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1. 发明授权

US06806002B2 Electrolytic composition with polymer base for electrochemical generator 失效
标题翻译：电化学发生器用电解质组合物
公开(公告)号：US06806002B2
公开(公告)日：2004-10-19
申请号：US09878356
申请日：2001-06-12
申请人： Alain Vallee , Michel Armand , Yves Choquette , Andre Belanger , Michel Gauthier , Michel Perrier , Karim Zaghib , Estelle Potvin , Simon Besner
发明人： Alain Vallee , Michel Armand , Yves Choquette , Andre Belanger , Michel Gauthier , Michel Perrier , Karim Zaghib , Estelle Potvin , Simon Besner
IPC分类号： H01M462
CPC分类号： H01M2/1686 , H01M2/1673 , H01M6/181 , Y10T29/49108 , Y10T29/49115
摘要： The invention concerns an aprotic electrolytic composition located in the separator and in at least one composite electrode containing a powder of an active electrode material, and if necessary an electronic conduction additive of an electrochemical generator. The electrolytic composition comprises a first polymer matrix consisting of a polyether and at least a second polymer matrix, macroscopically separated, and also at least an alkaline salt as well as a polar aprotic solvent: The polymer matrices are capable of being swollen by at least one of the polar aprotic solvents. The solvent or mixture of solvents is unevenly distributed between the polymer matrices. The invention also concerns an electrochemical generator comprising a negative electrode and positive electrode reversible to alkaline ions and a separator with polymer electrolyte, the electrolytic component of which is the composition described above. The invention further concerns the manufacture in two or three steps of a sub-assembly of an electrochemical generator by coating an electrode support with a composite electrode containing the second matrix, followed by a surface coating on the electrode resulting from the preceding step with a solution containing the first polymer matrix so as to form the separator wholly or partly.
摘要翻译：本发明涉及位于分离器中的非质子电解组合物和至少一个含有活性电极材料的粉末的复合电极，如果需要的话，电化学发生器的电子导电添加剂。电解质组合物包括由聚醚和至少第二聚合物基质组成的宏观分离的第一聚合物基质，以及至少一种碱性盐以及极性非质子溶剂。聚合物基质能够被至少一种的极性非质子溶剂。溶剂或溶剂混合物不均匀地分布在聚合物基质之间。本发明还涉及一种电化学发生器，其包括负极和碱性离子可逆的正极和具有聚合物电解质的隔膜，其电解组分是上述组成。本发明还涉及通过用包含第二基质的复合电极涂覆电极载体，然后在前述步骤中由溶液形成的电极上的表面涂层的方法，在电化学发生器的子组件的两个或三个步骤中制造两个或三个步骤含有第一聚合物基质以全部或部分形成隔膜。

