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1. 发明专利

JP2008258168A Heat-resistant polymer electrolyte 有权
标题翻译：耐热聚合物电解液
公开(公告)号：JP2008258168A
公开(公告)日：2008-10-23
申请号：JP2008104388
申请日：2008-04-14
申请人： Asahi Kasei Chemicals Corp , Toyota Central R&D Labs Inc , Toyota Motor Corp , トヨタ自動車株式会社 , 旭化成ケミカルズ株式会社 , 株式会社豊田中央研究所
发明人： TSUSAKA KYOKO , HASEGAWA NAOKI , KAWAKADO MASAYA , YAMAMOTO TAKASHI , KAMIYA ATSUSHI , KAWAHARA KAZUO , HONDA EIJI , TAKAHASHI YASUSHI
IPC分类号： H01M8/02 , C25B13/08 , H01B1/06 , H01M8/10
CPC分类号： Y02E60/521
摘要： PROBLEM TO BE SOLVED: To provide a heat-resistant polymer electrolyte having superior heat resistance, strength, and ionic conductivity. SOLUTION: This heat-resistant polymer electrolyte 18 is provided with: a first layer 16 formed of a perfluoro-polymer electrolyte, having a strongly-acidic imide group and formed, by bringing a perfluoro-electrolyte precursor 10 into contact with a gas A, containing steam and/or alcohol gas, thereafter bringing the perfluoro-electrolyte precursor 10 into contact with a gas B containing ammonia gas and/or primary amine gas, and thereafter, converting the perfluoro-electrolyte precursor 10 to a proton type; and a second layer 14 formed on a surface of the first layer 16, and formed of a perfluoro-polymer electrolyte small in an introduction amount of the strongly-acidic imide group relative to the first layer 16 or without its introduction. COPYRIGHT: (C)2009,JPO&INPIT
摘要翻译：要解决的问题：提供具有优异的耐热性，强度和离子导电性的耐热聚合物电解质。解决方案：该耐热聚合物电解质18设置有：由全氟聚合物电解质形成的第一层16，其具有强酸性酰亚胺基并通过使全氟电解质前体10与气体A，含有蒸汽和/或醇气体，然后使全氟电解质前体10与含有氨气和/或伯胺气体的气体B接触，然后将全氟电解质前体10转化为质子型; 以及形成在第一层16的表面上的第二层14，并且由相对于第一层16引入强酸性酰亚胺基团的引导量小的全氟聚合物电解质形成，也可以不引入。版权所有（C）2009，JPO＆INPIT

2. 发明专利

JP2011241344A Polymer electrolyte, manufacturing method therefor, imide monomer, and battery 审中-公开
标题翻译：聚合物电解质，其制造方法，电子单体和电池
公开(公告)号：JP2011241344A
公开(公告)日：2011-12-01
申请号：JP2010116677
申请日：2010-05-20
申请人： Toyota Central R&D Labs Inc , Toyota Motor Corp , トヨタ自動車株式会社 , 株式会社豊田中央研究所
发明人： SHINOHARA AKIHIRO , HASEGAWA NAOKI , KAWAKADO MASAYA , TAKAMI MASAYOSHI , YOSHIDA TOSHIHIKO
IPC分类号： C08F228/00 , C07D285/00 , C08F234/00 , H01B1/06 , H01M4/86 , H01M8/02 , H01M8/10
CPC分类号： C08F14/18 , C07C311/48 , C07D285/01 , C07D285/15 , C07D285/36 , C07D513/08 , H01M8/1023 , H01M8/1039
摘要： PROBLEM TO BE SOLVED: To provide a polymer electrolyte having a high softening point and excellent in oxygen permeability and proton conductivity, to provide a manufacturing method therefor, to provide an imide monomer usable as a raw material of the polymer electrolyte, and to provide a battery using the polymer electrolyte.SOLUTION: There are provided a polymer electrolyte which includes a fluorine-containing structure having an alicyclic 1,3-disulfonimide in a principal chain or side chain of the polymer and a battery using the electrolyte. An imide monomer capable of introducing a fluorine-containing structure having an alicyclic 1,3-disulfonimide into a principal chain or side chain of a polymer through a polymerization reaction or a combination of a polymerization reaction and a fluorination reaction is provided. A manufacturing method for a polymer electrolyte, includes a polymerization step of polymerizing a raw material that includes one or more types of imide monomers capable of introducing a fluorine-containing structure having an alicyclic 1,3-disulfonimide into a principal chain or side chain of a polymer through a polymerization reaction or a combination of a polymerization reaction and a fluorination reaction.
摘要翻译：要解决的问题为了提供具有高软化点和优异的氧气渗透性和质子传导性的聚合物电解质，为了提供其制备方法，提供可用作聚合物电解质的原料的酰亚胺单体，以及以提供使用聚合物电解质的电池。解决方案：提供一种聚合物电解质，其包含在聚合物的主链或侧链中具有脂环族1,3-二磺酰亚胺的含氟结构和使用该电解质的电池。提供了能够通过聚合反应或聚合反应和氟化反应的组合将具有脂环族1,3-二磺酰亚胺的含氟结构引入聚合物的主链或侧链的酰亚胺单体。聚合物电解质的制造方法包括使包含能够将具有脂环式1,3-二磺酰亚胺的含氟结构物导入到主链或侧链的一种或多种类型的酰亚胺单体的原料聚合的聚合步骤通过聚合反应的聚合物或聚合反应和氟化反应的组合。版权所有（C）2012，JPO＆INPIT

