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1. 发明申请

WO2002096839A1 FISCHER-TROPSCH PROCESS 审中-公开
标题翻译： FISCHER-TROPSCH过程
公开(公告)号：WO2002096839A1
公开(公告)日：2002-12-05
申请号：PCT/GB2002/002310
申请日：2002-05-17
申请人： BP EXPLORATION OPERAING COMPANY LIMITED , DAVY PROCESS TECHNOLOGY LIMITED , FONT FREIDE, Josephus, Johannes, Helena, Maria , LENG, Stephen, Anthony , SHARP, Christopher
发明人： FONT FREIDE, Josephus, Johannes, Helena, Maria , LENG, Stephen, Anthony , SHARP, Christopher
IPC分类号： C07C1/06
CPC分类号： C07C1/06 , B01J8/228 , B01J19/26 , B01J23/80 , B01J2208/00256 , B01J2208/00274 , B01J2208/00283 , B01J2208/003 , B01J2208/00398 , B01J2208/00415 , B01J2219/00006 , B01J2219/185 , B01J2219/1943 , C07C2523/80 , C10G2/32 , C10G2300/1022 , C10G2300/4081 , C07C9/02
摘要： The present invention provides a process for the conversion of synthesis gas to hydrocarbons comprising the steps of: a) contacting synthesis gas at an elevated temperature and pressure with a particulate Fischer-Tropsch catalyst in a Fischer-Tropsch reactor system to generate hydrocarbons comprising gaseous and liquid hydrocarbons; b) in a gas separation zone, separating a gaseous phase comprising saturated gaseous hydrocarbons from a liquid phase comprising liquid hydrocarbons and from the particulate Fischer-Tropsch catalyst; c) passing at least a portion of the separated gaseous phase to a dehydrogenation reactor where at least a portion of the saturated gaseous hydrocarbons are converted to unsaturated hydrocarbons; and d) recycling at least a portion of said unsaturated hydrocarbons back to the Fischer-Tropsch reactor system.
摘要翻译：本发明提供了一种将合成气转化为烃的方法，包括以下步骤：a）在费 - 托反应器系统中将高温和高压的合成气与微量费 - 托催化剂接触以产生包含气态和液态烃; b）在气体分离区中，从包含液体烃的液相和来自微量费 - 托催化剂的液相中分离包含饱和气态烃的气相; c）将至少一部分分离的气相通入脱氢反应器，其中至少一部分饱和气态烃转化为不饱和烃; 和d）将至少一部分所述不饱和烃再循环回费 - 托反应器系统。

2. 发明申请

WO2002096837A3 FISCHER-TROPSCH PROCESS 审中-公开
公开(公告)号：WO2002096837A3
公开(公告)日：2002-12-05
申请号：PCT/GB2002/002332
申请日：2002-05-17
申请人： BP EXPLORATION OPERATING COMPANY LIMITED , DAVY PROCESS TECHNOLOGY LIMITED , FONT FREIDE, Josephus, Johannes, Helena, Maria , HENSMAN, John, Richard , NEWTON, David , SHARP, Christopher , SMITH, Geoffrey, Benedict
发明人： FONT FREIDE, Josephus, Johannes, Helena, Maria , HENSMAN, John, Richard , NEWTON, David , SHARP, Christopher , SMITH, Geoffrey, Benedict
IPC分类号： C10G2/00
摘要： A process for the conversion of synthesis gas to hydrocarbons by contacting the synthesis gas at an elevated temperature and pressure with a suspension comprising a solid particulate catalyst suspended in a liquid medium, which contacting takes place in a system comprising at least one high shear mixing zone and a reactor vessel wherein the volume of suspension present in the high shear mixing zone(s) is substantially less than the volume of suspension present in the reactor vessel, suspension is mixed with synthesis gas in the high shear mixing zone(s), the resulting mixture of suspension and synthesis gas is discharged from the high shear mixing zone(s) into the reactor vessel and wherein kinetic energy is dissipated to the suspension present in the high shear mixing zone(s) at a rate of at least 0.5 kW/m 3 relative to the total volume of suspension present in the system.

