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1. 发明授权

US09233359B2 Process for the hydroconversion of a low quality hydrocarbonaceous feedstock 有权
标题翻译：低品质含烃原料加氢转化的方法
公开(公告)号：US09233359B2
公开(公告)日：2016-01-12
申请号：US13808425
申请日：2011-07-05
申请人： Didier Borremans , Jean-Pierre Dath , Kai Hortmann
发明人： Didier Borremans , Jean-Pierre Dath , Kai Hortmann
IPC分类号： B01J31/16 , B01J27/051 , B01J23/745 , B01J31/22 , B01J37/20 , C10G49/12 , B01J27/043 , B01J31/00 , B01J31/12
CPC分类号： B01J27/051 , B01J23/745 , B01J27/043 , B01J31/2295 , B01J37/20 , B01J2231/60 , B01J2531/56 , B01J2531/64 , B01J2531/842 , C10G49/12 , C10G2300/107 , C10G2300/1077 , C10G2300/44 , C10G2300/703
摘要： The invention concerns a process for upgrading lower quality carbonaceous feedstock using a slurry catalyst composition. The use of particular organometallic compounds as precursors for the dispersed active catalyst allows for reduced coke formation.
摘要翻译：本发明涉及一种使用浆料催化剂组合物来提升低质量碳质原料的方法。使用特定的有机金属化合物作为分散的活性催化剂的前体允许减少焦炭形成。

2. 发明申请

US20130172638A1 PROCESS FOR THE HYDROCONVERSION OF A LOW QUALITY HYDROCARBONACEOUS FEEDSTOCK 有权
标题翻译：低品质石油天然气原料的降解方法
公开(公告)号：US20130172638A1
公开(公告)日：2013-07-04
申请号：US13808425
申请日：2011-07-05
申请人： Didier Borremans , Jean-Pierre Dath , Kai Hortmann
发明人： Didier Borremans , Jean-Pierre Dath , Kai Hortmann
IPC分类号： B01J27/051 , B01J27/043
CPC分类号： B01J27/051 , B01J23/745 , B01J27/043 , B01J31/2295 , B01J37/20 , B01J2231/60 , B01J2531/56 , B01J2531/64 , B01J2531/842 , C10G49/12 , C10G2300/107 , C10G2300/1077 , C10G2300/44 , C10G2300/703
摘要： The invention concerns a process for upgrading lower quality carbonaceous feedstock using a slurry catalyst composition. The use of particular organometallic compounds as precursors for the dispersed active catalyst allows for reduced coke formation.
摘要翻译：本发明涉及一种使用浆料催化剂组合物来提升低质量碳质原料的方法。使用特定的有机金属化合物作为分散的活性催化剂的前体允许减少焦炭形成。

3. 发明授权

US10493438B2 Method to purify olefin-containing hydrocarbon feedstocks 有权
公开(公告)号：US10493438B2
公开(公告)日：2019-12-03
申请号：US13141283
申请日：2009-12-22
申请人： William J. Gauthier , Olivier Miserque , George Vulpescu , Francine Genin , Kai Hortmann , Jean-Pierre Dath
发明人： William J. Gauthier , Olivier Miserque , George Vulpescu , Francine Genin , Kai Hortmann , Jean-Pierre Dath
IPC分类号： B01J23/755 , C07C7/167 , B01J35/00 , B01J35/10
CPC分类号： B01J23/755 , C07C7/167 , B01J35/0026 , B01J35/1014 , B01J35/1019 , C07C2523/755 , Y02P20/52 , C07C7/167 , C07C11/02 , C07C7/167 , C07C11/06
摘要： A process for purifying an olefin-containing hydrocarbon feedstock comprising the steps of:

(a) passing the said hydrocarbon feedstock in the presence of hydrogen over a first catalyst bed material comprising nickel deposited on a support material wherein said nickel is present as both nickel oxide and metallic nickel
(b) recovering the feedstock having a substantially reduced acetylenics (in particular methylacetylene) and allenes (in particular propadiene) content.