2. 发明授权

US06280882B1 Electrolytic composition with polymer base for electrochemical generator 有权
标题翻译：电化学发生器用电解质组合物
公开(公告)号：US06280882B1
公开(公告)日：2001-08-28
申请号：US09142055
申请日：1998-12-14
申请人： Alain Vallee , Michel Armand , Yves Choquette , Andre Belanger , Michel Gauthier , Michel Perrier , Karim Zaghib , Estelle Potvin , Simon Besner
发明人： Alain Vallee , Michel Armand , Yves Choquette , Andre Belanger , Michel Gauthier , Michel Perrier , Karim Zaghib , Estelle Potvin , Simon Besner
IPC分类号： H01M614
CPC分类号： H01M2/1686 , H01M2/1673 , H01M6/181 , Y10T29/49108 , Y10T29/49115
摘要： The invention concerns an aprotic electrolytic composition located in the separator and in at least one composite electrode containing a powder of an active electrode material, and if necessary an electronic conduction additive of an electrochemical generator The electrolytic composition comprises a first polymer matrix consisting of a polyether and at least a second polymer matrix, macroscopically separated, and also at least an alkaline salt as well as a polar aprotic solvent: The polymer matrices are capable of being swollen by at least one of the polar aprotic solvents. The solvent or mixture of solvents is unevenly distributed between the polymer matrices. The invention also concerns an electrochemical generator comprising a negative electrode and positive electrode reversible to alkaline ions and a separator with polymer electrolyte, the electrolytic component of which is the composition described above. The invention further concerns the manufacture in two or three steps of a sub-assembly of an electrochemical generator by coating an electrode support with a composite electrode containing the second matrix, followed by a surface coating on the electrode resulting from the preceding step with a solution containing the first polymer matrix so as to form the separator wholly or partly.
摘要翻译：本发明涉及位于分离器中的非质子电解组合物和至少一个含有活性电极材料粉末的复合电极，如果需要的话，电化学发生器的电子导电添加剂电解组合物包括由聚醚和至少第二聚合物基质，宏观上分离的，以及至少一种碱性盐以及极性非质子传递溶剂。聚合物基质能够被至少一种极性非质子传递溶剂溶胀。溶剂或溶剂混合物不均匀地分布在聚合物基质之间。本发明还涉及一种电化学发生器，其包括负极和碱性离子可逆的正极和具有聚合物电解质的隔膜，其电解组分是上述组成。本发明还涉及通过用包含第二基质的复合电极涂覆电极载体，然后在前述步骤中由溶液形成的电极上的表面涂层的方法，在电化学发生器的子组件的两个或三个步骤中制造两个或三个步骤含有第一聚合物基质以全部或部分形成隔膜。

3. 发明申请

US20050234177A1 Highly-stable polymeric electrolyte and use thereof in electrochemical systems 有权
标题翻译：高度稳定的聚合物电解质及其在电化学系统中的应用
公开(公告)号：US20050234177A1
公开(公告)日：2005-10-20
申请号：US10501844
申请日：2003-01-15
申请人： Karim Zaghib , Michel Perrier , Abdelbast Guerfi , Elisabeth Dupuis , Patrick Charest , Francois Allaire , Michel Armand
发明人： Karim Zaghib , Michel Perrier , Abdelbast Guerfi , Elisabeth Dupuis , Patrick Charest , Francois Allaire , Michel Armand
IPC分类号： C08J3/24 , C08K3/00 , C08L33/12 , C08L33/20 , C08L101/02 , H01G11/32 , H01G11/56 , H01M4/48 , H01M4/485 , H01M4/50 , H01M4/505 , H01M4/52 , H01M4/525 , H01M4/58 , H01M4/587 , H01M10/052 , H01M10/0525 , H01M10/0565 , H01M10/36 , C08L1/00
CPC分类号： H01G9/038 , C08F283/00 , C08F290/062 , C08G65/2609 , C08G65/33348 , C08L33/12 , C08L71/02 , C09D133/12 , H01G11/56 , H01M4/485 , H01M4/505 , H01M4/525 , H01M4/587 , H01M10/052 , H01M10/0525 , H01M10/0565 , H01M2300/0091 , Y02E60/13 , C08L2666/04
摘要： Polymer electrolyte for an electrochemical generator based on at least a four branched polymer, at least a poly(vinylyldienefluoride), a poly(vinyldiene fluoro-co-hexafluoropropene copolymer), a poly(tetrafluoroethylene), a poly(ethylene-co-propylene-co-5-methylene-2-norbornene) or an ethylene propylene-diene copolymer, a polyol, a poly(methylmethacrylate, a poly(acrylonitrile), SiO2Al2O3, or nano TiO2 non coated or coated with an organic material. This electrolyte allows to prepare electrolytic compositions that can be used in high performance electrochemical devices.
摘要翻译：至少四种支链聚合物，至少一种聚（乙烯基二氟化物），聚（乙烯基二烯氟 - 共 - 六氟丙烯共聚物），聚（四氟乙烯），聚（乙烯 - 共 - 丙烯 - 共 - 5-亚甲基-2-降冰片烯）或乙烯丙烯 - 二烯共聚物，多元醇，聚甲基丙烯酸甲酯，聚（丙烯腈），SiO 2 Al 2 O 2， O 3或非有机材料的纳米TiO 2，该电解质允许制备可用于高性能电化学装置的电解质组合物。

