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1. 发明专利

JP2002114815A ZIEGLER-NATTA TYPE CATALYST COMPOSITION AND METHOD FOR PRODUCING THE SAME 审中-公开
公开(公告)号：JP2002114815A
公开(公告)日：2002-04-16
申请号：JP2001247639
申请日：2001-08-17
申请人： BASELL POLYOLEFINE GMBH
发明人： FOETTINGER KLAUS , HUEFFER STEPHAN DR , KARER RAINER
IPC分类号： C08F4/658 , C08F4/646 , C08F4/654 , C08F4/656 , C08F10/00 , C08F110/02
摘要： PROBLEM TO BE SOLVED: To obtain a catalyst composition free from a disadvantage of reduction in activity when a polysiloxane is used. SOLUTION: This Ziegler-Natta type catalyst composition suitable for an olefin polymerization is produced by (A) a process for bringing an inorganic metal oxide of precipitated magnesium compound into contact with a tetravalent titanium compound, (B) optionally, a process for bringing an intermediate obtained by the method into contact with an electron donor and (C) a process for bringing the intermediate obtained by the process (A) or the process (B) into contact with a polysiloxane. This method for polymerizing or copolymerizing an olefin in the presence of an aluminum compound as a cocatalyst is provided.

2. 发明申请

WO0232969A3 CATALYTIC SYSTEMS OF THE ZIEGLER-NATTA TYPE AND METHOD FOR PRODUCTION THEREOF 审中-公开
标题翻译： Ziegler-Natta催化剂催化剂系统类型及其制备方法
公开(公告)号：WO0232969A3
公开(公告)日：2002-07-25
申请号：PCT/EP0112048
申请日：2001-10-18
申请人： BASELL POLYOLEFINE GMBH , FOETTINGER KLAUS , FUNK GUIDO , KOELLE PETER , WULFF-DOERING JOACHIM
发明人： FOETTINGER KLAUS , FUNK GUIDO , KOELLE PETER , WULFF-DOERING JOACHIM
IPC分类号： C08F4/646 , C08F4/658 , C08F10/00
CPC分类号： C08F10/00 , C08F4/6555
摘要： A method for production of catalytic systems of the Ziegler-Natta type is characterised in comprising the following steps: A) bringing an inorganic metal oxide and a magnesium compound of formula MgRnX2-n into contact, where X = independently, fluorine, chlorine, bromine, iodine, hydrogen, NR2, OR, SR, SO3R or OC(O)R and R = independently, C1-C20 linear, branched, or cyclic alkyl, a C2-C10 alkenyl, an alkylaryl with 1-10 C atoms in the alkyl group and 6-20 C atoms in the aryl group, or a C6-C18 aryl and n =1 or 2, then, B) bringing the intermediate product obtained in step A) into contact with a halogenating reagent, C) bringing the intermediate product obtained in step B) into contact with a) a tetravalent titanium compound, b) a metallo-organic compound of group 3 of the periodic system and c) optionally, an electron-donor compound and D) washing the product obtained in step C) with an aprotic solvent. The invention further relates to a catalytic system obtained as above and a method for the polymerisation of olefins.
摘要翻译：一种用于制备齐格勒 - 纳塔催化剂的催化剂体系，方法，其特征在于它包括以下步骤：A）与镁化合物MgRnX2-n其中X独立地是氟，氯，溴，碘，氢使无机金属氧化物， NR 2，OR，SR，SO 3 R，或OC（O）R，和R独立地表示C1-C20直链，支链或环状烷基，C2-C10链烯基，在烷基部分和6-20个C 1-10个碳原子的烷芳 -atoms在芳基部分或C6-C18芳基，和n是1或2，然后，B）接触得到的，根据与卤化试剂，C）使在步骤B中得到的中间体）与步骤a）中间体）四价钛化合物，b）周期表和c）任选的电子供体，以及d）。步骤C后获得的产物的洗涤）的3组的与非质子LO一个mallorganischen化合物溶剂，从而使可用的催化剂体系和用于烯烃聚合的方法。

