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1. 发明申请

US20070111025A1 Use of platinum ll complexes as luminescent materials in organic light-emitting diodes (oleds) 审中-公开
标题翻译：在有机发光二极管（oleds）中使用铂II配合物作为发光材料
公开(公告)号：US20070111025A1
公开(公告)日：2007-05-17
申请号：US10580836
申请日：2004-12-08
申请人： Christian Lennartz , Arnd Vogler , Valeri Pawlowski
发明人： Christian Lennartz , Arnd Vogler , Valeri Pawlowski
IPC分类号： H01L51/54 , C09K11/06
CPC分类号： C09K11/06 , C09K2211/185 , H01L51/0087 , H01L51/5012 , H01L51/5016 , H05B33/14
摘要： The present invention relates to the use of platinum(II) complexes of the formulae I, II and III as emitter molecules in organic light-emitting diodes (OLEDs), where the radicals are defined in the claims and in the description. Furthermore, the present invention relates to the use of the platinum(II) complexes as light-emitting layer in OLEDs, a light-emitting layer comprising at least one platinum(II) complex, an OLED comprising this light-emitting layer and devices comprising an OLED according to the invention.
摘要翻译：本发明涉及式I，II和III的铂（II）配合物在有机发光二极管（OLED）中作为发射体分子的用途，其中自由基在权利要求书和说明书中定义。此外，本发明涉及铂（II）配合物作为OLED中的发光层的用途，包含至少一种铂（II）络合物的发光层，包含该发光层的OLED以及包含根据本发明的OLED。

2. 发明授权

US07858208B2 Use of a copper (I) complexes for organic luminescent diodes 有权
标题翻译：铜（I）配合物用于有机发光二极管
公开(公告)号：US07858208B2
公开(公告)日：2010-12-28
申请号：US11575554
申请日：2005-09-20
申请人： Arnd Vogler , Valeri Pawlowski , Hans-Werner Schmidt , Mukundan Thelakkat , Markus Baete
发明人： Arnd Vogler , Valeri Pawlowski , Hans-Werner Schmidt , Mukundan Thelakkat , Markus Baete
IPC分类号： H01J1/63 , C07F9/28
CPC分类号： C07F1/005 , C08G73/00 , C09K11/06 , C09K2211/188 , H01L51/0059 , H01L51/0062 , H01L51/0077 , H01L51/5012 , H01L51/5096 , H05B33/14
摘要： The present invention relates to the use of copper(I) complexes of the formula I where X is nitrogen or a C—R group, R is alkyl or aryl, Ar is phenyl or naphthyl, each of which is optionally substituted by from one to three radicals selected from the group consisting of alkoxy, alkylthio, alkylamino, dialkylamino, alkoxycarbonyl, alkoxysulfonyl, halogen, cyano, carboxyl, hydroxysulfonyl and nitro, and the two optionally substituted phenyl or naphthyl radicals may be joined to one another by a chemical single bond via the carbon atoms in the α- and α′-position relative to the phosphorus atom, n is 1, 2 or 3, and Y is halogen, cyano, thiocyanato, alkoxy, aryloxy, alkylthio, arylthio, alkylamino, dialkylamino, arylamino or diarylamino, in organic light-emitting diodes (OLEDs), The present invention further relates to light-emitting layers which comprise at least one copper(I) complex of the formula I, to OLEDs which comprise at least one copper(I) complex of the formula I or an inventive light-emitting layer, and to stationary visual display units which comprise inventive OLEDs.Furthermore, the present invention relates to novel copper(I) complexes of the formula Ia and Ib where R, Ar and n are each as defined in formula I, Y in formula Ia is defined as cyano, thiocyanato, alkoxy, aryloxy, alkylthio, arylthio, alkylamino, dialkylamino, arylamino or diarylamino, and Y in formula Ib is defined as halogen, cyano, thiocyanato, alkoxy, aryloxy, alkylthio, arylthio, alkylamino, dialkylamino, arylamino or diarylamino.
摘要翻译：本发明涉及式I的铜（I）络合物，其中X是氮或C-R基，R是烷基或芳基，Ar是苯基或萘基，其各自任选被一个选自烷氧基，烷硫基，烷基氨基，二烷基氨基，烷氧基羰基，烷氧基磺酰基，卤素，氰基，羧基，羟基磺酰基和硝基的三个基团和两个任选取代的苯基或萘基可以通过化学单键彼此连接通过相对于磷原子的α-和α'-位的碳原子，n是1,2或3，Y是卤素，氰基，氰硫基，烷氧基，芳氧基，烷硫基，芳硫基，烷基氨基，二烷基氨基，芳基氨基或在有机发光二极管（OLED）中的二芳基氨基，本发明还涉及包含至少一种式I的铜（I）配合物的发光层与包含至少一种铜（I）络合物公式I或者inve 发光层，以及包括本发明的OLED的固定的视觉显示单元。此外，本发明涉及式Ia和Ib的新型铜（I）络合物，其中R，Ar和n各自如式I中所定义，式Ia中的Y定义为氰基，氰硫基，烷氧基，芳氧基，烷硫基，氰基，氰硫基，烷氧基，芳氧基，烷硫基，芳硫基，烷氨基，二烷基氨基，芳基氨基或二芳基氨基。