3. 发明申请

WO2002097011A2 FISCHER-TROPSCH PROCESS 审中-公开
标题翻译： FISCHER-TROPSCH过程
公开(公告)号：WO2002097011A2
公开(公告)日：2002-12-05
申请号：PCT/GB2002/002328
申请日：2002-05-17
申请人： BP EXPLORATION OPERATING COMPANY LIMITED , DAVY PROCESS TECHNOLOGY LIMITED , FONT FREIDE, Josephus, Johannes, Helena, Maria , NAY, Barry , SHARP, Christopher
发明人： FONT FREIDE, Josephus, Johannes, Helena, Maria , NAY, Barry , SHARP, Christopher
IPC分类号： C10G2/00
CPC分类号： C10G2/332 , C10G2/342
摘要： A process which comprises contacting a gaseous reactant stream comprising synthesis gas at elevated temperature and pressure with a suspension of a particulate Fischer-Tropsch catalyst comprising cobalt in a liquid medium in a reactor system comprising at least one high shear mixing zone and a reactor vessel wherein the process comprises the steps of: a) contacting the particulate Fischer-Tropsch catalyst with a reducing gas at elevated temperature and pressure outside of the high shear mixing zone(s) and the reactor vessel and subsequently suspending the particulate Fischer-Tropsch catalyst in the liquid medium; b) passing the suspension from step a) through the high shear mixing zone(s) where the gaseous reactant stream comprising synthesis gas is mixed with the suspension; c) discharging a mixture comprising the synthesis gas and the suspension from the high shear mixing zone(s) into the reactor vessel; and d) converting the synthesis gas to liquid hydrocarbons in the reactor vessel to form a product suspension comprising the particulate Fischer-Tropsch catalyst suspended in the liquid medium and liquid hydrocarbons.
摘要翻译：一种方法，其包括使包含合成气体的气态反应物流在升高的温度和压力下与包含钴的微粒费 - 托催化剂的悬浮液在包含至少一个高剪切混合区和反应器容器的反应器系统中的液体介质中接触，该方法包括以下步骤：a）在高剪切混合区和反应器容器外的升高的温度和压力下使微量费 - 托催化剂与还原气体接触，随后将颗粒状费 - 托催化剂悬浮在液体介质; b）将来自步骤a）的悬浮液通过高剪切混合区，其中包含合成气的气态反应物流与悬浮液混合; c）将包含合成气和悬浮液的混合物从高剪切混合区排出到反应器容器中; 和d）将合成气转化为反应器容器中的液体烃，以形成悬浮在液体介质中的包含微量费 - 托催化剂和液体烃的产物悬浮液。

4. 发明申请

WO2002096833A3 FISCHER-TROPSCH PROCESS 审中-公开
公开(公告)号：WO2002096833A3
公开(公告)日：2002-12-05
申请号：PCT/GB2002/002256
申请日：2002-05-17
申请人： BP EXPLORATION OPERATING COMPANY LIMITED , DAVY PROCESS TECHNOLOGY LIMITED , FONT-FREIDE, Josephus, Johannes, Helena, Maria , NEWTON, David , SHARP, Christopher
发明人： FONT-FREIDE, Josephus, Johannes, Helena, Maria , NEWTON, David , SHARP, Christopher
IPC分类号： C10G2/00
摘要： A process for the conversion of synthesis gas to higher hydrocarbons by contacting a gaseous stream comprising synthesis gas, at an elevated temperature and pressure, with a suspension comprising a particulate Fischer-Tropsch catalyst suspended in a liquid medium, in a reactor system comprising at least one high shear mixing zone and a tubular loop reactor wherein the process comprises: a) passing the suspension and the gaseous stream through the high shear mixing zone(s) wherein the gaseous stream is broken down into gas bubbles and/or irregularly shaped gas voids; b) discharging suspension having gas bubbles and/or irregularly shaped gas voids dispersed therein from the high shear mixing zone(s) into the tubular loop reactor; c) circulating the discharged suspension around the tubular loop reactor; and d) withdrawing a product suspension stream comprising at least a portion of the circulating suspension from the tubular loop reactor.

5. 发明申请

WO2002097012A3 FISCHER-TROPSCH PROCESS 审中-公开
公开(公告)号：WO2002097012A3
公开(公告)日：2002-12-05
申请号：PCT/GB2002/002334
申请日：2002-05-17
申请人： BP EXPLORATION OPERATING COMPANY LIMITED , DAVY PROCESS TECHNOLOGY LIMITED , LENG, Stephen, Anthony , SHARP, Christopher
发明人： LENG, Stephen, Anthony , SHARP, Christopher
IPC分类号： C10G2/00
摘要： A process for the conversion of synthesis gas to product comprising liquid hydrocarbons wherein said process comprises contacting synthesis gas at an elevated temperature and pressure with a mixed particulate catalyst comprising a mixture of a particulate Fischer-Tropsch catalyst and a particulate hydrocracking and/or isomerisation catalyst.