4. 发明申请

US20120046512A1 METHOD TO PURIFY OLEFIN-CONTAINING HYDROCARBON FEEDSTOCKS 审中-公开
标题翻译：含有含烯烃的碳氢化合物的方法
公开(公告)号：US20120046512A1
公开(公告)日：2012-02-23
申请号：US13141283
申请日：2008-12-22
申请人： William J. Gauthier , Olivier Miserque , George Vulpescu , Francine Genin , Kai Hortmann , Jean-Pierre Dath
发明人： William J. Gauthier , Olivier Miserque , George Vulpescu , Francine Genin , Kai Hortmann , Jean-Pierre Dath
IPC分类号： C07C7/148
CPC分类号： B01J23/755 , B01J35/0026 , B01J35/1014 , B01J35/1019 , C07C7/167 , C07C2523/755 , Y02P20/52 , C07C11/02 , C07C11/06
摘要： A process for purifying an olefin-containing hydrocarbon feedstock comprising the steps of: (a) passing the said hydrocarbon feedstock in the presence of hydrogen over a first catalyst bed material comprising nickel deposited on a support material wherein said nickel is present as both nickel oxide and metallic nickel (b) recovering the feedstock having a substantially reduced acetylenics (in particular methylacetylene) and allenes (in particular propadiene) content.
摘要翻译：一种用于纯化含烯烃的原料的方法，包括以下步骤：（a）使所述烃原料在氢存在下通过沉积在载体材料上的包含镍的第一催化剂床材料，其中所述镍作为氧化镍和金属镍（b）回收具有显着降低的炔属（特别是甲基乙炔）和丙烯（特别是丙二烯）含量的原料。

5. 发明授权

US09162937B2 Process to make olefins from organics with reduced side reactions 有权
标题翻译：从有机物制备烯烃，减少副反应的方法
公开(公告)号：US09162937B2
公开(公告)日：2015-10-20
申请号：US13055019
申请日：2009-07-03
申请人： Giacomo Grasso , Nikolai Nesterenko , Sander Van Donk , Jean-Pierre Dath , Eric Duchesne
发明人： Giacomo Grasso , Nikolai Nesterenko , Sander Van Donk , Jean-Pierre Dath , Eric Duchesne
IPC分类号： C07C1/20
CPC分类号： C07C1/20 , Y02P30/42 , C07C11/02 , C07C11/06
摘要： The present invention is a process for making an olefin product from an oxygen-containing organic feedstock comprising: providing a mixture of said oxygen-containing feedstock, an hydrocarbon and optionally an inert diluent, contacting said mixture in a reaction zone having an inner surface (the MTO reactor) with a zeolitic catalyst at conditions effective to convert at least a part of the oxygen-containing organic feedstock to olefin products (the MTO reactor effluent), recovering a reactor effluent comprising light olefins, a heavy hydrocarbon fraction and undesired by-products, wherein: at least a part of the inner surface is passivated such that the undesired by-products are reduced by comparison with a non passivated inner surface and/or one or more sulphur compound is co-injected with the said oxygen-containing feedstock and the hydrocarbon and said sulphur compound is capable to reduce the undesired by-products by comparison with a non injection of sulphur compound. The present invention is of high interest for the catalyst of the ZSM type such as ZSM-5 optionally containing phosphorus and regenerated in the MTO reactor.
摘要翻译：本发明是从含氧有机原料制备烯烃产物的方法，包括：提供所述含氧原料，烃和任选的惰性稀释剂的混合物，使所述混合物在具有内表面的反应区 MTO反应器），在有效地将至少一部分含氧有机原料转化为烯烃产物（MTO反应器流出物）的条件下使用沸石催化剂，回收包含轻质烯烃，重质烃馏分和不希望的副产物的反应器流出物，产品，其中：所述内表面的至少一部分被钝化，使得通过与非钝化内表面相比减少不需要的副产物和/或一种或多种硫化合物与所述含氧原料共注入并且烃和所述硫化合物能够通过与非注射硫化合物相比而减少不期望的副产物。本发明对ZSM型催化剂如ZSM-5任选含磷并在MTO反应器中再生而感兴趣。