4. 发明授权

US09293769B2 Electrode coated with a film obtained from an aqueous solution comprising a water-soluble binder, production method thereof and uses of same 有权
公开(公告)号：US09293769B2
公开(公告)日：2016-03-22
申请号：US10534697
申请日：2003-11-13
申请人： Karim Zaghib , Michel Armand , Abdelbast Guerfi , Michel Perrier , Elisabeth Dupuis , Patrick Charest
发明人： Karim Zaghib , Michel Armand , Abdelbast Guerfi , Michel Perrier , Elisabeth Dupuis , Patrick Charest
IPC分类号： H01M4/62 , H01G11/42 , H01G11/46 , H01G11/86 , H01M2/14 , H01M2/16 , H01M4/04 , H01M4/139 , H01M4/1391 , H01M4/1393 , H01M4/1397 , H01M4/36 , H01G11/24 , H01G11/28 , H01G11/30 , H01G11/32 , H01M4/58 , H01M10/0569
CPC分类号： H01M4/0404 , H01G11/06 , H01G11/24 , H01G11/28 , H01G11/30 , H01G11/32 , H01G11/42 , H01G11/46 , H01G11/86 , H01M2/145 , H01M2/1653 , H01M4/04 , H01M4/0409 , H01M4/0471 , H01M4/133 , H01M4/136 , H01M4/139 , H01M4/1391 , H01M4/1393 , H01M4/1397 , H01M4/366 , H01M4/5825 , H01M4/587 , H01M4/621 , H01M4/622 , H01M4/623 , H01M4/625 , H01M4/66 , H01M4/661 , H01M10/0525 , H01M10/0565 , H01M10/0568 , H01M10/0569 , H01M2004/027 , H01M2004/028 , H01M2300/0028 , H01M2300/0037 , H01M2300/004 , H01M2300/0042 , H01M2300/0082 , Y02E60/122 , Y02E60/13 , Y02P70/54
摘要： The invention relates to a method of preparing an electrochemical electrode which is partially or totally covered with a film that is obtained by spreading an aqueous solution comprising a water-soluble binder over the electrode and subsequently drying same. The production cost of the electrodes thus obtained is reduced and the surface porosity thereof is associated with desirable resistance values.

5. 发明授权

US07897674B2 Polymer electrolyte with high stability, its use in electrochemical systems 有权
标题翻译：聚合物电解质具有高稳定性，其在电化学系统中的应用
公开(公告)号：US07897674B2
公开(公告)日：2011-03-01
申请号：US10501844
申请日：2003-01-15
申请人： Karim Zaghib , Michel Perrier , Abdelbast Guerfi , Elisabeth Dupuis , Patrick Charest , Francois Allaire , Michel Armand
发明人： Karim Zaghib , Michel Perrier , Abdelbast Guerfi , Elisabeth Dupuis , Patrick Charest , Francois Allaire , Michel Armand
IPC分类号： C08L1/00
CPC分类号： H01G9/038 , C08F283/00 , C08F290/062 , C08G65/2609 , C08G65/33348 , C08L33/12 , C08L71/02 , C09D133/12 , H01G11/56 , H01M4/485 , H01M4/505 , H01M4/525 , H01M4/587 , H01M10/052 , H01M10/0525 , H01M10/0565 , H01M2300/0091 , Y02E60/13 , C08L2666/04
摘要： Polymer electrolyte for an electrochemical generator based on at least a four branched polymer, at least a poly(vinylyldienefluoride), a poly(vinyldiene fluoro-co-hexafluoropropene copolymer), a poly(tetrafluoroethylene), a poly(ethylene-co-propylene-co-5-methylene-2-norbornene) or an ethylene propylene-diene copolymer, a polyol, a poly(methylmethacrylate, a poly(acrylonitrile), SiO2Al2O3, or nano TiO2 non coated or coated with an organic material. This electrolyte allows to prepare electrolytic compositions that can be used in high performance electrochemical devices.
摘要翻译：至少四种支链聚合物，至少一种聚（乙烯基二氟化物），聚（乙烯基二烯氟 - 共 - 六氟丙烯共聚物），聚（四氟乙烯），聚（乙烯 - 共 - 丙烯 - 共聚-5-亚甲基-2-降冰片烯）或乙烯丙烯 - 二烯共聚物，多元醇，聚（甲基丙烯酸甲酯，聚（丙烯腈），SiO 2 Al 2 O 3或纳米TiO 2），未涂覆或涂覆有机材料，该电解质允许制备可用于高性能电化学装置的电解质组合物。