3. 发明专利

JP2009187936A Electrolyte as well as manufacturing method thereof, electrolyte membrane as well as manufacturing method thereof, catalyst layer, and fuel cell 有权
标题翻译：电解质作为其制造方法，电解质膜作为其制造方法，催化层和燃料电池
公开(公告)号：JP2009187936A
公开(公告)日：2009-08-20
申请号：JP2008328792
申请日：2008-12-24
申请人： Toyota Central R&D Labs Inc , Toyota Motor Corp , トヨタ自動車株式会社 , 株式会社豊田中央研究所
发明人： HOSHIKAWA HISAHIRO , HOSOKAWA YOICHI , HASEGAWA NAOKI , KAWAKADO MASAYA , SHINOHARA AKIHIRO , TANAKA HIROMITSU , YOSHIDA TOSHIHIKO , TAKAMI MASAYOSHI
IPC分类号： H01B1/06 , C08G75/30 , C08G81/00 , H01B13/00 , H01M4/86 , H01M8/02 , H01M8/10
CPC分类号： Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide an electrolyte with high conductivity and hardly dissolving in or swelling against water, to provide a manufacturing method thereof, to provide an electrolyte membrane using the electrolyte, to provide a catalyst layer, and to provide a fuel cell. SOLUTION: The electrolyte has a structure where a fluorinated hydrophilic segment A represented by formula (1): -E 2 -[Rf-E 1 ] m -, and a hydrocarbon hydrophobic segment B are alternately bonded to each other through chemical bond. In the formula (1), Rf is a linear or a branched perfluoro chain having a carbon number of one or more, E1 and E2 are each a proton conductive portion represented by the formula α: -(CONM) i1 (CO) i2 (SO 2 NM) i3 (SO 2 ) i4 -, (In the formula α, 0≤i1, 0≤i2≤1, 0≤i3, 0≤i4≤1, 0 COPYRIGHT: (C)2009,JPO&INPIT
摘要翻译：要解决的问题：为了提供高导电性并且难以溶解或溶胀的电解质，以提供其制造方法，提供使用电解质的电解质膜，以提供催化剂层，并提供一种燃料电池。解决方案：电解质具有以下结构：式（1）表示的氟化亲水性链段A：-E 2 - [Rf -E 1 烃疏水链段B通过化学键彼此交替键合。式（1）中，Rf为碳数为1以上的直链或支链全氟链，E1和E2分别为由式α表示的质子传导部分： - （CONM） SB>（CO） i2 （SO 2 NM）（SO SB SB2） SB> - ，（式中，0≤i1,0≤i2≤1,0≤i3,0≤i4≤1,0