6. 发明授权

US09126183B2 Modified Y-type zeolites having a trimodal intracrystalline structure, method for making same, and use thereof 有权
标题翻译：具有三峰晶体结构的改性Y型沸石，其制备方法及其用途
公开(公告)号：US09126183B2
公开(公告)日：2015-09-08
申请号：US13141281
申请日：2009-12-22
申请人： Sander Van Donk , Maxime Lacroix , Régine Kenmogne-Gatchuissi , François Fajula , Métin Bulut , Jean-Pierre Dath , Krijn Pieter De Jong , Petra Elisabeth De Jongh , Jovana Zecevic , Adrianus Nicolaas Cornelis Van Laak
发明人： Sander Van Donk , Maxime Lacroix , Régine Kenmogne-Gatchuissi , François Fajula , Métin Bulut , Jean-Pierre Dath , Krijn Pieter De Jong , Petra Elisabeth De Jongh , Jovana Zecevic , Adrianus Nicolaas Cornelis Van Laak
IPC分类号： B01J29/84 , B01J29/08 , B01J29/12 , C01B39/02 , C01B39/24 , C10G47/16
CPC分类号： B01J29/084 , B01J29/126 , B01J2229/16 , B01J2229/18 , B01J2229/20 , B01J2229/22 , B01J2229/38 , B01J2229/40 , B01J2229/42 , C01B39/026 , C01B39/24 , C10G47/16
摘要： The invention relates to a Y-type zeolite having a modified faujasite structure, the intracrystalline structure of which includes at least one network of micropores, at least one network of small mesopores having an average diameter ranging from 2 to 5 nm, and at least one network of large mesopores having an average diameter ranging from 10 to 50 nm. The invention also relates to particles including such zeolites and to the use thereof in a method for processing crude oil, particularly as a hydrocracking catalyst.
摘要翻译：本发明涉及具有改性的八面沸石结构的Y型沸石，其结晶结构包括至少一个微孔网络，至少一个平均直径范围为2-5nm的小介孔网络，以及至少一个具有10至50nm平均直径的大介孔的网络。本发明还涉及包括这种沸石的颗粒以及其在用于加工原油，特别是加氢裂化催化剂的方法中的用途。

7. 发明授权

US09056807B2 Process to make olefins from isobutanol 有权
标题翻译：从异丁醇制备烯烃的方法
公开(公告)号：US09056807B2
公开(公告)日：2015-06-16
申请号：US13813168
申请日：2011-07-08
申请人： Cindy Adam , Delphine Minoux , Nikolai Nesterenko , Sander Van Donk , Jean-Pierre Dath
发明人： Cindy Adam , Delphine Minoux , Nikolai Nesterenko , Sander Van Donk , Jean-Pierre Dath
IPC分类号： C07C1/22 , C07C1/24 , C07C4/06 , C07C6/04 , C10G3/00 , C12P5/02 , C12P7/16 , B01J29/40
CPC分类号： C07C1/24 , B01J29/40 , B01J2229/42 , C07C1/22 , C07C4/06 , C07C6/04 , C07C2529/40 , C08F10/02 , C10G3/42 , C10G3/44 , C10G3/49 , C10G2300/1014 , C10G2300/1022 , C10G2300/201 , C10G2300/4081 , C10G2400/20 , C10G2400/22 , C12P5/026 , C12P7/16 , Y02E50/10 , Y02P20/52 , Y02P30/20 , Y02P30/42 , C07C11/08 , C07C11/06
摘要： The present invention relates to a process for the conversion of an alcohol mixture (A) comprising about 20 w % to 100% isobutanol to make essentially propylene, comprising: a) introducing in a reactor (A) a stream comprising the mixture (A), optionally water, optionally an inert component, b) contacting said stream with a catalyst (A1) at a temperature above 450° C. in said reactor (A) at conditions effective to dehydrate at least a part of the isobutanol and other alcohols, if any, and make a cracking, c) recovering from said reactor (A) an effluent comprising: ethylene, propylene, water, optionally unconverted alcohols of the mixture (A), various hydrocarbons, and the optional inert component of step a), d) fractionating said effluent of step c) to produce at least an ethylene stream, a propylene stream, a fraction consisting essentially of hydrocarbons having 4 carbon atoms or more, water and the optional inert component of step a), optionally recycling ethylene in whole or in part at the inlet of the reactor (A), optionally recycling the fraction consisting essentially of hydrocarbons having 4 carbon atoms or more at the inlet of the reactor (A).
摘要翻译：本发明涉及一种将包含约20％至100％异丁醇的醇混合物（A）转化成基本上丙烯的方法，其包括：a）在反应器（A）中引入包含混合物（A）的料流，任选的水，任选的惰性组分，b）在有效使至少一部分异丁醇和其它醇脱水的条件下，使所述物流与催化剂（A1）在高于450℃的温度下在所述反应器（A）中接触， c）从所述反应器（A）回收包含乙烯，丙烯，水，任选未转化的混合物（A）的醇，各种烃和步骤a）的任选的惰性组分的流出物， d）将步骤c）的所述流出物分馏以产生至少一种乙烯流，丙烯流，基本上由具有4个碳原子或更多的烃组成的级分，水和步骤a）的任选的惰性组分，任选地将乙烯全部回收或在par 在反应器（A）的入口处，任选地在反应器（A）的入口处循环基本上由具有4个或更多个碳原子的烃组成的馏分。