3. 发明专利

DE10163075A1 未知
公开(公告)号：DE10163075A1
公开(公告)日：2003-07-10
申请号：DE10163075
申请日：2001-12-20
申请人： BASELL POLYOLEFINE GMBH
发明人： FOETTINGER KLAUS , SCHNEIDER MARTIN-JULIUS , KARER RAINER
IPC分类号： C08F4/655 , C08F4/658 , C08F10/02 , C08F36/04 , C08F210/16
摘要： The present invention relates to catalyst systems of the Ziegler-Natta type, to a process for preparing them, to their use for the polymerization of olefins and to ethylene copolymers which can be prepared using this catalyst system.

4. 发明专利

AT467647T 未知
公开(公告)号：AT467647T
公开(公告)日：2010-05-15
申请号：AT08701494
申请日：2008-01-15
申请人： BASELL POLYOLEFINE GMBH
发明人： FOETTINGER KLAUS , HECKER MANFRED , BERGER LOTHAR , KARER RAINER , LILGE DIETER
IPC分类号： C08F210/02
摘要： Monomodal copolymers of ethylene and molding compositions comprising such copolymers, wherein the copolymers have a density determined according to DIN EN ISO 1183-1, variant A in the range from 0.938 to 0.944 g/cm3, a melt index MFR21 determined according to ISO 1133 at 190° C. under a load of 21.6 kg in the range from 12 to 17 g/10 min, a weight average molar mass Mw in the range from 140 000 g/mol to 330 000 g/mol, a polydispersity Mw/Mn in the range from 9 to 17, and a content of comonomer side chains per 1000 carbon atoms Cx equal to or above a value defined via equation (I) Cx=128.7−134.62×d′, wherein d′ is the numerical value of the density of the copolymer in g/cm3, the use of the copolymers for producing injection-molded articles, as well as injection-molded articles comprising the copolymers, and process for the preparation of such monomodal copolymers.

5. 发明专利

DE602008001250D1 EINMODUS-COPOLYMER VON ETHYLEN ZUM SPRITZGIESSEN UND VERFAHREN ZU DESSEN HERSTELLUNG 未知
公开(公告)号：DE602008001250D1
公开(公告)日：2010-06-24
申请号：DE602008001250
申请日：2008-01-15
申请人： BASELL POLYOLEFINE GMBH
发明人： FOETTINGER KLAUS , HECKER MANFRED , BERGER LOTHAR , KARER RAINER , LILGE DIETER
IPC分类号： C08F210/02

6. 发明专利

AR044022A1 SISTEMAS CATALIZADORES DEL TIPO ZIEGLER-NATTA Y UN PROCESO PARA PREPARARLOS 未知
公开(公告)号：AR044022A1
公开(公告)日：2005-08-24
申请号：ARP040101271
申请日：2004-04-15
申请人： BASELL POLYOLEFINE GMBH
发明人： FOETTINGER KLAUS
IPC分类号： C08F4/02 , C08F4/656 , C08F10/00 , C08F110/02 , C08F210/16 , C08F4/64 , C08F4/654
摘要： Un proceso para preparar sistemas catalizadores del tipo Ziegler-Natta, que comprende los siguientes pasos: A) poner en contacto un óxido de metal inorgánico con un compuesto de titanio tetravalente, y B) poner en contacto el compuesto intermedio obtenido del paso A) con un compuesto de magnesio MgR1nX12-n, en donde X1 son cada uno, independientemente del otro, flúor, cloro, bromo, yodo, hidrógeno, NRx2, ORx, SRx, SO3Rx u OC(O)Rx, y R1 y Rx son, cada uno, independientemente del otro, un alquilo C1-20 cíclico, ramificado o lineal, un alquenilo C2-10, un alquilarilo C1-10 en la parte de alquilo y C6-20 en la parte de arilo o un arilo C6-18 y n es 1 ó 2; C) poner en contacto el compuesto intermedio obtenido del paso B) con un reactivo de halogenación de la fórmula Rys-E-Y4-5, en donde Ry son cada uno, independientemente del otro, hidrógeno, un alquilo C1-20 cíclico, ramificado o lineal, un alquenilo C2-10, un alquilarilo C1-10 en la parte de alquilo y C6-20 en la parte de arilo o un arilo C6-18m, E es carbono o silicio, Y es flúor, cloro, bromo o yodo y s es 0, 1, 2 ó 3 cuando E es carbono y s es 1,2 ó 3 cuando E es silicio. Sistema catalizador del tipo Ziegler-Natta y sistema catalizador prepolimerizado que comprende un sistema catalizador obtenido según el proceso anterior. Proceso para la polimerización o copolimerización de olefinas y uso del sistema catalizador descripto para la polimerización o copolimerización de olefinas.