3. 发明申请

US20080199731A1 Use of a Copper (I) Complexes For Organic Luminescent Diodes 有权
标题翻译：用于有机发光二极管的铜（I）配合物
公开(公告)号：US20080199731A1
公开(公告)日：2008-08-21
申请号：US11575554
申请日：2005-09-20
申请人： Arnd Vogler , Valeri Pawlowski , Hans-Werner Schmidt , Mukundan Thelakkat , Markus Bate
发明人： Arnd Vogler , Valeri Pawlowski , Hans-Werner Schmidt , Mukundan Thelakkat , Markus Bate
IPC分类号： H01J1/63 , C07F9/28
CPC分类号： C07F1/005 , C08G73/00 , C09K11/06 , C09K2211/188 , H01L51/0059 , H01L51/0062 , H01L51/0077 , H01L51/5012 , H01L51/5096 , H05B33/14
摘要： The present invention relates to the use of copper(I) complexes of the formula I where X is nitrogen or a C—R group, R is alkyl or aryl, Ar is phenyl or naphthyl, each of which is optionally substituted by from one to three radicals selected from the group consisting of alkoxy, alkylthio, alkylamino, dialkylamino, alkoxycarbonyl, alkoxysulfonyl, halogen, cyano, carboxyl, hydroxysulfonyl and nitro, and the two optionally substituted phenyl or naphthyl radicals may be joined to one another by a chemical single bond via the carbon atoms in the α- and α′-position relative to the phosphorus atom, n is 1, 2 or 3, and Y is halogen, cyano, thiocyanato, alkoxy, aryloxy, alkylthio, arylthio, alkylamino, dialkylamino, arylamino or diarylamino, in organic light-emitting diodes (OLEDs), The present invention further relates to light-emitting layers which comprise at least one copper(I) complex of the formula I, to OLEDs which comprise at least one copper(I) complex of the formula I or an inventive light-emitting layer, and to stationary visual display units which comprise inventive OLEDs.Furthermore, the present invention relates to novel copper(I) complexes of the formula Ia and Ib where R, Ar and n are each as defined in formula I, Y in formula Ia is defined as cyano, thiocyanato, alkoxy, aryloxy, alkylthio, arylthio, alkylamino, dialkylamino, arylamino or diarylamino, and Y in formula Ib is defined as halogen, cyano, thiocyanato, alkoxy, aryloxy, alkylthio, arylthio, alkylamino, dialkylamino, arylamino or diarylamino.
摘要翻译：本发明涉及式I的铜（I）络合物，其中X是氮或CR基团，R是烷基或芳基，Ar是苯基或萘基，其各自任选被1-3个基团取代选自烷氧基，烷硫基，烷基氨基，二烷基氨基，烷氧基羰基，烷氧基磺酰基，卤素，氰基，羧基，羟基磺酰基和硝基，并且两个任选取代的苯基或萘基可以通过化学单键经由氰基，氰硫基，烷氧基，芳氧基，烷硫基，芳硫基，烷基氨基，二烷基氨基，芳基氨基或二芳基氨基，其中R 1，R 2，在有机发光二极管（OLED）中，本发明还涉及包含至少一种式I的铜（I）络合物的发光层与包含至少一种式（I）的络合物我还是一个透气发光层，以及包括本发明的OLED的静止视觉显示单元。此外，本发明涉及式Ia和Ib的新型铜（I）络合物，其中R，Ar和n各自如式I中所定义，式Ia中的Y定义为氰基，氰硫基，烷氧基，芳氧基，烷硫基，氰基，氰硫基，烷氧基，芳氧基，烷硫基，芳硫基，烷氨基，二烷基氨基，芳基氨基或二芳基氨基。

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