4. 发明专利

JP2012169042A Inorganic-organic composite solid electrolyte 审中-公开
标题翻译：无机有机复合固体电解质
公开(公告)号：JP2012169042A
公开(公告)日：2012-09-06
申请号：JP2011026558
申请日：2011-02-09
申请人： Toyota Central R&D Labs Inc , Toyota Motor Corp , トヨタ自動車株式会社 , 株式会社豊田中央研究所
发明人： MIURA FUSAYOSHI , ASANO TAKASHI , KAWAKADO MASAYA , FUJITA KEISUKE , TAKAMI MASAYOSHI
IPC分类号： H01B1/06 , H01M8/02 , H01M8/10
CPC分类号： Y02E60/521
摘要： PROBLEM TO BE SOLVED: To provide an inorganic-organic composite electrolyte which can enhance hydrogen peroxide resistance of a hydrocarbon-based electrolyte or a perfluoro-based electrolyte, and is less likely to degrade a battery performance.SOLUTION: The inorganic-organic composite electrolyte is obtained by bringing an additive solution, produced by dissolving an organic metal compound into an organic solvent having a dielectric constant of 10 or less, into contact with a solid polymer electrolyte, and then bringing the solid polymer electrolyte into contact with water or a solution containing cation having an action to enhance the hydrogen peroxide resistance of the solid polymer electrolyte.
摘要翻译：解决的问题：提供一种能够提高烃系电解质或全氟系电解质的耐过氧化氢性的无机 - 有机复合电解质，不太可能劣化电池性能。解决方案：通过将通过将有机金属化合物溶解到介电常数为10以下的有机溶剂中制成的添加剂溶液与固体聚合物电解质接触而获得无机 - 有机复合电解质，然后将固体聚合物电解质与水接触或含有阳离子的溶液，其具有增强固体聚合物电解质的耐过氧化氢性的作用。版权所有（C）2012，JPO＆INPIT

5. 发明专利

JP2011140605A High oxygen-permeable electrolyte, method for producing the same, and sulfonimide monomer 审中-公开
标题翻译：高氧可渗透电解质，其生产方法和磺化单体
公开(公告)号：JP2011140605A
公开(公告)日：2011-07-21
申请号：JP2010003369
申请日：2010-01-08
申请人： Toyota Central R&D Labs Inc , Toyota Motor Corp , トヨタ自動車株式会社 , 株式会社豊田中央研究所
发明人： SHINOHARA AKIHIRO , HASEGAWA NAOKI , KAWAKADO MASAYA , KUDO KENJI , KINJO TOMOYUKI , TAKAMI MASAYOSHI , YOSHIDA TOSHIHIKO
IPC分类号： C08F234/02 , C08F8/34 , C08F224/00 , H01B1/06 , H01B1/12 , H01B13/00 , H01M4/86 , H01M8/02 , H01M8/10
CPC分类号： Y02E60/521
摘要： PROBLEM TO BE SOLVED: To provide a high oxygen-permeable electrolyte high in softening temperature and excellent in oxygen permeability and proton conductivity, to provide a method for producing the same, and to provide a sulfonimide monomer usable as a raw material for such high oxygen-permeable electrolyte.
SOLUTION: The high oxygen-permeable electrolyte includes the structure represented by formula (A) (wherein P is a perfluorocarbon provided with an alicyclic structure; P' is a perfluorocarbon provided with an alicyclic structure or with an alicyclic structure and a chain-like structure; Q is a direct bond or a perfluorocarbon provided with a chain-like structure or an alicyclic structure; a is an integer of 1 or greater; n is an integer of 1 or greater, provided that n's may be different among the repeating units; and R
1 is OH or a sulfonimide group-linked perfluorocarbon group (-NHSO
2 Rf
1 )).
COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：为了提供高的软化温度的高透氧性电解质，透氧性和质子传导性优异，可以提供其制造方法，提供可用作原料的磺酰亚胺单体这种高透氧电解质。解决方案：高透氧性电解质包括由式（A）表示的结构（其中P是具有脂环结构的全氟化碳; P'是具有脂环结构或具有脂环结构和链的全氟化碳 Q是具有链状结构或脂环结构的直接键或全氟化碳; a为1以上的整数，n为1以上的整数，条件是n的整数为1以上重复单元; R“SP 1”是OH或与磺酰亚胺基相连的全氟化碳基团（-NHSO 2 SBR 2，R f＆lt; SP＆gt; 1））。版权所有（C）2011，JPO＆INPIT