7. 发明专利

AR044021A1 SISTEMAS CATALIZADORES DEL TIPO ZIEGLER-NATTA Y UN PROCESO PARA PREPARARLOS 未知
公开(公告)号：AR044021A1
公开(公告)日：2005-08-24
申请号：ARP040101270
申请日：2004-04-15
申请人： BASELL POLYOLEFINE GMBH
发明人： FOETTINGER KLAUS , SCHNEIDER MARTIN
IPC分类号： C08F4/02 , C08F110/02 , C08F210/16 , C08F4/64 , C08F4/654 , C08F10/00
摘要： Un proceso para preparar sistemas catalizadores del tipo Ziegler-Natta, que comprende los siguientes pasos: A) poner en contacto un óxido de metal inorgánico con un compuesto de titanio tetravalente, y B) poner en contacto el compuesto intermedio obtenido del paso A) con un compuesto de magnesio MgR1nX12-n, en donde X1 son cada uno, independientemente del otro, flúor, cloro, bromo, yodo, hidrógeno, NRx2, ORx, SRx, SO3Rx u OC(O)Rx, y R1 y Rx son, cada uno, independientemente del otro, un alquilo C1-20 cíclico, ramificado o lineal, un alquenilo C2-10, un alquilarilo C1-10 en la parte de alquilo y C6-20 en la parte de arilo o un arilo C6-18 y n es 1 ó 2; C) poner en contacto el compuesto intermedio obtenido del paso B) con un reactivo de halogenación; y D) poner en contacto el intermedio obtenido del paso C) con un compuesto donador. Sistema catalizador del tipo Ziegler-Natta y sistema catalizador prepolimerizado que comprende el sistema catalizador obtenido según el proceso anterior. Proceso para la polimerización o copolimerización de olefinas y uso del sistema catalizador descripto para la polimerización o copolimerización de olefinas.

8. 发明专利

BRPI0806786A2 未知
公开(公告)号：BRPI0806786A2
公开(公告)日：2011-09-13
申请号：BRPI0806786
申请日：2008-01-15
申请人： BASELL POLYOLEFINE GMBH
发明人： FOETTINGER KLAUS , HECKER MANFRED , BERGER LOTHAR , KARER RAINER , LILGE DIETER
IPC分类号： C08F210/02
摘要： Monomodal copolymers of ethylene and molding compositions comprising such copolymers, wherein the copolymers have a density determined according to DIN EN ISO 1183-1, variant A in the range from 0.938 to 0.944 g/cm3, a melt index MFR21 determined according to ISO 1133 at 190° C. under a load of 21.6 kg in the range from 12 to 17 g/10 min, a weight average molar mass Mw in the range from 140 000 g/mol to 330 000 g/mol, a polydispersity Mw/Mn in the range from 9 to 17, and a content of comonomer side chains per 1000 carbon atoms Cx equal to or above a value defined via equation (I) Cx=128.7−134.62×d′, wherein d′ is the numerical value of the density of the copolymer in g/cm3, the use of the copolymers for producing injection-molded articles, as well as injection-molded articles comprising the copolymers, and process for the preparation of such monomodal copolymers.