8. 发明申请

US20140076780A1 CATALYST FOR USE IN HYDROTREATMENT, COMPRISING METALS FROM GROUPS VIII AND VIB, AND PREPARATION WITH CITRIC ACID AND C1-C4 DIALKYL SUCCINATE 审中-公开
标题翻译：用于水力发电的催化剂，包含来自组VIII和VIB的金属，以及用柠檬酸和C 1 -C 4二烷基磺酸钠的制备
公开(公告)号：US20140076780A1
公开(公告)日：2014-03-20
申请号：US14005936
申请日：2012-02-10
申请人： Bertrand Guichard , Laurent Simon , Valentina De Grandi , Delphine Minoux , Jean-Pierre Dath
发明人： Bertrand Guichard , Laurent Simon , Valentina De Grandi , Delphine Minoux , Jean-Pierre Dath
IPC分类号： B01J31/34 , C10G45/10 , C10G47/14 , C10G45/12 , C10G45/54 , C10G47/18
CPC分类号： B01J31/34 , B01J21/04 , B01J21/12 , B01J23/85 , B01J23/882 , B01J23/883 , B01J23/94 , B01J31/0201 , B01J31/0209 , B01J31/04 , B01J35/002 , B01J37/0009 , B01J37/0203 , B01J37/20 , B01J38/52 , B01J38/62 , C10G45/04 , C10G45/06 , C10G45/08 , C10G45/10 , C10G45/12 , C10G45/50 , C10G45/54 , C10G45/68 , C10G47/12 , C10G47/14 , C10G47/18 , C10G2300/1055 , C10G2300/202
摘要： A catalyst which comprises an amorphous support based on alumina, a C1-C4 dialkyl succinate, citric acid and optionally acetic acid, phosphorus and a hydrodehydrogenating function comprising at least one element from group VIII and at least one element from group VIB; the most intense bands comprised in the Raman spectrum of the catalyst are characteristic of Keggin heteropolyanions (974 and/or 990 cm−1), C1-C4 dialkyl succinate and citric acid (in particular 785 and 956 cm−1). Also a process for preparing said catalyst in which a catalytic precursor in the dried, calcined or regenerated state containing the elements of the hydrodehydrogenating function, and optionally phosphorus, is impregnated with an impregnation solution comprising at least one C1-C4 dialkyl succinate, citric acid and optionally at least one compound of phosphorus and optionally acetic acid, and is then dried. Further, the use of said catalyst in any hydrotreatment process.
摘要翻译：一种催化剂，其包含基于氧化铝的无定形载体，琥珀酸C1-C4二烷基酯，柠檬酸和任选的乙酸，磷和氢化脱氢功能，其包含来自VIII族的至少一种元素和至少一种来自VIB族的元素; 包含在催化剂的拉曼光谱中的最强烈的条带是Keggin杂多阴离子（974和/或990cm -1），C 1 -C 4二烷基琥珀酸酯和柠檬酸（特别是785和956cm -1）的特征。还有一种制备所述催化剂的方法，其中将含有脱氢官能团元素的干燥，煅烧或再生状态的催化前体以及任选的磷浸渍在浸渍溶液中，所述浸渍溶液包含至少一种琥珀酸C 1 -C 4二烷基酯，柠檬酸和任选的至少一种磷和任选的乙酸化合物，然后干燥。此外，在任何加氢处理方法中使用所述催化剂。