6. 发明专利

JP2013056920A Noncrosslinking type layered phosphonic acid metal compound and method for production of the same 有权
标题翻译：非交联型层状磷酸金属化合物及其制造方法
公开(公告)号：JP2013056920A
公开(公告)日：2013-03-28
申请号：JP2012253644
申请日：2012-11-19
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： OGATA SHINICHI , FUKUSHIMA YOSHIAKI , KAWAKADO MASAYA
IPC分类号： C07F19/00 , C07F7/00 , C07F9/38
摘要： PROBLEM TO BE SOLVED: To provide a novel noncrosslinking type layered phosphonic acid metal compound which has high crystallinity and a uniformly introduced multicomponent phosphonic acid and is free of a fluorine atom, and to provide a method for the production of the same.SOLUTION: The method for the production of the noncrosslinking type layered phosphonic acid metal compound includes a reaction step of reacting two or more monophosphonic acids or derivatives thereof having predetermined conditions with a metal source that can generate a hexacoordinated metal atom ion to be a central atom (M) of a metal oxide octahedron upon reaction in the presence of a sulfuric acid catalyst. The noncrosslinking type layered phosphonic acid metal compound obtained by the production method is also provided.
摘要翻译：待解决的问题：提供一种具有高结晶度和均匀引入的多组分膦酸并且不含氟原子的新型非交联型层状膦酸金属化合物，并提供其制备方法。解决方案：制备非交联型层状膦酸金属化合物的方法包括使具有预定条件的两种或更多种单膦酸或其衍生物与能够产生六配位金属原子离子的金属源反应的反应步骤在硫酸催化剂存在下反应时，金属氧化物八面体的中心原子（M）。还提供了通过制备方法获得的非交联型层状膦酸金属化合物。版权所有（C）2013，JPO＆INPIT

7. 发明专利

JP2011129380A Lamella porous electrolyte 有权
标题翻译： LAMELLA多孔电解质
公开(公告)号：JP2011129380A
公开(公告)日：2011-06-30
申请号：JP2009286970
申请日：2009-12-17
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： FUJITA SATORU , OSUNA SATORU , KAWAKADO MASAYA , INAGAKI SHINJI
IPC分类号： H01B1/06 , C25B13/04 , H01M8/02
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide a lamella porous electrolyte showing a high proton conductivity even in a low humidity environment (in particular, low humidity in which aqueous capillary condensation is not caused). SOLUTION: A lamella porous electrolyte includes a lamella porous body having silica layers arranged in parallel at predetermined intervals and a silica pillar connecting between the silica layers and an organic sulfonate group decorating an inner surface of the silica layer. Preferably, a ratio (=D/L) of a distance D between the silica layers to a molecular length L of the organic sulfonate group is 1≤D/L≤3. COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：即使在低湿度环境（特别是没有引起水中毛细管冷凝的低湿度）下，也可提供显示出高质子传导性的薄片多孔电解质。解决方案：薄片多孔电解质包括具有以预定间隔平行布置的二氧化硅层和连接在二氧化硅层和装饰二氧化硅层的内表面的有机磺酸盐基团之间的二氧化硅柱的薄片多孔体。优选地，二氧化硅层之间的距离D与有机磺酸盐基团的分子长度L之比（= D / L）为1≤D/L≤3。版权所有（C）2011，JPO＆INPIT