9. 发明专利

DE10317398A1 Preparation of Ziegler-Natta type catalyst systems involves contacting inorganic metal oxide with tetravalent titanium compound, and contacting obtained intermediate with magnesium compound and then with halogenating reagent 未知
公开(公告)号：DE10317398A1
公开(公告)日：2004-11-04
申请号：DE10317398
申请日：2003-04-15
申请人： BASELL POLYOLEFINE GMBH
发明人： FOETTINGER KLAUS
IPC分类号： C08F10/00 , C08F110/02 , C08F210/16 , C08F4/658 , C08F4/651 , C08F4/654 , C08F4/656 , C08F10/02
摘要： Ziegler-Natta type catalyst systems are prepared by bringing an inorganic metal oxide into contact with a tetravalent titanium compound; bringing the obtained intermediate into contact with a magnesium compound; and then, bringing the obtained intermediate into contact with a halogenating reagent. Preparation of Ziegler-Natta type catalyst systems includes bringing an inorganic metal oxide into contact with a tetravalent titanium compound; bringing the obtained intermediate into contact with a magnesium compound of formula: MgR 1> nX 1> 2 - n; and then, bringing the obtained intermediate into contact with a halogenating reagent of formula: (R-Y) s-E-Y 4 - s. X 1>F, Cl, Br, I, H, N(R ->X) 2, O(R-X), S(R-X), SO 3(R-X) or OC(O)(R-X); R 1>, R-X, R-Y : 1-20C alkyl, 2-10C alkenyl, alkylaryl having 1-10C in the alkyl part and 6-20C in the aryl part or 6-18C aryl; n : 1 or 2; E : C or Si; Y : F, Cl, Br or I; s : 0, 1, 2 or 3 when E is carbon; and s : 1, 2 or 3 when E is silicon. Independent claims are also included for: (1) a prepolymerized catalyst system, comprising a catalyst system prepared as above; and linear 2-10C 1-alkene polymerized onto it in a mass ratio of 1:0.1-1:200; and (2) a process for the polymerization or copolymerization of olefins at 20-150[deg]C and pressures of 1-100 bar in the presence of catalyst system(s) as above and, if appropriate, an aluminum compound as co-catalyst.

10. 发明专利

DE10317395A1 Preparation of Ziegler-Natta type catalyst systems by contacting inorganic metal oxide with tetravalent titanium compound, and contacting obtained intermediate with magnesium compound, with halogenating reagent and then with donor compound 未知
公开(公告)号：DE10317395A1
公开(公告)日：2004-11-04
申请号：DE10317395
申请日：2003-04-15
申请人： BASELL POLYOLEFINE GMBH
发明人： FOETTINGER KLAUS , SCHNEIDER MARTIN
IPC分类号： C08F110/02 , C08F210/16 , C08F4/654 , C08F4/02 , C08F4/642 , C08F4/651 , C08F10/02
摘要： Preparation of Ziegler-Natta type catalyst systems includes bringing an inorganic metal oxide into contact with a tetravalent titanium compound; bringing the obtained intermediate into contact with a magnesium compound; bringing the obtained intermediate into contact with a halogenating reagent; and then, bringing the obtained intermediate into contact with a donor compound. Preparation of Ziegler-Natta type catalyst systems includes bringing an inorganic metal oxide into contact with a tetravalent titanium compound; bringing the obtained intermediate into contact with a magnesium compound MgR 1> nX 1> 2 - n; bringing the obtained intermediate into contact with a halogenating reagent; and then, bringing the obtained intermediate into contact with a donor compound. X 1>F, Cl, Br, I, H, N(R-X) 2, O(R-X), SO 3(R-X) or OC(O)R-X; R 1>, R-X : 1-20C alkyl, 2-10C alkenyl, alkylaryl having 1-10C in the alkyl part and 6-20C in the aryl part or 6-18C aryl;and n : 1 or 2. Independent claims are also included for: (1) a prepolymerized catalyst system, comprising a catalyst system as prepared by the above process; and linear 2-10C-1-alkenes polymerized onto the catalyst system in a mass ratio of 1:0.1-1:200; and (2) a process for the polymerization or copolymerization of olefins at 20-150[deg]C and pressures of 1-100 bar in the presence of catalyst system(s) as above and, if appropriate, an aluminum compound as co-catalyst.

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