6. 发明申请

US20060166093A1 Electrode coated with a film obtained from an aqueous solution comprising a water-soluble binder, production method thereof and uses of same 有权
标题翻译：用由包含水溶性粘合剂的水溶液获得的膜涂覆的电极，其制备方法和用途
公开(公告)号：US20060166093A1
公开(公告)日：2006-07-27
申请号：US10534697
申请日：2003-11-13
申请人： Karim Zaghib , Michel Armand , Abdelbast Guerfi , Michel Perrier , Elisabeth Dupuis , Patrick Charest
发明人： Karim Zaghib , Michel Armand , Abdelbast Guerfi , Michel Perrier , Elisabeth Dupuis , Patrick Charest
IPC分类号： H01M4/62 , B05D5/12 , H01M4/74 , H01M4/66
CPC分类号： H01M4/0404 , H01G11/06 , H01G11/24 , H01G11/28 , H01G11/30 , H01G11/32 , H01G11/42 , H01G11/46 , H01G11/86 , H01M2/145 , H01M2/1653 , H01M4/04 , H01M4/0409 , H01M4/0471 , H01M4/133 , H01M4/136 , H01M4/139 , H01M4/1391 , H01M4/1393 , H01M4/1397 , H01M4/366 , H01M4/5825 , H01M4/587 , H01M4/621 , H01M4/622 , H01M4/623 , H01M4/625 , H01M4/66 , H01M4/661 , H01M10/0525 , H01M10/0565 , H01M10/0568 , H01M10/0569 , H01M2004/027 , H01M2004/028 , H01M2300/0028 , H01M2300/0037 , H01M2300/004 , H01M2300/0042 , H01M2300/0082 , Y02E60/122 , Y02E60/13 , Y02P70/54
摘要： The invention relates to a method of preparing an electrochemical electrode which is partially or totally covered with a film that is obtained by spreading an aqueous solution comprising a water-soluble binder over the electrode and subsequently drying same. The production cost of the electrodes thus obtained is reduced and the surface porosity thereof is associated with desirable resistance values.
摘要翻译：本发明涉及一种制备电化学电极的方法，其部分或全部被膜覆盖，所述膜通过在电极上铺展包含水溶性粘合剂的水溶液并随后干燥而获得。由此获得的电极的生产成本降低，并且其表面孔隙率与期望的电阻值相关联。