8. 发明专利

JP2011040363A Reforming electrolyte and method of manufacturing the same, and reforming agent 有权
标题翻译：改性电解质及其制备方法和改性剂
公开(公告)号：JP2011040363A
公开(公告)日：2011-02-24
申请号：JP2009283472
申请日：2009-12-14
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： SHINOHARA AKIHIRO , HASEGAWA NAOKI , KAWAKADO MASAYA , KUDO KENJI , TANAKA HIROMITSU
IPC分类号： H01M8/02 , C08J5/22 , H01B1/06 , H01B13/00 , H01M8/10
CPC分类号： Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide a reforming electrolyte with a low EW capable of exhibiting a high proton conductivity, having a high solubility in a solvent, and applicable to a catalyst layer ionomer, a method of manufacturing the same, and a reforming agent.
SOLUTION: The invention relates to the method of manufacturing the reforming electrolyte including a reaction process of reacting sulfonamide polymer containing a sulfonamide group with the reforming agent represented by a general formula: X-[(SO
2 )(CF
2 )
n SO
2 NH]
a -SO
2 R
4 (where X is a halogen, n is an integer no smaller than 1, a is an integer no smaller than 1, R
4 is OH or perfluorocarbon) and combining the sulfonamide polymer with the reforming agent via a sulfonylimide group (-SO
2 NHSO
2 -), the reforming electrolyte obtained through the method, and the reforming agent used to manufacture such a reforming electrolyte.
COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：提供一种能够显示高质子传导性的低EW，在溶剂中溶解性高，适用于催化剂层离聚物的重整电解质，其制造方法和改性剂。解决方案：本发明涉及重整电解质的制造方法，其包括使含有磺酰胺基团的磺酰胺聚合物与由以下通式表示的重整剂反应的反应方法：X - [（SO 2 ）（CF 2 ）名词 SO 2 NH] 一 -SO 2 R 4 （其中X为卤素，n为不小于1的整数，a为不小于1的整数，R 4为OH或全氟化碳）通过磺酰亚胺基团（-SO 2 SBR 2 NHSO 2 SBB）的重整剂的磺酰胺聚合物，通过该方法获得的重整电解质和用于制造这种改性剂重整电解质。版权所有（C）2011，JPO＆INPIT

9. 发明专利

JP2013216518A Solid electrolyte 有权
标题翻译：固体电解液
公开(公告)号：JP2013216518A
公开(公告)日：2013-10-24
申请号：JP2012086892
申请日：2012-04-05
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： FUJITA SATORU , HASEGAWA NAOKI , KAWAKADO MASAYA , ASAOKA MASAHIKO
IPC分类号： C01F7/16
摘要： PROBLEM TO BE SOLVED: To provide a novel solid electrolyte that shows conductivity equivalent to that of YSZ and more.SOLUTION: A solid electrolyte comprises Co substitutional mayenite in which a part of a Ca site of the mayenite (CaAlO) in which an oxygen ion is subsumed in a structure is substituted with Co, wherein a Co/Ca ratio (molar ratio) is 0.03≤Co/Ca≤0.10. In the Co/Ca ratio, 0.05≤Co/Ca≤0.10 is desirable, and 0.07≤Co/Ca≤0.10 is more desirable.
摘要翻译：要解决的问题：提供一种显示与YSZ等效的电导率的新型固体电解质。解决方案：固体电解质包含Co替代钙铝石，其中一部分钙铝矿（CaAlO）的Ca位置，其中氧离子被Co取代，其中Co / Ca比（摩尔比）为0.03≤Co/Ca≤0.10。在Co / Ca比中，希望为0.05≤Co/Ca≤0.10，更优选为0.07≤Co/Ca≤0.10。

10. 发明专利

JP2010238598A Mesoporous electrolyte 有权
标题翻译： MOPOPOROUS电解质
公开(公告)号：JP2010238598A
公开(公告)日：2010-10-21
申请号：JP2009086627
申请日：2009-03-31
申请人： Toyota Central R&D Labs Inc , 株式会社豊田中央研究所
发明人： FUJITA SATORU , KAWAKADO MASAYA , INAGAKI SHINJI , TANI TAKAO
IPC分类号： H01M8/02 , H01B1/06
CPC分类号： Y02E60/50
摘要： PROBLEM TO BE SOLVED: To provide mesoporous electrolyte of an organic/inorganic hybrid type in which a threshold value for the amount of acid radicals which is introduced is dramatically great compared with the conventional. SOLUTION: The mesoporous electrolyte includes a mesoporous body composed from silica with mesopores in an ordered array and a perfluoro sulfonic acid group that is expressed by formula (1) that modifies the inner surfaces of the mesopores. The formula (1) is -[C(H,F) 2 ] n -X-(CF 2 ) m -SO 3 H when X is O or a direct bond and n, m are respectively integers of 1 or more and 3 or less. COPYRIGHT: (C)2011,JPO&INPIT

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