6. 发明申请

WO2002097010A2 FISCHER-TROPSCH PROCESS 审中-公开
标题翻译： FISCHER-TROPSCH过程
公开(公告)号：WO2002097010A2
公开(公告)日：2002-12-05
申请号：PCT/GB2002/002326
申请日：2002-05-17
申请人： BP EXPLORATION OPERATING COMPANY LIMITED , DAVY PROCESS TECHNOLOGY LIMITED , NAY, Barry , SHARP, Christopher
发明人： NAY, Barry , SHARP, Christopher
IPC分类号： C10G2/00
CPC分类号： C10G2/342
摘要： A process for the conversion of synthesis gas to hydrocarbons, at least a portion of which are liquid at ambient temperature and pressure, by contacting the synthesis gas at an elevated temperature and pressure with a suspension comprising a solid particulate Fischer-Tropsch catalyst suspended in a liquid medium, which contacting takes place in a reactor system comprising at least one high shear mixing zone and a reactor vessel wherein the volume of suspension present in the high shear mixing zone(s) is substantially less than the volume of suspension present in the reactor vessel, which process comprises: mixing the suspension with synthesis gas in the high shear mixing zone(s) and dissipating kinetic energy to the suspension present in the high shear mixing zone(s) at a rate of at least 0.5kW/m 3 relative to the total volume of suspension present in the reactor system; discharging the resulting mixture of synthesis gas and suspension from the high shear mixing zone(s) into the reactor vessel; withdrawing suspension from the reactor vessel and, at least in part, recycling the suspension to the high shear mixing zone(s); wherein the suspension which is recycled to the high shear mixing zone(s) is cooled to a temperature which is not more than 100°C below the temperature of the suspension in the reactor vessel with the proviso that the temperature of the cooled suspension is at least 150°C.
摘要翻译：一种将合成气转化为烃的方法，其中至少一部分在环境温度和压力下为液态，通过使合成气在升高的温度和压力下与悬浮在一种固体颗粒状费托催化剂中的悬浮液液体介质，其在包括至少一个高剪切混合区和反应器容器的反应器系统中进行，其中存在于高剪切混合区中的悬浮体的体积基本上小于存在于反应器中的悬浮液的体积容器，该方法包括：将混合物与合成气混合在高剪切混合区中，并以至少0.5kW / m 3的速率向存在于高剪切混合区域中的悬浮液释放动能 >相对于存在于反应器系统中的悬浮体的总体积; 将所得的合成气和悬浮液的混合物从高剪切混合区排出到反应器容器中; 从反应器容器中取出悬浮液，并且至少部分地将悬浮液再循环到高剪切混合区域; 其中循环到高剪切混合区的悬浮液被冷却到低于反应器容器中悬浮液温度不超过100℃的温度，条件是冷却的悬浮液的温度在至少150℃

7. 发明公开

EP1392622A2 FISCHER-TROPSCH PROCESS 有权
标题翻译： FISCHER-TROPSCH过程
公开(公告)号：EP1392622A2
公开(公告)日：2004-03-03
申请号：EP02730434.4
申请日：2002-05-17
申请人： BP EXPLORATION OPERATING COMPANY LIMITED , Davy Process Technology Limited
发明人： FONT FREIDE, Josephus, Johannes, Helena, Maria , HENSMAN, John, Richard , NEWTON, David , SHARP, Christopher , SMITH, Geoffrey, Benedict
IPC分类号： C07C1/00
CPC分类号： C10G2/342 , B01J8/228 , B01J2208/00132 , B01J2208/00256 , B01J2208/003 , C07C1/0485
摘要： A process for the conversion of synthesis gas to hydrocarbons by contacting the synthesis gas at an elevated temperature and pressure with a suspension comprising a solid particulate catalyst suspended in a liquid medium, which contacting takes place in a system comprising at least one high shear mixing zone and a reactor vessel wherein the volume of suspension present in the high shear mixing zone(s) is substantially less than the volume of suspension present in the reactor vessel, suspension is mixed with synthesis gas in the high shear mixing zone(s), the resulting mixture of suspension and synthesis gas is discharged from the high shear mixing zone(s) into the reactor vessel and wherein kinetic energy is dissipated to the suspension present in the high shear mixing zone(s) at a rate of at least 0.5 kW/m3 relative to the total volume of suspension present in the system.
摘要翻译：通过使合成气在升高的温度和压力下与包含悬浮在液体介质中的固体颗粒催化剂的悬浮液接触而将合成气转化为烃的方法，该方法发生在包含至少一个高剪切混合区和反应器容器，其中存在于高剪切混合区中的悬浮液的体积基本上小于存在于反应器容器中的悬浮液的体积，悬浮液在合成气的高剪切混合区中与混合气混合，得到的悬浮液和合成气的混合物从高剪切混合区排出到反应器容器中，并且其中动能以至少0.5kW / s的速率消散到存在于高剪切混合区中的悬浮液中。 m3相对于系统中存在的悬浮液的总体积。