7. 发明授权

US6030421A Ultra thin solid state lithium batteries and process of preparing same 失效
标题翻译：超薄固态锂电池及其制备方法
公开(公告)号：US6030421A
公开(公告)日：2000-02-29
申请号：US64821
申请日：1998-04-23
申请人： Michel Gauthier , Ginette Lessard , Guy Vassort , Patrick Bouchard , Alain Vallee , Michel Perrier
发明人： Michel Gauthier , Ginette Lessard , Guy Vassort , Patrick Bouchard , Alain Vallee , Michel Perrier
IPC分类号： H01M4/64 , H01M4/04 , H01M6/18 , H01M6/40 , H01M10/04 , H01M10/40 , H01M6/16 , H01M6/00
CPC分类号： H01M10/052 , H01M10/0436 , H01M10/0565 , H01M4/04 , H01M6/188 , H01M6/40 , Y10T29/49108 , Y10T29/49112
摘要： There is provided a mother-battery containing at least the following films: an anode of metallic lithium or sodium, a polymer electrolyte which is conductive towards the alkaline ions of the anode and also acts as a separator between the electrodes, and a composite cathode consisting of a compound which is reducible to lithium or sodium, an additive of electronic conduction and a polymer electrolyte binder. The mother battery also includes an electronically conductive thin coating on the external face of the anode and, possibly of the cathode, in which the conductive material is chemically inert towards the electrode material and which also serves to establish permanent electrical contacts on the external faces. The laminated mother-battery of larger surface area and at least partially charged is thereafter subjected to a sharp mechanical cutting out to give thin polymer electrolyte batteries with lithium or sodium anode. The thus cut out batteries preserve substantially their voltage after mechanical cutting out which is recovered by a mechanism of self-healing.
摘要翻译：提供了至少包含以下膜的母体电池：金属锂或钠的阳极，朝向阳极的碱性离子导电并且还用作电极之间的隔板的聚合物电解质，以及包含的可还原成锂或钠的化合物，电子传导添加剂和聚合物电解质粘合剂。母电池还包括在阳极的外表面上以及可能的阴极的电子导电薄涂层，其中导电材料对于电极材料具有化学惰性，并且还用于在外表面上建立永久性电接触。然后将具有较大表面积并且至少部分带电的叠层母电池进行锋利的机械切割以得到具有锂或钠阳极的薄聚合物电解质电池。这样切出的电池在机械切割之后基本保持其电压，其通过自愈机制回收。

8. 发明申请

US20060147790A1 Particle Containing a Graphite Based Nucleus Covered with at Least One Continuous or Discontinuous Layer, Processes for Preparing the Same and Their Uses 有权
标题翻译：含有以至少一个连续或不连续层覆盖的基于石墨的核的粒子，其制备方法及其用途的方法
公开(公告)号：US20060147790A1
公开(公告)日：2006-07-06
申请号：US10532793
申请日：2003-10-23
申请人： Karim Zaghib , Patrick Charest , Abdelbast Querfi , Michel Perrier , Kimio Kinoshita
发明人： Karim Zaghib , Patrick Charest , Abdelbast Querfi , Michel Perrier , Kimio Kinoshita
IPC分类号： B05D5/12 , B05D7/00 , H01B1/04 , H01M4/96 , H01M4/90
CPC分类号： H01M4/90 , C01P2004/03 , C01P2006/40 , C08K3/04 , C08K9/04 , C09C1/46 , C09C1/56 , C09D5/24 , C09D7/62 , H01M4/362 , H01M4/587 , H01M4/625 , H01M4/96 , Y10T428/2991 , Y10T428/2993 , Y10T428/2995 , Y10T428/2996 , Y10T428/2998
摘要： Process for preparing by crushing, a homogenous mixture of particles containing a conductive nucleus including at least one graphite and continuously or discontinuously coated with at least one material that is different from the one constituting the nucleus, the size of the particles of the nucleus being larger than the particles used for coating the nuclei by crushing the particles together. The mixtures of particles obtained show electrochemical and mechanical properties that enable them to be advantageously used in electrochemical batteries and in paints.
摘要翻译：通过粉碎制备包含至少一种石墨的导电核的颗粒的均匀混合物的方法，并连续地或不连续地涂覆有至少一种与构成核的材料不同的材料，核的颗粒尺寸更大比用于通过将颗粒粉碎在一起来涂覆核的颗粒。获得的颗粒的混合物显示出电化学和机械性能，使得它们有利地用于电化学电池和涂料中。