9. 发明申请

US20130204059A1 PROCESS TO MAKE OLEFINS FROM ISOBUTANOL 有权
标题翻译：从ISOBUTANOL制造OLEFINS的过程
公开(公告)号：US20130204059A1
公开(公告)日：2013-08-08
申请号：US13813115
申请日：2011-07-08
申请人： Cindy Adam , Delphine Minoux , Nikolai Nesterenko , Sander Van Donk , Jean-Pierre Dath
发明人： Cindy Adam , Delphine Minoux , Nikolai Nesterenko , Sander Van Donk , Jean-Pierre Dath
IPC分类号： C07C1/22 , C07C2/12
CPC分类号： C07C1/24 , C07C1/20 , C07C1/22 , C07C2/12 , C07C4/06 , C07C11/06 , C07C29/00 , C07C2529/40 , C07C2529/85 , C08F210/02 , C08F210/06 , C12P7/16 , Y02P30/42
摘要： The present invention relates to a process for the conversion of an alcohols mixture (A) comprising about 20 w % to 100% isobutanol to make essentially propylene, comprising: a) introducing in a reactor (A) a stream comprising the mixture (A), mixed with a stream (D1) comprising olefins having 4 carbon atoms or more (C4+ olefins), optionally water, optionally an inert component, b) contacting said stream with a catalyst (A1) at a temperature above 500° C. in said reactor (A) at conditions effective to dehydrate at least a part of the isobutanol and other alcohols, if any, and make a cracking, c) recovering from said reactor (A) an effluent comprising: ethylene, propylene, water, optionally unconverted alcohols of the mixture (A), various hydrocarbons, and the optional inert component of step a), d) fractionating said effluent of step c) to produce at least an ethylene stream, a propylene stream, a fraction consisting essentially of hydrocarbons having 4 carbon atoms or more, water and the optional inert component of step a), optionally recycling ethylene in whole or in part at the inlet of the reactor (A), optionally recycling the fraction consisting essentially of hydrocarbons having 4 carbon atoms or more at the inlet of the reactor (A).
摘要翻译：本发明涉及一种将包含约20％至100％异丁醇的醇混合物（A）转化成基本上丙烯的方法，其包括：a）在反应器（A）中引入包含混合物（A）的料流，与包含具有4个或更多碳原子的烯烃（C 4 +烯烃），任选的水，任选的惰性组分的流（D1）混合，b）在所述的温度高于500℃的温度下使所述料流与催化剂（A1）接触反应器（A）在有效使至少一部分异丁醇和其它醇脱水的条件下（如果有的话）并且产生裂化，c）从所述反应器（A）回收包含乙烯，丙烯，水，任选未转化的醇混合物（A），各种烃和步骤a）的任选的惰性组分，d）将步骤c）的所述流出物分馏以产生至少一种乙烯流，丙烯料流，基本上由具有4碳原子的烃组成的馏分原子或更多，水和步骤a）的任选的惰性组分，任选地在反应器（A）的入口处全部或部分地循环乙烯，任选地在反应器（A）的入口处循环基本上由具有4个或更多碳原子的烃组成的馏分，。

10. 发明申请

US20120271085A1 METHOD FOR PRODUCING DISTILLATE FROM A HYDROCARBON FEED, COMPRISING ALCOHOL CONDENSATION 审中-公开
标题翻译：用于生产来自油料进料的蒸馏物的方法，包含酒精浓缩
公开(公告)号：US20120271085A1
公开(公告)日：2012-10-25
申请号：US13501382
申请日：2010-10-13
申请人： Nikolai Nesterenko , Delphine Minoux , Sander Van Donk , Jean-Pierre Dath
发明人： Nikolai Nesterenko , Delphine Minoux , Sander Van Donk , Jean-Pierre Dath
IPC分类号： C07C1/20
CPC分类号： C07C29/34 , B01J29/40 , C07C2529/40 , C10G3/42 , C10G3/45 , C10G50/00 , C10G2300/1011 , C10G2300/1088 , C10G2300/4018 , C10G2300/4081 , C10G2300/70 , C10G2400/22 , Y02P30/42 , C07C31/12 , C07C31/125
摘要： The invention relates to a method for converting a hydrocarbon feed containing C3-C10 olefins into a distillate, whereby the quantities of olefins having a chain length that is too short can be reduced in order to be exploited (typically C10 or even less) and the C10+ molecule yields can be increased, while controlling the exothermicity of the oligomerisation reactions. This effect is obtained by oligomerising the hydrocarbon feed in the presence of at least one part of the products resulting from the pre-conversion, by means of condensation, of light oxygen molecules (comprising at least one alcohol having at least two carbon atoms) which can originate from biomass.
摘要翻译：本发明涉及一种将含有C 3 -C 10烯烃的烃进料转化成馏出物的方法，由此可以减少链长过短的烯烃的用量（通常为C10或更小），并且可以增加C10 +分子的产率，同时控制低聚反应的放热。这种效果是通过在至少一部分产物的存在下，通过缩合产生的轻氧分子（包含至少一种具有至少两个碳原子的至少一个醇）而产生的产物的低聚来获得的。可以源自生物量。

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