8. 发明公开

EP1390444A2 FISCHER-TROPSCH PROCESS 审中-公开
标题翻译： FISCHER-TROPSCH过程
公开(公告)号：EP1390444A2
公开(公告)日：2004-02-25
申请号：EP02727733.4
申请日：2002-05-17
申请人： BP EXPLORATION OPERATING COMPANY LIMITED , Davy Process Technology Limited
发明人： FONT FREIDE, Josephus Johannes Helena Maria , NAY, Barry,"Little Wissett" , SHARP, Christopher
IPC分类号： C10G2/00
CPC分类号： C10G2/332 , C10G2/342
摘要： A process which comprises contacting a gaseous reactant stream comprising synthesis gas at elevated temperature and pressure with a suspension of a particulate Fischer-Tropsch catalyst comprising cobalt in a liquid medium in a reactor system comprising at least one high shear mixing zone and a reactor vessel wherein the process comprises the steps of: a) contacting the particulate Fischer-Tropsch catalyst with a reducing gas at elevated temperature and pressure outside of the high shear mixing zone(s) and the reactor vessel and subsequently suspending the particulate Fischer-Tropsch catalyst in the liquid medium; b) passing the suspension from step a) through the high shear mixing zone(s) where the gaseous reactant stream comprising synthesis gas is mixed with the suspension; c) discharging a mixture comprising the synthesis gas and the suspension from the high shear mixing zone(s) into the reactor vessel; and d) converting the synthesis gas to liquid hydrocarbons in the reactor vessel to form a product suspension comprising the particulate Fischer-Tropsch catalyst suspended in the liquid medium and liquid hydrocarbons.
摘要翻译：一种方法，包括在升高的温度和压力下使包含合成气的气态反应物流与包含钴的颗粒费 - 托催化剂在液体介质中的悬浮液在包含至少一个高剪切混合区和反应器容器的反应器系统中接触，其中该方法包括以下步骤：a）使颗粒费 - 托催化剂与还原性气体在高剪切混合区和反应器容器外的高温高压下接触，随后将颗粒费 - 托催化剂悬浮于液体介质; b）使来自步骤a）的悬浮液通过高剪切混合区，其中含有合成气的气态反应物流与悬浮液混合; c）将包含合成气和悬浮液的混合物从高剪切混合区排出到反应器中; 和d）在反应器容器中将合成气转化为液态烃以形成包含悬浮在液体介质中的颗粒费 - 托催化剂和液态烃的产物悬浮液。

9. 发明公开

EP1392794A2 FISCHER-TROPSCH PROCESS 审中-公开
标题翻译： FISCHER-TROPSCH过程
公开(公告)号：EP1392794A2
公开(公告)日：2004-03-03
申请号：EP02727734.2
申请日：2002-05-17
申请人： BP EXPLORATION OPERATING COMPANY LIMITED , Davy Process Technology Limited
发明人： LENG, Stephen Anthony , SHARP, Christopher
IPC分类号： C10G2/00
CPC分类号： C10G2/332 , C10G2/342 , C10G45/66 , C10G47/26
摘要： A process for the conversion of synthesis gas to product comprising liquid hydrocarbons wherein said process comprises contacting synthesis gas at an elevated temperature and pressure with a mixed particulate catalyst comprising a mixture of a particulate Fischer-Tropsch catalyst and a particulate hydrocracking and/or isomerisation catalyst.
摘要翻译：一种将合成气转化成包含液态烃的产物的方法，其中所述方法包括使合成气在升高的温度和压力下与混合的颗粒状催化剂接触，所述混合的颗粒状催化剂包含颗粒费 - 托催化剂和颗粒状加氢裂化和/或异构化催化剂。

10. 发明授权

EP1392622B1 FISCHER-TROPSCH PROCESS 有权
标题翻译： FISCHER TROPSCHVERFAHREN
公开(公告)号：EP1392622B1
公开(公告)日：2005-01-12
申请号：EP02730434.4
申请日：2002-05-17
申请人： BP EXPLORATION OPERATING COMPANY LIMITED , Davy Process Technology Limited
发明人： FONT FREIDE, Josephus, Johannes, Helena, Maria , HENSMAN, John, Richard , NEWTON, David , SHARP, Christopher , SMITH, Geoffrey, Benedict
IPC分类号： C07C1/00
CPC分类号： C10G2/342 , B01J8/228 , B01J2208/00132 , B01J2208/00256 , B01J2208/003 , C07C1/0485
摘要： A process for the conversion of synthesis gas to hydrocarbons by contacting the synthesis gas at an elevated temperature and pressure with a suspension comprising a solid particulate catalyst suspended in a liquid medium, which contacting takes place in a system comprising at least one high shear mixing zone and a reactor vessel wherein the volume of suspension present in the high shear mixing zone(s) is substantially less than the volume of suspension present in the reactor vessel, suspension is mixed with synthesis gas in the high shear mixing zone(s), the resulting mixture of suspension and synthesis gas is discharged from the high shear mixing zone(s) into the reactor vessel and wherein kinetic energy is dissipated to the suspension present in the high shear mixing zone(s) at a rate of at least 0.5 kW/m3 relative to the total volume of suspension present in the system.

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