9. 发明授权

US07588826B2 Particle containing a graphite based nucleus with at least one continuous or discontinuous layer, processes for preparing the same and their uses 有权
标题翻译：含有至少一个连续或不连续层的基于石墨的核的颗粒，其制备方法及其用途
公开(公告)号：US07588826B2
公开(公告)日：2009-09-15
申请号：US10532793
申请日：2003-10-23
申请人： Karim Zaghib , Patrick Charest , Abdelbast Guerfi , Michel Perrier , Kimio Kinoshita
发明人： Karim Zaghib , Patrick Charest , Abdelbast Guerfi , Michel Perrier , Kimio Kinoshita
IPC分类号： B32B5/66
CPC分类号： H01M4/90 , C01P2004/03 , C01P2006/40 , C08K3/04 , C08K9/04 , C09C1/46 , C09C1/56 , C09D5/24 , C09D7/62 , H01M4/362 , H01M4/587 , H01M4/625 , H01M4/96 , Y10T428/2991 , Y10T428/2993 , Y10T428/2995 , Y10T428/2996 , Y10T428/2998
摘要： Process for preparing by crushing, a homogenous mixture of particles containing a conductive nucleus including at least one graphite and continuously or discontinuously coated with at least one material that is different from the one constituting the nucleus, the size of the particles of the nucleus being larger than the particles used for coating the nuclei by crushing the particles together. The mixtures of particles obtained show electrochemical and mechanical properties that enable them to be advantageously used in electrochemical batteries and in paints.
摘要翻译：通过粉碎制备包含至少一种石墨的导电核的颗粒的均匀混合物的方法，并连续地或不连续地涂覆有至少一种与构成核的材料不同的材料，核的颗粒尺寸更大比用于通过将颗粒粉碎在一起来涂覆核的颗粒。获得的颗粒的混合物显示出电化学和机械性能，使得它们有利地用于电化学电池和涂料中。

10. 发明申请

US20090017378A1 COATED METAL OXIDE PARTICLES WITH LOW DISSOLUTION RATE, METHODS FOR PREPARING SAME AND USE THEREOF IN ELECTROCHEMICAL SYSTEMS 审中-公开
标题翻译：具有低溶解速率的涂覆金属氧化物颗粒，其制备方法及其在电化学体系中的应用
公开(公告)号：US20090017378A1
公开(公告)日：2009-01-15
申请号：US12162095
申请日：2007-01-24
申请人： Patrick Charest , Michel Perrier , Martin Dontigny , Michel Petitclerc , Abdelbast Guerfi , Karim Zaghib
发明人： Patrick Charest , Michel Perrier , Martin Dontigny , Michel Petitclerc , Abdelbast Guerfi , Karim Zaghib
IPC分类号： H01M4/60 , H01B1/12 , H01M4/88 , B05D5/12 , H01M6/00
CPC分类号： H01M4/621 , H01M4/131 , H01M4/136 , H01M4/139 , H01M4/366 , H01M4/485 , H01M4/5825 , H01M4/625 , H01M10/052 , H01M10/0565 , Y10T29/49108
摘要： Particles comprising a core and a coat covering at least part of the core surface. The core has more than 50% of an acidic metal oxide and the core coating is based on a polymer, preferably based on a soiled polymer with high electrochemical stability. The particle has a solubility rate (ts), in fixed time, of the metal oxide migrating towards the electrolyte, per cycle, which is less than 5 per 10000. The particles are obtained by mixing the polymer and a metal oxide, via dry process with addition of solvent. The electrodes constituting an electrode substrate at least partly coated with a mixture consisting of at least 40 of those particles have remarkable electrochemical properties, in particular regarding the lifetime of batteries in which they are incorporated.
摘要翻译：颗粒包括芯和覆盖芯表面的至少一部分的涂层。核心具有超过50％的酸性金属氧化物，核心涂层基于聚合物，优选基于具有高电化学稳定性的污染聚合物。颗粒在固定时间内的溶解速率（ts）在金属氧化物向电解质迁移的循环中，每周期小于5。通过干法将该聚合物与金属氧化物混合得到颗粒加入溶剂。构成至少部分地涂覆有由这些颗粒中的至少40个的混合物组成的电极基底的电极具有显着的电化学特性，特别是关于它们掺入的电池的寿命。

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