nitride arranged in contact with one another and in a stack having a side near the gas to be measured so that, when there is one seal element comprised of steatite, the one seal element comprised of steatite is positioned on the side of the stack near the gas to be measured, and so that, when there are two seal elements comprised of steatite, the additional seal element is positioned between the two seal elements comprised of steatite, wherein the at least one seal element comprised of steatite and the additional seal element comprised of boron nitride are inserted into the longitudinal bore of the housing as deformable rings and are pressed-in therein, and wherein, during the pressing-in, the deformable rings are deformed in such a way that the at least one seal element comprised of steatite and the additional seal element comprised of boron nitride are pushed against the sensor element and the housing.
摘要翻译： PCT No.PCT / DE96 / 00567 Sec。 371日期1997年04月29日 102（e）日期1997年4月29日PCT 1996年3月21日PCT公布。公开号WO97 / 08542 日期1997年3月6日用于气体传感器的传感器元件的密封件，用于确定包括内燃机废气的待测气体中的氧含量，所述密封件包括金属壳体，其中限定有纵向孔; 插入纵向孔中的传感器元件; 以及设置在所述纵向孔中的密封装置，围绕所述传感器元件的至少一部分，并且包括至少一个由滑石组成的密封元件和由氮化硼组成的另外的密封元件，所述氮化硼彼此接触并且在堆叠具有靠近要测量的气体的一侧，使得当存在由滑石组成的一个密封元件时，由滑石组成的一个密封元件位于靠近待测量气体的堆叠侧，并且当那里是由滑石组成的两个密封元件，附加的密封元件位于由滑石组成的两个密封元件之间，其中由滑石组成的至少一个密封元件和由氮化硼组成的另外的密封元件被插入到壳体作为可变形环并被压入其中，并且其中，在压入期间，可变形环以这样的方式变形，使得至少一个由滑石组成的气体元件和由氮化硼组成的另外的密封元件被推靠在传感器元件和壳体上。

9. 发明授权

US5795454A Seal for a sensor element of a gas sensor 失效
标题翻译：气体传感器传感器元件的密封
公开(公告)号：US5795454A
公开(公告)日：1998-08-18
申请号：US569074
申请日：1995-12-04
申请人： Karl-Hermann Friese , Helmut Weyl , Romuald Fries , Hans-Martin Wiedenmann , Anton Hans
发明人： Karl-Hermann Friese , Helmut Weyl , Romuald Fries , Hans-Martin Wiedenmann , Anton Hans
IPC分类号： G01N27/409 , G01N27/12 , G01N27/407 , F16J15/14
CPC分类号： G01N27/4078 , G01N27/407 , G01N27/4077 , Y10S277/936 , Y10S277/938 , Y10S277/939 , Y10S277/941 , Y10S277/943
摘要： A seal for a sensor element of a gas sensor for determining the oxygen content in gases including exhaust gases of an internal combustion engine, which seal seals the sensor element in a longitudinal bore of a housing, the seal including a sealing stack which is positioned within the longitudinal bore of the housing and around the sensor element in use and which is comprised of two sealing bodies and an additional seal positioned between the two sealing bodies. The two sealing bodies are comprised of a pre-sintered ceramic material. The additional seal is comprised of a pre-pressed powder material and has a porosity which is lower than that of the two sealing bodies. The two sealing bodies and the additional seal are compressed together within the longitudinal bore in use, whereby at least the additional seal is deformed so that the sensor element is sealed in a gap-free manner within the longitudinal bore. The pre-pressed powder material of the additional seal may consist essentially of a ductile metal, which may be one of nickel or copper, or graphite which may be fiber-reinforced.
摘要翻译： PCT No.PCT / DE94 / 00537 Sec。 371 1995年12月4日第 102（e）日期1995年12月4日PCT 1994年5月11日PCT公布。公开号WO94 / 29710 日期1994年12月22日用于确定包括内燃机的废气在内的气体中的氧含量的气体传感器的传感器元件的密封件，该密封件将传感器元件密封在壳体的纵向孔中，所述密封件包括密封件堆叠，其位于壳体的纵向孔内并且在使用中围绕传感器元件，并且由两个密封体和位于两个密封体之间的附加密封件组成。两个密封体由预烧结的陶瓷材料组成。附加密封件由预压粉末材料组成，并且具有低于两个密封体的孔隙率。两个密封体和附加密封件在使用中在纵向孔内压缩在一起，由此至少附加的密封件变形，使得传感器元件以无间隙的方式密封在纵向孔内。附加密封件的预压粉末材料可以由可以是镍或铜之一的延性金属或可以是纤维增强的石墨组成。

10. 发明授权

US5172466A Process for producing PTC temperature sensor elements for PTC temperature sensor 失效
标题翻译：用于生产PTC温度传感器PTC温度传感器元件的工艺
公开(公告)号：US5172466A
公开(公告)日：1992-12-22
申请号：US715798
申请日：1991-06-14
申请人： Karl-Hermann Friese , Hans-Martin Wiedenmann , Gunther Stecher
发明人： Karl-Hermann Friese , Hans-Martin Wiedenmann , Gunther Stecher
IPC分类号： G01K7/16 , G01J5/02 , G01J5/20 , G01K7/18 , G01K7/22 , G01N27/416 , G01N27/417 , H01C1/024 , H01C1/034 , H01C7/02
CPC分类号： G01K7/183 , H01C7/021 , Y10T29/49085
摘要： A PTC temperature sensor and a process for producing PTC temperature sensing elements from ceramic films for a PTC temperature sensor are proposed. The PTC temperature sensing elements are so designed that the PTC resistor track is hermetically encapsulated with respect to the gas being measured and the ambient air. Ceramic films based on an insulator ceramic, in particular based on Al.sub.2 O.sub.3, and ceramic films based on a solid electrolyte can be used to produce the temperature sensing elements. The PTC temperature sensor according to the invention is distinguished, in particular, by the fact that, while the manufacturing procedure is cheap, it is not subject to aging due to the effect of varying O.sub.2 partial pressures, has a high resistance to aging of the resistance characteristic in rich and lean gas mixtures, for example in motor vehicle exhaust gases, at 300.degree.-1000.degree. C. and has a construction free from extraneous potential, is characterized by short response times owning to its low heat capacity and is suitable for incorportion in very narrow housing as a consequence of small dimensions.
摘要翻译：提出了一种用于PTC温度传感器的PTC温度传感器和用于从陶瓷膜生产PTC温度传感元件的工艺。 PTC温度感测元件被设计成使得PTC电阻轨道相对于被测量的气体和环境空气被气密地封装。可以使用基于绝缘体陶瓷，特别是基于Al 2 O 3的陶瓷膜和基于固体电解质的陶瓷膜来制造温度感测元件。根据本发明的PTC温度传感器的特征在于，特别是由于制造过程便宜，由于变化的O2分压的影响，其不会老化，因此具有高耐老化性富含和贫气混合物的阻力特性，例如在机动车排气中，在300°-1000℃，具有无外力的结构，其特征在于具有低热容量的响应时间短，适用于由于小尺寸，狭窄房屋的配额不合。

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